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J. L. Bohn

Publications and source records attributed to J. L. Bohn.

36 records · Page 2Linked to original sources

Pseudo-potential treatment of two aligned dipoles under external harmonic confinement

Dipolar Bose and Fermi gases, which are currently being studied extensively experimentally and theoretically, interact through anisotropic, long-range potentials. Here, we replace the long-range potential by a zero-range pseudo-potential that simplifies the theoretical treatment of two dipolar particles in a harmonic trap. Our zero-range pseudo-potential description reproduces the energy spectrum of two dipoles interacting through a shape-dependent potential under external confinement very well, provided that sufficiently many partial waves are included, and readily leads to a classification scheme of the energy spectrum in terms of approximate angular momentum quantum numbers. The results may be directly relevant to the physics of dipolar gases loaded into optical lattices.

physics.atom-ph↗

Ultracold Rb-OH collisions and prospects for sympathetic cooling

We have computed ab inito cross sections for cold collisions of Rb atoms with OH radicals. We predict collision rate constants of order 10^{-11} cm^3/s at temperatures in the range 10-100 mK at which molecules have already been produced experimentally. However, we also find that in these collisions the molecules have a strong propensity for changing their internal state, which could make sympathetic cooling of OH in a Rb buffer gas problematic in magnetostatic or electrostatic traps.

physics.atom-ph↗

Dipolar Bose gases: Many-body versus mean-field description

We characterize zero-temperature dipolar Bose gases under external spherical confinement as a function of the dipole strength using the essentially exact many-body diffusion Monte Carlo (DMC) technique. We show that the DMC energies are reproduced accurately within a mean-field framework if the variation of the s-wave scattering length with the dipole strength is accounted for properly. Our calculations suggest stability diagrams and collapse mechanisms of dipolar Bose gases that differ significantly from those previously proposed in the literature.

cond-mat.stat-mech↗

Ultracold Collisions of Fermionic OD Radicals

We discuss consequences of Fermi exchange symmetry on collisions of polar molecules at low temperatures (below 1 K), considering the OD radical as a prototype. At low fields and low temperatures, Fermi statistics can stabilize a gas of OD molecules against state-changing collisions. We find, however, that this stability does not extend to temperatures high enough to assist with evaporative cooling. In addition, we establish that a novel ``field-linked'' resonance state of OD dimers exists, in analogy with the similar states predicted for bosonic OH.

physics.atom-ph↗

Observation of Heteronuclear Feshbach Resonances in a Bose-Fermi Mixture

Three magnetic-field induced heteronuclear Feshbach resonances were identified in collisions between bosonic 87Rb and fermionic 40K atoms in their absolute ground states. Strong inelastic loss from an optically trapped mixture was observed at the resonance positions of 492, 512, and 543 +/- 2 G. The magnetic-field locations of these resonances place a tight constraint on the triplet and singlet cross-species scattering lengths, yielding -281 +/- 15 Bohr and -54 +/- 12 Bohr, respectively. The width of the loss feature at 543 G is 3.7 +/- 1.5 G wide; this broad Feshbach resonance should enable experimental control of the interspecies interactions.

cond-mat.soft↗

Pair Wave Functions in Atomic Fermi Condensates

Recent experiments have observed condensation behavior in a strongly interacting system of fermionic atoms. We interpret these observations in terms of a mean-field version of resonance superfluidity theory. We find that the objects condensed are not bosonic molecules composed of bound fermion pairs, but are rather spatially correlated Cooper pairs whose coherence length is comparable to the mean spacing between atoms. We propose experiments that will help to further probe these novel pairs.

cond-mat.soft↗

Multiplet Structure of Feshbach Resonances in non-zero partial waves

We report a unique feature of magnetic field Feshbach resonances in which atoms collide with non-zero orbital angular momentum. P-wave ($l=1$) Feshbach resonances are split into two components depending on the magnitude of the resonant state's projection of orbital angular momentum onto the field axis. This splitting is due to the magnetic dipole-dipole interaction between the atoms and it offers a means to tune anisotropic interactions of an ultra-cold gas of atoms. A parameterization of the resonance in terms of an effective range expansion is given.

physics.atom-ph↗

Field-linked States of Ultracold Polar Molecules

We explore the character of a novel set of ``field-linked'' states that were predicted in [A. V. Avdeenkov and J. L. Bohn, Phys. Rev. Lett. 90, 043006 (2003)]. These states exist at ultralow temperatures in the presence of an electrostatic field, and their properties are strongly dependent on the field's strength. We clarify the nature of these quasi-bound states by constructing their wave functions and determining their approximate quantum numbers. As the properties of field-linked states are strongly defined by anisotropic dipolar and Stark interactions, we construct adiabatic surfaces as functions of both the intermolecular distance and the angle that the intermolecular axis makes with the electric field. Within an adiabatic approximation we solve the 2-D Schrodinger equation to find bound states, whose energies correlate well with resonance features found in fully-converged multichannel scattering calculations.

physics.atom-ph↗

Detection of spatial correlations in an ultracold gas of fermions

Spatial correlations are observed in an ultracold gas of fermionic atoms close to a Feshbach resonance. The correlations are detected by inducing spin-changing rf transitions between pairs of atoms. We observe the process in the strongly interacting regime for attractive as well as for repulsive atom-atom interactions and both in the regime of high and low quantum degeneracy. The observations are compared with a two-particle model that provides theoretical predictions for the measured rf transition rates.

cond-mat.soft↗

Photoassociation of a Quantum Degenerate Gas

We have measured the intensity dependent rate and frequency shift of a photoassociation transition in a quantum degenerate gas of 7Li. The rate increases linearly with photoassociation laser intensity for low intensities, whereas saturation is observed at higher intensities. The measured rates and shifts agree reasonably well with theory within the estimated systematic uncertainties. Several theoretically predicted saturation mechanisms are discussed, but a theory in which saturation arises because of quantum mechanical unitarity agrees well with the data.

cond-mat.soft↗

Creation of ultracold molecules from a Fermi gas of atoms

Since the realization of Bose-Einstein condensates (BEC) in atomic gases an experimental challenge has been the production of molecular gases in the quantum regime. A promising approach is to create the molecular gas directly from an ultracold atomic gas; for example, atoms in a BEC have been coupled to electronic ground-state molecules through photoassociation as well as through a magnetic-field Feshbach resonance. The availability of atomic Fermi gases provides the exciting prospect of coupling fermionic atoms to bosonic molecules, and thus altering the quantum statistics of the system. This Fermi-Bose coupling is closely related to the pairing mechanism for a novel fermionic superfluid proposed to occur near a Feshbach resonance. Here we report the creation and quantitative characterization of exotic, ultracold $^{40}$K$_2$ molecules. Starting with a quantum degenerate Fermi gas of atoms at T < 150 nanoKelvin we scan over a Feshbach resonance to adiabatically create over a quarter million trapped molecules, which we can convert back to atoms by reversing the scan. The small binding energy of the molecules is controlled by detuning from the Feshbach resonance and can be varied over a wide range. We directly detect these weakly bound molecules through rf photodissociation spectra that probe the molecular wavefunction and yield binding energies that are consistent with theory.

cond-mat↗

Tuning p-wave interactions in an ultracold Fermi gas of atoms

We have measured a p-wave Feshbach resonance in a single-component, ultracold Fermi gas of potassium atoms. We have used this resonance to enhance the normally suppressed p-wave collision cross-section to values larger than the background s-wave cross-section between potassium atoms in different spin-states. In addition to the modification of two-body elastic processes, the resonance dramatically enhances three-body inelastic collisional loss.

cond-mat↗

Linking Ultracold Polar Molecules

We predict that pairs of polar molecules can be weakly bound together in an ultracold environment, provided that a dc electric field is present. The field that links the molecules together also strongly influences the basic properties of the resulting dimer, such as its binding energy and predissociation lifetime. Because of their long-range character these dimers will be useful in disentangling cold collision dynamics of polar molecules. As an example, we estimate the microwave photoassociation yield for OH-OH cold collisions.

physics.atom-ph↗

Rotational Feshbach Resonances in Ultracold Molecular Collisions

In collisions at ultralow temperatures, molecules will possess Feshbach resonances, foreign to ultracold atoms, whose virtual excited states consist of rotations of the molecules. We estimate the mean spacing and mean widths of these resonant states, exploiting the fact the molecular collisions at low energy display chaotic motion. As examples, we consider the experimentally relevant molecules O_2, OH, and PbO. The density of s-wave resonant states for these species is quite high, implying that a large number of narrow resonant states will exist.

physics.atom-ph↗

Resonant control of elastic collisions in an optically trapped Fermi gas of atoms

We have loaded an ultracold gas of fermionic atoms into a far off resonance optical dipole trap and precisely controlled the spin composition of the trapped gas. We have measured a magnetic-field Feshbach resonance between atoms in the two lowest energy spin-states, |9/2, -9/2> and |9/2, -7/2>. The resonance peaks at a magnetic field of 201.5 plus or minus 1.4 G and has a width of 8.0 plus or minus 1.1 G. Using this resonance we have changed the elastic collision cross section in the gas by nearly 3 orders of magnitude.

cond-mat.stat-mech↗

On the nature of spinor Bose-Einstein condensates in rubidium

We perform detailed close-coupling calculations for the rubidium isotopes 85Rb and 87Rb to ascertain the nature of their spinor Bose-Einstein condensates. These calculations predict that the spinor condensate for the spin-1 boson 87Rb has a ferromagnetic nature. The spinor condensates for the spin-2 bosons 85Rb and 87Rb, however, are both predicted to be polar. The nature of a spin-1 condensate hinges critically on the sign of the difference between the s-wave scattering lengths for total spin 0 and 2 while the nature of a spin-2 condensate depends on the values of the differences between s-wave scattering lengths for the total spin 0, 2 and 4. These scattering lengths were extracted previously and found to have overlapping uncertainties for all three cases, thus leaving the nature of the spinor condensates ambiguous. The present study exploits a refined uncertainty analysis of the scattering lengths based on recently improved result from experimental work by Roberts et al., which permits us to extract an unambiguous result for the nature of the ground state spinor condensates.

physics.atom-ph↗

Geometry and symmetries of multi-particle systems

The quantum dynamical evolution of atomic and molecular aggregates, from their compact to their fragmented states, is parametrized by a single collective radial parameter. Treating all the remaining particle coordinates in d dimensions democratically, as a set of angles orthogonal to this collective radius or by equivalent variables, bypasses all independent-particle approximations. The invariance of the total kinetic energy under arbitrary d-dimensional transformations which preserve the radial parameter gives rise to novel quantum numbers and ladder operators interconnecting its eigenstates at each value of the radial parameter. We develop the systematics and technology of this approach, introducing the relevant mathematics tutorially, by analogy to the familiar theory of angular momentum in three dimensions. The angular basis functions so obtained are treated in a manifestly coordinate-free manner, thus serving as a flexible generalized basis for carrying out detailed studies of wavefunction evolution in multi-particle systems.

physics.atm-clus↗

Observation of p-wave Threshold Law Using Evaporatively Cooled Fermionic Atoms

We have measured independently both s-wave and p-wave cross-dimensional thermalization rates for ultracold potassium-40 atoms held in a magnetic trap. These measurements reveal that this fermionic isotope has a large positive s-wave triplet scattering length in addition to a low temperature p-wave shape resonance. We have observed directly the p-wave threshold law which, combined with the Fermi statistics, dramatically suppresses elastic collision rates at low temperatures. In addition, we present initial evaporative cooling results that make possible these collision measurements and are a precursor to achieving quantum degeneracy in this neutral, low-density Fermi system.

cond-mat↗