arXiv subjects

J. A. Devlin

Publications and source records attributed to J. A. Devlin.

17 recordsLinked to original sources

arXiv2024

Orders of Magnitude Improved Cyclotron-Mode Cooling for Non-Destructive Spin Quantum Transition Spectroscopy with Single Trapped Antiprotons

We demonstrate efficient sub-thermal cooling of the modified cyclotron mode of a single trapped antiproton and reach particle temperatures $T_+=E_+/k_\text{B}$ below $200\,$mK in preparation times shorter than $500\,$s. This corresponds to the fastest resistive single-particle cyclotron cooling to sub-thermal temperatures ever demonstrated. By cooling trapped particles to such low energies, we demonstrate the detection of antiproton spin transitions with an error-rate $<0.000025$, more than three orders of magnitude better than in previous best experiments. This method will have enormous impact on multi-Penning-trap experiments that measure magnetic moments with single nuclear spins for tests of matter/antimatter symmetry, high-precision mass-spectrometry, and measurements of electron $g$-factors bound to highly-charged ions that test quantum electrodynamics.

physics.atom-ph↗

arXiv2023

A 16 Parts per Trillion Comparison of the Antiproton-to-Proton q/m Ratios

The Standard Model (SM) of particle physics is both incredibly successful and glaringly incomplete. Among the questions left open is the striking imbalance of matter and antimatter in the observable universe which inspires experiments to compare the fundamental properties of matter/antimatter conjugates with high precision. Our experiments deal with direct investigations of the fundamental properties of protons and antiprotons, performing spectroscopy in advanced cryogenic Penning-trap systems. For instance, we compared the proton/antiproton magnetic moments with 1.5 ppb fractional precision, which improved upon previous best measurements by a factor of >3000. Here we report on a new comparison of the proton/antiproton charge-to-mass ratios with a fractional uncertainty of 16ppt. Our result is based on the combination of four independent long term studies, recorded in a total time span of 1.5 years. We use different measurement methods and experimental setups incorporating different systematic effects. The final result, $-(q/m)_{\mathrm{p}}/(q/m)_{\bar{\mathrm{p}}}$ = $1.000\,000\,000\,003 (16)$, is consistent with the fundamental charge-parity-time (CPT) reversal invariance, and improves the precision of our previous best measurement by a factor of 4.3. The measurement tests the SM at an energy scale of $1.96\cdot10^{-27}\,$GeV (C$.$L$.$ 0.68), and improves 10 coefficients of the Standard Model Extension (SME). Our cyclotron-clock-study also constrains hypothetical interactions mediating violations of the clock weak equivalence principle (WEP$_\text{cc}$) for antimatter to a level of $|α_{g}-1| < 1.8 \cdot 10^{-7}$, and enables the first differential test of the WEP$_\text{cc}$ using antiprotons \cite{hughes1991constraints}. From this interpretation we constrain the differential WEP$_\text{cc}$-violating coefficient to $|α_{g,D}-1|<0.030$.

physics.atom-ph↗

arXiv2023

Image-current mediated sympathetic laser cooling of a single proton in a Penning trap down to 170 mK axial temperature

We demonstrate a new temperature record for image-current mediated sympathetic cooling of a single proton in a cryogenic Penning trap by laser-cooled $^9$Be$^+$. An axial mode temperature of 170 mK is reached, which is a 15-fold improvement compared to the previous best value. Our cooling technique is applicable to any charged particle, so that the measurements presented here constitute a milestone towards the next generation of high-precision Penning-trap measurements with exotic particles.

physics.atom-ph↗

arXiv2023

Ultra thin polymer foil cryogenic window for antiproton deceleration and storage

We present the design and characterisation of a cryogenic window based on an ultra-thin aluminised PET foil at T < 10K, which can withstand a pressure difference larger than 1bar at a leak rate < $1\times 10^{-9}$ mbar$\cdot$ l/s. Its thickness of approximately 1.7 $μ$m makes it transparent to various types of particles over a broad energy range. To optimise the transfer of 100keV antiprotons through the window, we tested the degrading properties of different aluminium coated PET foils of thicknesses between 900nm and 2160nm, concluding that 1760nm foil decelerates antiprotons to an average energy of 5 keV. We have also explicitly studied the permeation as a function of coating thickness and temperature, and have performed extensive thermal and mechanical endurance and stress tests. Our final design integrated into the experiment has an effective open surface consisting of 7 holes with 1 mm diameter and will transmit up to 2.5% of the injected 100keV antiproton beam delivered by the AD/ELENA-facility of CERN.

physics.ins-det↗

arXiv2023

BASE-STEP: A transportable antiproton reservoir for fundamental interaction studies

Currently, the only worldwide source of low-energy antiprotons is the AD/ELENA facility located at CERN. To date, all precision measurements on single antiprotons have been conducted at this facility and provide stringent tests of the fundamental interactions and their symmetries. However, the magnetic field fluctuations from the facility operation limit the precision of upcoming measurements. To overcome this limitation, we have designed the transportable antiproton trap system BASE-STEP to relocate antiprotons to laboratories with a calm magnetic environment. We anticipate that the transportable antiproton trap will facilitate enhanced tests of CPT invariance with antiprotons, and provide new experimental possibilities of using transported antiprotons and other accelerator-produced exotic ions. We present here the technical design of the transportable trap system. This includes the transportable superconducting magnet, the cryogenic inlay consisting of the trap stack and the detection systems, and the differential pumping section to suppress the residual gas flow into the cryogenic trap chamber.

physics.ins-det↗

arXiv2023

Testing CPT Invariance by High-Precision Comparisons of Fundamental Properties of Protons and Antiprotons at BASE

The BASE collaboration at the Antiproton Decelerator facility of CERN compares the fundamental properties of protons and antiprotons using advanced Penning-trap systems. In previous measurement campaigns, we measured the magnetic moments of the proton and the antiproton, reaching (sub-)parts-in-a-billion fractional uncertainty. In the latest campaign, we have compared the proton and antiproton charge-to-mass ratios with a fractional uncertainty of 16 parts in a trillion. In this contribution, we give an overview of the measurement campaign, and detail how its results are used to constrain nine spin-independent coefficients of the Standard-Model Extension in the proton and electron sector.

hep-ex↗

arXiv2021

Sympathetic cooling schemes for separately trapped ions coupled via image currents

Cooling of particles to mK-temperatures is essential for a variety of experiments with trapped charged particles. However, many species of interest lack suitable electronic transitions for direct laser cooling. We study theoretically the remote sympathetic cooling of a single proton with laser-cooled $^9$Be$^+$ in a double-Penning-trap system. We investigate three different cooling schemes and find, based on analytical calculations and numerical simulations, that two of them are capable of achieving proton temperatures of about 10 mK with cooling times on the order of 10 s. In contrast, established methods such as feedback-enhanced resistive cooling with image-current detectors are limited to about 1 K in 100 s. Since the studied techniques are applicable to any trapped charged particle and allow spatial separation between the target ion and the cooling species, they enable a variety of precision measurements based on trapped charged particles to be performed at improved sampling rates and with reduced systematic uncertainties.

physics.atom-ph↗

arXiv2021

Sympathetic cooling of a trapped proton mediated by an LC circuit

Efficient cooling of trapped charged particles is essential to many fundamental physics experiments, to high-precision metrology, and to quantum technology. Until now, sympathetic cooling has required close-range Coulomb interactions, but there has been a sustained desire to bring laser-cooling techniques to particles in macroscopically separated traps, extending quantum control techniques to previously inaccessible particles such as highly charged ions, molecular ions and antimatter. Here we demonstrate sympathetic cooling of a single proton using laser-cooled Be+ ions in spatially separated Penning traps. The traps are connected by a superconducting LC circuit that enables energy exchange over a distance of 9 cm. We also demonstrate the cooling of a resonant mode of a macroscopic LC circuit with laser-cooled ions and sympathetic cooling of an individually trapped proton, reaching temperatures far below the environmental temperature. Notably, as this technique uses only image-current interactions, it can be easily applied to an experiment with antiprotons, facilitating improved precision in matter-antimatter comparisons and dark matter searches.

physics.atom-ph↗

arXiv2021

Laser cooling and magneto-optical trapping of molecules analyzed using optical Bloch equations and the Fokker-Planck-Kramers equation

We study theoretically the behavior of laser-cooled calcium monofluoride (CaF) molecules in an optical molasses and magneto-optical trap (MOT), and compare our results to recent experiments. We use multi-level optical Bloch equations to estimate the force and the diffusion constant, followed by a Fokker-Planck-Kramers equation to calculate the time-evolution of the velocity distribution. The calculations are done in three-dimensions, and we include all the relevant energy levels of the molecule and all the relevant frequency components of the light. Similar to simpler model systems, the velocity-dependent force curve exhibits Doppler and polarization-gradient forces of opposite signs. We show that the temperature of the MOT is governed mainly by the balance of these two forces. Our calculated MOT temperatures and photon scattering rates are in broad agreement with those measured experimentally over a wide range of parameters. In a blue-detuned molasses, the temperature is determined by the balance of polarization gradient cooling, and heating due to momentum diffusion, with no significant contribution from Doppler heating. In the molasses, we calculate a damping rate similar to the measured one, and steady-state temperatures that have the same dependence on laser intensity and applied magnetic field as measured experimentally, but are consistently a few times smaller than measured. We attribute the higher temperatures in the experiments to fluctuations of the dipole force which are not captured by our model. We show that the photon scattering rate is strongly influenced by the presence of dark states in the system, but that the scattering rate does not go to zero even for stationary molecules because of the transient nature of the dark states.

physics.atom-ph↗

arXiv2020

Direct limits on the interaction of antiprotons with axion-like dark matter

Astrophysical observations indicate that there is roughly five times more dark matter in the Universe than ordinary baryonic matter, with an even larger amount of the Universe's energy content due to dark energy. So far, the microscopic properties of these dark components have remained shrouded in mystery. In addition, even the five percent of ordinary matter in our Universe has yet to be understood, since the Standard Model of particle physics lacks any consistent explanation for the predominance of matter over antimatter. Inspired by these central problems of modern physics, we present here a direct search for interactions of antimatter with dark matter, and place direct constraints on the interaction of ultra-light axion-like particles $-$ one of the dark-matter candidates $-$ and antiprotons. If antiprotons exhibit a stronger coupling to these dark-matter particles than protons, such a CPT-odd coupling could provide a link between dark matter and the baryon asymmetry in the Universe. We analyse spin-flip resonance data acquired with a single antiproton in a Penning trap [Smorra et al., Nature 550, 371 (2017)] in the frequency domain to search for spin-precession effects from ultra-light axions with a characteristic frequency governed by the mass of the underlying particle. Our analysis constrains the axion-antiproton interaction parameter $f_a/C_{\overline{p}}$ to values greater than $0.1$ to $0.6$ GeV in the mass range from $2 \times 10^{-23}$ to $4 \times 10^{-17}\,$eV/$c^2$, improving over astrophysical antiproton bounds by up to five orders of magnitude. In addition, we derive limits on six combinations of previously unconstrained Lorentz-violating and CPT-violating terms of the non-minimal Standard Model Extension.

physics.atom-ph↗

arXiv2020

New techniques for a measurement of the electron's electric dipole moment

The electric dipole moment of the electron (eEDM) can be measured with high precision using heavy polar molecules. In this paper, we report on a series of new techniques that have improved the statistical sensitivity of the YbF eEDM experiment. We increase the number of molecules participating in the experiment by an order of magnitude using a carefully designed optical pumping scheme. We also increase the detection efficiency of these molecules by another order of magnitude using an optical cycling scheme. In addition, we show how to destabilise dark states and reduce backgrounds that otherwise limit the efficiency of these techniques. Together, these improvements allow us to demonstrate a statistical sensitivity of $1.8 \times 10^{-28}$ e cm after one day of measurement, which is 1.2 times the shot-noise limit. The techniques presented here are applicable to other high-precision measurements using molecules.

physics.atom-ph↗

arXiv2019

Deep laser cooling and efficient magnetic compression of molecules

We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and characterise the method experimentally, reaching a temperature of 5.4(7) $μ$K. We solve a general problem of measuring low temperatures for large clouds by rotating the phase-space distribution and then directly imaging the complete velocity distribution. Using the same phase-space rotation method, we rapidly compress the cloud. Applying the cooling method a second time, we compress both the position and velocity distributions.

physics.atom-ph↗

arXiv2019

Measurement of ultra-low heating rates of a single antiproton in a cryogenic Penning trap

We report on the first detailed study of motional heating in a cryogenic Penning trap using a single antiproton. Employing the continuous Stern-Gerlach effect we observe cyclotron quantum transition rates of 6(1) quanta/h and an electric field noise spectral density below $7.5(3.4)\times 10^{-20}\,\text{V}^{2}\text{m}^{-2} \text{Hz}^{-1}$, which corresponds to a scaled noise spectral density below $8.8(4.0)\times 10^{-12}\,\text{V}^{2}\text{m}^{-2}$, results which are more than two orders of magnitude smaller than those reported by other ion trap experiments.

physics.atom-ph↗

arXiv2017

Blue-detuned magneto-optical trap

We present the properties and advantages of a new magneto-optical trap (MOT) where blue-detuned light drives `type-II' transitions that have dark ground states. Using $^{87}$Rb, we reach a radiation-pressure-limited density exceeding $10^{11}$cm$^{-3}$ and a temperature below 30$μ$K. The phase-space density is higher than in normal atomic MOTs, and a million times higher than comparable red-detuned type-II MOTs, making it particularly attractive for molecular MOTs which rely on type-II transitions. The loss of atoms from the trap is dominated by ultracold collisions between Rb atoms. For typical trapping conditions, we measure a loss rate of $1.8(4)\times10^{-10}$cm$^{3}$s$^{-1}$.

physics.atom-ph↗

arXiv2017

Ultracold molecules for measuring the electron's electric dipole moment

We demonstrate one-dimensional sub-Doppler laser cooling of a beam of YbF molecules to 100 $μ$K. This is a key step towards a measurement of the electron's electric dipole moment using ultracold molecules. We compare the effectiveness of magnetically-assisted and polarization-gradient sub-Doppler cooling mechanisms. We model the experiment and find good agreement with our data.

physics.atom-ph↗

arXiv2017

Three-dimensional Doppler, polarization-gradient, and magneto-optical forces for atoms and molecules with dark states

We theoretically investigate the damping and trapping forces in a three-dimensional magneto-optical trap (MOT), by numerically solving the optical Bloch equations. We focus on the case where there are dark states because the atom is driven on a "type-II" system where the angular momentum of the excited state, $F'$, is less than or equal to that of the ground state, $F$. For these systems we find that the force in a three-dimensional light field has very different behaviour to its one dimensional counterpart. This differs from the more commonly used "type-I" systems ($F'=F+1$) where the 1D and 3D behaviours are similar. Unlike type-I systems where, for red-detuned light, both Doppler and sub-Doppler forces damp the atomic motion towards zero velocity, in type-II systems in 3D, the Doppler force and polarization gradient force have opposite signs. As a result, the atom is driven towards a non-zero equilibrium velocity, $v_{0}$, where the two forces cancel. We find that $v_{0}^{2}$ scales linearly with the intensity of the light and is fairly insensitive to the detuning from resonance. We also discover a new magneto-optical force that alters the normal MOT force at low magnetic fields and whose influence is greatest in the type-II systems. We discuss the implications of these findings for the laser cooling and magneto-optical trapping of molecules where type-II transitions are unavoidable in realising closed optical cycling transitions.

physics.atom-ph↗

arXiv2016

Low magnetic Johnson noise electric field plates for precision measurement

We describe a parallel pair of high voltage electric field plates designed and constructed to minimise magnetic Johnson noise. They are formed by laminating glass substrates with commercially available polyimide (Kapton) tape, covered with a thin gold film. Tested in vacuum, the outgassing rate is less than $5\times10^{-5}$ mbar.l/s. The plates have been operated at electric fields up to 8.3 kV/cm, when the leakage current is at most a few hundred pA. The design is discussed in the context of a molecular spin precession experiment to measure the permanent electric dipole moment of the electron.

physics.ins-det↗