arXiv subjects

J. Billowes

Publications and source records attributed to J. Billowes.

At least 19 recordsLinked to original sources

arXiv2026

Energy-differential measurement of the $^{\mathrm{nat}}$C(n,p) and $^{\mathrm{nat}}$C(n,d) reactions at the n_TOF facility at CERN

Energy-differential cross section of the $^{\mathrm{nat}}$C(n,p) and $^{\mathrm{nat}}$C(n,d) reactions was measured at the neutron time of flight facility n_TOF at CERN. The measurement was performed in the first experimental area (EAR1; flight path of 182.5 m). Two position-sensitive $\Delta E$-$E$ silicon telescopes were used. Two naturally occurring carbon isotopes, $^{12}$C and $^{13}$C, contribute to the reactions on natural carbon, with the (n,p) reaction threshold at 13.7 MeV and the (n,d) threshold at 14.9 MeV (determined by the $^{12}$C isotope for both reactions). This paper provides the details of the analysis leading to the final results published previously as a Letter. The cross section results are reported up to 25 MeV. During the data analysis the population of the excited states in the daughter nuclei $^{11}$B, $^{12}$B, $^{13}$B had to be considered, requiring the adoption of the branching ratios and angular distributions of the emitted particles from an external source of information. TALYS-2.0 calculations were used as the main source and an in-depth analysis of the model-related uncertainties was performed. The n_TOF results are largely inconsistent with the major evaluation libraries. On the other hand, an unexpected agreement is found with TALYS-2.0 calculations. Specifically, the obtained cross section for the (n,p) reaction is significantly higher than in the available evaluations, fully supporting the earlier finding from an integral measurement at n_TOF.

nucl-ex↗

arXiv2025

Measurement of the $^\text{nat}$C(n,p) and $^\text{nat}$C(n,d) reactions from n_TOF at CERN

The energy dependence of the cross section of the (n,p) and (n,d) reactions on $^\text{nat}$C has been studied for the first time at the n_TOF facility at CERN, from the particle detection threshold up to 25 MeV. The measurement was performed with two telescopes made of position-sensitive silicon $\Delta E$-$E$ detectors, covering the angular range from 20{\deg} to 140{\deg}. A detector efficiency has been determined by means of Monte Carlo simulations of the experimental setup. Various assumptions on the angular distributions and branching ratios of the excited levels of the residual $^{11}$B, $^{12}$B, $^{13}$B nuclei were considered. In particular, theoretical calculations based on the TALYS-2.0 code were used and the systematic uncertainties in the analysis results were determined from the variations in these distributions. The n_TOF data on the (n,p) and (n,d) reaction on carbon are characterized by a higher accuracy and wider energy range than currently available in literature. A comparison with current evaluations from different libraries reveals a rather significant disagreement with the n_TOF results, while a remarkable agreement is observed with the prediction of TALYS-2.0 for this light element.

nucl-ex↗

arXiv2025

Reduction in nuclear size and quadrupole deformation of high-spin isomers of 127,129In

We employed laser spectroscopy of atomic transitions to measure the nuclear charge radii and electromagnetic properties of the high-spin isomeric states in neutron-rich indium isotopes (Z = 49) near the closed proton and neutron shells at Z = 50 and N = 82. Our data reveal a reduction in the nuclear charge radius and intrinsic quadrupole moment when protons and neutrons are fully aligned in 129In(N = 80), to form the high spin isomer. Such a reduction is not observed in 127In(N = 78), where more complex configurations can be formed by the existence of four neutron-holes. These observations are not consistently described by nuclear theory.

nucl-ex↗

arXiv2025

Charge radii of neutron-rich scandium isotopes and the seniority symmetry in the $0f_{7/2}$ shell

Nuclear charge radii of neutron-rich $^{47-49}$Sc isotopes were measured using collinear laser spectroscopy at CERN-ISOLDE. The new data reveal that the charge radii of scandium isotopes exhibit a distinct trend between $N=20$ and $N=28$, with $^{41}$Sc and $^{49}$Sc isotopes having similar values, mirroring the closeness of the charge radii of $^{40}$Ca and $^{48}$Ca. Theoretical models that successfully interpret the radii of calcium isotopes could not account for the observed behavior in scandium radii, in particular the reduced odd-even staggering. Remarkably, the inclusion of the new $^{49}$Sc radius data has unveiled a similar trend in the charge radii of $N=28$ isotones and $Z=20$ isotopes when adding the neutrons atop the $^{40}$Ca core and the protons atop the $^{48}$Ca core, respectively. We demonstrate that this trend is consistent with the prediction of the seniority model.

nucl-ex↗

arXiv2024

Radiative neutron capture cross section of $^{242}$Pu measured at n_TOF-EAR1 in the unresolved resonance region up to 600 keV

Accurate neutron capture cross sections are essential for the design and operation of fast reactors using MOX fuels. For $^{242}$Pu, the Nuclear Energy Agency (NEA) recommends 8--12% accuracy in the fast energy region (2--500 keV), compared to the current uncertainty of 35%. Moreover, integral experiments and previous measurements suggest the evaluated $^{242}$Pu(n,$\gamma$) cross section is overestimated, particularly in the JEFF-3.3 library, which shows a 14% overestimation between 1 keV and 1 MeV. Recent measurements from LANSCE reported a 20--30% reduction in the 1--40 keV range relative to evaluations. To solve these discrepancies, the $^{242}$Pu(n,$\gamma$) cross section was measured from 1 to 600 keV at CERN n_TOF-EAR1 facility using a 95(4) mg $^{242}$Pu target, enriched to 99.959%. Gamma rays from neutron capture were detected with an array of C$_6$D$_6$ scintillators and a novel application of the Pulse Height Weighting Technique was employed. The resulting cross section presents a systematic uncertainty between 8 and 12%, reducing the current uncertainties of 35\% and achieving the accuracy requested by the NEA. Analysis using FITACS produced average resonance parameters, consistent with the analysis of the resolved resonance region. Our data align well with Wisshak and Kaeppeler, and are 10--14\% lower than JEFF-3.3 in the 1--250 keV range, helping to achieve consistency with integral benchmarks. At higher energies, our results are in reasonable agreement with ENDF/B-VIII.1 and JEFF-3.3. In contrast, DANCE results appear to underestimate the cross section by a factor of 2--3 above a few keV.

nucl-ex↗

arXiv2024

Measurement and analysis of the $^{246}$Cm and $^{248}$Cm neutron capture cross-sections at the EAR2 of the n TOF facility

The $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) cross-sections have been measured at the Experimental Area 2 (EAR2) of the n_TOF facility at CERN with three C$_6$D$_6$ detectors. This measurement is part of a collective effort to improve the capture cross-section data for Minor Actinides (MAs), which are required to estimate the production and transmutation rates of these isotopes in light water reactors and innovative reactor systems. In particular, the neutron capture in $^{246}$Cm and $^{248}$Cm open the path for the formation of other Cm isotopes and heavier elements such as Bk and Cf and the knowledge of (n,$\gamma$) cross-sections of these Cm isotopes plays an important role in the transport, transmutation and storage of the spent nuclear fuel. The reactions $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) have been the two first capture measurements analyzed at n_TOF EAR2. Until this experiment and two recent measurements performed at J-PARC, there was only one set of data of the capture cross-sections of $^{246}$Cm and $^{248}$Cm, that was obtained in 1969 in an underground nuclear explosion experiment. In the measurement at n_TOF a total of 13 resonances of $^{246}$Cm between 4 and 400 eV and 5 of $^{248}$Cm between 7 and 100 eV have been identified and fitted. The radiative kernels obtained for $^{246}$Cm are compatible with JENDL-5, but some of them are not with JENDL-4, which has been adopted by JEFF-3.3 and ENDF/B-VIII.0. The radiative kernels obtained for the first three $^{248}$Cm resonances are compatible with JENDL-5, however, the other two are not compatible with any other evaluation and are 20% and 60% larger than JENDL-5.

nucl-ex↗

arXiv2024

Electromagnetic moments of the odd-mass nickel isotopes $^{59-67}$Ni

The magnetic dipole and the spectroscopic quadrupole moments of the nuclear ground states in the odd-mass nickel isotopes $^{59-67}$Ni have been determined using collinear laser spectroscopy at the CERN-ISOLDE facility. They are compared to ab initio valence-space in-medium similarity renormalization group (VS-IMSRG) calculations including contributions of two-body currents as well as to shell-model calculations. The two-body-current contributions significantly improve the agreement with experimental data, reducing the mean-square deviation from the experimental moments by a factor of 3 to 5, depending on the employed interaction. For all interactions, the largest contributions are obtained for the $5/2^-$ ($7/2^-$) isotopes $^{65}$Ni ($^{55}$Ni), which is ascribed to the high angular momentum of the $f$ orbitals. Our results demonstrate that the inclusion of two-body-current contributions to the magnetic moment in an isotopic chain of complex nuclei can be handled by the VS-IMSRG and can outperform phenomenological shell-model calculations using effective $g$-factors in the nickel region.

nucl-ex↗

arXiv2024

Nuclear charge radii of germanium isotopes around $N$ = 40

Collinear laser spectroscopy measurements were performed on $^{68-74}$Ge isotopes ($Z = 32$) at ISOLDE-CERN, by probing the $4s^2 4p^2 \, ^3\!P_1 \rightarrow 4s^2 4p 5s \, ^3\!P_1^o$ atomic transition (269~nm) of germanium. Nuclear charge radii are determined via the measured isotope shifts, revealing a larger local variation than the neighboring isotopic chains. Nuclear density functional theory with the Fayans functionals Fy($\Delta r$,HFB) and Fy(IVP), and the SV-min Skyrme describes the experimental data for the differential charge radii $\delta\langle r^{2} \rangle$ and charge radii $R_{\rm c}$ within the theoretical uncertainties. The observed large variation in the charge radii of germanium isotopes is better accounted for by theoretical models incorporating ground state quadrupole correlations. This suggests that the polarization effects due to pairing and deformation contribute to the observed large odd-even staggering in the charge radii of the Ge isotopic chain.

nucl-ex↗

arXiv2023

Electromagnetic Properties of Indium Isotopes Elucidate the Doubly Magic Character of $^{100}$Sn

Our understanding of nuclear properties in the vicinity of $^{100}$Sn, suggested to be the heaviest doubly magic nucleus with equal numbers of protons (Z=50) and neutrons (N=50), has been a long-standing challenge for experimental and theoretical nuclear physics. Contradictory experimental evidence exists on the role of nuclear collectivity in this region of the nuclear chart. Using precision laser spectroscopy, we measured the ground-state electromagnetic moments of indium (Z=49) isotopes approaching the N=50 neutron number down to 101In, and nuclear charge radii of 101-131In spanning almost the complete range between the two major neutron closed-shells at N=50 and N=82. Our results for both nuclear charge radii and quadrupole moments reveal striking parabolic trends as a function of the neutron number, with a clear reduction toward these two neutron closed-shells, thus supporting a doubly magic character of $^{100}$Sn. Two complementary nuclear many-body frameworks, density functional theory and ab initio methods, elucidate our findings. A detailed comparison with our experimental results exposes deficiencies of nuclear models, establishing a benchmark for future theoretical developments.

nucl-ex↗

arXiv2022

Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV

Background: The $^{14}$N(n,p)$^{14}$C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s-process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region and resonance region. Purpose: Measuring the 14N(n,p)14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and providing calculations of Maxwellian averaged cross sections (MACS). Method: Time-of-flight technique. Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. $^{10}$B(n,${\alpha}$)$^7$Li and $^{235}$U(n,f) reactions as references. Two detection systems running simultaneously, one on-beam and another off-beam. Description of the resonances with the R-matrix code sammy. Results: The cross section has been measured from sub-thermal energy to 800 keV resolving the two first resonances (at 492.7 and 644 keV). A thermal cross-section (1.809$\pm$0.045 b) lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations has been obtained. A 1/v energy dependence of the cross section has been confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed to determine the $^{14}$N(n,p) cross-section over a wide energy range for the first time. We have obtained cross-sections with high accuracy (2.5 %) from sub-thermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.

nucl-ex↗

arXiv2022

Electromagnetic moments of scandium isotopes and $N=28$ isotones in the distinctive $0f_{7/2}$ orbit

The electric quadrupole moment of $^{49}$Sc was measured by collinear laser spectroscopy at CERN-ISOLDE to be $Q_{\rm s}=-0.159(8)$ $e$b, and a nearly tenfold improvement in precision was reached for the electromagnetic moments of $^{47,49}$Sc. The single-particle behavior and nucleon-nucleon correlations are investigated with the electromagnetic moments of $Z=21$ isotopes and $N=28$ isotones as valence neutrons and protons fill the distinctive $0f_{7/2}$ orbit, respectively, located between magic numbers, 20 and 28. The experimental data are interpreted with shell-model calculations using an effective interaction, and ab-initio valence-space in-medium similarity renormalization group calculations based on chiral interactions. These results highlight the sensitivity of nuclear electromagnetic moments to different types of nucleon-nucleon correlations, and establish an important benchmark for further developments of theoretical calculations.

nucl-ex↗

arXiv2022

High accuracy, high resolution 235U(n,f) cross section from n_TOF (CERN) in the thermal to 10 keV energy range

The 235U(n,f) cross section was measured in a wide energy range (25 meV - 170 keV) at the n_TOF facility at CERN, relative to 6Li(n,t) and 10B(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between thermal and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the n_TOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement is found in average between the new results and the latest evaluated data files ENDF-B/VIII and JEFF-3.3, as well as with respect to the IAEA reference files. However, some discrepancies are still present in some specific energy regions. The new dataset here presented, characterized by unprecedented resolution and accuracy, can help improving the evaluations in the Resolved Resonance Region and up to 10 keV, and reduce the uncertainties that affect this region.

nucl-ex↗

arXiv2022

The $^{7}$Be(n,p)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

nucl-ex↗

arXiv2021

Nuclear Charge Radii of the Nickel Isotopes $^{58-68,70}$Ni

Collinear laser spectroscopy is performed on the nickel isotopes $^{58-68,70}$Ni, using a time-resolved photon counting system. From the measured isotope shifts, nuclear charge radii $R_c$ are extracted and compared to theoretical results. Three ab initio approaches all employ, among others, the chiral interaction NNLO$_{\rm sat}$, which allows an assessment of their accuracy. We find agreement with experiment in differential radii $δ\left\langle r_\mathrm{c}^2 \right\rangle$ for all employed ab initio methods and interactions, while the absolute radii are consistent with data only for NNLO$_{\rm sat}$. Within nuclear density functional theory, the Skyrme functional SV-min matches experiment more closely than the Fayans functional Fy($Δr$,HFB).

nucl-ex↗

arXiv2021

Charge radii, moments and masses of mercury isotopes across the N = 126 shell closure

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predominantly in the particle-hole channel in CDFT, since both are present in the calculations without pairing. However, the magnitude of the kink is still affected by the occupation of the $1i_{11/2}$ and $2g_{9/2}$ orbitals with a dependence on the relative energies as well as pairing.

nucl-ex↗

arXiv2021

Isotope Shifts of Radium Monofluoride Molecules

Isotope shifts of $^{223-226,228}$Ra$^{19}$F were measured for different vibrational levels in the electronic transition $A^{2}{}Π_{1/2}\leftarrow X^{2}{}Σ^{+}$. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.

nucl-ex↗

arXiv2020

Laser spectroscopy of neutron-rich $^{207,208}$Hg isotopes: Illuminating the kink and odd-even staggering in charge radii across the $N=126$ shell closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is demonstrated that both the kink at $N=126$ and the odd-even staggering (OES) in its vicinity can be described predominately at the mean-field level, and that pairing does not need to play a crucial role in their origin. A new OES mechanism is suggested, related to the staggering in the occupation of the different neutron orbitals in odd- and even-$A$ nuclei, facilitated by particle-vibration coupling for odd-$A$ nuclei.

nucl-ex↗

arXiv2020

Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,\gamma$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,\gamma$) and $^{56}$Fe($n, \gamma$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.

physics.ins-det↗