arXiv subjects

J. E. Moore

Publications and source records attributed to J. E. Moore.

At least 19 recordsLinked to original sources

arXiv2026

Optical Depths from the Thermal Sunyaev-Zel'dovich Effect with ACT DR6 and DESI DR1 Spectroscopic Galaxies and Optically-Selected Clusters

We present stacked thermal Sunyaev-Zel'dovich (tSZ) effect measurements for three samples of galaxy groups and clusters: those traced by the Dark Energy Spectroscopic Intstrument Data Release 1 (DESI DR1) luminous red galaxies (LRG) and the DESI DR1 Bright Galaxy Sample (BGS), and an eROMaPPer optically-selected sample from the DESI Legacy Imaging Survey. We use the latest Atacama Cosmology Telescope DR6 (ACT)+Planck component-separated internal linear combination (ILC) Compton-$y$ maps and ACT+Planck coadded 90, 150, and 220 GHz temperature maps to extract the tSZ signal within a $\sim2'$ disk aperture for sources binned by luminosity, richness, or mass. We measure the average tSZ signal with high statistical significance, with signal-to-noise ratios surpassing 38 for LRG, 27 for BGS, and 39 for the eROMaPPer sample using the 90 GHz ACT DR6+Planck map. We conduct a detailed study of systematics and foregrounds such as dust and cosmic infrared background (CIB) contamination, which remain a core challenge for tSZ analysis. For the LRG and BGS samples, we find that dust and radio source emission dominate the tSZ signal at scales near and below the disk aperture radius. Large-scale ($R>4'$) contamination from the CIB is less significant. We mitigate these contaminants to isolate the tSZ signal and use a combination of simulated and real measurements to develop Compton-$y-$optical depth ($\bar y-\bar \tau$) scaling relations to infer optical depths, which are found to be in agreement with values measured using the pairwise kinematic SZ effect for the same tracer samples. The $\bar y-\bar \tau$ scaling relation for the eROMaPPer sample is the first such relationship to be derived directly from SZ measurements.

astro-ph.CO↗

arXiv2026

Spectrum and low-temperature bulk properties of triangular quantum spin liquid candidate NaYbSe$_2$

We report neutron scattering, pressure-dependent AC calorimetry, and AC magnetic susceptibility measurements of triangular lattice NaYbSe$_2$. We observe a continuum of scattering, which is reproduced by matrix product simulations, and no phase transition is detected in any bulk measurements. Comparison to heat capacity simulations suggest the material is within the Heisenberg spin liquid phase. AC Susceptibility shows a frequency-dependent peak at 40 mK, as has been observed in several triangular magnets.

cond-mat.str-el↗

arXiv2026

Nonlinear light cone spreading of correlations in a triangular quantum magnet: a hard quantum simulation target

Dynamical correlations of quantum many-body systems are typically analyzed in the momentum space and frequency basis. However, quantum simulators operate more naturally in real space, real time settings. Here we analyze the real-space time-dependent van Hove spin correlations $G(r,t)$ of the 2D triangular antiferromagnet KYbSe$_2$ as obtained from high-resolution Fourier-transformed neutron spectroscopy. We compare this to $G(r,t)$ from five theoretical simulations of the well-established spin Hamiltonian. Our analysis reveals non-linear sub-ballistic low-temperature transport in KYbSe$_2$ which none of the current state-of-the-art numerical or field-theoretical methods reproduce. Our observation signals an emergent collective hydrodynamics, perhaps associated with the quantum critical phase of a quantum spin liquid, and provides an ideal benchmark for future quantum simulations.

cond-mat.str-el↗

arXiv2023

Symmetry-breaking pathway towards the unpinned broken helix

One of the prime material candidates to host the axion insulator state is EuIn$_{2}$As$_{2}$. First-principles calculations predicted the emergence of this exotic topological phase based on the assumption of a collinear antiferromagnetic structure. However, neutron scattering measurements revealed a more intricate magnetic ground state, characterized by two coexisting magnetic wavevectors, reached by successive thermal phase transitions. The proposed high and low temperature phases were a spin helix and a state with interpenetrating helical and antiferromagnetic order, termed a broken helix, respectively. Despite its complexity, the broken helix still protects the axion state because the product of time-reversal and a rotational symmetry is preserved. Here we identify the magnetic structure associated with these two phases using a multimodal approach that combines symmetry-sensitive optical probes, scattering, and group theoretical analysis. We find that the higher temperature phase hosts a nodal structure rather than a helix, characterized by a variation of the magnetic moment amplitude from layer to layer, with the moment vanishing entirely in every third Eu layer. The lower temperature structure is similar to the broken helix, with one important difference: the relative orientation of the magnetic structure and the lattice is not fixed, resulting in an `unpinned broken helix'. As a result of the breaking of rotational symmetry, the axion phase is not generically protected. Nevertheless, we show that it can be restored if the magnetic structure is tuned with externally-applied uniaxial strain. Finally, we present a spin Hamiltonian that identifies the spin interactions needed to account for the complex magnetic order in EuIn$_{2}$As$_{2}$. Our work highlights the importance of the multimodal approach in determining the symmetry of complex order-parameters.

cond-mat.str-el↗

arXiv2023

Witnessing quantum criticality and entanglement in the triangular antiferromagnet KYbSe$_2$

The Heisenberg triangular lattice quantum spin liquid and the phase transitions to nearby magnetic orders have received much theoretical attention, but clear experimental manifestations of these states are rare. This work investigates a new spin-half Yb$^{3+}$ delafossite material, KYbSe$_2$, whose inelastic neutron scattering spectra reveal a diffuse continuum with a sharp lower bound. Applying entanglement witnesses to the data reveals significant multipartite entanglement spread between its neighbors, and analysis of its magnetic exchange couplings shows close proximity to the triangular lattice Heisenberg quantum spin liquid. Key features of the data are reproduced by Schwinger-boson theory and tensor network calculations with a significant second-neighbor coupling $J_2$. The strength of the dynamical structure factor at the $K$ point shows a scaling collapse in $\hbarω/k_\mathrm{B}T$ down to 0.3 K, indicating a second-order quantum phase transition. Comparing this to previous theoretical work suggests that the proximate phase at larger $J_2$ is a gapped $\mathbb{Z}_2$ spin liquid, resolving a long-debated issue. We thus show that KYbSe$_2$ is close to a spin liquid phase, which in turn sheds light on the theoretical phase diagram itself.

cond-mat.str-el↗

arXiv2022

Observation of a phase transition within the domain walls of ferromagnetic Co3Sn2S2

The ferromagnetic phase of Co$_3$Sn$_2$S$_2$ is widely considered to be a topological Weyl semimetal, with evidence for momentum-space monopoles of Berry curvature from transport and spectroscopic probes. As the bandstructure is highly sensitive to the magnetic order, attention has focused on anomalies in magnetization, susceptibility and transport measurements that are seen well below the Curie temperature, leading to speculation that a "hidden" phase coexists with ferromagnetism. Here we report spatially-resolved measurements by Kerr effect microscopy that identify this phase. We find that the anomalies coincide with a deep minimum in domain wall (DW) mobility, indicating a crossover between two regimes of DW propagation. We demonstrate that this crossover is a manifestation of a 2D phase transition that occurs within the DW, in which the magnetization texture changes from continuous rotation to unidirectional variation. We propose that the existence of this 2D transition deep within the ferromagnetic state of the bulk is a consequence of a giant quality factor for magnetocrystalline anisotropy unique to this compound. This work broadens the horizon of the conventional binary classification of DWs into Bloch and Néel walls, and suggests new strategies for manipulation of domain walls and their role in electron and spin transport.

cond-mat.mes-hall↗

arXiv2020

Detection of Kardar-Parisi-Zhang hydrodynamics in a quantum Heisenberg spin-$1/2$ chain

Classical hydrodynamics is a remarkably versatile description of the coarse-grained behavior of many-particle systems once local equilibrium has been established. The form of the hydrodynamical equations is determined primarily by the conserved quantities present in a system. Some quantum spin chains are known to possess, even in the simplest cases, a greatly expanded set of conservation laws, and recent work suggests that these laws strongly modify collective spin dynamics even at high temperature. Here, by probing the dynamical exponent of the one-dimensional Heisenberg antiferromagnet KCuF$_3$ with neutron scattering, we find evidence that the spin dynamics are well described by the dynamical exponent $z=3/2$, which is consistent with the recent theoretical conjecture that the dynamics of this quantum system are described by the Kardar-Parisi-Zhang universality class. This observation shows that low-energy inelastic neutron scattering at moderate temperatures can reveal the details of emergent quantum fluid properties like those arising in non-Fermi liquids in higher dimensions.

cond-mat.str-el↗

arXiv2020

NWChem: Past, Present, and Future

Specialized computational chemistry packages have permanently reshaped the landscape of chemical and materials science by providing tools to support and guide experimental efforts and for the prediction of atomistic and electronic properties. In this regard, electronic structure packages have played a special role by using first-principledriven methodologies to model complex chemical and materials processes. Over the last few decades, the rapid development of computing technologies and the tremendous increase in computational power have offered a unique chance to study complex transformations using sophisticated and predictive many-body techniques that describe correlated behavior of electrons in molecular and condensed phase systems at different levels of theory. In enabling these simulations, novel parallel algorithms have been able to take advantage of computational resources to address the polynomial scaling of electronic structure methods. In this paper, we briefly review the NWChem computational chemistry suite, including its history, design principles, parallel tools, current capabilities, outreach and outlook.

physics.chem-ph↗

arXiv2019

Observation of Topological Photocurrents in the Chiral Weyl Semimetal RhSi

Weyl semimetals are crystals in which electron bands cross at isolated points in momentum space. Associated with each crossing point (or Weyl node) is an integer topological invariant known as the Berry monopole charge. The discovery of new classes of Weyl materials is driving the search for novel properties that derive directly from the Berry charge. The circular photogalvanic effect (CPGE), whereby circular polarized light generates a current whose direction depends on the helicity of the absorbed photons, is a striking example of a macroscopic property that emerges from Weyl topology. Recently, it was predicted that the rate of current generation associated with optical transitions near a Weyl node is proportional to its monopole charge and independent of material-specific parameters. In Weyl semimetals that retain mirror symmetry this universal photogalvanic current is strongly suppressed by opposing contributions from energy equivalent nodes of opposite charge. However, when all mirror symmetries are broken, as in chiral Weyl systems, nodes with opposite topological charge are no longer degenerate, opening a window of photon energies where the topological CPGE can emerge. In this work we test this theory through measurement of the photon-energy dependence of the CPGE in the chiral Weyl semimetal RhSi. The spectrum is fully consistent with a topological CPGE, as it reveals a response in a low-energy window that closes at 0.65 eV, in quantitative agreement with the theoretically-derived bandstucture.

cond-mat.mes-hall↗

arXiv2018

Imaging stress and magnetism at high pressures using a nanoscale quantum sensor

Pressure alters the physical, chemical and electronic properties of matter. The development of the diamond anvil cell (DAC) enables tabletop experiments to investigate a diverse landscape of high-pressure phenomena ranging from the properties of planetary interiors to transitions between quantum mechanical phases. In this work, we introduce and utilize a novel nanoscale sensing platform, which integrates nitrogen-vacancy (NV) color centers directly into the culet (tip) of diamond anvils. We demonstrate the versatility of this platform by performing diffraction-limited imaging (~600 nm) of both stress fields and magnetism, up to pressures ~30 GPa and for temperatures ranging from 25-340 K. For the former, we quantify all six (normal and shear) stress components with accuracy $<0.01$ GPa, offering unique new capabilities for characterizing the strength and effective viscosity of solids and fluids under pressure. For the latter, we demonstrate vector magnetic field imaging with dipole accuracy $<10^{-11}$ emu, enabling us to measure the pressure-driven $α\leftrightarrowε$ phase transition in iron as well as the complex pressure-temperature phase diagram of gadolinium. In addition to DC vector magnetometry, we highlight a complementary NV-sensing modality using T1 noise spectroscopy; crucially, this demonstrates our ability to characterize phase transitions even in the absence of static magnetic signatures. By integrating an atomic-scale sensor directly into DACs, our platform enables the in situ imaging of elastic, electric and magnetic phenomena at high pressures.

cond-mat.mes-hall↗

arXiv2018

Resonance-enhanced optical nonlinearity in the Weyl semimetal TaAs

While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $σ^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is broken. Second order nonlinear optical responses are powerful tools in basic research, as probes of symmetry breaking, and in optical technology as the basis for generating currents from far-infrared to X-ray wavelengths. The recent surge of interest in Weyl semimetals with acentric crystal structures has led to the discovery of a host of $σ^{(2)}$ -related phenomena in this class of materials, such as polarization-selective conversion of light to dc current (photogalvanic effects) and the observation of giant second-harmonic generation (SHG) efficiency in TaAs at photon energy 1.5 eV. Here, we present measurements of the SHG spectrum of TaAs revealing that the response at 1.5 eV corresponds to the high-energy tail of a resonance at 0.7 eV, at which point the second harmonic conductivity is approximately 200 times larger than seen in the standard candle nonlinear crystal, GaAs. This remarkably large SHG response provokes the question of ultimate limits on $σ^{(2)}$ , which we address by a new theorem relating frequency-integrated nonlinear response functions to the third cumulant (or "skewness") of the polarization distribution function in the ground state. This theorem provides considerable insight into the factors that lead to the largest possible second-order nonlinear response, specifically showing that the spectral weight is unbounded and potentially divergent when the possibility of next-neighbor hopping is included.

cond-mat.mtrl-sci↗

arXiv2017

Giant anisotropic nonlinear optical response in transition metal monopnictide Weyl semimetals

Although Weyl fermions have proven elusive in high-energy physics, their existence as emergent quasiparticles has been predicted in certain crystalline solids in which either inversion or time-reversal symmetry is broken\cite{WanPRB2011,BurkovPRL2011, WengPRX2015,HuangNatComm2015}. Recently they have been observed in transition metal monopnictides (TMMPs) such as TaAs, a class of noncentrosymmetric materials that heretofore received only limited attention \cite{XuScience2015, LvPRX2015, YangNatPhys2015}. The question that arises now is whether these materials will exhibit novel, enhanced, or technologically applicable electronic properties. The TMMPs are polar metals, a rare subset of inversion-breaking crystals that would allow spontaneous polarization, were it not screened by conduction electrons \cite{anderson1965symmetry,shi2013ferroelectric,kim2016polar}. Despite the absence of spontaneous polarization, polar metals can exhibit other signatures of inversion-symmetry breaking, most notably second-order nonlinear optical polarizability, $χ^{(2)}$, leading to phenomena such as optical rectification and second-harmonic generation (SHG). Here we report measurements of SHG that reveal a giant, anisotropic $χ^{(2)}$ in the TMMPs TaAs, TaP, and NbAs. With the fundamental and second harmonic fields oriented parallel to the polar axis, the value of $χ^{(2)}$ is larger by almost one order of magnitude than its value in the archetypal electro-optic materials GaAs \cite{bergfeld2003second} and ZnTe \cite{wagner1998dispersion}, and in fact larger than reported in any crystal to date.

cond-mat.mtrl-sci↗

arXiv2016

Thermodynamic Anomaly Above the Superconducting Critical Temperature in the Quasi One-Dimensional Superconductor Ta$_4$Pd$_3$Te$_{16}$

We study the intrinsic transport anisotropy and fermiology of the quasi one-dimensional superconductor Ta$_4$Pd$_3$Te$_{16}$. Below $T^*=20$ K we detect a thermodynamic phase transition that predominantly affects the conductivity perpendicular to the quasi one-dimensional chains, consistent with a thermodynamic transition related to the presence of charge order that precedes superconductivity. Remarkably the Fermi surface pockets detected by de Haas-van Alphen (dHvA) oscillations are unaffected by this transition, suggesting that the ordered state does not break any translational symmetries but rather alters the scattering of the quasiparticles themselves.

cond-mat.supr-con↗

arXiv2015

Approaching Many-Body Localization from Disordered Luttinger Liquids via the Functional Renormalization Group

We study the interplay of interactions and disorder in a one-dimensional fermion lattice coupled adiabatically to infinite reservoirs. We employ both the functional renormalization group (FRG) as well as matrix product state techniques, which serve as an accurate benchmark for small systems. Using the FRG, we compute the length- and temperature-dependence of the conductance averaged over $10^4$ samples for lattices as large as $10^{5}$ sites. We identify regimes in which non-ohmic power law behavior can be observed and demonstrate that the corresponding exponents can be understood by adapting earlier predictions obtained perturbatively for disordered Luttinger liquids. In presence of both disorder and isolated impurities, the conductance has a universal single-parameter scaling form. This lays the groundwork for an application of the functional renormalization group to the realm of many-body localization.

cond-mat.str-el↗

arXiv2015

Quantum revivals and many-body localization

We show that the magnetization of a single `qubit' spin weakly coupled to an otherwise isolated disordered spin chain exhibits periodic revivals in the localized regime, and retains an imprint of its initial magnetization at infinite time. We demonstrate that the revival rate is strongly suppressed upon adding interactions after a time scale corresponding to the onset of the dephasing that distinguishes many-body localized phases from Anderson insulators. In contrast, the ergodic phase acts as a bath for the qubit, with no revivals visible on the time scales studied. The suppression of quantum revivals of local observables provides a quantitative, experimentally observable alternative to entanglement growth as a measure of the `non-ergodic but dephasing' nature of many-body localized systems.

cond-mat.str-el↗

arXiv2014

Quasi Many-body Localization in Translation Invariant Systems

It is typically assumed that disorder is essential to realize Anderson localization. Recently, a number of proposals have suggested that an interacting, translation invariant system can also exhibit localization. We examine these claims in the context of a one-dimensional spin ladder. At intermediate time scales, we find slow growth of entanglement entropy consistent with the phenomenology of many-body localization. However, at longer times, all finite wavelength spin polarizations decay in a finite time, independent of system size. We identify a single length scale which parametrically controls both the eventual spin transport times and the divergence of the susceptibility to spin glass ordering. We dub this long pre-thermal dynamical behavior, intermediate between full localization and diffusion, quasi-many body localization.

cond-mat.dis-nn↗

arXiv2014

Universal nonequilibrium signatures of Majorana zero modes in quench dynamics

The quantum evolution after a metallic lead is suddenly connected to an electron system contains information about the excitation spectrum of the combined system. We exploit this type of "quantum quench" to probe the presence of Majorana fermions at the ends of a topological superconducting wire. We obtain an algebraically decaying overlap (Loschmidt echo) ${\cal L}(t)=| < ψ(0) | ψ(t) > |^2\sim t^{-α}$ for large times after the quench, with a universal critical exponent $α$=1/4 that is found to be remarkably robust against details of the setup, such as interactions in the normal lead, the existence of additional lead channels or the presence of bound levels between the lead and the superconductor. As in recent quantum dot experiments, this exponent could be measured by optical absorption, offering a new signature of Majorana zero modes that is distinct from interferometry and tunneling spectroscopy.

cond-mat.mes-hall↗

arXiv2014

Transport properties of the one-dimensional Hubbard model at finite temperature

We study finite-temperature transport properties of the one-dimensional Hubbard model using the density matrix renormalization group. Our aim is two-fold: First, we compute both the charge and the spin current correlation function of the integrable model at half filling. The former decays rapidly, implying that the corresponding Drude weight is either zero or very small. Second, we calculate the optical charge conductivity sigma(omega) in presence of small integrability-breaking next-nearest neighbor interactions (the extended Hubbard model). The DC conductivity is finite and diverges as the temperature is decreased below the gap. Our results thus suggest that the half-filled, gapped Hubbard model is a normal charge conductor at finite temperatures. As a testbed for our numerics, we compute sigma(omega) for the integrable XXZ spin chain in its gapped phase.

cond-mat.str-el↗