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J. I. Climente

Publications and source records attributed to J. I. Climente.

11 recordsLinked to original sources

Anisotropy of spin-orbit induced electron spin relaxation in [001] and [111] grown GaAs quantum dots

We report a systematic study of the spin relaxation anisotropy between single electron Zeeman sublevels in cuboidal GaAs quantum dots (QDs). The QDs are subject to an in-plane magnetic field. As the field orientation varies, the relaxation rate oscillates periodically, showing ``magic'' angles where the relaxation rate is suppressed by several orders of magnitude. This behavior is found in QDs with different shapes, heights, crystallographic orientations and external fields. The origin of these angles can be traced back to the symmetries of the spin admixing terms of the Hamiltonian. In [001] grown QDs, the suppression angles are different for Rashba and Dresselhaus spin-orbit terms. By contrast, in [111] grown QDs they are the same, which should facilitate a thorough suppression of spin-orbit induced relaxation. Our results evidence that cubic Dresselhaus terms play a critical role in determining the spin relaxation anisotropy even in quasi-2D QDs.

cond-mat.mes-hall

Effect of interface alloying and band-alignment on the Auger recombination of heteronanocrystals

We report a numerical study of the effect of interface alloying and band-alignment on the Auger recombination processes of core/shell nanocrystals. Numerical calculations are carried out using a two-band Kane Hamiltonian. Smooth interfaces are found to suppress Auger recombination, the strength of the suppression being very sensitive to the core size. The use of type-II structures constitutes an additional source of suppression, especially when the shell confines electrons rather than holes. We show that "magic" sizes leading to negligible Auger recombination [Cragg and Efros, Nano Letters 10 (2010) 313] should be easier to realize experimentally in nanocrystals with extended interface alloying and wide band gap.

cond-mat.mes-hall

Charge control in laterally coupled double quantum dots

We investigate the electronic and optical properties of InAs double quantum dots grown on GaAs (001) and laterally aligned along the [110] crystal direction. The emission spectrum has been investigated as a function of a lateral electric field applied along the quantum dot pair mutual axis. The number of confined electrons can be controlled with the external bias leading to sharp energy shifts which we use to identify the emission from neutral and charged exciton complexes. Quantum tunnelling of these electrons is proposed to explain the reversed ordering of the trion emission lines as compared to that of excitons in our system.

cond-mat.mes-hall

Hole Spin Mixing in InAs Quantum Dot Molecules

Holes confined in single InAs quantum dots have recently emerged as a promising system for the storage or manipulation of quantum information. These holes are often assumed to have only heavy-hole character and further assumed to have no mixing between orthogonal heavy hole spin projections (in the absence of a transverse magnetic field). The same assumption has been applied to InAs quantum dot molecules formed by two stacked InAs quantum dots that are coupled by coherent tunneling of the hole between the two dots. We present experimental evidence of the existence of a hole spin mixing term obtained with magneto-photoluminescence spectroscopy on such InAs quantum dot molecules. We use a Luttinger spinor model to explain the physical origin of this hole spin mixing term: misalignment of the dots along the stacking direction breaks the angular symmetry and allows mixing through the light-hole component of the spinor. We discuss how this novel spin mixing mechanism may offer new spin manipulation opportunities that are unique to holes.

cond-mat.mtrl-sci

Antibonding ground states in semiconductor artificial molecules

The spin-orbit interaction is a crucial element of many semiconductor spintronic technologies. Here we report the first experimental observation, by magneto-optical spectroscopy, of a remarkable consequence of the spin-orbit interaction for holes confined in the molecular states of coupled quantum dots. As the thickness of the barrier separating two coupled quantum dots is increased, the molecular ground state changes character from a bonding orbital to an antibonding orbital. This result is counterintuitive, and antibonding molecular ground states are never observed in natural diatomic molecules. We explain the origin of the reversal using a four band k.p model that has been validated by numerical calculations that account for strain. The discovery of antibonding molecular ground states provides new opportunities for the design of artificially structured materials with complex molecular properties that cannot be achieved in natural systems.

cond-mat.mtrl-sci

Electron states in quantum rings with defects under axial or in-plane magnetic fields

A comprehensive study of anisotropic quantum rings, QRs, subject to axial and in-plane magnetic field, both aligned and transverse to the anisotropy direction, is carried out. Elliptical QRs for a wide range of eccentricity values and also perfectly circular QRs including one or more barriers disturbing persistent QR current are considered. These models mimic anisotropic geometry deformations and mass diffusion occuring in the QR fabrication process. Symmetry considerations and simplified analytical models supply physical insight into the obtained numerical results. Our study demonstrates that, except for unusual extremely large eccentricities, QR geometry deformations only appreciably influence a few low-lying states, while the effect of barriers disturbing the QR persistent current is stronger and affects all studied states to a similar extent. We also show that the response of the electron states to in-plane magnetic fields provides accurate information on the structural anisotropy.

cond-mat.mes-hall

Electronic states of laterally coupled quantum rings

The conduction band electron states of laterally-coupled semiconductor quantum rings are studied within the frame of the effective mass envelope function theory. We consider the effect of axial and in-plane magnetic fields for several inter-ring distances, and find strong changes in the energy spectrum depending on the coupling regime. Our results indicate that the magnetic response accurately monitors the quantum ring molecule dissociation process. Moreover, the anisotropic response of the electron states to in-plane magnetic fields provides information on the orientation of the quantum ring molecule.

cond-mat.mes-hall

Phonon-induced electron relaxation in weakly-confined single and coupled quantum dots

We investigate charge relaxation rates due to acoustic phonons in weakly-confined quantum dot systems, including both deformation potential and piezoelectric field interactions. Single-electron excited states lifetimes are calculated for single and coupled quantum dot structures, both in homonuclear and heteronuclear devices. Piezoelectric field scattering is shown to be the dominant relaxation mechanism in many experimentally relevant situations. On the other hand, we show that appropriate structure design allows to minimize separately deformation potential and piezolectric field interactions, and may bring electron lifetimes in the range of microseconds.

cond-mat.mes-hall

Electronic structure of few-electron concentric double quantum rings

The ground state structure of few-electron concentric double quantum rings is investigated within the local spin density approximation. Signatures of inter-ring coupling in the addition energy spectrum are identified and discussed. We show that the electronic configurations in these structures can be greatly modulated by the inter-ring distance: At short and long distances the low-lying electron states localize in the inner and outer rings, respectively, and the energy structure is essentially that of an isolated single quantum ring. However, at intermediate distances the electron states localized in the inner and the outer ring become quasi-degenerate and a rather entangled, strongly-correlated system is formed.

cond-mat.mes-hall

Magnetic field dependence of hole levels in self-assembled InAs quantum dots

Recent magneto-transport experiments of holes in InGaAs quantum dots [D. Reuter, P. Kailuweit, A.D. Wieck, U. Zeitler, O. Wibbelhoff, C. Meier, A. Lorke, and J.C. Maan, Phys. Rev. Lett. 94, 026808 (2005)] are interpreted by employing a multi-band kp Hamiltonian, which considers the interaction between heavy hole and light hole subbands explicitely. No need of invoking an incomplete energy shell filling is required within this model. The crucial role we ascribe to the heavy hole-light hole interaction is further supported by one-band local-spin-density functional calculations, which show that Coulomb interactions do not induce any incomplete hole shell filling and therefore cannot account for the experimental magnetic field dispersion.

cond-mat.mes-hall

Aharonov-Bohm effect for pedestrian

When a magnetic field pierces a multiple-connected quantum system, the corresponding wavefunction is altered although no net Lorentz force acts upon its carriers. This is the so called Aharonov-Bohm effect. The most simple multiply-connected quantum system is a quantum ring QR. Nowadays it is possible to obtain QRs in the nanoscopic range providing spectroscopic data vs. and applied external magnetic field. We describe here the most significant quantum effects induced by the magnetic field in a QR by means of simple quantum mechanical models.

cond-mat.mes-hall