arXiv subjects

J. Arlt

Publications and source records attributed to J. Arlt.

At least 19 recordsLinked to original sources

arXiv2026

Hierarchical Interdiffusion Kinetics in Nanoscale Ni/Al Multilayers

Reactive metallic multilayers store chemical energy that can be released rapidly through interdiffusion and intermetallic formation. Predictive control of this heat release requires distinguishing transport and phase-formation processes that occur in rapid succession. Here we combine free-standing nanoscale Ni/Al multilayers with chip-based flash calorimetry and isoconversional kinetic analysis over five orders of magnitude in heating rate. Selected reaction states are quenched and examined by scanning transmission electron microscopy. This workflow separates pre-ignition interdiffusion into two regimes and quantifies activation energies of (81 $\pm$ 24) and (168 $\pm$ 17) kJ/mol, consistent with grain-boundary and lattice diffusion of Ni in Al, respectively. Microscopy supports this assignment: no significant compositional changes are observed after the first regime, whereas the second increases the Ni content of the Al layers and produces Ni-enriched features spaced by 5$-$10 nm, matching the Al grain size. These results identify the Al grain-boundary network as the dominant low-barrier pathway, providing rapid transport across the Al layers and priming lattice-mediated mixing and intermetallic phase formation. More broadly, the workflow links calorimetric signatures to pathway-specific kinetics and transient microstructures, enabling direct assessment of how microstructural design redirects coupled transport and reaction pathways in reactive multilayers and other materials driven far from equilibrium.

cond-mat.mtrl-sci↗

arXiv2026

Spontaneous phase separation and pattern formation in a lyotropic nematic mixture

Lyotropic liquid crystals can display rich phase behaviour and self-organisation, yet the physical principles underlying their self-assembly into large scale patterns remains understudied. Here, we combine theory, simulations and experiments on Sunset Yellow-water chromonic mixtures to show that such materials spontaneously phase separate, even without assuming any underlying microscopic attraction between the molecular species. In our minimal model, demixing depends solely on the Onsager-like coupling between local nematogen density and orientational order. If such a coupling is sufficiently strong, nematic defects trigger the nucleation of isotropic droplets, which then coalesce due to elastic or interfacial tensions. We further show that strong anchoring of the director field at the interface arrests this coarsening process, resulting in a stable microphase separated lamellar pattern. This self-assembled smectic phase has striking and unusual features, including spontaneous undulations, heterogeneous layer spacing, long-lived glassy defect patterns and lamellar onions. Our results identify orientational-density coupling and elastocapillarity as fundamental mechanisms to guide self-assembly in lyotropic and chromonic liquid crystals.

cond-mat.soft↗

arXiv2025

Advancing Atom Probe Tomography of SrTiO$_3$: Measurement Methodology and Impurity Detection Limits

Strontium titanate (STO) possesses promising properties for applications in thermoelectricity, catalysis, fuel cells, and more, but its performance is highly dependent on stoichiometry and impurity levels. While atom probe tomography (APT) can provide detailed three-dimensional atomic-scale chemical information, STO specimens have been challenging to analyze due to premature specimen fracture. In this study, we show that by applying a thin metal coating to atom probe tips, STO specimens can be analyzed with nearly 100% success. Using this approach, we investigate both undoped STO and 1 at% Nb-doped STO, achieving sufficient sensitivity to detect Nb concentrations as low as 0.7 at%. This work establishes a reliable APT method for high-resolution chemical analysis of STO at the nanoscale.

cond-mat.mtrl-sci↗

arXiv2023

Fock State Sampling Method -- Characteristic temperature of maximal fluctuations for interacting bosons in box potentials

We study the statistical properties of a gas of interacting bosons trapped in a box potential in two and three dimensions. Our primary focus is the characteristic temperature $\tchar$, i.e. the temperature at which the fluctuations of the number of condensed atoms (or, in 2D, the number of motionless atoms) is maximal. Using the Fock State Sampling method, we show that $\tchar$ increases due to interaction. In 3D, this temperature converges to the critical temperature in the thermodynamic limit. In 2D we show the general applicability of the method by obtaining a generalized dependence of the characteristic temperature on the interaction strength. Finally, we discuss the experimental conditions necessary for the verification of our theoretical predictions.

quant-ph↗

arXiv2019

Preparation of mesoscopic atomic ensembles with single-particle resolution

The analysis of entangled atomic ensembles and their application for interferometry beyond the standard quantum limit requires an accurate determination of the number of atoms. We present an accurate fluorescence detection technique for atoms that is fully integrated into an experimental apparatus for the production of many-particle entangled quantum states. Single-particle resolving fluorescence measurements for $1$ up to $30$ atoms are presented. According to our noise analysis, we extrapolate that the single-atom resolution extends to a limiting atom number of $390(20)$ atoms. We utilize the accurate atom number detection for a number stabilization of the laser-cooled atomic ensemble. For a target ensemble size of $7$ atoms prepared on demand, we achieve a $92(2)\,\%$ preparation fidelity and reach number fluctuations $18(1)\,\mathrm{dB}$ below the shot noise level using real-time feedback on the magneto-optical trap.

quant-ph↗

arXiv2016

0.75 atoms improve the clock signal of 10,000 atoms

Since the pioneering work of Ramsey, atom interferometers are employed for precision metrology, in particular to measure time and to realize the second. In a classical interferometer, an ensemble of atoms is prepared in one of the two input states, whereas the second one is left empty. In this case, the vacuum noise restricts the precision of the interferometer to the standard quantum limit (SQL). Here, we propose and experimentally demonstrate a novel clock configuration that surpasses the SQL by squeezing the vacuum in the empty input state. We create a squeezed vacuum state containing an average of 0.75 atoms to improve the clock sensitivity of 10,000 atoms by 2.05 dB. The SQL poses a significant limitation for today's microwave fountain clocks, which serve as the main time reference. We evaluate the major technical limitations and challenges for devising a next generation of fountain clocks based on atomic squeezed vacuum.

quant-ph↗

arXiv2015

Satisfying the Einstein-Podolsky-Rosen criterion with massive particles

In 1935, Einstein, Podolsky and Rosen (EPR) questioned the completeness of quantum mechanics by devising a quantum state of two massive particles with maximally correlated space and momentum coordinates. The EPR criterion qualifies such continuous-variable entangled states, where a measurement of one subsystem seemingly allows for a prediction of the second subsystem beyond the Heisenberg uncertainty relation. Up to now, continuous-variable EPR correlations have only been created with photons, while the demonstration of such strongly correlated states with massive particles is still outstanding. Here, we report on the creation of an EPR-correlated two-mode squeezed state in an ultracold atomic ensemble. The state shows an EPR entanglement parameter of 0.18(3), which is 2.4 standard deviations below the threshold 1/4 of the EPR criterion. We also present a full tomographic reconstruction of the underlying many-particle quantum state. The state presents a resource for tests of quantum nonlocality and a wide variety of applications in the field of continuous-variable quantum information and metrology.

quant-ph↗

arXiv2015

Interaction-free measurements by quantum Zeno stabilisation of ultracold atoms

Quantum mechanics predicts that our physical reality is influenced by events that can potentially happen but factually do not occur. Interaction-free measurements (IFMs) exploit this counterintuitive influence to detect the presence of an object without requiring any interaction with it. Here we propose and realize an IFM concept based on an unstable many-particle system. In our experiments, we employ an ultracold gas in an unstable spin configuration which can undergo a rapid decay. The object - realized by a laser beam - prevents this decay due to the indirect quantum Zeno effect and thus, its presence can be detected without interacting with a single atom. Contrary to existing proposals, our IFM does not require single-particle sources and is only weakly affected by losses and decoherence. We demonstrate confidence levels of 90%, well beyond previous optical experiments.

quant-ph↗

arXiv2015

A continuously pumped reservoir of ultracold atoms

Typical sources of ultracold atoms operate with a considerable delay between the delivery of ensembles due to sequential trapping and cooling schemes. Therefore, alternative schemes for the continuous generation of ultracold atoms are highly desirable. Here, we demonstrate the continuous loading of a magnetic trap from a quasi-continuous atom beam. We achieve a steady state with $3.8 \times 10^7$ magnetically trapped atoms and a temperature of $102 μ$K. The ensemble is protected from laser light sources, a requirement for its application for metrological tasks or sympathetic cooling. The continuous scheme is robust and applicable to a wide range of particles and trapping potentials.

quant-ph↗

arXiv2014

Filling an emulsion drop with motile bacteria

We have measured the spatial distribution of motile Escherichia coli inside spherical water droplets emulsified in oil. At low cell concentrations, the cell density peaks at the water-oil interface; at increasing concentration, the bulk of each droplet fills up uniformly while the surface peak remains. Simulations and theory show that the bulk density results from a `traffic' of cells leaving the surface layer, increasingly due to cell-cell scattering as the surface coverage rises above $\sim 10\%$. Our findings show similarities with the physics of a rarefied gas in a spherical cavity with attractive walls.

cond-mat.soft↗

arXiv2013

Evolutionary optimization of an experimental apparatus

In recent decades, cold atom experiments have become increasingly complex. While computers control most parameters, optimization is mostly done manually. This is a time-consuming task for a high-dimensional parameter space with unknown correlations. Here we automate this process using a genetic algorithm based on Differential Evolution. We demonstrate that this algorithm optimizes 21 correlated parameters and that it is robust against local maxima and experimental noise. The algorithm is flexible and easy to implement. Thus, the presented scheme can be applied to a wide range of experimental optimization tasks.

quant-ph↗

arXiv2011

Extended coherence time on the clock transition of optically trapped Rubidium

Optically trapped ensembles are of crucial importance for frequency measurements and quantum memories, but generally suffer from strong dephasing due to inhomogeneous density and light shifts. We demonstrate a drastic increase of the coherence time to 21 s on the magnetic field insensitive clock transition of Rb-87 by applying the recently discovered spin self-rephasing. This result confirms the general nature of this new mechanism and thus shows its applicability in atom clocks and quantum memories. A systematic investigation of all relevant frequency shifts and noise contributions yields a stability of 2.4E-11 x tau^(-1/2), where tau is the integration time in seconds. Based on a set of technical improvements, the presented frequency standard is predicted to rival the stability of microwave fountain clocks in a potentially much more compact setup.

quant-ph↗

arXiv2010

A slow gravity compensated Atom Laser

We report on a slow guided atom laser beam outcoupled from a Bose-Einstein condensate of 87Rb atoms in a hybrid trap. The acceleration of the atom laser beam can be controlled by compensating the gravitational acceleration and we reach residual accelerations as low as 0.0027 g. The outcoupling mechanism allows for the production of a constant flux of 4.5x10^6 atoms per second and due to transverse guiding we obtain an upper limit for the mean beam width of 4.6 μ\m. The transverse velocity spread is only 0.2 mm/s and thus an upper limit for the beam quality parameter is M^2=2.5. We demonstrate the potential of the long interrogation times available with this atom laser beam by measuring the trap frequency in a single measurement. The small beam width together with the long evolution and interrogation time makes this atom laser beam a promising tool for continuous interferometric measurements.

cond-mat.quant-gas↗

arXiv2010

Parametric amplification of matter waves in dipolar spinor Bose-Einstein condensates

Spin-changing collisions may lead under proper conditions to the parametric amplification of matter waves in spinor Bose-Einstein condensates. Magnetic dipole-dipole interactions, although typically very weak in alkaline atoms, are shown to play a very relevant role in the amplification process. We show that these interactions may lead to a strong dependence of the amplification dynamics on the angle between the trap axis and the magnetic-field orientation. We analyze as well the important role played by magnetic-field gradients, which modify also strongly the amplification process. Magnetic-field gradients must be hence carefully controlled in future experiments, in order to observe clearly the effects of the dipolar interactions in the amplification dynamics.

cond-mat.quant-gas↗

arXiv2009

Multi-resonant spinor dynamics in a Bose-Einstein condensate

We analyze the spinor dynamics of a Rb-87 F=2 condensate initially prepared in the m_F=0 Zeeman sublevel. We show that this dynamics, characterized by the creation of correlated atomic pairs in m_F=+/-1, presents an intriguing multi-resonant magnetic field dependence induced by the trap inhomogeneity. This dependence is directly linked to the most unstable Bogoliubov spin excitations of the initial m_F = 0 condensate, showing that, in general, even a qualitative understanding of the pair creation efficiency in a spinor condensate requires a careful consideration of the confinement.

quant-ph↗

arXiv2008

Radio frequency association of heteronuclear Feshbach molecules

We present a detailed analysis of the production efficiency of weakly bound heteronuclear KRb-Feshbach molecules using radio frequency association in a harmonic trap. The efficiency was measured in a wide range of temperatures, binding energies and radio frequencies. A comprehensive analytical model is presented, explaining the observed asymmetric spectra and achieving good quantitative agreement with the measured production rates. This model provides a deep understanding of the molecule association process and paves the way for future experiments which rely on Feshbach molecules e.g. for the production of deeply bound molecules.

quant-ph↗

arXiv2008

Transport of a quantum degenerate heteronuclear Bose-Fermi mixture in a harmonic trap

We report on the transport of mixed quantum degenerate gases of bosonic 87Rb and fermionic 40K in a harmonic potential provided by a modified QUIC trap. The samples are transported over a distance of 6 mm to the geometric center of the anti-Helmholtz coils of the QUIC trap. This transport mechanism was implemented by a small modification of the QUIC trap and is free of losses and heating. It allows all experiments using QUIC traps to use the highly homogeneous magnetic fields that can be created in the center of a QUIC trap and improves the optical access to the atoms, e.g., for experiments with optical lattices. This mechanism may be cascaded to cover even larger distances for applications with quantum degenerate samples.

cond-mat.other↗

arXiv2007

Dynamics of Bloch Oscillations in Disordered Lattice Potentials

We present a detailed analysis of the dynamics of Bloch oscillations of Bose-Einstein condensates in disordered lattice potentials. Due to the disorder and the interparticle interactions these oscillations undergo a dephasing, reflected in a damping of the center of mass oscillations, which should be observable under realistic experimental conditions. The interplay between interactions and disorder is far from trivial, ranging from an interaction-enhanced damping due to modulational instability for strong interactions, to an interaction-reduced damping due to a dynamical screening of the disorder potential.

cond-mat.other↗