arXiv subjects

J. Kačmarčík

Publications and source records attributed to J. Kačmarčík.

11 recordsLinked to original sources

arXiv2024

Two-gap superconductivity in the noncentrosymmetric La$_3$Se$_4$ compound

Point-contact Andreev reflection spectroscopy at low temperatures and high magnetic fields has been performed on a noncentrosymmetric La$_3$Se$_4$ superconductor with a critical temperature $T_c$ = 8 K. Two superconducting energy gaps $Δ_1$ and $Δ_2$ with $2Δ_{1}/k_{B} T_{c}$ ~ 5.8 and $2Δ_{2}/k_{B} T_{c}$ ~ 2.3, are directly observed in some of the spectra. The temperature and magnetic field effects help to resolve a two-gap structure even on the most frequent spectra where at low temperatures only a single gap is apparent, reflected in a pair of maxima around the zero bias. Two-gap superconductivity consistently with the point contact Andreev reflection spectroscopy is also supported by the heat capacity and the Hall probe magnetization measurements.

cond-mat.supr-con↗

arXiv2021

Extreme in-plane upper critical magnetic fields of heavily doped quasi-two-dimensional transition metal dichalcogenides

Extreme in-plane upper critical magnetic fields $B_{c2//ab}$ strongly violating the Pauli paramagnetic limit have been observed in the misfit layer $(LaSe)_{1.14}(NbSe_2)$ and $(LaSe)_{1.14}(NbSe_2)_2$ single crystals with $T_c$ = 1.23 K and 5.7 K, respectively. The crystals show a two-dimensional to three-dimensional transition at temperatures slightly below $T_c$ with an upturn in the temperature dependence of $B_{c2//ab}$, a temperature dependent huge superconducting anisotropy and a cusplike behavior of the angular dependence of $B_{c2}$. Both misfits are characterized by a strong charge transfer from LaSe to $NbSe_2$. As shown in our previous work, $(LaSe)_{1.14}(NbSe_2)$ is electronically equivalent to the highly doped $NbSe_2$ monolayers. Then, the strong upper critical field can be attributed to the Ising coupling recently discovered in atomically thin transition metal dichalcogenides with strong spin-orbit coupling and a lack of inversion symmetry. A very similar behavior is found in $(LaSe)_{1.14}(NbSe_2)_2$, where the charge transfer is nominally twice as big, which could eventually lead to complete filling of the $NbSe_2$ conduction band and opening superconductivity in LaSe. Whatever the particular superconducting mechanism would be, a common denominator in both misfits is that they behave as a stack of almost decoupled superconducting atomic layers, proving that Ising superconductivity can also exist in bulk materials.

cond-mat.supr-con↗

arXiv2021

Zeeman driven superconductor insulator transition in strongly disordered MoC film. STM and transport studies in transverse magnetic field

Superconductor insulator transition in transverse magnetic field is studied in the highly disordered MoC film with the product of the Fermi momentum and the mean free path $k_F*l$ close to unity. Surprisingly, the Zeeman paramagnetic effects dominate over orbital coupling on both sides of the transition. In superconducting state it is evidenced by a high upper critical magnetic field $B_{c2}$, by its square root dependence on temperature, as well as by the Zeeman splitting of the quasiparticle density of states (DOS) measured by scanning tunneling microscopy. At $B_{c2}$ a logarithmic anomaly in DOS is observed. This anomaly is further enhanced in increasing magnetic field, which is explained by the Zeeman splitting of the Altshuler-Aronov DOS driving the system into a more insulating or resistive state. Spin dependent Altshuler-Aronov correction is also needed to explain the transport behavior above $B_{c2}$.

cond-mat.supr-con↗

arXiv2019

Single-gap superconductivity in Mo$_8$Ga$_{41}$

In this paper, potential two-gap superconductivity in Mo$_8$Ga$_{41}$ is addressed in detail by means of thermodynamic and spectroscopic measurements. Combination of highly sensitive ac-calorimetry and scanning tunneling spectroscopy (STS), as bulk and surface sensitive probes, utilized on the same piece of crystal reveals that there is only one intrinsic gap in the system featuring strong electron-phonon coupling. Traces of multiple superconducting phases seen by STS and also in the heat capacity measured in high magnetic fields on a high-quality and seemingly single-phase crystal might mimic the multigap superconductivity of Mo$_8$Ga$_{41}$ suggested recently in several studies.

cond-mat.supr-con↗

arXiv2018

On the origin of in-gap states in homogeneously disordered ultrathin films. MoC case

Many disordered superconducting films exhibit smeared tunneling spectra with evident in-gap states. We demonstrated that the tunneling density of states in ultrathin MoC films is gapless and can be described by the Dynes version of the BCS density of states with a strong broadening parameter Gamma accounting for the suppression of coherence peaks and increased in-gap states. The thinner the film, the lower the Tc and the superconducting energy gap Delta and the larger the Gamma. MoC films of 3 nm thickness deposited simultaneously on silicon and sapphire substrates reveal very similar scalar disorder, evidenced by the equal sheet resistance, but exhibit different superconducting characteristics of Tc, Delta and Gamma, suggesting that pair breaking responsible for the dissipation channel and the suppression of superconductivity originates on the film-substrate interface. It indicates that sapphire is a stronger pair breaker. Interface pair breaking can be operative in other cases as well.

cond-mat.supr-con↗

arXiv2018

Thermodynamic signatures of quantum criticality in cuprates

The three central phenomena of cuprate superconductors are linked by a common doping $p^{\star}$, where the enigmatic pseudogap phase ends, around which the superconducting phase forms a dome, and at which the resistivity exhibits an anomalous linear dependence on temperature as $T \to 0$. However, the fundamental nature of $p^{\star}$ remains unclear, in particular whether it marks a true quantum phase transition. We have measured the specific heat $C$ of the cuprates Eu-LSCO and Nd-LSCO at low temperature in magnetic fields large enough to suppress superconductivity, over a wide doping range across $p^{\star}$. As a function of doping, we find that the electronic term $C_{\rm el}$ is strongly peaked at $p^{\star}$, where it exhibits a $-T$log$T$ dependence as $T \to 0$. These are the classic signatures of a quantum critical point, as observed in heavy-fermion and iron-based superconductors where their antiferromagnetic phase ends. We conclude that the pseudogap phase of cuprates ends at a quantum critical point, whose associated fluctuations are most likely involved in the $d$-wave pairing and the anomalous scattering.

cond-mat.supr-con↗

arXiv2017

Unconventional superconductivity in the strong-coupling limit for the heavy fermion system CeCoIn$_5$

We present scanning tunneling spectroscopy measurements of the local quasiparticles' excitation spectra of CeCoIn$_5$ between 440mK and 3K in samples with a bulk $T_{\rm c}=2.25$K. The spectral shape of our low-temperature tunneling data, quite textbook nodal-gap conductance, allow us to confidently fit the spectra with a d-wave density of states considering also a shortening of quasiparticles' lifetime term $Γ$. The $Δ(0)$ value obtained from the fits yields a BCS ratio $2Δ/kT_{\rm c} =7.73$ suggesting that CeCoIn$_5$ is an unconventional superconductor in the strong coupling limit. The fits also suggest that the height of coherence peaks in CeCoIn$_5$ is reduced with respect to a pure BCS spectra and therefore the coupling of quasiparticles with spin excitations should play a relevant role. In addition, the tunneling conductance shows a depletion at energies smaller than $Δ$ for temperatures larger than the bulk $T_{\rm c}$, giving further support to the existence of a pseudogap phase that in our samples span up to $T^{*}\sim 1.2 T_{\rm c}$. The phenomenological scaling of the pseudogap temperature observed in various families of cuprates, $2Δ/kT^{*} \sim 4.3 $, is not fulfilled in our measurements. This suggests that in CeCoIn$_5$ the strong magnetic fluctuations might conspire to close the local superconducting gap at a smaller pesudogap temperature-scale than in cuprates.

cond-mat.supr-con↗

arXiv2017

Magnetic and thermodynamic properties of Cu$_x$TiSe$_2$ single crystals

We present a detailed study of the phase diagram of copper intercalated TiSe$_2$ single crystals, combining local Hall-probe magnetometry, tunnel diode oscillator technique (TDO), specific-heat, and angle-resolved photoemission spectroscopy measurements. A series of the Cu$_x$TiSe$_2$ samples from three different sources with various copper content $x$ and superconducting critical temperatures $T_c$ have been investigated. We first show that the vortex penetration mechanism is dominated by geometrical barriers enabling a precise determination of the lower critical field, $H_{c1}$. We then show that the temperature dependence of the superfluid density deduced from magnetic measurements (both $H_{c1}$ and TDO techniques) clearly suggests the existence of a small energy gap in the system, with a coupling strength $2Δ_s \sim [2.4-2.8]k_BT_c$, regardless of the copper content, in puzzling contradiction with specific heat measurements which can be well described by one single large gap $2Δ_l \sim [3.7-3.9]k_BT_c$. Finally, our measurements reveal a non-trivial doping dependence of the condensation energy, which remains to be understood.

cond-mat.supr-con↗

arXiv2017

Puzzling evidence for surface superconductivity in the layered dichalcogenide Cu$_{10\%}$TiSe$_2$

We report on specific heat and magnetotransport measurements performed on superconducting Cu$_{10\%}$TiSe$_2$ single crystals. We show that superconductivity persists in transport measurements up to magnetic fields $H_R$ well above the upper critical field $H_{c2}$ deduced from the calorimetric measurements. Surprisingly this "surface" superconductivity is present for all magnetic field orientations, either parallel or perpendicular to the layers. For $H\|ab$, the temperature dependence of the $H_R/H_{c2}$ ratio can be well reproduced by solving the Ginzburg-Landau equations in presence of a surface layer with reduced superconducting properties. Unexpectedly this temperature dependence does not depend on the field orientation.

cond-mat.supr-con↗

arXiv2016

Single gap superconductivity in beta-Bi2Pd

beta-Bi2Pd compound has been proposed as another example of a multi-gap superconductor [Y. Imai et al., J. Phys. Soc. Jap. 81, 113708 (2012)]. Here, we report on measurements of several important physical quantities capable to show a presence of multiple energy gaps on our superconducting single crystals of beta-Bi2Pd with the critical temperature Tc close to 5 K. The calorimetric study via a sensitive ac technique shows a sharp anomaly at the superconducting transition, however only a single energy gap is detected. Also other characteristics inferred from calorimetric measurements as the field dependence of the Sommerfeld coefficient and the temperature and angular dependence of the upper critical magnetic field point unequivocally to standard single s-wave gap superconductivity. The Hall-probe magnetometry provides the same result from the analysis of the temperature dependence of the lower critical field. A single-gapped BCS density of states is detected by the scanning tunneling spectroscopy measurements. Then, the bulk as well as the surface sensitive probes evidence a standard conventional superconductivity in this system where the topologically protected surface states have been recently detected by ARPES [M. Sakano et al., Nature Comm. 6, 8595 (2015)] .

cond-mat.supr-con↗

arXiv2016

Fermionic scenario for the destruction of superconductivity in ultrathin MoC films evidenced by STM measurements

We use sub-Kelvin scanning tunneling spectroscopy to investigate the suppression of superconductivity in homogeneously disordered ultrathin MoC films. We observe that the superconducting state remains spatially homogeneous even on the films of 3 nm thickness. The vortex imaging suggests the global phase coherence in our films. Upon decreasing thickness, when the superconducting transition drops from 8.5 to 1.2 K, the superconducting energy gap follows perfectly Tc. All this is pointing to a two-stage fermionic scenario of the superconductor-insulator transition (SIT) via a metallic state as an alternative to the direct bosonic SIT scenario with a Cooper-pair insulating state evidenced by the last decade STM experiments.

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