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J. Kuttruff

Publications and source records attributed to J. Kuttruff.

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Quantum tomography of free electrons

Determining the quantum state of a given quantum-mechanical system is a fundamental task in physics. Quantum-state tomography has been pivotal for establishing quantum optics [1-4] and for revealing the properties of bound charges in materials [5-7]. An emerging other object for studying and utilizing quantum effects are free electrons, elementary particles that are central to high-resolution microscopy [8,9], electron-based quantum optics [10-17], ul-trafast electron microscopy [18-24] and particle accelerators [25-27]. However, free electrons are intrinsically incoherent, and we lack a broadly applicable method to measure and control their quantum state beyond special cases with discrete energy sidebands [28,29]. Here, we report a universal approach to measure arbitrary free-electron quantum states in continuous variables. Two monochromatic but spectrally shifted laser waves produce interfering quan-tum paths that directly reveal the density matrix and thus all essential properties of the pure wavepackets, the ensemble, and their interlinks. As a first application, we show how the quantum state of a single electron is modified by many-body Coulomb interactions of a sur-rounding electron gas. The reported concepts and results provide insight into otherwise hid-den correlations in electron beams and enable the controlled optimization of exceptional quantum states for free-electron quantum optics or quantum electron microscopy.

quant-ph

Electron modulation and ultrafast near-field imaging with vectorial laser fields

Controlled interaction of laser light with electron beams is fundamental for ultrafast electron microscopy and electron-based quantum optics, yet their direct coupling is forbidden in free space. Here we use longitudinally polarized light at a thin membrane and show that the emerging focal fields can modulate the electron beam in a direct, coherent and linear way, without the need for nanostructured materials or slanted interaction geometries. Also, we use vectorial polarizations to excite and probe three-dimensional nanophotonic near-fields in metallic mesocrystals by coherent electron energy gain and loss. We find that longitudinal electric fields excite axial near-fields in a direct way while longitudinal magnetic fields excite oscillating ring currents via azimuthal electric fields. These possibilities enable tilt-free, collinear generation of attosecond electron pulses or free-electron qubits and provide novel imaging modes in ultrafast electron microscopy and metamaterial tomography.

physics.optics

Stronger femtosecond excitation causes slower electron-phonon coupling in silicon

Electron-hole pairs in semiconductors are essential for solar cells and fast electronic circuitry, but the competition between carrier transport and relaxation into heat limits the efficiency and speed. Here we use ultrafast electron diffraction with terahertz pulse compression to measure the electron-phonon decay rate in single-crystal silicon as a function of laser excitation strength. We find that the excited electrons relax slower into phonons for higher carrier densities. The electron-phonon scattering rate changes in a nonlinear way from 400 fs at ~$2 \times 10^{20} \text{ cm}^{-3}$ to 1.2 ps at ~$4 \times 10^{20} \text{ cm}^{-3}$. These results indicate that a hot electron gas quenches the scattering into phonons in a temperature-dependent way. Ultrafast electronic circuitry of silicon therefore should work faster and provide higher bandwidths at lower carrier densities.

cond-mat.mtrl-sci

Electron matter waves with internal torque

Angular momentum and torque are important principles for basic and applied physics on any spatial scales, for example, in elementary particles, cold gases, optical tweezers, quantum information technology, metamaterials, gyroscopes or astrophysical entities. Investigating or controlling angular momentum in atoms or sub-atomic structures requires torque on femtosecond and picometer scales, far below the capabilities of laser light. Here we shape the electrons in an electron microscope into wave packets with a time-dependent chirality and internal torque. We intersect the electron beam with chiral laser light to create discrete energy sidebands by multiple helical photon absorptions that create a correlation between orbital angular momentum and kinetic energy. Dispersion of these partial waves due to the electron rest mass then converts each single electron into a wave function with internal torque. Under our control, a left-handed matter wave becomes right-handed in femtosecond times. Such quantum objects will facilitate research on angular momentum and chirality on atomic and sub-atomic scales.

physics.optics

Terahertz control in a transmission electron microscope

Ultrafast electron microscopy provides a movie-like access to structural dynamics of materials in space and time, but fundamental atomic motions or electron dynamics are, so far, too quick to be resolved. Here we report the all-optical control, compression and characterization of electron pulses in a transmission electron microscope by the single optical cycles of laser-generated terahertz light. This concept provides isolated electron pulses and merges the spatial resolution of a transmission electron microscope with the temporal resolution that is offered by a single cycle of laser light. Central to these achievements is a perforated parallel-plate metallic waveguide in which transverse velocity mismatch and magnetic forces are mitigated by electrically constructive and magnetically destructive interferences of incoming and reflected terahertz half-cycles from a displaced waveguide termination. Measurements of spatial chirp via energy-filtered imaging reveal flat pulses with no transversal deflection or temporal aberrations at the specimen. We also report the all-optical control of multi-electron states and discover a substantial two-electron and three-electron anti-correlation in the time domain. These results open up the possibility to visualize atomic and electronic motions together with their quantum correlations on fundamental dimensions in space and time.

physics.optics