arXiv subjects

J. Kono

Publications and source records attributed to J. Kono.

At least 19 recordsLinked to original sources

arXiv2023

Development of the Thomson scattering measurement system for cascade arc device with indirectly heated hollow cathode

We have developed a Thomson scattering measurement system for the cascade arc discharge device designed for the plasma window (PW) application study. The PW is one of the plasma application techniques that sustain the steep pressure gradient between high pressure (10-100 kPa) and a vacuum environment due to the thermal energy of the plasma. Since the plasma thermal energy is the essential parameter for the pressure separation capability of PW, we installed the Thomson scattering measurement system to observe the electron density and temperature within the anode and cathode of the PW for the detailed analysis of the pressure separation capability. The frequency-doubled Nd:YAG laser (532 nm, 200 mJ, 8 ns) was employed for the probe laser. The scattered light was fed to the triple grating spectrometer. The notch filter between the first and second grating eliminated the stray light, realizing a sufficiently high signal-to-noise ratio. The Thomson scattering measurement system successfully obtained the electron density and temperature of the cascade arc plasma at 20 mm downstream from the tip of the cathode. The installed system successfully obtained the Thomson scattering spectrum and showed that the electron density increased from $2\times10^{19} {\rm m}^{-3}$ to $7\times10^{19} {\rm m}^{-3}$ with the discharge power, while the electron temperature was almost constant at about 2 eV. The obtained data successfully contributed to the study of the pressure separation capability of the PW.

physics.plasm-ph↗

arXiv2020

Observation of Photoinduced Terahertz Gain in GaAs Quantum Wells: Evidence for Radiative Two-Exciton-to-Biexciton Scattering

We have observed photoinduced negative optical conductivity, or gain, in the terahertz frequency range in a GaAs multiple-quantum-well structure in a strong perpendicular magnetic field at low temperatures. The gain is narrow-band: it appears as a sharp peak (linewidth $<$0.45 meV) whose frequency shifts with applied magnetic field. The gain has a circular-polarization selection rule: a strong line is observed for hole-cyclotron-resonance-active polarization. Furthermore, the gain appears only when the exciton $1s$ state is populated, which rules out intraexcitonic transitions to be its origin. Based on these observations, we propose a possible process in which the stimulated emission of a terahertz photon occurs while two free excitons scatter into one biexciton in an energy and angular-momentum conserving manner.

cond-mat.mes-hall↗

arXiv2020

Guided Mode Resonances in Flexible 2D THz Photonic Crystals

In terahertz (THz) photonics, there is an ongoing effort to develop thin, compact devices such as dielectric photonic crystal (PhC) slabs with desirable light matter interactions. However, previous works in THz PhC slabs are limited to rigid substrates with thicknesses $\sim$ 100s of micrometers. Dielectric PhC slabs have been shown to possess in-plane modes that are excited by external radiation to produce sharp guided mode resonances with minimal absorption for applications in sensors, optics and lasers. Here, we confirm the existence of guided resonances in a membrane-type THz PhC slab with subwavelength ($λ_{0}$/6 - $λ_{0}$/12) thicknesses of flexible dielectric polyimide films. The transmittance of the guided resonances was measured for different structural parameters of the unit cell. Furthermore, we exploited the flexibility of the samples to modulate the linewidth of the guided modes down to 1.5 GHz for bend angle of $θ$ $\geq 5^{\circ}$; confirmed experimentally by the suppression of these modes. The mechanical flexibility of the device allows for an additional degree of freedom in system design for optical components for high-speed communications, soft wearable photonics and implantable medical devices.

physics.app-ph↗

arXiv2019

Ultrastrong coupling regimes of light-matter interaction

Recent experiments have demonstrated that light and matter can mix together to an extreme degree, and previously uncharted regimes of light-matter interactions are currently being explored in a variety of settings. The so-called ultrastrong coupling (USC) regime is established when the light-matter interaction energy is a comparable fraction of the bare frequencies of the uncoupled systems. Furthermore, when the interaction strengths become larger than the bare frequencies, the deep-strong coupling (DSC) regime emerges. This article reviews advances in the field of the USC and DSC regimes, in particular, for light modes confined in cavities interacting with two-level systems. An overview is first provided on the theoretical progress since the origins from the semiclassical Rabi model until recent developments of the quantum Rabi model. Next, several key experimental results from a variety of quantum platforms are described, including superconducting circuits, semiconductor quantum wells, and other hybrid quantum systems. Finally, anticipated applications are highlighted utilizing USC and DSC regimes, including novel quantum optical phenomena, quantum simulation, and quantum computation.

quant-ph↗

arXiv2018

Singular charge fluctuations at a magnetic quantum critical point

Strange metal behavior is ubiquitous to correlated materials ranging from cuprate superconductors to bilayer graphene. There is increasing recognition that it arises from physics beyond the quantum fluctuations of a Landau order parameter which, in quantum critical heavy fermion antiferromagnets, may be realized as critical Kondo entanglement of spin and charge. The dynamics of the associated electronic delocalization transition could be ideally probed by optical conductivity, but experiments in the corresponding frequency and temperature ranges have remained elusive. We present terahertz time-domain transmission spectroscopy on molecular beam epitaxy-grown thin films of YbRh$_2$Si$_2$, a model strange metal compound. We observe frequency over temperature scaling of the optical conductivity as a hallmark of beyond-Landau quantum criticality. Our discovery implicates critical charge fluctuations as playing a central role in the strange metal behavior, thereby elucidating one of the longstanding mysteries of correlated quantum matter.

cond-mat.str-el↗

arXiv2016

Probing the semiconductor to semimetal transition in InAs/GaSb double quantum wells by magneto-infrared spectroscopy

We perform a magneto-infrared spectroscopy study of the semiconductor to semimetal transition of InAs/GaSb double quantum wells from the normal to the inverted state. We show that owing to the low carrier density of our samples (approaching the intrinsic limit), the magneto-absorption spectra evolve from a single cyclotron resonance peak in the normal state to multiple absorption peaks in the inverted state with distinct magnetic field dependence. Using an eight-band Pidgeon-Brown model, we explain all the major absorption peaks observed in our experiment. We demonstrate that the semiconductor to semimetal transition can be realized by manipulating the quantum confinement, the strain, and the magnetic field. Our work paves the way for band engineering of optimal InAs/GaSb structures for realizing novel topological states as well as for device applications in the terahertz regime.

cond-mat.mes-hall↗

arXiv2014

Rapid Scanning Terahertz Time-Domain Magnetospectroscopy with a Table-Top Repetitive Pulsed Magnet

We have performed terahertz time-domain magnetospectroscopy by combining a rapid scanning terahertz time-domain spectrometer based on the electronically coupled optical sampling method with a table-top mini-coil pulsed magnet capable of producing magnetic fields up to 30 T. We demonstrate the capability of this system by measuring coherent cyclotron resonance oscillations in a high-mobility two-dimensional electron gas in GaAs and interference-induced terahertz transmittance modifications in a magnetoplasma in lightly doped n-InSb.

cond-mat.mtrl-sci↗

arXiv2014

High-Ampacity Power Cables of Tightly-Packed and Aligned Carbon Nanotubes

We characterize the current-carrying capacity (CCC), or ampacity, of highly-conductive, light, and strong carbon nanotube (CNT) fibers by measuring their failure current density (FCD) and continuous current rating (CCR) values. We show, both experimentally and theoretically, that the CCC of these fibers is determined by the balance between current-induced Joule heating and heat exchange with the surroundings. The measured FCD values of the fibers range from 10$^7$ to 10$^9$ A/m$^2$ and are generally higher than the previously reported values for aligned buckypapers, carbon fibers, and CNT fibers. To our knowledge, this is the first time the CCR for a CNT fiber has been reported. We demonstrate that the specific CCC (i.e., normalized by the linear mass density) of our CNT fibers are higher than those of copper.

cond-mat.mtrl-sci↗

arXiv2013

Plasmonic Nature of the Terahertz Conductivity Peak in Single-Wall Carbon Nanotubes

Plasmon resonance is expected to occur in metallic and doped semiconducting carbon nanotubes in the terahertz frequency range, but its convincing identification has so far been elusive. The origin of the terahertz conductivity peak commonly observed for carbon nanotube ensembles remains controversial. Here we present results of optical, terahertz, and DC transport measurements on highly enriched metallic and semiconducting nanotube films. A broad and strong terahertz conductivity peak appears in both types of films, whose behaviors are consistent with the plasmon resonance explanation, firmly ruling out other alternative explanations such as absorption due to curvature-induced gaps.

cond-mat.mes-hall↗

arXiv2013

Ultrafast Generation of Fundamental and Multiple-order Phonon Excitations in Highly-Enriched (6,5) Single-Wall Carbon Nanotubes

Using a macroscopic ensemble of highly-enriched (6,5) single-wall carbon nanotubes, combined with high signal-to-noise ratio, time-dependent differential transmission spectroscopy, we have generated vibrational modes in an ultrawide spectral range (10-3000 cm^{-1}). A total of fourteen modes were clearly resolved and identified, including fundamental modes of A, E1, and E2 symmetries and their combinational modes involving two and three phonons. Through comparison with CW Raman spectra as well as calculations based on an extended tight-binding model, we were able to identify all the observed peaks and determine the frequencies of the individual and combined modes. We provide a full summary of phonon frequencies for (6,5) nanotubes that can serve as a basic reference with which to refine our understanding of nanotube phonon spectra as well as a testbed for new theoretical models.

cond-mat.mes-hall↗

arXiv2013

Fermi-Edge Superfluorescence from a Quantum-Degenerate Electron-Hole Gas

We report on the observation of spontaneous bursts of coherent radiation from a quantum-degenerate gas of nonequilibrium electron-hole pairs in semiconductor quantum wells. Unlike typical spontaneous emission from semiconductors, which occurs at the band edge, the observed emission occurs at the quasi-Fermi edge of the carrier distribution. As the carriers are consumed by recombination, the quasi-Fermi energy goes down toward the band edge, and we observe a continuously red-shifting streak. We interpret this emission as cooperative spontaneous recombination of electron-hole pairs, or superfluorescence, which is enhanced by Coulomb interactions near the Fermi edge. This novel many-body enhancement allows the magnitude of the spontaneously developed macroscopic polarization to exceed the maximum value for ordinary superfluorescence, making electron-hole superfluorescence even more "super" than atomic superfluorescence.

cond-mat.mes-hall↗

arXiv2013

Terahertz Science and Technology of Carbon Nanomaterials

The diverse applications of terahertz radiation and its importance to fundamental science makes finding ways to generate, manipulate, and detect terahertz radiation one of the key areas of modern applied physics. One approach is to utilize carbon nanomaterials, in particular, single-wall carbon nanotubes and graphene. Their novel optical and electronic properties offer much promise to the field of terahertz science and technology. This article describes the past, current, and future of the terahertz science and technology of carbon nanotubes and graphene. We will review fundamental studies such as terahertz dynamic conductivity, terahertz nonlinearities, and ultrafast carrier dynamics as well as terahertz applications such as terahertz sources, detectors, modulators, antennas, and polarizers.

cond-mat.mes-hall↗

arXiv2013

Spin Relaxation Times of Single-Wall Carbon Nanotubes

We have measured temperature ($T$)- and power-dependent electron spin resonance in bulk single-wall carbon nanotubes to determine both the spin-lattice and spin-spin relaxation times, $T_1$ and $T_2$. We observe that $T_1^{-1}$ increases linearly with $T$ from 4 to 100 K, whereas $T_2^{-1}$ {\em decreases} by over a factor of two when $T$ is increased from 3 to 300 K. We interpret the $T_1^{-1} \propto T$ trend as spin-lattice relaxation via interaction with conduction electrons (Korringa law) and the decreasing $T$ dependence of $T_2^{-1}$ as motional narrowing. By analyzing the latter, we find the spin hopping frequency to be 285 GHz. Last, we show that the Dysonian lineshape asymmetry follows a three-dimensional variable-range hopping behavior from 3 to 20 K; from this scaling relation, we extract a localization length of the hopping spins to be $\sim$100 nm.

cond-mat.mes-hall↗

arXiv2013

Measurement of Filling-Factor-Dependent Magnetophonon Resonances in Graphene Using Raman Spectroscopy

We perform polarization-resolved Raman spectroscopy on graphene in magnetic fields up to 45T. This reveals a filling-factor-dependent, multi-component anticrossing structure of the Raman G peak, resulting from magnetophonon resonances between magnetoexcitons and E$_{2g}$ phonons. This is explained with a model of Raman scattering taking into account the effects of spatially inhomogeneous carrier densities and strain. Random fluctuations of strain-induced pseudo-magnetic fields lead to increased scattering intensity inside the anti-crossing gap, consistent with the experiment.

cond-mat.mes-hall↗

arXiv2013

Review of Anisotropic Terahertz Material Response

Anisotropy is ubiquitous in solids and enhanced in low-dimensional materials. In response to an electromagnetic wave, anisotropic absorptive and refractive properties result in dichroic and birefringent optical phenomena both in the linear and nonlinear optics regimes. Such material properties have led to a diverse array of useful polarization components in the visible and near-infrared, but mature technology is non-existent in the terahertz (THz). Here, we review several novel types of anisotropic material responses observed in the THz frequency range, including both linear and circular anisotropy, which have long-term implications for the development of THz polarization optics. We start with the extreme linear anisotropy of macroscopically aligned carbon nanotubes, arising from their intrinsically anisotropic dynamic conductivity. Magnetically induced anisotropy will then be reviewed, including the giant Faraday effects observed in semiconductors, semimetals, and two-dimensional electron systems.

cond-mat.mtrl-sci↗

arXiv2013

Effects of Electron-Electron Interactions on Electronic Raman Scattering of Graphite in High Magnetic Fields

We report the observation of strongly temperature-dependent, asymmetric spectral lines in electronic Raman scattering spectra of graphite in a high magnetic field up to 45 T applied along the c-axis. The magnetic field quantizes the in-plane motion, while the out-of-plane motion remains free, effectively reducing the system dimension from three to one. Optically created electron-hole pairs interact with, or shake up, the one-dimensional Fermi sea in the lowest Landau subbands. Based on the Tomonaga-Luttinger liquid theory, we show that interaction effects modify the van Hove singularity to the form $(ω-Δ)^{2α-1/2}$ at zero temperature. At finite temperature, we predict a thermal broadening factor that increases linearly with the temperature. Our model reproduces the observed temperature-dependent line-shape, determining $α$ to be $\sim$0.05 at 40 T.

cond-mat.mes-hall↗

arXiv2013

Midinfrared Third Harmonic Generation from Macroscopically Aligned Ultralong Single-Wall Carbon Nanotubes

We report the observation of strong third harmonic generation from a macroscopic array of aligned ultralong single-wall carbon nanotubes (SWCNTs) with intense midinfrared radiation. Through power-dependent experiments, we determined the absolute value of the third-order nonlinear optical susceptibility, $χ^{(3)}$, of our SWCNT film to be 5.53 $\times$ 10$^{-12}$ esu, three orders of magnitude larger than that of the fused silica reference we used. Taking account of the filling factor of 8.75% for our SWCNT film, we estimate a $χ^{(3)}$ of 6.32 $\times$ 10$^{-11}$ esu for a fully dense film. Furthermore, through polarization-dependent experiments, we extracted all the nonzero elements of the $χ^{(3)}$ tensor, determining the magnitude of the weaker tensor elements to be $\sim$1/6 of that of the dominant $χ^{(3)}_{zzzz}$ component.

cond-mat.mes-hall↗

arXiv2013

Collective Antenna Effects in the Terahertz and Infrared Response of Highly Aligned Carbon Nanotube Arrays

We study macroscopically-aligned single-wall carbon nanotube arrays with uniform lengths via polarization-dependent terahertz and infrared transmission spectroscopy. Polarization anisotropy is extreme at frequencies less than $\sim$3 THz with no sign of attenuation when the polarization is perpendicular to the alignment direction. The attenuation for both parallel and perpendicular polarizations increases with increasing frequency, exhibiting a pronounced and broad peak around 10 THz in the parallel case. We model the electromagnetic response of the sample by taking into account both radiative scattering and absorption losses. We show that our sample acts as an effective antenna due to the high degree of alignment, exhibiting much larger radiative scattering than absorption in the mid/far-infrared range. Our calculated attenuation spectrum clearly shows a non-Drude peak at $\sim$10 THz in agreement with the experiment.

cond-mat.mes-hall↗