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J. A. Mydosh

Publications and source records attributed to J. A. Mydosh.

At least 73 records · Page 4Linked to original sources
arXiv2004

Ferromagnetism makes a doped semiconductor less shiny

Magnetic semiconductors have attracted interest because of the question of how a magnetic metal can be derived from a paramagnetic insulator. Here our approach is to carrier dope insulating FeSi and we show that the magnetic half-metal which emerges has unprecedented optical properties, unlike those of other low carrier density magnetic metals. All traces of the semiconducting gap of FeSi are obliterated and the material is unique in being less reflective in the ferromagnetic than in the paramagnetic state, corresponding to larger rather than smaller electron scattering in the ordered phase.

cond-mat.str-el↗
arXiv2003

Magnetotransport in Single Crystal Half-Heusler Compounds

We present the results of electrical resistivity and Hall effect measurements on single crystals of HfNiSn, TiPtSn, and TiNiSn. Semiconducting behavior is observed in each case, involving the transport of a small number of highly compensated carriers. Magnetization measurements suggest that impurities and site disorder create both localized magnetic moments and extended paramagnetic states, with the susceptibility of the latter increasing strongly with reduced temperature. The magnetoresistance is sublinear or linear in fields ranging from 0.01 - 9 Tesla at the lowest temperatures. As the temperature increases, the normal quadratic magnetoresistance is regained, initially at low fields, and at the highest temperatures extending over the complete range of fields. The origin of the vanishingly small field scale implied by these measurements remains unknown, presenting a challenge to existing classical and quantum mechanical theories of magnetoresistance.

cond-mat.str-el↗
arXiv2003

Divergence of the Grueneisen Ratio at Quantum Critical Points in Heavy Fermion Metals

We present low-temperature volume thermal expansion, $β$, and specific heat, $C$, measurements on high-quality single crystals of CeNi2Ge2 and YbRh2(Si$_{0.95}$Ge$_{0.05}$)$_2$ which are located very near to quantum critical points. For both systems, $β$ shows a more singular temperature dependence than $C$, and thus the Grueneisen ratio ${Γ\propto β/C}$ diverges as T --> 0. For CeNi2Ge2, our results are in accordance with the spin-density wave (SDW) scenario for three-dimensional critical spin-fluctuations. By contrast, the observed singularity in YbRh2$(Si$_{0.95}$Ge$_{0.05}$)$_2$ cannot be explained by the itinerant SDW theory but is qualitatively consistent with a locally quantum critical picture.

cond-mat.str-el↗
arXiv2003

Magnetic field and pressure effects on charge density wave, superconducting, and magnetic states in Lu$_5$Ir$_4$Si$_{10}$ and Er$_5$Ir$_4$Si$_{10}$

We have studied the charge-density-wave (CDW) state for the superconducting Lu$_5$Ir$_4$Si$_{10}$ and the antiferromagnetic Er$_5$Ir$_4$Si$_{10}$ as variables of temperature, magnetic field, and hydrostatic pressure. For Lu$_5$Ir$_4$Si$_{10}$, the application of pressure strongly suppresses the CDW phase but weakly enhances the superconducting phase. For Er$_5$Ir$_4$Si$_{10}$, the incommensurate CDW state is pressure independent and the commensurate CDW state strongly depends on the pressure, whereas the antiferromagnetic ordering is slightly depressed by applying pressure. In addition, Er$_5$Ir$_4$Si$_{10}$ shows negative magnetoresistance at low temperatures, compared with the positive magnetoresistance of Lu$_5$Ir$_4$Si$_{10}$.

cond-mat.str-el↗
arXiv2003

A Hierarchically-Organized Phase Diagram near a Quantum Critical Point in URu2Si2

A comprehensive transport study, as a function of both temperature and magnetic field in continuous magnetic fields up to 45 T reveals that URu2Si2 possesses all the essential hallmarks of quantum criticality at temperatures above 5.5 K and fields around 38 T, but then collapses into multiple low temperature phases in a hierarchically-organized phase diagram as the temperature is reduced. Although certain generic features of the phase diagram are very similar to those in the cuprates and heavy fermion superconductors, the existence of multiple ordered hysteretic phases near the field-tuned quantum critical point is presently unique to URu2Si2. This finding suggests the existence of many competing order parameters separated by small energy difference in URu2Si2.

cond-mat.str-el↗
arXiv2003

The Case for Phase Separation in $URu_2Si_2$

Motivated by experiment, we review the case for phase inhomogeneity in URu_2Si_2. In this scenario, the paramagnetic hidden order phase coexists with small distinct domains of antiferromagnetism whose volume fraction increases with pressure. The implications for the nature of the hidden order are discu ssed.

cond-mat.str-el↗
arXiv2003

Heavy Carriers and Non-Drude Optical Conductivity in MnSi

Optical properties of the weakly helimagnetic metal MnSi have been determined in the photon energy range from 2 meV to 4.5 eV using the combination of grazing incidence reflectance at 80 degrees (2 meV to 0.8 eV) and ellipsometry (0.8 to 4.5 eV). As the sample is cooled below 100 K the effective mass becomes strongly frequency dependent at low frequencies, while the scattering rate developes a linear frequency dependence. The complex optical conductivity can be described by the phenomenological relation σ(ω,T) \propto (Γ(T)+iω)^{-1/2} used for cuprates and ruthenates.

cond-mat.str-el↗
arXiv2003

Re-entrant hidden order at a metamagnetic quantum critical end point

Magnetization measurements of URu2Si2 in pulsed magnetic fields of 44 T reveal that the hidden order phase is destroyed before appearing in the form of a re-entrant phase between ~ 36 and 39 T. Evidence for conventional itinerant electron metamagnetism at higher temperatures suggests that the re-entrant phase is created in the vicinity of a quantum critical end point.

cond-mat.str-el↗
arXiv2002

Nonequilibrium Antiferromagnetic State in the Heavy Electron Compound URu_2Si_2

We have investigated the nature of the antiferromagnetic (AF) phase induced by uniaxial stress sigma in URu2Si2, by performing elastic neutron scattering measurements up to 0.4 GPa. We have found that the AF Bragg-peak intensity shows a clear hysteresis loop with sigma under the zero-stress cooling condition. The result strongly suggests that the sigma-induced AF phase is metastable and separated from the coexisting "hidden ordered" phase by a first-order phase transition. We also present the analyses of the crystalline strain effects, and suggest that the c/a ratio plays an important role in the competition between these two phases.

cond-mat.str-el↗
arXiv2002

non-Local Quantum Criticality in Ce(Ru_{1-x} Fe_x)_2 Ge_2 (x = x_c = 0.76)

We present the results of inelastic neutron scattering measurements, performed near the antiferromagnetic quantum critical point in Ce(Ru_{0.24} Fe_{0.76})_2 Ge_2. Both local and long range fluctuations of the local moments are observed, but due to the Kondo effect only the latter are critical. We propose a phenomenological expression which fits the energy $E$, temperature T and wave vector q dependences of the generalized susceptibility chi(q,E,T), describing the non-Fermi liquid E/T scaling found at every wave vector.

cond-mat.str-el↗
arXiv2002

Search for novel order in URu2Si2 by neutron scattering

We have made extensive reciprocal space maps in the heavy-fermion superconductor URu2Si2 using high-resolution time-of-flight single-crystal neutron diffraction to search for signs of a hidden order parameter related to the 17.5 K phase transition. Within the present sensitivity of the experiment (0.007 uB/U-ion for sharp peaks), no additional features such as incommensurate structures or short-range order have been found in the (h0l) or (hhl) scattering planes. The only additional low-temperature scattering observed was the well-known tiny antiferromagnetic moment of 0.03 uB/U-ion.

cond-mat.str-el↗
arXiv2002

Effects of Uniaxial Stress on Antiferromagnetic Moment in the Heavy Electron Compound URu_2Si_2

We have performed the elastic neutron scattering experiments under uniaxial stress σalong the tetragonal [100], [110] and [001] directions for URu2Si2. For σ// [100] and [110], the antiferromagnetic moment μ_o is strongly enhanced from 0.02 μ_B (σ=0) to 0.22 μ_B (σ=2.5 kbar) at 1.5 K. The rate of increase dμ_o/dσis roughly estimated to be ~ 0.1 μ_B/kbar, which is much larger than that for the hydrostatic pressure (~ 0.025 μ_B/kbar). Above 2.5 kbar, μ_o shows a tendency to saturate similar to the behavior in the hydrostatic pressure. For σ// [001], on the other hand, μ_o shows only a slight increase to 0.028 μ_B (σ= 4.6 kbar) with a rate of ~ 0.002 μ_B/kbar. The observed anisotropy suggests that the competition between the hidden order and the antiferromagnetic state in URu2Si2 is strongly coupled with the tetragonal four-fold symmetry and the c/a ratio, or both.

cond-mat.str-el↗
arXiv2002

Hidden Orbital Order in $URu_{2}Si_{2}$

When matter is cooled from high temperatures, collective instabilities develop amongst its constituent particles that lead to new kinds of order. An anomaly in the specific heat is a classic signature of this phenomenon. Usually the associated order is easily identified, but sometimes its nature remains elusive. The heavy fermion metal $URu_2Si_2$ is one such example, where the order responsible for the sharp specific heat anomaly at $T_0=17 K$ has remained unidentified despite more than seventeen years of effort. In $URu_{2}Si_{2}$, the coexistence of large electron-electron repulsion and antiferromagnetic fluctuations in $URu_2Si_2$ leads to an almost incompressible heavy electron fluid, where anisotropically paired quasiparticle states are energetically favored. In this paper we use these insights to develop a detailed proposal for the hidden order in $URu_2Si_2$. We show that incommensurate orbital antiferromagnetism, associated with circulating currents between the uranium ions, can account for the local fields and entropy loss observed at the $17 K$ transition; furthermore we make detailed predictions for neutron scattering measurements.

cond-mat.str-el↗
arXiv2001

Pressure-Induced Magnetism and Hidden Order in URu_2Si_2

We discuss the discovery of pressure-induced antiferromagnetism in URu_2Si_2, in the context of neutron, NMR and μSR results. The identification of a critical pressure separating mean-field and Ising phase transitions leads us to propose that the system lies close to a bicritical point associated with magnetic and (non-magnetic) hidden order. We conclude that the recent observation of an isotropic, field-independent component in the silicon NMR line-width implies that the hidden order parameter breaks time-reversal invariance and present a preliminary discussion of the underlying nature of the hidden order parameter.

cond-mat.str-el↗
arXiv2001

Thickness dependence of the ground-state properties in thin films of the heavy-fermion compound CeCu_6

High-quality thin polycrystalline films of the heavy-fermion compound CeCu_6 were prepared by sputter deposition. The thicker of these films (with thickness up to around 200 nm) reproduce the properties of the bulk compound CeCu_6. As the thickness of the films is decreased, our measurements display strong deviations from the bulk properties, namely, a suppression of the heavy-fermion state. We show that possible `external' effects, like disorder, oxidation and morphology can be excluded and that this size effect is therefore an intrinsic property of CeCu_6. In addition, we investigate possible scenarios explaining the size effect, and find that the proximity of CeCu_6 to a quantum phase transition can account for this striking result.

cond-mat.str-el↗
arXiv2001

29-Si NMR and Hidden Order in URu2Si2

We present new 29-Si NMR spectra in URu2Si2 for varying temperature T, and external field H. On lowering T, the systematics of the low-field lineshape and width reveal an extra component (lambda) to the linewidth below T_N ~ 17 K not observed previously. We find that lambda is magnetic-field independent and dominates the low-field lineshape for all orientations of H with respect to the tetragonal c axis. The behavior of lambda indicates a direct relationship between the 29-Si spin and the transition at T_N, but it is inconsistent with a coupling of the nuclei to static antiferromagnetic order/disorder of the U-spin magnetization. This leads us to conjecture that lambda is due to a coupling of 29-Si to the system's hidden-order parameter. A possible coupling mechanism involving charge degrees of freedom and indirect nuclear spin/spin interactions is proposed. We also propose further experiments to test for the existence of this coupling mechanism.

cond-mat.str-el↗
arXiv2001

Magnetic properties of hexagonal YMnO$_3$, LuMnO$_3$ and ScMnO$_3$ Magnetic susceptibility, specific heat and dielectric constant of hexagonal YMnO_3, LuMnO_3 and ScMnO_3

We report the magnetic susceptibility, specific heat and dielectric constant on high purity polycrystalline samples of three hexagonal manganites: YMnO_3, LuMnO_3 and ScMnO_3. These materials can exhibit a ferroelectric transition at very high temperatures (T_{FE} > 700K). At lower temperatures there is magnetic ordering of the frustrated Mn^{3+} spins (S=2) on a triangular Mn lattice (YMnO_3:T_N=71K; LuMnO$_3:T_N=90K and ScMnO_3:T_N=130K). The transition is characterized by a sharp kink in the magnetic susceptibility at T_N below which it continues to increase due to the frustration on the triangular lattice. The specific heat shows one clear continuous phase transition at T_N, which is independent of external magnetic field up to 9T with an entropy content as expected for Mn^{3+} ions. The temperature dependent dielectric constant displays a distinct anomaly at T_N.

cond-mat.mtrl-sci↗