arXiv subjects
Publications and source records attributed to J. J. Alonso.
This is the reply to a Comment by I.S.Tupitsyn and P.C.E. Stamp (PRL v92,119701 (2004)) on a letter of ours (J.F.Fernandez and J.J.Alonso, PRL v91, 047202 (2003)).
Can magnetic interactions between single-molecule magnets (SMMs) in a crystal establish long-range magnetic order at low temperatures deep in the quantum regime, where the only electron spin-fluctuations are due to incoherent magnetic quantum tunneling (MQT)? Put inversely: can MQT provide the temperature dependent fluctuations needed to destroy the ordered state above some finite Tc, although it should basically itself be a T-independent process? Our experiments on two novel Mn4 SMMs provide a positive answer to the above, showing at the same time that MQT in the SMMs has to involve spin-lattice coupling at a relaxation rate equaling that predicted and observed recently for nuclear spin-mediated quantum relaxation.
We model magnetization processes that take place through tunneling in crystals of single-molecule magnets, such as Mn_12 and Fe_8. These processes take place when a field H is applied after quenching to very low temperatures. Magnetic dipolar interactions and spin flipping rules are essential ingredients of the model. The results obtained follow from Monte Carlo simulations and from the stochastic model we propose for dipole field diffusion. Correlations established before quenching are shown to later drive the magnetization process. We also show that in simple cubic lattices, m \propto sqrt(t) at time t after H is applied, as observed in Fe_8, but only for 1+2\log_10(h_d/h_w) time decades, where h_d is some near-neighbor magnetic dipolar field and a spin reversal can occur only if the magnetic field acting on it is within some field window (-h_w,h_w). However, the sqrt(t) behavior is not universal. For BCC and FCC lattices, m \propto t^p, but p \simeq 0.7 . An expression for p in terms of lattice parameters is derived. At later times the magnetization levels off to a constant value. All these processes take place at approximately constant magnetic energy if the annealing energy epsilon_a is larger than the tunneling window's energy width (i.e., if epsilon_a \gtrsim gμ_B h_w S). Thermal processes come in only later on to drive further magnetization growth.
We report results from Monte Carlo simulations of systems of magnetic dipoles that relax through quantum tunneling, much as Fe_8 crystals at very low temperature.For short times, a hole develops in suitably defined magnetic field pseudo--distributions, which matches the shape of the tunnel window (TW). Much later, ordinary field distributions P(h) develop similar holes if thermal energies are not much larger than the TW's energy. Still later, below the long--range ordering (LRO) temperature, P(h) exhibits the signature of LRO.
We show that correlations established before quenching to very low temperatures, later drive the magnetization process of systems of single molecule magnets, after a magnetic field is applied at t=0. We also show that in SC lattices, m \propto sqrt(t), as observed in Fe_8, but only for 1+2*log_10(h_d/h_w) time decades, where h_d is a nearest neighbor dipolar magnetic field and a spin reversal can occur only if the field on it is within (-h_w,h_w). However, the sqrt(t) behavior is not universal. For BCC and FCC lattices, m \propto t^p, but p \simeq 0.7. The value to which m finally levels off is also given.
We study Ising systems of spins with dipolar interactions. We find a simple approximate relation for the interaction energy between pairs of parallel lattice columns of spins running along the Ising spin direction. This relation provides insight into the relation between lattice geometry and the nature of the ordered state. It can be used to calculate ground state energies. We have also obtained ground state energies and ordering temperatures T_0 from Monte Carlo simulations. Simple empirical relations, that give T_0 for simple and body centered tetragonal lattices in terms of lattice parameters are also established. Finally, the nature of the ordered state and T_0 are determined for Fe_8 clusters, which crystallize on a triclinic lattice.
Reply to comment appeared on hep-lat/9912014.
We analyze the percolation properties of certain clusters defined on configurations of the 2--dimensional Heisenberg model. We find that, given any direction \vec{n} in O(3) space, the spins almost perpendicular to \vec{n} form a percolating cluster. This result gives indications of how the model can avoid a previously conjectured Kosterlitz-Thouless phase transition at finite temperature T.
Evidence for the existence of van der Waals loops in pressure p versus volume v plots has for some time supported the belief that melting in two dimensions is a first order phase transition. We report rather accurate equilibrium p(v) curves for systems of hard disks obtained from long Monte Carlo simulations. These curves, obtained in the constant volume ensemble, using periodic boundary conditions, exhibit well defined van der Waals loops. We illustrate their existence for finite systems that are known to undergo a continuous transition in the thermodynamic limit. To this end, we obtain magnetization m versus applied field curves from Monte Carlo simulations of the 2D Ising model, in the constant m ensemble, at the critical point. Whether van der Waals loops for disk systems behave in the thermodynamic limit as they do for the 2D Ising model at the critical point cannot be ruled out. Thus, the often made claim that melting in 2D is a first order phase transition, based on the evidence that van der Waals loops exist, is not sound.
We study the shape of the tail of a heap of granular material. A simple theoretical argument shows that the tail adds a logarithmic correction to the slope given by the angle of repose. This expression is in good agreement with experiments. We present a cellular automaton that contains gravity, dissipation and surface roughness and its simulation also gives the predicted shape.