arXiv subjects

J. E. Lang

Publications and source records attributed to J. E. Lang.

9 recordsLinked to original sources

arXiv2019

Quantum bath control with nuclear spin state selectivity via pulse-adjusted dynamical decoupling

Dynamical decoupling (DD) is a powerful method for controlling arbitrary open quantum systems. In quantum spin control, DD generally involves a sequence of timed spin flips ($π$ rotations) arranged to average out or selectively enhance coupling to the environment. Experimentally, errors in the spin flips are inevitably introduced, motivating efforts to optimise error-robust DD. Here we invert this paradigm: by introducing particular control "errors" in standard DD, namely a small constant deviation from perfect $π$ rotations (pulse adjustments), we show we obtain protocols that retain the advantages of DD while introducing the capabilities of quantum state readout and polarisation transfer. We exploit this nuclear quantum state selectivity on an ensemble of nitrogen-vacancy centres in diamond to efficiently polarise the $^{13}$C quantum bath. The underlying physical mechanism is generic and paves the way to systematic engineering of pulse-adjusted protocols with nuclear state selectivity for quantum control applications.

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arXiv2019

The non-vanishing effect of detuning errors in dynamical decoupling based quantum sensing experiments

Characteristic dips appear in the coherence traces of a probe qubit when dynamical decoupling (DD) is applied in synchrony with the precession of target nuclear spins, forming the basis for nanoscale nuclear magnetic resonance (NMR). The frequency of the microwave control pulses is chosen to match the qubit transition but this can be detuned from resonance by experimental errors, hyperfine coupling intrinsic to the qubit, or inhomogeneous broadening. The detuning acts as an additional static field which is generally assumed to be completely removed in Hahn echo and DD experiments. Here we demonstrate that this is not the case in the presence of finite pulse-durations, where a detuning can drastically alter the coherence response of the probe qubit, with important implications for sensing applications. Using the electronic spin associated with a nitrogen-vacancy centre in diamond as a test qubit system, we analytically and experimentally study the qubit coherence response under CPMG and XY8 dynamical decoupling control schemes in the presence of finite pulse-durations and static detunings. Most striking is the splitting of the NMR resonance under CPMG, whereas under XY8 the amplitude of the NMR signal is modulated. Our work shows that the detuning error must not be neglected when extracting data from quantum sensor coherence traces.

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arXiv2018

Dynamical decoupling protocols with nuclear spin state selectivity

The ability to initialise nuclear spins, which are typically in a mixed state even at low temperature, is a key requirement of many protocols used in quantum computing and simulations as well as in magnetic resonance spectroscopy and imaging. Yet, it remains a challenging task that typically involves complex and inefficient protocols, limiting the fidelity of ensuing operations or the measurement sensitivity. We introduce here a class of dynamical nuclear spin state selective (DNSS) protocols which, when applied to a polarised electron spin such as the nitrogen-vacancy (NV) centre in diamond, permit the addressing of selected nuclear states of the mixture. It works by splitting the underlying eigenstates into two distinct symmetries dependent on the nuclear spin state, and independent of the electron-nuclear coupling strength. As a particular example, we show that DNSS is achievable by simply introducing a detuning in the common Carr-Purcell-Meiboom-Gill (CPMG) protocol, where the state selection is then controlled by the inter-pulse spacing. This approach offers advantages in ultra-high fidelity initialisation of nuclear registers, ensemble polarisation and single-gate manipulation of nuclei.

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arXiv2018

Stochastic Langevin propagation for classical and quantum optomechanics

Interesting experimental signatures of quantum cavity optomechanics arise because the quantum back-action induces correlations between incident quantum shot noise and the cavity field. While the quantum linear theory of optomechanics (QLT) has provided vital understanding across many experimental platforms, in certain new set-ups it may be insufficient: analysis in the time domain may be needed, but QLT obtains only spectra in frequency space; and nonlinear behavior may be present. Direct solution of the stochastic equations of motion in time is an alternative, but unfortunately standard methods do not preserve the important optomechanical correlations. We introduce two-timescale stochastic Langevin (T2SL) propagation as an efficient and straightforward method to obtain time traces with the correct correlations. We show that T2SL, in contrast to standard stochastic simulations, can efficiently simulate correlation phenomena such as ponderomotive squeezing and reproduces accurately cavity sideband structures on the scale of the applied quantum noise and even complicated features entirely submerged below the quantum shot noise imprecision floor. We investigate nonlinear regimes and find where comparison is possible, that the method agrees with analytical results obtained with master equations at low temperatures and in perturbative regimes.

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arXiv2017

Imaging correlations in heterodyne-detected spectra for quantum sensing

The extraordinary sensitivity of the output field of an optical cavity to small quantum-scale displacements has led to breakthroughs such as the first detection of gravitational waves \cite{LIGO,LIGODC} and of the motions of quantum ground-state cooled mechanical oscillators \cite{Teufel2011,Chan2011}. While heterodyne detection of the cavity field preserves asymmetries which provide a key signature that mechanical oscillators has attained the quantum regime, detection of a rotating quadrature of the light averages out important quantum correlations, yielding a weaker signal and lower sensitivity than homodyne detection. In turn, homodyning, detects a single optical quadrature, but loses the important quantum sideband asymmetries. In the present work we present and experimentally demonstrate a technique, involving judicious construction of the autocorrelators of the output current using filter functions, which can restore the lost correlations (whether classical or quantum), drastically augmenting the useful information extracted: the filtering adjusts for moderate errors in the locking phase of the local oscillator, allowing efficient single-shot measurement of hundreds of different field quadratures and rapid mapping of detailed features from a simple heterodyne trace. One may also control whether the correlations are recovered in isolation or interfere with the usual stationary heterodyne sidebands. In the latter case we obtain a spectrum of hybrid homodyne-heterodyne character, with motional sidebands of combined amplitudes comparable to homodyne. We term such recovery of lost heterodyne correlations with filter functions r-heterodyning: although investigated here in a thermal regime, its robustness and generality represents a promising new approach to sensing of quantum-scale displacements.

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arXiv2017

Proposal for enhanced resolution in nanoscale NMR: quantum sensing with pulses of finite duration

The nitrogen vacancy (NV) color center in diamond is an enormously important platform for the development of quantum sensors, including for single spin and single molecule NMR. Detection of weak single-spin signals is greatly enhanced by repeated sequences of microwave pulses; in these dynamical decoupling (DD) techniques, the key control parameters swept in the experiment are the time intervals, $τ$, between pulses. Here we show that, in fact, the pulse duration offers a powerful additional control parameter. While previously, a non-negligible pulse-width has been considered simply a source of experimental error, here we elucidate the underlying quantum dynamics: we identify a landscape of quantum-state crossings which are usually closed (inactive) but may be controllably activated (opened) by adjusting the pulse-width from zero. We identify these crossings with recently observed but unexpected dips (so called spurious dips) seen in the quantum coherence of the NV spin. With this new understanding, both the position and strength of these sharp features may be accurately controlled; they co-exist with the usual broader coherence dips of short-duration microwave pulses, but their sharpness allows for higher resolution spectroscopy with quantum diamond sensors, or their analogues.

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arXiv2017

Recovering correlations in optomechanical heterodyne spectra for high-precision quantum displacement sensing

Homodyne and heterodyne detection represent "twin-pillars" of quantum displacement sensing using optical cavities, having permitted major breakthroughs including detection of gravitational waves and of the motion of quantum ground-state cooled mechanical oscillators. Both can suffer disadvantages as diagnostics in quantum optomechanics, either through symmetrisation (homodyne), or loss of correlations (heterodyne). We show that, for modest heterodyne beat frequencies ($Ω\sim ω_M/10 \gg Γ$), judicious construction of the autocorrelation of the measured current can either recover (i) a spectrum with strong sidebands but without an imprecision noise floor (ii) a spectrum which is a hybrid, combining both homodyne and heterodyne sideband features. We simulate an experimental realisation with stochastic numerics and find excellent agreement with analytical quantum noise spectra. We term such retrospective recovery of lost heterodyne correlations "r-heterodyning": as the method simply involves post-processing of a normal heterodyne time signal, there is no additional experimental constraint other than on the magnitude of $Ω$.

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arXiv2016

Decoherence of electron spins in isotopically enriched silicon near Clock Transitions

Despite the importance of isotopically purified samples in current experiments, there have been few corresponding studies of spin qubit decoherence using full quantum bath calculations. Isotopic purification eliminates the well-studied nuclear spin baths which usually dominate decoherence. We model the coherence of electronic spin qubits in silicon near so called Clock Transitions (CT) where experiments have electronic $T_{2e}$ times of seconds. Despite the apparent simplicity of the residual decoherence mechanism, this regime is not well understood: the state mixing which underpins CTs allows also a proliferation of contributions from usually forbidden channels (direct flip-flops with non-resonant spins); in addition, the magnitude and effects of the corresponding Overhauser fields and other detunings is not well quantified. For purely magnetic detunings, we identify a regime, potentially favourable for quantum computing, where forbidden channels are completely suppressed but spins in resonant states are fully released from Overhauser fields and applied magnetic field gradients. We show by a general argument that the enhancement between this regime and the high field limit is $< 8$, regardless of density, while enhancements of order 50 are measured experimentally. We propose that this discrepancy is likely to arise from strains of exclusively non-magnetic origin, underlining the potential of CTs for isolating and probing different types of inhomogeneities. We also identify a set of fields, "Dipolar Refocusing Points" (DRPs), where the Hahn echo fully refocuses the effect of the dipolar interaction.

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arXiv2016

Dynamical decoupling based quantum sensing: Floquet spectroscopy

Sensing the internal dynamics of individual nuclear spins or clusters of nuclear spins has recently become possible by observing the coherence decay of a nearby electronic spin: the weak magnetic noise is amplified by a periodic, multi-pulse decoupling sequence. However, it remains challenging to robustly infer underlying atomic-scale structure from decoherence traces in all but the simplest cases. We introduce Floquet spectroscopy as a versatile paradigm for analysis of these experiments, and argue it offers a number of general advantages. In particular, this technique generalises to more complex situations, offering physical insight in regimes of many-body dynamics, strong coupling and pulses of finite duration. As there is no requirement for resonant driving, the proposed spectroscopic approach permits physical interpretation of striking, but overlooked, coherence decay features in terms of the form of the avoided crossings of the underlying quasienergy eigenspectrum. This is exemplified by a set of "diamond" shaped features arising for transverse-field scans in the case of single-spin sensing by NV-centers in diamond. We investigate also applications for donors in silicon showing that the resulting tunable interaction strengths offer highly promising future sensors.

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