arXiv subjects

J. K. Freericks

Publications and source records attributed to J. K. Freericks.

At least 73 records · Page 4Linked to original sources

arXiv2016

Theoretical description of pump/probe experiments in electron mediated charge-density-wave insulators

In this review, we develop the formalism employed to describe charge-density-wave insulators in pump/probe experiments using ultra short driving pulses of light. The theory emphasizes exact results in the simplest model for a charge-density wave insulator (given by a noninteracting systems with two bands and a gap) and by employing nonequilibrium dynamical mean-field theory to solve the Falicov-Kimball model in its ordered phase. We show both how to develop the formalism and how the solutions behave. Care is taken to describe the details behind these calculations and to show how to verify their accuracy via sum-rule constraints.

cond-mat.str-el↗

arXiv2016

Review of the theoretical description of time-resolved angle-resolved photoemission spectroscopy in electron-phonon mediated superconductors

We review recent work on the theory for pump/probe photoemission spectroscopy of electron-phonon mediated superconductors in both the normal and the superconducting states. We describe the formal developments that allow one to solve the Migdal-Eliashberg theory in nonequilibrium for an ultrashort laser pumping field, and explore the solutions which illustrate the relaxation as energy is transferred from electrons to phonons. We focus on exact results emanating from sum rules and approximate numerical results which describe rules of thumb for relaxation processes. In addition, in the superconducting state, we describe how Higg's oscillations can be excited due to the nonlinear coupling with the electric field and how pumping the system can enhance superconductivity.

cond-mat.supr-con↗

arXiv2016

Time-domain pumping a quantum-critical charge-density-wave-ordered material

We determine the exact time-resolved photoemission spectroscopy for a nesting driven charge-density-wave (described by the spinless Falicov-Kimball model within dynamical mean-field theory). The pump-probe experiment involves two light pulses: the first is an ultrashort intense pump pulse that excites the system into nonequilibrium, and the second is a lower amplitude higher frequency probe pulse that photoexcites electrons. We examine three different cases: the strongly correlated metal, the quantum-critical charge density wave and the critical Mott insulator. Our results show that the quantum critical charge density wave has an ultra efficient relaxation channel that allows electrons to be de-excited during the pump pulse, resulting in little net excitation. In contrast, the metal and the Mott insulator show excitations that are closer to what one expects from these systems. In addition, the pump field produces spectral band narrowing, peak sharpening, and a spectral gap reduction, all of which rapidly return to their field free values after the pump is over.

cond-mat.str-el↗

arXiv2016

Generalized gradient expansion for inhomogeneous dynamical mean-field theory: Application to ultracold atoms in a harmonic trap

We develop a generalized gradient expansion of the inhomogeneous dynamical mean-field theory method for determining properties of ultracold atoms in a trap. This approach goes beyond the well-known local density approximation and at higher temperatures, in the normal phase, it shows why the local density approximation works so well, since the local density and generalized gradient approximations are essentially indistinguishable from each other (and from the exact solution within full inhomogeneous dynamical mean-field theory). But because the generalized gradient expansion only involves nearest-neighbor corrections, it does not work as well at low temperatures, when the systems enter into ordered phases. This is primarily due to the problem that ordered phases often satisfy some global constraints which determine the spatial ordering pattern, and the local density and generalized gradient approximations are not able to impose those kinds of constraints; they also overestimate the tendency to order. The theory is applied to phase separation of different mass fermionic mixtures represented by the Falicov-Kimball model and to determining the entropy per particle of a fermionic system represented by the Hubbard model. The generalized gradient approximation is a useful diagnostic for the accuracy of the local density approximation---when both methods agree, they are likely accurate, when they disagree, neither is likely to be correct.

cond-mat.quant-gas↗

arXiv2016

Energy dissipation in the time domain governed by bosons in a correlated material

In complex materials various interactions play important roles in determining the material properties. Angle Resolved Photoelectron Spectroscopy (ARPES) has been used to study these processes by resolving the complex single particle self energy $Σ(E)$ and quantifying how quantum interactions modify bare electronic states. However, ambiguities in the measurement of the real part of the self energy and an intrinsic inability to disentangle various contributions to the imaginary part of the self energy often leave the implications of such measurements open to debate. Here we employ a combined theoretical and experimental treatment of femtosecond time-resolved ARPES (tr-ARPES) and show how measuring the population dynamics using tr-ARPES can be used to separate electron-boson interactions from electron-electron interactions. We demonstrate the analysis of a well-defined electron-boson interaction in the unoccupied spectrum of the cuprate Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ characterized by an excited population decay time constant $τ_{QP}$ that maps directly to a discrete component of the equilibrium self energy not readily isolated by static ARPES experiments.

cond-mat.str-el↗

arXiv2016

Direct observation of Higgs mode oscillations in the pump-probe photoemission spectra of electron-phonon mediated superconductors

Using the non-equilibrium Keldysh formalism, we solve the equations of motion for electron-phonon superconductivity, including an ultrafast pump field. We present results for time-dependent photoemission spectra out of equilibrium which probes the dynamics of the superconducting gap edge. The partial melting of the order by the pump field leads to oscillations at twice the melted gap frequency, a hallmark of the Higgs or amplitude mode. Thus the Higgs mode can be directly excited through the nonlinear effects of an electromagnetic field and detected without any additional symmetry breaking.

cond-mat.supr-con↗

arXiv2015

Measuring nonequilibrium retarded spin-spin Green's functions in an ion-trap based quantum simulator

Recent work proposed a variant on Ramsey interferometry for coupled spin-$1/2$ systems that directly measures the retarded spin-spin Green's function. We expand on that work by investigating nonequilibrium retarded spin-spin Green's functions within the transverse-field Ising model. We derive the lowest four spectral moments to understand the short-time behavior and we employ a Lehmann-like representation to determine the spectral behavior. We simulate a Ramsey protocol for a nonequilibrium quantum spin system that consists of a coherent superposition of the ground state and diabatically excited higher-energy states via a temporally ramped transverse magnetic field. We then apply the Ramsey spectroscopy protocol to the final Hamiltonian, which has a constant transverse field. The short-time behavior directly relates to Lieb-Robinson bounds for the transport of many-body correlations, while the long-time behavior relates to the excitation spectra of the Hamiltonian. Compressive sensing is employed in the data analysis to efficiently extract that spectra.

quant-ph↗

arXiv2015

Bang-bang shortcut to adiabaticity in trapped ion quantum simulators

We model the bang-bang optimization protocol as a shortcut to adiabaticity in the ground-state preparation of an ion-trap-based quantum simulator. Compared to a locally adiabatic evolution, the bang-bang protocol produces a somewhat lower ground-state probability, but its implementation is so much simpler than the locally adiabatic approach, that it remains an excellent choice to use for maximizing ground-state preparation in systems that cannot be solved with conventional computers. We describe how one can optimize the shortcut and provide specific details for how it can be implemented with current ion-trap-based quantum simulators.

quant-ph↗

arXiv2015

Nonequilibrium response of an electron mediated charge-density-wave-ordered material to a large dc electric field

Using the Kadanoff-Baym-Keldysh formalism, we employ nonequilibrium dynamical mean-field theory to exactly solve for the nonlinear response of an electron-mediated charge-density-wave-ordered material. We examine both the dc current and the order parameter of the conduction electrons as the ordered system is driven by the electric field. Although the formalism we develop applies to all models, for concreteness, we examine the charge-density-wave phase of the Falicov-Kimball model, which displays a number of anomalous behaviors including the appearance of subgap density of states as the temperature increases. These subgap states should have a significant impact on transport properties, particularly the nonlinear response of the system to a large dc electric field.

cond-mat.str-el↗

arXiv2015

Creating thermal distributions from diabatic excitations in ion-trap-based quantum simulation

The goal of adiabatic ground-state preparation is to start a simple quantum system in its ground state and adiabatically evolve the Hamiltonian to a complex one, maintaining the ground state throughout the evolution. In ion-trap-based quantum simulations, coherence times are too short to allow for adiabatic evolution for large chains, so the system evolves diabatically, creating excitations to higher energy states. Because the probability for diabatic excitation depends exponentially on the excitation energy and because the thermal distribution also depends exponentially on the excitation energy, we investigate whether the diabatic excitation can create a thermal distribution; as this could serve as an alternative for creating thermal states of complex quantum systems without requiring contact with a heat bath. In this work, we explore this relationship and determine situations where diabatic excitation can approximately create such a thermal state.

quant-ph↗

arXiv2015

Anomalous longitudinal relaxation of nuclear spins in CaF$_2$

We consider the effect of non-secular resonances for interacting nuclear spins in solids which were predicted theoretically to exist in the presence of strong static and strong radio-frequency magnetic fields. These resonances imply corrections to the standard secular approximation for the nuclear spin-spin interaction in solids, which, in turn, should lead to an anomalous longitudinal relaxation in nuclear magnetic resonance experiments. In this article, we investigate the feasibility of the experimental observation of this anomalous longitudinal relaxation in calcium fluoride (CaF$_2$) and conclude that such an observation is realistic.

cond-mat.mes-hall↗

arXiv2015

Exact calculation of phonon effects on spin squeezing

Theoretical models of spins coupled to bosons provide a simple setting for studying a broad range of important phenomena in many-body physics, from virtually mediated interactions to decoherence and thermalization. In many atomic, molecular, and optical systems, such models also underlie the most successful attempts to engineer strong, long-ranged interactions for the purpose of entanglement generation. Especially when the coupling between the spins and bosons is strong---such that it cannot be treated perturbatively---the properties of such models are extremely challenging to calculate theoretically. Here, exact analytical expressions for nonequilibrium spin-spin correlation functions are derived for a specific model of spins coupled to bosons. The spatial structure of the coupling between spins and bosons is completely arbitrary, and thus the solution can be applied to systems in any number of dimensions. The explicit and nonperturbative inclusion of the bosons enables the study of entanglement generation (in the form of spin squeezing) even when the bosons are driven strongly and near-resonantly, and thus provides a quantitative view of the breakdown of adiabatic elimination that inevitably occurs as one pushes towards the fastest entanglement generation possible. The solution also helps elucidate the effect of finite temperature on spin squeezing. The model considered is relevant to a variety of atomic, molecular, and optical systems, such as atoms in cavities or trapped ions. As an explicit example, the results are used to quantify phonon effects in trapped ion quantum simulators, which are expected to become increasingly important as these experiments push towards larger numbers of ions.

cond-mat.quant-gas↗

arXiv2015

Determining the ground-state probability of a quantum simulation with product-state measurements

One of the goals in quantum simulation is to adiabatically generate the ground state of a complicated Hamiltonian by starting with the ground state of a simple Hamiltonian and slowly evolving the system to the complicated one. If the evolution is adiabatic and the initial and final ground states are connected due to having the same symmetry, then the simulation will be successful. But in most experiments, adiabatic simulation is not possible because it would take too long, and the system has some level of diabatic excitation. In this work, we quantify the extent of the diabatic excitation even if we do not know {\it a priori} what the complicated ground state is. Since many quantum simulator platforms, like trapped ions, can measure the probabilities to be in a product state, we describe techniques that can employ these measurements to estimate the probability of being in the ground state of the system after the diabatic evolution. These techniques do not require one to know any properties about the Hamiltonian itself, nor to calculate its eigenstate properties. All the information is derived by analyzing the product-state measurements as functions of time.

quant-ph↗

arXiv2015

Theoretical basis for quantum simulation with a planar ionic crystal in a Penning trap using a triangular rotating wall

One of the challenges with quantum simulation in ion traps is that the effective spin-spin exchange couplings are not uniform across the lattice. This can be particularly important in Penning trap realizations where the presence of an ellipsoidal boundary at the edge of the trap leads to dislocations in the crystal. By adding an additional anharmonic potential to better control interion spacing, and a triangular shaped rotating wall potential to reduce the appearance of dislocations, one can achieve better uniformity of the ionic positions. In this work, we calculate the axial phonon frequencies and the spin-spin interactions driven by a spin-dependent optical dipole force, and discuss what effects the more uniform ion spacing has on the spin simulation properties of Penning trap quantum simulators. Indeed, we find the spin-spin interactions behave more like a power law for a wide range of parameters.

quant-ph↗

arXiv2015

Nonequilibrium dynamical mean-field theory for the charge-density-wave phase of the Falicov-Kimball model

Nonequilibrium dynamical mean-field theory (DMFT) is developed for the case of the charge-density-wave ordered phase. We consider the spinless Falicov-Kimball model which can be solved exactly. This strongly correlated system is then placed in an uniform external dc electric field. We present a complete derivation for nonequilibrium dynamical mean-field theory Green's functions defined on the Keldysh-Schwinger time contour. We also discuss numerical issues involved in solving the coupled equations.

cond-mat.str-el↗

arXiv2014

The Nonequilibrium Many-Body Problem as a paradigm for extreme data science

Generating big data pervades much of physics. But some problems, which we call extreme data problems, are too large to be treated within big data science. The nonequilibrium quantum many-body problem on a lattice is just such a problem, where the Hilbert space grows exponentially with system size and rapidly becomes too large to fit on any computer (and can be effectively thought of as an infinite-sized data set). Nevertheless, much progress has been made with computational methods on this problem, which serve as a paradigm for how one can approach and attack extreme data problems. In addition, viewing these physics problems from a computer-science perspective leads to new approaches that can be tried to solve them more accurately and for longer times. We review a number of these different ideas here.

cond-mat.str-el↗

arXiv2014

Theory of pump-probe photoemission in graphene: Ultrafast tuning of Floquet bands and local pseudospin textures

The control of physical properties of solids with short laser pulses is an intriguing prospect of ultrafast materials science. Continuous-wave high-frequency laser driving with circular polarization was predicted to induce a light-matter coupled new state possessing a quasi-static band structure with an energy gap and a quantum Hall effect, coined "Floquet topological insulator". Whereas the envisioned Floquet topological insulator requires well separated Floquet bands and therefore high-frequency pumping, a natural follow-up question regards the creation of Floquet-like states in graphene with realistic pump laser pulses. Here we predict that with short low-frequency laser pulses attainable in pump-probe experiments, states with local spectral gaps at the Dirac points and novel pseudospin textures can be achieved in graphene using circular light polarization. We demonstrate that time- and angle-resolved photoemission spectroscopy can track these states by measuring sizeable energy gaps and quasi-Floquet energy bands that form on femtosecond time scales. By analyzing Floquet energy level crossings and snapshots of pseudospin textures near the Dirac points, we identify transitions to new states with optically induced nontrivial changes of sublattice mixing that can lead to Berry curvature corrections of electrical transport and magnetization.

cond-mat.mes-hall↗

arXiv2014

Effect of dynamical spectral weight redistribution on effective interactions in time-resolved spectroscopy

The redistribution of electrons in an ultrafast pump-probe experiment causes significant changes to the effective interaction between electrons and bosonic modes. We study the influence of these changes on pump-probe photoemission spectroscopy for a model electron-phonon coupled system using the nonequilibrium Keldysh formalism. We show that spectral rearrangement due to the driving field preserves an overall sum rule for the electronic self-energy, but modifies the effective electron-phonon scattering as a function of energy. Experimentally, this pump-modified scattering can be tracked by analyzing the fluence or excitation energy dependence of population decay rates and transient changes in dispersion kinks.

cond-mat.mes-hall↗