arXiv subjects

J. Demsar

Publications and source records attributed to J. Demsar.

42 records · Page 3Linked to original sources

arXiv1999

The superconducting gap Δ_{c}, the pseudogap Δ_{p} and pair fluctuations above Tc in overdoped YCaBaCuO from femtosecond time-domain spectroscopy

The low-energy electronic excitation spectrum and gap structure in optimally doped and overdoped Y_{1-x}Ca_{x}Ba_{2}Cu_{3}O_{7-δ} single crystals are investigated by real-time measurements of the quasiparticle relaxation dynamics with femtosecond optical spectroscopy. From the amplitude of the photoinduced reflectivity as a function of time, temperature and doping x we find clear evidence for the coexistence of two distinct gaps in the entire overdoped phase. One is a temperature-independent pseudogap $Δ_{p}$ and the other is a T-dependent collective gap $Δ_{c}(T)$ which has a BCS-like T-dependence closing at Tc. From quasiparticle relaxation time measurements above Tc we ascertain that fluctuations associated with the collective gap $Δ_{c}(T)$ are limited to a few K, consistent with time-dependent Ginzburg-Landau theory and are distinct from the pseudogap whose presence is apparent well above Tc for all x.

cond-mat.supr-con↗

arXiv1999

Time-Resolved Optical Studies of Quasiparticle Dynamics in High-Temperature Superconductors: Experiments and theory

Ultrafast time-resolved optical spectroscopy in high-temperature superconductors enables the direct real-time measurement of non-equilibrium quasiparticle recombination dynamics. In addition, it also gives detailed information about the symmetry of the superconducting gap and the "pseudogap", their doping dependence and their temperature dependence. Experimental data, together with theoretical models on the photoinduced transmission amplitude and relaxation time as a function of temperature and doping in YBa2Cu3O7-d gives a consistent picture of the evolution of low-energy structure, where a temperature-independent gap is shown to exist in the underdoped state which evolves with doping into a two-component state near optimum doping, where the dominant response is from a T-dependent BCS-like superconducting gap.

cond-mat.supr-con↗

arXiv1998

Evidence for crossover from a Bose-Einstein condensate to a BCS-like superconductor with doping in YBa2Cu3O(7-x) from quasiparticle relaxation dynamics experiments

Time resolved measurements of quasiparticle (QP) relaxation dynamics on the femtosecond timescale are reported as a function of temperature and doping in YBa2Cu3O(7-x) for (0.48 < x < 0.1). In the underdoped state (x > 0.15), there is no evidence for any changes in the low-energy gap structure at Tc from either photoinduced QP absorption or QP relaxation time data. In combination with the sum rule, this implies the existence of pre-formed pairs up to a much higher temperature T*. Near x = 0.1 a rapid cross-over is observed, to a state where the QP recombination time diverges and the photoinduced QP density falls to zero at Tc, indicating the existence of a temperature-dependent superconducting gap which closes at Tc.

cond-mat.supr-con↗

arXiv1998

Quasiparticle relaxation dynamics in superconductors with different gap structures: theory and experiments on YBa_{2}Cu_{3}O_{7-δ}

Photoexcited quasiparticle relaxation dynamics are investigated in a $YBa_{2}Cu_{3}O_{7-δ}$ superconductor as a function of doping $δ$ and temperature $T$ using ultrafast time-resolved optical spectroscopy. A model calculation is presented which describes the temperature dependence of the photoinduced quasiparticle population $n_{pe}$, photoinduced transmission $Δ{\cal T}/{\cal T}$ and relaxation time $τ$ for three different superconducting gaps: (i) a temperature-dependent collective gap such that ${\bf Δ}(T)\to 0$ as $T\to T_{c}$, (ii) a temperature-independent gap, which might arise for the case of a superconductor with pre-formed pairs and (iii) an anisotropic (e.g. d-wave) gap with nodes. Comparison of the theory with data of photoinduced transmission $| Δ{\cal T}/{\cal T} |$, reflection $| Delta{\cal R}/{\cal R}|$ and quasiparticle recombination time $τ$ in $YBa_{2}Cu_{3}O_{7-δ}$ over a very wide range of doping ($0.1 < δ<0.48)$ is found to give good quantitative agreement with a temperature-dependent BCS-like isotropic gap near optimum doping ($δ<0.1)$ and a temperature-independent isotropic gap in underdoped $YBa_{2}Cu_{3}O_{7-δ}$ ($0.15<δ<0.48$). A pure d-wave gap was found to be inconsistent with the data.

cond-mat.supr-con↗

arXiv1998

Divergence of the quasiparticle lifetime with doping and evidence for pre-formed pairs below T* in YBa_2Cu3$O_{7-δ}

We report new time-resolved data of quasiparticle relaxation and Cooper pair recombination dynamics in YBa_2Cu_3O_{7-δ}, measured as a function of temperature and doping δusing femtosecond optical spectroscopy. The data show the existence of a normal state pseudo-gap for in-plane charge excitations below T* and an unusual divergence of the quasiparticle relaxation time in the superconducting state τ_s with δtowards optimum doping. In the underdoped state, no change in the amplitude of the induced transmission (which is proportional to the DOS at E_F), or relaxation time τ_s is observed at T_c. From the sum rule, both observations signify that no gap opens at T_c in underdoped YBCO for δ>0.15. T_c in this case only signifies the onset of phase coherence. The presented data thus suggest pair formation with an associated redistribution of the DOS starting at T* and the establishment of phase coherence at T_c consistent with Bose-Einstein condensation. In the optimally doped material, δ~ 0.1, on the other hand, both a divergence in lifetime and a change of the DOS occur at T_c, signifying the opening of a gap and the occurence of pairing takes place simultaneously.

cond-mat.supr-con↗

arXiv1997

A study of photoexcited carrier relaxation in YBa_2Cu_3O_(7-d) by picosecond resonant Raman spectroscopy

The temperature dependence of the energy relaxation of photoexcited (PE) carriers is used as a probe of the electronic structure of YBa_2Cu_3O_(7-d) in the insulating d~0.8 and metallic d~0.1 phases. The energy relaxation rate to phonons is obtained by measuring the non-equilibrium phonon occupation number, n_neq, with pulsed Raman Stokes/anti-Stokes spectroscopy using 1.5 and 70 ps long laser pulses. We can distinguish between relaxation via extended band states and localized states, since theoretically in the former, the relaxation is expected to be virtually T-independent, while in the latter it is strongly T-dependent. From the experiment - which shows strong temperature dependence of n_neq - we deduce that at least part of the PE carrier relaxation proceeds via hopping between localized states and we propose a simple theoretical model of the relaxation process. In addition, we compare the coupling of different vibrational modes to the carriers to find that the apical O vibrational mode is significantly more involved in the energy relaxation process that the in-plane 340 cm^(-1}) mode. This implies that the localized states are mainly (but not entirely) coupled to out-of plane vibrations.

cond-mat.supr-con↗