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J. Jolie

Publications and source records attributed to J. Jolie.

At least 19 recordsLinked to original sources

Lifetime measurements in neutron-rich odd-A yttrium isotopes ($^{93-99}$Y): Investigation of shape coexistence and the intertwined quantum phase transition

Lifetimes of 16 excited states in the neutron-rich odd-$A$ nuclei $^{93-99}$Y were measured using fast-timing $\gamma$-$\gamma$ coincidence spectroscopy with fast scintillation detectors at the LOHENGRIN recoil separator. Particular attention is given to the region around $N \approx 59$, where rapid changes in nuclear deformation and shape coexistence occur. The lifetimes, determined using the generalized centroid difference method, are compared with interacting boson-fermion model calculations with configuration mixing, in which the odd-$A$ yttrium isotopes are described as a proton coupled to a bosonic core containing normal and intruder configurations. The results provide new constraints on theoretical descriptions of shape coexistence and structural evolution in neutron-rich nuclei near $A \approx 100$, particularly for odd-$A$ systems where experimental information remains limited.

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Multiple shape coexistence near Sn118: First 03+ lifetime measurement

The intruder bands in Sn isotopes, built on the 2p-2h excitation across the $Z = 50$ proton shell gap, are well-known examples of shape coexistence near the neutron mid-shell region. Spectroscopic signatures for shape coexistence include enhanced $E0$ transitions between the $0^+$ band heads. However, the underlying shape coexistence and mixing has been unclear because lifetime information for the excited $0^+$ states was incomplete in $^{118}$Sn. We thus present here the first measurement of the $0^+_3$ lifetime in $^{118}$Sn using the fast-timing technique following thermal-neutron capture. The observed enhancement in $\rho^2(E0; 0^+_3 \rightarrow 0^+_2)$ of 150(30) milliunits provides compelling indications for multiple shape coexistence in $^{118}$Sn. Additionally, three distinct shapes in $^{116,118,120}$Sn naturally emerged in theoretical calculations based on the quantum-number-projected generator coordinate method employing a relativistic energy density functional.

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Lifetime of the $4^+_1$ state of $^{132}$Te

The evolution of the collectivity of tellurium isotopes from mid-shell towards $N=82$ is currently based mainly on properties of the first excited $2^+$ states. To extend structural information in this isotopic chain, in particular with respect to the balance of microscopic, seniority-type and collective excitations, electric quadrupole transition strengths from $4^+$ states need to be considered. An experiment was performed to determine the $4_1^+$ lifetime of $^{132}$Te via the recoil-distance Doppler-shift method at the University of Cologne tandem accelerator. The isotope of interest was populated in the two neutron-transfer reaction $^{130}$Te($^{18}$O,$^{16}$O)$^{132}$Te$^*$. The $E2$ decay transition strength has been determined to be $B(E2; 4^+_1\rightarrow 2^+_1) = 9.3(10)\, \text{W.u.}$ and compares favourably to shell model calculations.

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Evidence for shape coexistence in $^{120}$Sn from the first $0^+_3$ lifetime measurement

The lifetime of the $0^+_3$ state in $^{120}$Sn was measured for the first time applying the fast-timing technique following thermal neutron capture. The mean lifetime of $τ= 50(7)$~ps leads to a $E0$ transition strength of $10^3\times ρ^2(E0;0^+_3\rightarrow0^+_2) = 120(50)$, suggesting shape coexistence and a high degree of mixing between the $0^+_2$ and $0^+_3$ states. With the newly measured lifetime, the $B(E2;0^+_3\rightarrow 2^+_1)$ value is 0.50(7)~W.u., which reveals that the $ρ^2(E0;0^+_3\rightarrow0^+_1)$ increases by a factor of $\approx 3.4$ from $^{116}$Sn to $^{120}$Sn.

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Revised $B(E2; 2^{+}_{1} \rightarrow 0^{+}_{1})$ value in the semi-magic nucleus $^{210}$Pb

The lifetime of the $2^+_1$ state of $^{210}$Pb was measured in the $^{208}$Pb($^{18}$O, $^{16}$O)$^{210}$Pb two-neutron transfer reaction by $\gamma$-ray spectroscopy employing the recoil-distance Doppler-shift method. The extracted absolute $B(E2)$$\downarrow$ value of ${119\;^{+\;9}_{-\;8}\;\hspace{-0pt}\,\text{e}^2\text{fm}^4}$ is consistent with previously reported measurements, but with significantly improved precision. The available experimental data for the $2^+_1$-$4^+_1$-$6^+_1$-$8^+_1$ multiplet are compared with shell-model calculations based on the well-established Kuo-Herling interaction. The new $B(E2)$$\downarrow$ value agrees well with the shell-model prediction, providing evidence that the properties of the $2^+_1$ and $8^+_1$ states of $^{210}$Pb can be consistently described together within the nuclear shell-model framework.

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Revealing the nature of yrast states in neutron-rich polonium isotopes

Polonium isotopes having two protons above the shell closure at $Z=82$ show a wide variety of low-lying high-spin isomeric states across the whole chain. The structure of neutron-deficient isotopes up to $^{210}$Po ($N=126$) is well established as they are easily produced through various methods. However, there is not much information available for the neutron-rich counterparts for which only selective techniques can be used for their production. We report on the first fast-timing measurements of yrast states up to the 8$^+$ level in $^{214,216,218}$Po isotopes produced in the $β^-$ decay of $^{214,216,218}$Bi at ISOLDE, CERN. In particular, our new half-life value of 607(14) ps for the 8$_1^+$ state in $^{214}$Po is nearly 20 times shorter than the one available in literature and comparable with the newly measured half-lives of 409(16) and 628(25) ps for the corresponding 8$_1^+$ states in $^{216,218}$Po, respectively. The measured $B(E2;8_1^+ \to 6_1^+)$ transition probability values follow an increasing trend relative to isotope mass, reaching a maximum for $^{216}$Po. The increase contradicts the previous claims of isomerism for the $8^+$ yrast states in neutron-rich $^{214}$Po and beyond. Together with the other measured yrast transitions, the $B(E2)$ values provide a crucial test of the different theoretical approaches describing the underlying configurations of the yrast band. The new experimental results are compared to shell-model calculations using the KHPE and H208 effective interactions and their pairing modified versions, showing an increase in configuration mixing when moving towards the heavier isotopes.

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Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $γγ$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $γγ$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $γγ$-coincidence and $γ$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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Investigating timing properties of modern digitizers utilizing interpolating CFD algorithms and the application to digital fast-timing lifetime measurement

The performance of two implementations of digital real-time interpolating constant fraction discriminator algorithms with respect to fast-timing lifetime measurements are investigated. The implementations integrated in two different digitizers were evaluated in terms of the effects of tuning parameters of the digital CFDs and the influence of different input amplitudes on the time resolution and time walk characteristics. Reference is made to the existing analog standard of fast-timing techniques. The study shows, that the timing performance of both modules is comparable to established fast-timing setups using analog constant fraction discriminators, but with the added benefit of digital processing. Both digitizer modules were found to be highly effective and user-friendly instruments for modern fast-timing requirements.

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Tests of collectivity in $^{98}$Zr by absolute transition rates

Lifetimes of low-spin excited states in $^{98}$Zr were measured using the recoil-distance Doppler-shift technique and the Doppler-shift attenuation method. The nucleus of interest was populated in a $^{96}$Zr($^{18}$O,$^{16}$O)$^{98}$Zr two-neutron transfer reaction at the Cologne FN Tandem accelerator. Lifetimes of six low-spin excited states, of which four are unknown, were measured. The deduced $B(E2)$ values were compared with Monte Carlo shell model and interacting boson model with configuration mixing calculations. Both approaches reproduce well most of the data but leave challenging questions regarding the structure of some low lying states.

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Detailed spectroscopy of doubly magic $^{132}$Sn

The structure of the doubly magic $^{132}_{50}$Sn$_{82}$ has been investigated at the ISOLDE facility at CERN, populated both by the $β^-$decay of $^{132}$In and $β^-$-delayed neutron emission of $^{133}$In. The level scheme of $^{132}$Sn is greatly expanded with the addition of 68 $γ$-transitions and 17 levels observed for the first time in the $β$ decay. The information on the excited structure is completed by new $γ$-transitions and states populated in the $β$-n decay of $^{133}$In. Improved delayed neutron emission probabilities are obtained both for $^{132}$In and $^{133}$In. Level lifetimes are measured via the Advanced Time-Delayed $βγγ$(t) fast-timing method. An interpretation of the level structure is given based on the experimental findings and the particle-hole configurations arising from core excitations both from the \textit{N} = 82 and \textit{Z} = 50 shells, leading to positive and negative parity particle-hole multiplets. The experimental information provides new data to challenge the theoretical description of $^{132}$Sn.

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Fast-timing study of $^{81}$Ga from the $β$ decay of $^{81}$Zn

The $β^{-}$ decay of $^{81}$Zn to the neutron magic $N=50$ nucleus $^{81}$Ga, with only three valence protons with respect to $^{78}$Ni, was investigated. The study was performed at the ISOLDE facility at CERN by means of $γ$ spectroscopy. The $^{81}$Zn half-life was determined to be $T_{1/2}=290(4)$ ms while the $β$-delayed neutron emission probability was measured as $P_n=23(4)\%$. The analysis of the $β$-gated $γ$-ray singles and $γ$-$γ$ coincidences from the decay of $^{81}$Zn provides 47 new levels and 70 new transitions in $^{81}$Ga. The $β^-$$n$ decay of $^{81}$Zn was observed and a new decay scheme into the odd-odd $^{80}$Ga nucleus was established. The half-lives of the first and second excited states of $^{81}$Ga were measured via the fast-timing method using LaBr$_3$(Ce) detectors. The level scheme and transition rates are compared to large-scale shell-model calculations. The low-lying structure of $^{81}$Ga is interpreted in terms of the coupling of the three valence protons outside the doubly-magic $^{78}$Ni core.

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Structure of even-even Cadmium isotopes from the beyond-mean-field interacting boson model

The structure of even-even $^{108-116}$Cd isotopes is investigated based on the self-consistent mean-field approach. By mapping the quadrupole-$(β,γ)$ deformation energy surface, obtained from the constrained self-consistent mean-field calculations with a choice of the Skyrme force and pairing property, onto the Hamiltonian of the interacting boson model with configuration mixing, the strength parameters of the Hamiltonian are determined. The low-lying excitation spectra and electric quadrupole transition rates for the considered Cd nuclei are computed by the resultant Hamiltonian, and are compared in detail with the experimental data. Our semi-microscopic prediction identifies several intruder states as suggested empirically, and overall, provides a reasonable qualitative description of the experimental energy levels and transition rates.

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A revised $B(E2; 2^+_1 \to 0^+_1)$ value in the semi-magic nucleus $^{210}$Po

The lifetimes of the $2^+_1$, the $2^+_2$ and the $3^-_1$ states of $^{210}$Po have been measured in the $^{208}$Pb($^{12}$C,$^{10}$Be)$^{210}$Po transfer reaction by the Doppler-shift attenuation method. The results for the lifetime of the $2^+_1$ state is about three times shorter than the adopted value. However, the new value still does not allow for consistent description of the properties of the yrast $2^+_1$, $4^+_1$, $6^+_1$, and $8^+_1$ states of $^{210}$Po in the framework of nuclear shell models. The Quasi-particle Phonon Model (QPM) calculations also cannot overcome this problem thus indicating the existence of a peculiarity which is neglected in both theoretical approaches.

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Shell model based deformation analysis of light Cadmium isotopes

Large-scale shell-model calculations for the even-even Cadmium isotopes 98 Cd - 108 Cd have been performed with the ANTOINE code in the π(2p 1/2 ; 1g 9/2 ) ν(2d 5/2 ; 3s 1/2 ; 2d 3/2 ; 1g 7/2 ; 1h 11/2 ) model space without further truncation. Known experimental energy levels and B(E2) values could be well reproduced. Taking these calculations as a starting ground we analyze the deformation parameters predicted for the Cd isotopes as a function of neutron number N and spin J using the methods of model independent invariants introduced by K. Kumar and D. Cline.

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The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus 133Sb

The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

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Partial dynamical symmetry in Bose-Fermi systems

We generalize the notion of partial dynamical symmetry (PDS) to a system of interacting bosons and fermions. In a PDS, selected states of the Hamiltonian are solvable and preserve the symmetry exactly, while other states are mixed. As a first example of such novel symmetry construction, spectral features of the odd-mass nucleus $^{195}$Pt are analyzed.

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Evolution of E2 transition strength in deformed hafnium isotopes from new measurements on $^{172}$Hf, $^{174}$Hf, and $^{176}$Hf

The available data for E2 transition strengths in the region between neutron-deficient Hf and Pt isotopes are far from complete. More and precise data are needed to enhance the picture of structure evolution in this region and to test state-of-the-art nuclear models. In a simple model, the maximum collectivity is expected at the middle of the major shell. However, for actual nuclei, this picture may no longer be the case, and one should use a more realistic nuclear-structure model. We address this point by studying the spectroscopy of Hf. We remeasure the 2^+_1 half-lives of 172,174,176Hf, for which there is some disagreement in the literature. The main goal is to measure, for the first time, the half-lives of higher-lying states of the rotational band. The new results are compared to a theoretical calculation for absolute transition strengths. The half-lives were measured using γ-γand conversion-electron-γdelayed coincidences with the fast timing method. For the determination of half-lives in the picosecond region, the generalized centroid difference method was applied. For the theoretical calculation of the spectroscopic properties, the interacting boson model is employed, whose Hamiltonian is determined based on microscopic energy-density functional calculations. The measured 2^+_1 half-lives disagree with results from earlier γ-γfast timing measurements, but are in agreement with data from Coulomb excitation experiments and other methods. Half-lives of the 4^+_1 and 6^+_1 states were measured, as well as a lower limit for the 8^+_1 states. We show the importance of the mass-dependence of effective boson charge in the description of E2 transition rates in chains of nuclei. It encourages further studies of the microscopic origin of this mass dependence. New data on transition rates in nuclei from neighboring isotopic chains could support these studies.

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Evidence for shape coexistence in $^{98}$Mo

A $γγ$ angular correlation experiment has been performed to investigate the low-energy states of the nucleus $^{98}$Mo. The new data, including spin assignments, multipole mixing ratios and lifetimes reveal evidence for shape coexistence and mixing in $^{98}$Mo, arising from a proton intruder configuration. This result is reproduced by a theoretical calculation within the proton-neutron interacting boson model with configuration mixing, based on microscopic energy density functional theory. The microscopic calculation indicates the importance of the proton particle-hole excitation across the Z=40 sub-shell closure and the subsequent mixing between spherical vibrational and the $γ$-soft equilibrium shapes in $^{98}$Mo.

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