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J. A. Swartz

Publications and source records attributed to J. A. Swartz.

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Low-energy collective structure of $^{92,94}$Zr and $^{94}$Mo from ($e,e^{\prime}$) and ($p,p^{\prime}$) scattering I. Experimental results

This is the first of two papers discussing a new signature of quadrupole mixed-symmetry states in the vibrational nuclei $^{92,94}$Zr and $^{94}$Mo based on proton and neutron transition densities derived from the comparison of inelastic electron and proton scattering experiments. Results of the $(e,e^\prime)$ and $(p,p^\prime)$ experiments on these nuclei as well as $(p,p^\prime)$ data for other potential cases $^{96}$Mo and $^{70}$Zn are presented. Spin and parity quantum numbers of excited states are assigned based on angular distributions from the proton scattering data in comparison to calculations employing form factors from the collective model in distorted-wave Born approximation. Possible candidates of one-phonon fully symmetric and mixed-symmetry states as well as members of two-phonon multiplets are identified.

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First Proton-Induced Cross Sections on a Stored Rare Ion Beam: Measurement of 118Te(p,γ) for Explosive Nucleosynthesis

We present the first nuclear cross-section measurements of (p,γ) and (p,n) reactions on 118Te at energies relevant for the γ-process nucleosynthesis. Absolute cross-section values for center-of-mass energies of 6, 7 and 10 MeV are provided, together with a theoretical extrapolation to the Gamow window. This experiment marks the first time that direct proton-induced reactions have been measured on a radioactive ion beam at the Experimental Storage Ring (ESR) at GSI, Darmstadt. This paves the way for a large variety of measurements, delivering new constraints for explosive nucleosynthesis and for physics beyond nuclear stability.

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First simultaneous measurement of the gamma-ray and neutron emission probabilities in inverse kinematics at a heavy-ion storage ring

The probabilities for gamma-ray and particle emission as a function of the excitation energy of a decaying nucleus are valuable observables for constraining the ingredients of the models that describe the de-excitation of nuclei near the particle emission threshold. These models are essential in nuclear astrophysics and applications. In this work, we have for the first time simultaneously measured the gamma-ray and neutron emission probabilities of 208Pb. The measurement was performed in inverse kinematics at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, where a 208Pb beam interacted through the 208Pb(p,p') reaction with a hydrogen gas jet target. Instead of detecting the gamma-rays and neutrons emitted by 208Pb, we detected the heavy beam-like residues produced after gamma and neutron emission. These heavy residues were fully separated by a dipole magnet of the ESR and were detected with outstanding efficiencies. The comparison of the measured probabilities with model calculations has allowed us to test and select different descriptions of the gamma-ray strength function and the nuclear level density available in the literature.

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First measurement of the neutron-emission probability with a surrogate reaction in inverse kinematics at a heavy-ion storage ring

Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the 208Pb(p,p') reaction as a surrogate for neutron capture on 207Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of 208Pb. We have used this probability to select different descriptions of the gamma-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of 207Pb at energies for which no experimental data exist.

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Measurement of the Isolated Nuclear Two-Photon Decay in $^{72}\mathrm{Ge}$

The nuclear two-photon or double-gamma ($2γ$) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the $2γ$ decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to $\sim100$\,keV and half-lives as short as $\sim10$\,ms. The half-life for the $2γ$ decay of the first-excited $0^+$ state in bare $^{72}\mathrm{Ge}$ ions was determined to be $23.9\left(6\right)$\,ms, which strongly deviates from expectations.

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Storage, Accumulation and Deceleration of Secondary Beams for Nuclear Astrophysics

Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.

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Damping of the isovector giant dipole resonance in $^{40,48}$Ca

The fine structure of the IsoVector Giant Dipole Resonance (IVGDR) in the doubly-magic nuclei $^{40,48}$Ca observed in inelastic proton scattering experiments under $0^\circ$ is used to investigate the role of different mechanisms contributing to the IVGDR decay width. Characteristic energy scales are extracted from the fine structure by means of wavelet analysis. The experimental scales are compared to different theoretical approaches allowing for the inclusion of complex configurations beyond the mean-field level. Calculations are performed in the framework of RPA and beyond-RPA in a relativistic approach based on an effective meson-exchange interaction, with the UCOM effective interaction and, for the first time, with realistic two- plus three-nucleon interactions from chiral effective field theory employing the in-medium similarity renormalization group. All models highlight the role of Landau fragmentation for the damping of the IVGDR, while the differences in the coupling strength between one particle-one hole (1p-1h) and two particle-two hole (2p-2h) correlated (relativistic) and non-correlated (non-relativistic) configurations lead to very different pictures of the importance of the spreading width resulting in wavelet scales being a sensitive measure of their interplay. The relativistic approach with particle-vibration coupling, in particular, shows impressive agreement with the number and absolute values of the scales extracted from the experimental data.

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Multi-probe study of excited states in $\mathrm{^{12}C}$: disentangling the sources of monopole strength between the Hoyle state and $E_{x} = 13$ MeV

Knowledge of the low-lying monopole strength in $\mathrm{^{12}C}$, the Hoyle state in particular, is crucial for our understanding of both the astrophysically important $3α$ reaction and of $α$-particle clustering. The $\mathrm{^{12}C}(α, α^{\prime})\mathrm{^{12}C}$ and $\mathrm{^{14}C}(p, t)\mathrm{^{12}C}$ reactions were employed to populate states in $^{12}$C. A self-consistent, simultaneous analysis of the inclusive spectra with lineshapes was performed, which accounted for distortion due to nuclear dynamics and experimental effects. Clear evidence was found for excess monopole strength at $E_{x} \sim 9$ MeV, particularly in the $\mathrm{^{12}C}(α, α^{\prime})\mathrm{^{12}C}$ reaction at $0^{\circ}$. This additional strength cannot be reproduced by the previously established monopole states between $E_{x} = 7$ and 13 MeV. An additional $0^{+}$ state at $E_{x} \sim 9$ MeV yielded a significantly improved fit of the data and is the leading candidate for the predicted breathing-mode excitation of the Hoyle state. Alternatively, the results may suggest that a more sophisticated, physically motivated parameterization of the astrophysically important monopole strengths in $\mathrm{^{12}C}$ is required.

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Investigating the predicted breathing-mode excitation of the Hoyle state

Knowledge of the low-lying monopole strength in $\mathrm{^{12}C}$ $-$ the Hoyle state in particular $-$ is crucial for our understanding of both the astrophysically important $3α$ reaction and of $α$-particle clustering. Multiple theoretical models have predicted a breathing mode of the Hoyle State at $E_{x} \approx 9$ MeV, corresponding to a radial in-phase oscillation of the underlying $α$ clusters. The $\mathrm{^{12}C}(α, α^{\prime})\mathrm{^{12}C}$ and $\mathrm{^{14}C}(p, t)\mathrm{^{12}C}$ reactions were employed to populate states in $^{12}$C in order to search for this predicted breathing mode. A self-consistent, simultaneous analysis of the inclusive spectra with R-matrix lineshapes, together with angular distributions of charged-particle decay, yielded clear evidence for excess monopole strength at $E_{x} \approx 9$ MeV which is highly collective. Reproduction of the experimentally observed inclusive yields using a fit, with consistent population ratios for the various broad states, required an additional source of monopole strength. The interpretation of this additional monopole resonance as the breathing-mode excitation of the Hoyle state would provide evidence supporting a $\mathcal{D}_{3h}$ symmetry for the Hoyle state itself. The excess monopole strength may complicate analysis of the properties of the Hoyle state, modifying the temperature dependence of the $3α$ rate at $T_{9} \gtrsim 2$ and ultimately, the predicted nucleosynthesis in explosive stars.

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Fine Structure of the Isovector Giant Dipole Resonance in $^{142-150}$Nd and $^{152}$Sm

Background: Inelastic proton scattering at energies of a few hundred MeV and very-forward angles including $0^\circ$ has been established as a tool to study electric-dipole strength distributions in nuclei. The present work reports a systematic investigation of the chain of stable even-mass Nd isotopes representing a transition from spherical to quadrupole-deformed nuclei. Purpose: Extraction of the equivalent photo-absorption cross sections and analysis of their fine structure in the energy region of the IsoVector Giant Dipole Resonance (IVGDR). Method: Proton inelastic scattering reactions of 200 MeV protons were measured at iThemba LABS in Cape Town, South Africa. The scattering products were momentum-analysed by the K600 magnetic spectrometer positioned at $θ_{\mathrm{Lab}}=0^\circ$. Using dispersion-matching techniques, energy resolutions of $ΔE \approx 40 - 50$ keV were obtained. After subtraction of background and contributions from other multipoles, the spectra were converted to photo-absorption cross sections using the equivalent virtual-photon method. Results: Wavelet-analysis techniques are used to extract characteristic energy scales of the fine structure of the IVGDR from the experimental data. Comparisons with the Quasiparticle-Phonon Model (QPM) and Skyrme Separable Random Phase Approximation (SSRPA) predictions provide insight into the role of different giant resonance damping mechanisms. Conclusions: Fine structure is observed even for the most deformed nuclei studied. Fragmentation of the one particle-one hole ($1p1h$) strength seems to be the main source of fine structure in both spherical and deformed nuclei. Some impact of the spreading due to coupling of the two particle-two hole ($2p2h$) states to the $1p1h$ doorway states is seen in the spherical/transitional nuclei, where calculations beyond the $1p1h$ level are available.

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Measurement of the $2^+\rightarrow 0^+$ ground-state transition in the $β$ decay of $^{20}$F

We report the first detection of the second-forbidden, non-unique, $2^+\rightarrow 0^+$, ground-state transition in the $β$ decay of $^{20}$F. A low-energy, mass-separated $^{20}\rm{F}^+$ beam produced at the IGISOL facility in Jyväskylä, Finland, was implanted in a thin carbon foil and the $β$ spectrum measured using a magnetic transporter and a plastic-scintillator detector. The $β$-decay branching ratio inferred from the measurement is $b_β = [ 0.41\pm 0.08\textrm{(stat)}\pm 0.07\textrm{(sys)}] \times 10^{-5}$ corresponding to $\log ft = 10.89(11)$, making this one of the strongest second-forbidden, non-unique $β$ transitions ever measured. The experimental result is supported by shell-model calculations and has significant implications for the final evolution of stars that develop degenerate oxygen-neon cores. Using the new experimental data, we argue that the astrophysical electron-capture rate on $^{20}$Ne is now known to within better than 25% at the relevant temperatures and densities.

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Studies of the Giant Dipole Resonance in $^{27}$Al, $^{40}$Ca, $^{56}$Fe, $^{58}$Ni and $^{208}$Pb with high energy-resolution inelastic proton scattering under 0$^\circ$

A survey of the fine structure of the Isovector Giant Dipole Resonance (IVGDR) was performed, using the recently commissioned zero-degree facility of the K600 magnetic spectrometer at iThemba LABS. Inelastic proton scattering at an incident energy of 200 MeV was measured on $^{27}$Al, $^{40}$Ca, $^{56}$Fe, $^{58}$Ni and $^{208}$Pb. A high energy resolution ($\rmΔ\it{E} \simeq$ 40 keV FWHM) could be achieved after utilising faint-beam and dispersion-matching techniques. Considerable fine structure is observed in the energy region of the IVGDR and characteristic energy scales are extracted from the experimental data by means of a wavelet analysis. The comparison with Quasiparticle-Phonon Model (QPM) calculations provides insight into the relevance of different giant resonance decay mechanisms. Photoabsorption cross sections derived from the data assuming dominance of relativistic Coulomb excitation are in fair agreement with previous work using real photons.

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Investigating 16O with the 15N(p,α)12C reaction

The 16O nucleus was investigated through the 15N(p,α)12C reaction at excitation energies from Ex = 12 231 to 15 700 keV using proton beams from a 5 MeV Van de Graaff accelerator at beam energies of Ep = 331 to 3800 keV. Alpha decay from resonant states in 16O was strongly observed for ten known excited states in this region. The candidate 4-alpha cluster state at Ex = 15.1 MeV was investigated particularly intensely in order to understand its particle decay channels.

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First Accurate Normalization of the $β$-delayed $α$ Decay of $^{16}$N and Implications for the $^{12}$C$(α,γ)^{16}$O Astrophysical Reaction Rate

The $^{12}\text{C}(α,γ){}^{16}\text{O}$ reaction plays a central role in astrophysics, but its cross section at energies relevant for astrophysical applications is only poorly constrained by laboratory data. The reduced $α$ width, $γ_{11}$, of the bound $1^-$ level in $^{16}$O is particularly important to determine the cross section. The magnitude of $γ_{11}$ is determined via sub-Coulomb $α$-transfer reactions or the $β$-delayed $α$ decay of $^{16}$N, but the latter approach is presently hampered by the lack of sufficiently precise data on the $β$-decay branching ratios. Here we report improved branching ratios for the bound $1^-$ level [$b_{β,11} = (5.02\pm 0.10)\times 10^{-2}$] and for $β$-delayed $α$ emission [$b_{βα} = (1.59\pm 0.06)\times 10^{-5}$]. Our value for $b_{βα}$ is 33% larger than previously held, leading to a substantial increase in $γ_{11}$. Our revised value for $γ_{11}$ is in good agreement with the value obtained in $α$-transfer studies and the weighted average of the two gives a robust and precise determination of $γ_{11}$, which provides significantly improved constraints on the $^{12}$C$(α,γ)$ cross section in the energy range relevant to hydrostatic He burning.

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Wavelet signatures of $K$-splitting of the Isoscalar Giant Quadrupole Resonance in deformed nuclei from high-resolution (p,p$'$) scattering off $^{146,148,150}$Nd

The phenomenon of fine structure of the Isoscalar Giant Quadrupole Resonance (ISGQR) has been studied with high energy-resolution proton inelastic scattering at iThemba LABS in the chain of stable even-mass Nd isotopes covering the transition from spherical to deformed ground states. A wavelet analysis of the background-subtracted spectra in the deformed 146,148,150Nd isotopes reveals characteristic scales in correspondence with scales obtained from a Skyrme RPA calculation using the SVmas10 parameterization. A semblance analysis shows that these scales arise from the energy shift between the main fragments of the K = 0, 1 and K = 2 components.

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Deformation dependence of the isovector giant dipole resonance: The neodymium isotopic chain revisited

Proton inelastic scattering experiments at energy E_p = 200 MeV and a spectrometer scattering angle of 0 degree were performed on 144,146,148,150Nd and 152Sm exciting the IsoVector Giant Dipole Resonance (IVGDR). Comparison with results from photo-absorption experiments reveals a shift of resonance maxima towards higher energies for vibrational and transitional nuclei. The extracted photo-absorption cross sections in the most deformed nuclei, 150Nd and 152Sm, exhibit a pronounced asymmetry rather than a distinct double-hump structure expected as a signature of K-splitting. This behaviour can be related to the proximity of these nuclei to the critical point of the phase shape transition from vibrators to rotors with a soft quadrupole deformation potential. Self-consistent random-phase approximation (RPA) calculations using the SLy6 Skyrme force provide a relevant description of the IVGDR shapes deduced from the present data

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Characterization of the proposed 4-α cluster state candidate in 16O

The $\mathrm{^{16}O}(α, α^{\prime})$ reaction was studied at $θ_{lab} = 0^\circ$ at an incident energy of $\textrm{E}_{lab}$ = 200 MeV using the K600 magnetic spectrometer at iThemba LABS. Proton and $α$-decay from the natural parity states were observed in a large-acceptance silicon-strip detector array at backward angles. The coincident charged particle measurements were used to characterize the decay channels of the $0_{6}^{+}$ state in $\mathrm{^{16}O}$ located at $E_{x} = 15.097(5)$ MeV. This state is identified by several theoretical cluster calculations to be a good candidate for the 4-$α$ cluster state. The results of this work suggest the presence of a previously unidentified resonance at $E_{x}\approx15$ MeV that does not exhibit a $0^{+}$ character. This unresolved resonance may have contaminated previous observations of the $0_{6}^{+}$ state.

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No evidence of an 11.16 MeV 2+ state in 12C

An experiment using the 11B(3He,d)12C reaction was performed at iThemba LABS at an incident energy of 44 MeV and analyzed with a high energy-resolution magnetic spectrometer, to re-investigate states in 12C published in 1971. The original investigation reported the existence of an 11.16 MeV state in 12C that displays a 2+ nature. In the present experiment data were acquired at laboratory angles of 25-, 30- and 35- degrees, to be as close to the c.m. angles of the original measurements where the clearest signature of such a state was observed. These new low background measurements revealed no evidence of the previously reported state at 11.16 MeV in 12C.

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