arXiv subjects

J. -V. Kim

Publications and source records attributed to J. -V. Kim.

At least 19 recordsLinked to original sources

arXiv2026

Time-resolved observation of magnon splitting into vortex gyration and Floquet spin waves

Forced excitations at frequencies in the range of the first order azimuthal spin waves of a magnetic disk in the vortex state are known to scatter into the vortex gyration mode, thereby allowing the growth of Floquet spin waves forming a frequency comb. We study the temporal emergence of this dynamical state using time-resolved microwave electrical measurements. The most intense Floquet mode emerges synchronously with the gyration mode after a common incubation delay which diverges at the scattering threshold. This delay is minimal when the drive is resonant with one of the first order azimuthal spin waves. It can be as short as 3 ns for the maximum investigated power. We conclude that the first-to-occur scattering mechanism is the three-wave splitting of a regular azimuthal eigenmode into a coherent pair formed by a gyration magnon and a Floquet spin wave.

cond-mat.mtrl-sci↗

arXiv2026

Field-driven triggering of self-induced Floquet magnons in a magnetic vortex

We report the experimental control of Floquet magnons in a magnetic vortex. Using microwave spectroscopy of vortex state magnetic tunnel junctions (MTJs), we find that self-induced Floquet sidebands form frequency combs whose existence depend on the vortex core orbit. By shifting the vortex core with an applied magnetic field, we switch the system between regular and Floquet magnons at identical drive conditions, demonstrating hysteretic control of the Floquet spectrum. A nonlinear vortex-magnon model shows that this behavior originates from multiple stable vortex gyration radii created by Floquet-mediated feedback. These results establish magnetic state initialization as a means to switch between regular and Floquet magnons.

cond-mat.mtrl-sci↗

arXiv2025

Experimental observation of vortex gyrotropic mode excited by surface acoustic waves

The traditional method for exciting spin-wave dynamics in magnetic materials involves microwave magnetic fields generated by current injection into inductive antennas. However, there is a growing interest in non-inductive excitation methods. Magneto-acoustic effects present a viable alternative, where strains produced by applying voltages to a piezoelectric substrate can couple to spin-waves in a magnetic film. Recently, it has been proposed that surface acoustic waves (SAWs) can excite the gyrotropic mode of the vortex state in a magnetic disk. Here we report on experiments utilizing a magnetic resonance force microscope to investigate magnetization dynamics in CoFeB sub-micrometer disks in the vortex state, grown on a Z-cut LiNbO$_3$ substrate. The device design enables excitation of the gyrotropic mode either inductively, using an antenna on top of the disks, or acoustically via SAWs launched from an interdigital transducer. Our modelling indicates that the lattice rotation ωxz generates a localized magneto-acoustic field that displaces the vortex core from the disk center, initiating the gyration motion. Tuning of the magneto-acoustic torque acting on the vortex structure is achieved by a perpendicular magnetic field. These results demonstrate the clear excitation of the vortex gyrotropic mode by magneto-acoustic excitation.

cond-mat.mtrl-sci↗

arXiv2023

Unidirectionality of spin waves in Synthetic Antiferromagnets

We study the frequency non-reciprocity of the spin waves in symmetric CoFeB/Ru/CoFeB synthetic antiferromagnets stacks set in the scissors state by in-plane applied fields. Using a combination of Brillouin Light Scattering and propagating spin wave spectroscopy experiments, we show that the acoustical spin waves in synthetic antiferromagnets possess a unique feature if their wavevector is parallel to the applied field: the frequency non-reciprocity due to layer-to-layer dipolar interactions can be so large that the acoustical spin waves transfer energy in a unidirectional manner for a wide and bipolar interval of wavevectors. Analytical modeling and full micromagnetic calculations are conducted to account for the dispersion relations of the optical and acoustical spin waves for arbitrary field orientations. Our formalism provides a simple and direct method to understand and design devices harnessing unidirectional propagation of spin waves in synthetic antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2022

Exchange energies in CoFeB/Ru/CoFeB Synthetic Antiferromagnets

The interlayer exchange coupling confers specific properties to Synthetic Antiferromagnets that make them suitable for several applications of spintronics. The efficient use of this magnetic configuration requires an in-depth understanding of the magnetic properties and their correlation with the material structure. Here we establish a reliable procedure to quantify the interlayer exchange coupling and the intralayer exchange stiffness in synthetic antiferromagnets; we apply it to the ultrasmooth and amorphous Co$_{40}$Fe$_{40}$B$_{20}$ (5-40 nm)/Ru/ Co$_{40}$Fe$_{40}$B$_{20}$ material platform. The complex interplay between the two exchange interactions results in a gradient of the magnetization orientation across the thickness of the stack which alters the hysteresis and the spin wave eigenmodes of the stack in a non trivial way. We measured the field-dependence of the frequencies of the first four spin waves confined within the thickness of the stack. We modeled these frequencies and the corresponding thickness profiles of these spin waves using micromagnetic simulations. The comparison with the experimental results allows to deduce the magnetic parameters that best account for the sample behavior. The exchange stiffness is established to be 16 $\pm$ 2 pJ/m, independently of the Co$_{40}$Fe$_{40}$B$_{20}$ thickness. The interlayer exchange coupling starts from -1.7 mJ/m$^2$ for the thinnest layers and it can be maintained above -1.3 mJ/m$^2$ for CoFeB layers as thick as 40 nm. The comparison of our method with earlier characterizations using the sole saturation fields argues for a need to revisit the tabulated values of interlayer exchange coupling in thick synthetic antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2022

Measuring a population of spin waves from the electrical noise of an inductively coupled antenna

We study how a population of spin waves can be characterized from the analysis of the electrical microwave noise delivered by an inductive antenna placed in its vicinity. The measurements are conducted on a synthetic antiferromagnetic thin stripe covered by a micron-sized antenna that feeds a spectrum analyser after amplification. The antenna noise contains two contributions. The population of incoherent spin waves generates a fluctuating field that is sensed by the antenna: this is the "magnon noise". The antenna noise also contains the contribution of the electronic fluctuations: the Johnson-Nyquist noise. The latter depends on all impedances within the measurement circuit, which includes the antenna self-inductance. As a result, the electronic noise contains information about the magnetic susceptibility of the stripe, though it does not inform on the absolute amplitude of the magnetic fluctuations. For micrometer-sized systems at thermal equilibrium, the electronic noise dominates and the pure magnon noise cannot be determined. If in contrast the spinwave bath is not at thermal equilibrium with the measurement circuit, and if the spin wave population can be changed then one could measure a mode-resolved effective magnon temperature provided specific precautions are implemented.

cond-mat.mtrl-sci↗

arXiv2020

Real-space imaging of non-collinear antiferromagnetic order with a single spin magnetometer

While ferromagnets are at the heart of daily life applications, their large magnetization and resulting energy cost for switching bring into question their suitability for reliable low-power spintronic devices. Non-collinear antiferromagnetic systems do not suffer from this problem and often possess remarkable extra functionalities: non-collinear spin order may break space-inversion symmetry and thus allow electric-field control of magnetism, or produce emergent spin-orbit effects, which enable efficient spin-charge interconversion. To harness these unique traits for next-generation spintronics, the nanoscale control and imaging capabilities that are now routine for ferromagnets must be developed for antiferromagnetic systems. Here, using a non-invasive scanning nanomagnetometer based on a single nitrogen-vacancy (NV) defect in diamond, we demonstrate the first real-space visualization of non-collinear antiferromagnetic order in a magnetic thin film, at room temperature. We image the spin cycloid of a multiferroic BiFeO$_3$ thin film and extract a period of $\sim70$ nm, consistent with values determined by macroscopic diffraction. In addition, we take advantage of the magnetoelectric coupling present in BiFeO$_3$ to manipulate the cycloid propagation direction by an electric field. Besides highlighting the unique potential of NV magnetometry for imaging complex antiferromagnetic orders at the nanoscale, these results demonstrate how BiFeO$_3$ can be used as a versatile platform for the design of reconfigurable nanoscale spin textures.

cond-mat.mtrl-sci↗

arXiv2020

Quantifying the thermal stability in perpendicularly magnetized ferromagnetic nanodisks with forward flux sampling

The thermal stability in nanostructured magnetic systems is an important issue for applications in information storage. From a theoretical and simulation perspective, an accurate prediction of thermally-activated transitions is a challenging problem because desired retention times are on the order of 10 years, while the characteristic time scale for precessional magnetization dynamics is of the order of nanoseconds. Here, we present a theoretical study of the thermal stability of magnetic elements in the form of perpendicularly-magnetized ferromagnetic disks using the forward flux sampling method, which is useful for simulating rare events. We demonstrate how rates of thermally-activated switching between the two uniformly-magnetized ``up'' and ``down'' states, which occurs through domain wall nucleation and propagation, vary with the interfacial Dzyaloshinskii-Moriya interaction, which affect the energy barrier separating these states. Moreover, we find that the average lifetimes differ by several orders of magnitude from estimates based on the commonly assumed value of 1 GHz for the attempt frequency.

cond-mat.mes-hall↗

arXiv2020

Entropy-reduced retention times in magnetic memory elements: A case of the Meyer-Neldel Compensation Rule

We compute mean waiting times between thermally-activated magnetization reversals in a nanodisk with parameters similar to a free CoFeB layer used in magnetic random access memories. By combining Langer's theory and forward flux sampling simulations, we show that the Arrhenius prefactor can take values up to 10$^{21}$ Hz, orders of magnitude beyond the value of 10$^{9}$ Hz typically assumed, and varies drastically as a function of material parameters. We show that the prefactor behaves like an exponential of the activation energy, which highlights a case of the Meyer-Neldel compensation rule. This suggests that modeling information retention times with a barrier-independent prefactor in such magnetic storage elements is not justified.

cond-mat.mes-hall↗

arXiv2020

Path sampling for lifetimes of metastable magnetic skyrmions and direct comparison with Kramers' method

We perform a direct comparison between Kramers' method in many dimensions -- i.e., Langer's theory -- adapted to magnetic spin systems, and a path sampling method in the form of forward flux sampling, as a means to compute collapse rates of metastable magnetic skyrmions. We show that a good agreement is obtained between the two methods. We report variations of the attempt frequency associated with skyrmion collapse by three to four orders of magnitude when varying the applied magnetic field by 5$\%$ of the exchange strength, which confirms the existence of a strong entropic contribution to the lifetime of skyrmions. This demonstrates that in complex systems, the knowledge of the rate prefactor, in addition to the internal energy barrier, is essential in order to properly estimate a lifetime.

cond-mat.mes-hall↗

arXiv2019

Paths to annihilation of first and second-order (anti)skyrmions via (anti)meron nucleation on the frustrated square lattice

We study annihilation mechanisms of small first- and second-order skyrmions and antiskyrmions on the frustrated $J_1-J_2-J_3$ square lattice with broken inversion symmetry (DMI). We find that annihilation happens via the injection of the opposite topological charge in the form of meron or antimeron nucleation. Overall, the exchange frustration generates a complex energy landscape with not only many (meta)stable and unstable local energy solutions, but also many possible paths connecting them. Whenever possible, we compute the activation energy and attempt frequency for the annihilation of isolated topological defects. In particular, we compare the average lifetime of the antiskyrmion calculated with transition state theory with direct Langevin simulations, where an excellent agreement is obtained.

cond-mat.mes-hall↗

arXiv2019

Determining key spin-orbitronic parameters by means of propagating spin waves

We characterize spin wave propagation and its modification by an electrical current in Permalloy(Py)/Pt bilayers with Py thickness between 4 and 20 nm. First, we analyze the frequency non-reciprocity of surface spin waves and extract from it the interfacial Dzyaloshinskii-Moriya interaction constant $D_s$ accounting for an additional contribution due to asymmetric surface anisotropies. Second, we measure the spin-wave relaxation rate and deduce from it the Py/Pt spin mixing conductance $g^{\uparrow\downarrow}_{eff}$. Last, applying a \textit{dc} electrical current, we extract the spin Hall conductivity $σ_{SH}$ from the change of spin wave relaxation rate due to the spin-Hall spin transfer torque. We obtain a consistent picture of the spin wave propagation data for different film thicknesses using a single set of parameters $D_s=0.25$ pJ/m, $g^{\uparrow\downarrow}_{eff} = 3.2\times 10^{19}$ m$^{-2}$ and $σ_{SH}=4\times10^{5}$ S/m.

cond-mat.mtrl-sci↗

arXiv2016

Direct measurement of interfacial Dzyaloshinskii-Moriya interaction in X/CoFeB/MgO heterostructures with a scanning-NV magnetometer

The Dzyaloshinskii-Moriya Interaction (DMI) has recently attracted considerable interest owing to its fundamental role in the stabilization of chiral spin textures in ultrathin ferromagnets, which are interesting candidates for future spintronic technologies. Here we employ a scanning nano-magnetometer based on a single nitrogen-vacancy (NV) defect in diamond to locally probe the strength of the interfacial DMI in CoFeB/MgO ultrathin films grown on different heavy metal underlayers X=Ta,TaN, and W. By measuring the stray field emanating from DWs in micron-long wires of such materials, we observe deviations from the Bloch profile for TaN and W underlayers that are consistent with a positive DMI value favoring right-handed chiral spin structures. Moreover, our measurements suggest that the DMI constant might vary locally within a single sample, illustrating the importance of local probes for the study of magnetic order at the nanoscale.

cond-mat.mes-hall↗

arXiv2016

Probing the Dzyaloshinskii-Moriya interaction in CoFeB ultrathin films using domain wall creep and Brillouin light spectroscopy

We have characterized the strength of the interfacial Dyzaloshinskii-Moriya interaction (DMI) in ultrathin perpendicularly magnetized CoFeB/MgO films, grown on different underlayers of W, TaN, and Hf, using two experimental methods. First, we determined the effective DMI field from measurements of field-driven domain wall motion in the creep regime, where applied in-plane magnetic fields induce an anisotropy in the wall propagation that is correlated with the DMI strength. Second, Brillouin light spectroscopy was employed to quantify the frequency non-reciprocity of spin waves in the CoFeB layers, which yielded an independent measurement of the DMI. By combining these results, we show that DMI estimates from the different techniques only yield qualitative agreement, which suggests that open questions remain on the underlying models used to interpret these results.

cond-mat.mtrl-sci↗

arXiv2016

Spin wave amplification using the spin Hall effect in permalloy/platinum bilayers

We investigate the effect of an electrical current on the attenuation length of a 900 nm wavelength spin-wave in a permalloy/Pt bilayer using propagating spin-wave spectroscopy. The modification of the spin-wave relaxation rate is linear in current density, reaching up to 14% for a current density of 2.3$\times10^{11} $A/m$^2$ in Pt. This change is attributed to the spin transfer torque induced by the spin Hall effect and corresponds to an effective spin Hall angle of 0.13, which is among the highest values reported so far. The spin Hall effect thus appears as an efficient way of amplifying/attenuating propagating spin waves.

cond-mat.mtrl-sci↗

arXiv2016

Exchange stiffness in ultrathin perpendicularly-magnetized CoFeB layers determined using spin wave spectroscopy

We measure the frequencies of spin waves in nm-thick perpendicularly magnetized FeCoB systems, and model the frequencies to deduce the exchange stiffness of this material in the ultrathin limit. For this, we embody the layers in magnetic tunnel junctions patterned into circular nanopillars of diameters ranging from 100 to 300 nm and we use magneto-resistance to determine which rf-current frequencies are efficient in populating the spin wave modes. Micromagnetic calculations indicate that the ultrathin nature of the layer and the large wave vectors used ensure that the spin wave frequencies are predominantly determined by the exchange stiffness, such that the number of modes in a given frequency window can be used to estimate the exchange. For 1 nm layers the experimental data are consistent with an exchange stiffness A= 20 pJ/m, which is slightly lower that its bulk counterpart. The thickness dependence of the exchange stiffness has strong implications for the numerous situations that involve ultrathin films hosting strong magnetization gradients, and the micromagnetic description thereof.

cond-mat.str-el↗

arXiv2016

A skyrmion-based spin-torque nano-oscillator

A model for a spin-torque nano-oscillator based on the self-sustained oscillation of a magnetic skyrmion is presented. The system involves a circular nanopillar geometry comprising an ultrathin film free magnetic layer with a strong Dzyaloshinkii-Moriya interaction and a polariser layer with a vortex-like spin configuration. It is shown that spin-transfer torques due to current flow perpendicular to the film plane leads to skyrmion gyration that arises from a competition between geometric confinement due to boundary edges and the vortex-like polarisation of the spin torques. A phenomenology for such oscillations is developed and quantitative analysis using micromagnetics simulations is presented. It is also shown that weak disorder due to random anisotropy variations does not influence the main characteristics of the steady-state gyration.

cond-mat.mes-hall↗

arXiv2014

The nature of domain walls in ultrathin ferromagnets revealed by scanning nanomagnetometry

The recent observation of current-induced domain wall (DW) motion with large velocity in ultrathin magnetic wires has opened new opportunities for spintronic devices. However, there is still no consensus on the underlying mechanisms of DW motion. Key to this debate is the DW structure, which can be of Bloch or Néel type, and dramatically affects the efficiency of the different proposed mechanisms. To date, most experiments aiming to address this question have relied on deducing the DW structure and chirality from its motion under additional in-plane applied fields, which is indirect and involves strong assumptions on its dynamics. Here we introduce a general method enabling direct, in situ, determination of the DW structure in ultrathin ferromagnets. It relies on local measurements of the stray field distribution above the DW using a scanning nanomagnetometer based on the Nitrogen-Vacancy defect in diamond. We first apply the method to a Ta/Co40Fe40B20(1 nm)/MgO magnetic wire and find clear signature of pure Bloch DWs. In contrast, we observe left-handed Néel DWs in a Pt/Co(0.6 nm)/AlOx wire, providing direct evidence for the presence of a sizable Dzyaloshinskii-Moriya interaction (DMI) at the Pt/Co interface. This method offers a new path for exploring interfacial DMI in ultrathin ferromagnets and elucidating the physics of DW motion under current.

cond-mat.mes-hall↗