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J. Guillot

Publications and source records attributed to J. Guillot.

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Evolution of Spectroscopic Factors in Neutron-deficient $p$-shell Nuclei in connection with Short-Range Correlations

We report an uncertainty-controlled determination of neutron-removal spectroscopic factors in the neutron-deficient $p$-shell nuclei $^{12}\mathrm{C}$, $^{10}\mathrm{C}$, $^{9}\mathrm{C}$, and $^{8}\mathrm{B}$, all measured under uniform conditions through exclusive ground-state-to-ground-state $(p,d)$ reactions at about 50 MeV/nucleon in a liquid hydrogen target at the GANIL/LISE facility. The deuterons were detected in the highly-segmented MUST2 detector placed at forward angles and the excitation energy was reconstructed by the missing mass method. Several transitions, including a new state in $^7\mathrm{B}$, were observed. Differential cross sections, which display an $L=1$ pattern for all nuclei, were fitted with 416 sets of uncertainty-quantified optical-model potential parameters and considering various single-particle bound-state wavefunctions to derive $C^2S$ values. The ratio between experimental and shell-model calculated values, $R_S$, is found to be slightly decreasing as a function of increasing proton to neutron separation energy asymmetry $\Delta S$, with a slope of $-0.0049(36)_{\rm stat}(13)_{\rm omp}(8)_{\rm s.p.}$. The observed trend is compatible with the phenomenological expectation that the short-range correlation effect on $C^2S$ increases with the degree of nucleon minority. The present data set delivers a high-precision benchmark that will tightly constrain future microscopic descriptions of short-range correlations in asymmetric nuclei.

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Data sorting modes of phoswich detector array

The different data-sorting modes of the phoswich detector array PARIS used for detecting high-energy (4$-$10 MeV) $\gamma$ rays are investigated. The characteristics including time resolution, energy resolution and detection efficiency under various modes are studied. The present study shows that PARIS has capabilities of rejecting escape and pileup events when used for decay spectroscopy. Notably, the methods presented in this work refer specifically to the $\beta$-decay experiment of $^{80g+m}$Ga conducted with three PARIS clusters comprising 27 phoswich detectors, rather than to a general report on the PARIS array or its overall performance for in-beam spectroscopy. Compared with the 2"$\times$2"$\times$2" LaBr$_3$(Ce) detector (Ciema{\l}a et al., 2009), even in individual mode, PARIS provides significant suppression of single- and double-escape peaks and reduces background via vetoing function of the outer-volume NaI(Tl) crystals. In contrast to the common approach of adding back the energies in LaBr$_3$(Ce) and NaI(Tl) to increase the detection efficiency of the full-energy peak, using NaI(Tl) as a veto shield provides a superior trade-off for applications where spectral purity is essential. Employing add-back analysis within each cluster of nine phoswiches or between all phoswiches could enhance full-energy peak efficiency and further suppress escape peaks and background. Applying a multiplicity condition provides a further suppression but simultaneously lowers the statistics of full-energy peaks.

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$\beta$-delayed spectroscopy of $^{80}$Ge$_{48}$ and competition between Gamow-Teller and first-forbidden transitions in $^{80g+m}$Ga$_{49}$ $\beta$ decay

The $\beta$-delayed spectroscopy of $^{80}$Ge has been studied using sources of ground and low-lying isomeric states of $^{80}$Ga. A hybrid $\gamma$-ray spectrometer was used, composed of high-purity germanium (HPGe) detectors for low-energy $\gamma$-ray detection, phoswich detectors from the PARIS array for high-energy $\gamma$ rays and a plastic detector for $\beta$ tagging. The new decay level schemes are presented, with 13 and 14 states $\beta$ populated by $^{80g}$Ga and $^{80m}$Ga, respectively, being reported for the first time. We quantitatively compare summed intensities of first-forbidden and previously reported Gamow-Teller $\beta$ transitions [R. Li et al., \href{https://doi.org/10.1103/PhysRevC.111.034303}{Phys. Rev. C 111, 034303 (2025)}]. The upper-limit fractions of first-forbidden transitions contributing to the decays of $^{80g}$Ga and $^{80m}$Ga are (48.0 $\pm$ 2.7)$\%$ and (47.9 $\pm$ 3.3)$\%$ of the observed total $\beta$ transition intensities of (78.2 $\pm$ 2.5)$\%$ and (82.2 $\pm$ 3.7)$\%$, respectively. Notably, the half-lives decrease in accordance with the upper limits of (48.0 $\pm$ 6.0)$\%$ [3.67(20) s $\rightarrow$ 1.91(3) s] and (47.9 $\pm$ 7.2)$\%$ [3.01(19) s $\rightarrow$ 1.57(1) s] for $^{80g}$Ga and $^{80m}$Ga, respectively, when including first-forbidden transitions, in contrast to those by Gamow-Teller transitions only.

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Simultaneous impacts of nuclear shell structure and collectivity on $\beta$ decay: Evidence from $^{80}$Ga$_{49}$

The Gamow-Teller strength distribution covering the entire $\beta$-decay window, up to 10.312(4) MeV, of $^{80g+m}$Ga was measured for the first time in photo fission of UC$_x$ induced by a 50 MeV electron beam. The new data show significant enhancement in the high-energy region with a jump structure. Simultaneously, the $\gamma$ deexciting behavior of $\beta$-populated states presents a competition between deexcitation to 2$_1^+$ [$\beta_2$ = 0.155(9)] and to 2$_2^+$ [$\beta_2$ = 0.053$_{0.009}^{0.008}$)] in $^{80}$Ge. To understand these data, we performed a realistic shell-model calculation and systematic analysis of log $\it{ft}$ ratios between precursors' $\beta$ decay to 2$_2^+$ and to 2$_1^+$ of Ga isotopes. We conclude that these phenomena evidence simultaneous impacts of nuclear shell structure and collectivity on $\it{B}$(GT) distribution and therefore the half-life of the precursor.

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N=16 magicity revealed at the proton drip-line through the study of 35Ca

The last proton bound calcium isotope $^{35}$Ca has been studied for the first time, using the $^{37}$Ca($p, t$)$^{35}$Ca two neutron transfer reaction. The radioactive $^{37}$Ca nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid hydrogen target CRYPTA, to produce tritons $t$ that were detected in the MUST2 detector array, in coincidence with the heavy residues Ca or Ar. The atomic mass of $^{35}$Ca and the energy of its first 3/2$^+$ state are reported. A large $N=16$ gap of 4.61(11) MeV is deduced from the mass measurement, which together with other measured properties, makes $^{36}$Ca a doubly-magic nucleus. The $N = 16$ shell gaps in $^{36}$Ca and $^{24}$O are of similar amplitude, at both edges of the valley of stability. This feature is discussed in terms of nuclear forces involved, within state-of-the-art shell model calculations. Even though the global agreement with data is quite convincing, the calculations underestimate the size of the $N = 16$ gap in 36Ca by 840(110) keV.

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The structure of $^{36}$Ca under the Coulomb magnifying glass

Detailed spectroscopy of the neutron-deficient nucleus $^{36}$Ca was obtained up to 9 MeV using the $^{37}$Ca($p$,$d$)$^{36}$Ca and the $^{38}$Ca($p$,$t$)$^{36}$Ca transfer reactions. The radioactive nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid Hydrogen target CRYPTA, to produce light ejectiles (the deuteron $d$ or triton $t$) that were detected in the MUST2 detector array, in coincidence with the heavy residues %identified by a zero degree detection system. %States have been measured up to 9 MeV. Our main findings are: i) a similar shift in energy for the 1$^+_1$ and 2$^+_1$ states by about -250 keV, as compared to the mirror nucleus $^{36}$S, ii) the discovery of an intruder 0$^+_2$ state at 2.83(13) MeV, which appears below the first 2$^+$ state, in contradiction with the situation in $^{36}$S, and iii) a tentative 0$^+_3$ state at 4.83(17) MeV, proposed to exhibit a bubble structure with two neutron vacancies in the 2s$_{1/2}$ orbit. The inversion between the 0$^+_2$ and 2$^+_1$ states is due to the large mirror energy difference (MED) of -516(130) keV for the former. This feature is reproduced by Shell Model (SM) calculations, using the $sd$-$pf$ valence space, predicting an almost pure intruder nature for the 0$^+_2$ state, with two protons (neutrons) being excited across the $Z$=20 magic closure in $^{36}$Ca ($^{36}$S). This mirror system has the largest MEDs ever observed, if one excludes the few cases induced by the effect of the continuum.

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Evaluation of the $^{35}$K($p$,$γ$)$^{36}$Ca reaction rate using the $^{37}$Ca($p$,$d$)$^{36}$Ca transfer reaction

A recent sensitivity study has shown that the $^{35}$K$(p,γ)^{36}$Ca reaction is one of the ten $(p,γ)$ reaction rates that could significantly impact the shape of the calculated X-ray burst light curve. In this work, we propose to reinvestigate the $^{35}$K$(p,γ)^{36}$Ca reaction rate, as well as related uncertainties, by determining the energies and decay branching ratios of $^{36}$Ca levels, within the Gamow window, in the 0.5 to 2 GK X-ray burst temperature range. These properties were studied using the one neutron pick-up transfer reaction $^{37}$Ca$(p,d)^{36}$Ca in inverse kinematics using a radioactive beam of $^{37}$Ca at 48 MeV nucleon$^{-1}$. The experiment performed at GANIL, used the liquid Hydrogen target CRYPTA, the MUST2 detector array for the detection of the light charged particles and a zero degree detection system for the outgoing heavy ions. The atomic mass of $^{36}$Ca is confirmed and new resonances have been proposed together with their proton decay branching ratios. This spectroscopic information, used in combination with recent theoretical predictions for the $γ$-width, were used to calculate the $^{35}$K$(p,γ)^{36}$Ca reaction rate. The recommended rate of the present work was obtain within a uncertainty factor of 2 at 1 sigma. This is consistent, with the previous estimate in the X-ray burst temperature range. A large increase of the reaction rate was found at higher temperatures due to two newly discovered resonances. The $^{35}$K$(p,γ)^{36}$Ca thermonuclear reaction rate is now well constrained by the present work in a broad range of temperatures. Our results show that the $^{35}$K$(p,γ)^{36}$Ca reaction does not affect the shape of the X-ray burst light curve, and that it can be removed from the list of the few influential proton radiative captures reactions having a strong impact on the light curve.

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Neutron-proton pairing in the N=Z radioactive fp-shell nuclei 56Ni and 52Fe probed by pair transfer

The isovector and isoscalar components of neutron-proton pairing are investigated in the N=Z unstable nuclei of the \textit{fp}-shell through the two-nucleon transfer reaction (p,$^3$He) in inverse kinematics. The combination of particle and gamma-ray detection with radioactive beams of $^{56}$Ni and $^{52}$Fe, produced by fragmentation at the GANIL/LISE facility, made it possible to carry out this study for the first time in a closed and an open-shell nucleus in the \textit{fp}-shell. The transfer cross-sections for ground-state to ground-state (J=0$^+$,T=1) and to the first (J=1$^+$,T=0) state were extracted for both cases together with the transfer cross-section ratios $σ$(0$^+$,T=1) /$σ$(1$^+$,T=0). They are compared with second-order distorted-wave born approximation (DWBA) calculations. The enhancement of the ground-state to ground-state pair transfer cross-section close to mid-shell, in $^{52}$Fe, points towards a superfluid phase in the isovector channel. For the "deuteron-like" transfer, very low cross-sections to the first (J=1$^+$,T=0) state were observed both for \Ni\phe\, and \Fe\phe\, and are related to a strong hindrance of this channel due to spin-orbit effect. No evidence for an isoscalar deuteron-like condensate is observed.

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Charged-particle branching ratios above the neutron threshold in $^{19}$F: constraining $^{15}$N production in core-collapse supernovae

Spatially-correlated overabundances of $^{15}$N and $^{18}$O observed in some low-density graphite meteoritic grains have been connected to nucleosynthesis taking place in the helium-burning shell during core-collapse supernovae. Two of the reactions which have been identified as important to the final abundances of $^{15}$N and $^{18}$O are $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O. The relative strengths of the $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O reactions depend on the relative $α_0$ and $p_0$ decays from states above the neutron threshold in $^{19}$F in addition to other properties. Experimental data on the charged-particle decays from these highly excited states are lacking or inconsistent. Two experiments were performed using proton inelastic scattering from LiF targets and magnetic spectrographs. The first experiment used the high-resolution Q3D spectrograph at Munich to constrain properties of levels in $^{19}$F. A second experiment using the Orsay Split-Pole spectrograph and an array of silicon detectors was performed in order to measure the charged-particle decays of neutron-unbound levels in $^{19}$F. A number of levels in $^{19}$F have been identified along with their corresponding charged-particle decays. The first state above the neutron threshold which has an observed proton-decay branch to the ground state of $^{18}$O lies 68 keV above the neutron threshold while the $α$-particle decays from the neutron-unbound levels are generally observed to be much stronger than the proton decays. Neutron-unbound levels in $^{19}$F are observed to decay predominantly by $α$-particle emission, supporting the role of $^{18}$F($n,α$)$^{15}$N in the production of $^{15}$N in the helium-burning shell of supernovae. Improved resonant-scattering reaction data are required in order to be able to determine the reaction rates accurately.

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Probing nuclear forces beyond the nuclear drip line: The cases of $^{16}$F and $^{15}$F

The unbound proton-rich nuclei $^{16}$F and $^{15}$F are investigated experimentally and theoretically. Several experiments using the resonant elastic scattering method were performed at GANIL with radioactive beams to determine the properties of the low lying states of these nuclei. Strong asymmetry between $^{16}$F-$^{16}$N and $^{15}$F-$^{15}$C mirror nuclei is observed. The strength of the $nucleon-nucleon$ effective interaction involving the loosely bound proton in the $s_{1/2}$ orbit is significantly modified with respect to their mirror nuclei $^{16}$N and $^{15}$C. The reduction of the effective interaction is estimated by calculating the interaction energies with a schematic zero-range force. It is found that, after correcting for the effects due to changes in the radial distribution of the single-particle wave functions, the mirror symmetry of the $n-p$ interaction is preserved between $^{16}$F and $^{16}$N, while a difference of 63\% is measured between the $p-p$ versus $n-n$ interactions in the second excited state of $^{15}$F and $^{15}$C nuclei. Several explanations are proposed.

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Charged-particle decays of highly excited states in $^{19}$F

Neutron-capture reactions on $^{18}$F in the helium-burning shell play an important role in the production of $^{15}$N during core-collapse supernovae. The competition between the $^{18}$F($n,p/α$)$^{18}$O/$^{15}$N reactions controls the amount of $^{15}$N produced. The strengths of these reactions depend on the decay branching ratios of states in $^{19}$F above the neutron threshold. We report on an experiment investigating the decay branching ratios of these states in order to better constrain the strengths of the reactions.

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Experimental study of the two-body spin-orbit force

Energies and spectroscopic factors of the first $7/2^-$, $3/2^-$, $1/2^-$ and $5/2^-$ states in the $^{35}$Si$_{21}$ nucleus were determined by means of the (d,p) transfer reaction in inverse kinematics at GANIL using the MUST2 and EXOGAM detectors. By comparing the spectroscopic information on the $^{35}$Si and $^{37}$S isotones, a reduction of the $p_{3/2} - p_{1/2}$ spin-orbit splitting by about 25% is proposed, while the $f_{7/2} -f_{5/2}$ spin-orbit splitting seems to remain constant. These features, derived after having unfolded nuclear correlations using shell model calculations, have been attributed to the properties of the 2-body spin-orbit interaction, the amplitude of which is derived for the first time in an atomic nucleus. The present results, remarkably well reproduced by using several realistic nucleon-nucleon forces, provide a unique touchstone for the modeling of the spin-orbit interaction in atomic nuclei.

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Structure of unbound neutron-rich $^{9}$He studied using single-neutron transfer

The 8He(d,p) reaction was studied in inverse kinematics at 15.4A MeV using the MUST2 Si-CsI array in order to shed light on the level structure of 9He. The well known 16O(d,p)17O reaction, performed here in reverse kinematics, was used as a test to validate the experimental methods. The 9He missing mass spectrum was deduced from the kinetic energies and emission angles of the recoiling protons. Several structures were observed above the neutron-emission threshold and the angular distributions were used to deduce the multipolarity of the transitions. This work confirms that the ground state of 9He is located very close to the neutron threshold of 8He and supports the occurrence of parity inversion in 9He.

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Emergence of the N=16 shell gap in 21O

The spectroscopy of 21O has been investigated using a radioactive 20O beam and the (d,p) reaction in inverse kinematics. The ground and first excited states have been determined to be Jpi=5/2+ and Jpi=1/2+ respectively. Two neutron unbound states were observed at excitation energies of 4.76 +- 0.10 and 6.16 +- 0.11. The spectroscopic factor deduced for the lower of these interpreted as a 3/2+ level, reveals a rather pure 0d3/2 single-particle configuration. The large energy difference between the 3/2+ and 1/2+ states is indicative of the emergence of the N=16 magic number. For the higher lying resonance, which has a character consistent with a spin-parity assignment of 3/2+ or 7/2-, a 71% branching ratio to the first 2+ state in 20O has been observed. The results are compared with new shell model calculations.

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