arXiv subjects

J. L. Iguain

Publications and source records attributed to J. L. Iguain.

13 recordsLinked to original sources

arXiv2025

Fractal conduction pathways governing ionic transport in a glass

We present a systematic characterization of the fractal conduction pathways governing ionic transport in a non-crystalline solid below the glass-transition temperature. Using classical molecular dynamics simulations of lithium metasilicate, we combine mobility-resolved dynamical analysis with a real-space description of the regions explored by lithium ions. Ensemble-averaged velocity autocorrelation functions rapidly decorrelate and do not resolve the pronounced dynamic heterogeneity of the system, whereas single-ion analysis reveals short-lived episodes of nearly collinear motion. By mapping active-site clusters over increasing time windows, we show that ion-conducting pathways are quasi one-dimensional at short times and evolve into larger, branched structures characterized by a robust fractal dimension $d_f\simeq1.7$. This geometry persists while the silicate backbone remains structurally arrested, whereas near the glass-transition temperature the loss of structural memory leads to the reappearance of small clusters. These results provide a real-space structural interpretation of ionic transport in non-crystalline solids and support fractal pathway models of high-frequency ionic response.

cond-mat.soft↗

arXiv2022

Local Einstein relation for fractals

We study single random walks and the electrical resistance for fractals obtained as the limit of a sequence of periodic structures. In the long-scale regime, power laws describe both the mean-square displacement of a random walk as a function of time and the electrical resistance as a function of length. We show that the corresponding power-law exponents satisfy the Einstein relation. For shorter scales, where these exponents depend on length, we find how the Einstein relation can be generalized to hold locally. All these findings were analytically derived and confirmed by numerical simulations.

cond-mat.stat-mech↗

arXiv2019

Roughening of the anharmonic Larkin model

We study the roughening of $d$-dimensional directed elastic interfaces subject to quenched random forces. As in the Larkin model, random forces are considered constant in the displacement direction and uncorrelated in the perpendicular direction. The elastic energy density contains an harmonic part, proportional to $(\partial_x u)^2$, and an anharmonic part, proportional to $(\partial_x u)^{2n}$, where $u$ is the displacement field and $n>1$ an integer. By heuristic scaling arguments, we obtain the global roughness exponent $ζ$, the dynamic exponent $z$, and the harmonic to anharmonic crossover length scale, for arbitrary $d$ and $n$, yielding an upper critical dimension $d_c(n)=4n$. We find a precise agreement with numerical calculations in $d=1$. For the $d=1$ case we observe, however, an anomalous "faceted" scaling, with the spectral roughness exponent $ζ_s$ satisfying $ζ_s > ζ> 1$ for any finite $n>1$, hence invalidating the usual single-exponent scaling for two-point correlation functions, and the small gradient approximation of the elastic energy density in the thermodynamic limit. We show that such $d=1$ case is directly related to a family of Brownian functionals parameterized by $n$, ranging from the random-acceleration model for $n=1$, to the Lévy arcsine-law problem for $n = \infty$. Our results may be experimentally relevant for describing the roughening of non-linear elastic interfaces in a Matheron-de Marsilly type of random flow.

cond-mat.dis-nn↗

arXiv2017

Creep and thermal rounding close to the elastic depinning threshold

We study the slow stochastic dynamics near the depinning threshold of an elastic interface in a random medium by solving a particularly suited model of hopping interacting particles that belongs to the quenched-Edwards-Wilkinson depinning universality class. The model allows us to compare the cases of uniformly activated and Arrhenius activated hops. In the former case, the velocity accurately follows a standard scaling law of the force and noise intensity with the analog of the thermal rounding exponent satisfying a modified "hyperscaling" relation. For the Arrhenius activation, we find, both numerically and analytically, that the standard scaling form fails for any value of the thermal rounding exponent. We propose an alternative scaling incorporating logarithmic corrections that appropriately fits the numerical results. We argue that this anomalous scaling is related to the strong correlation between activated hops that, alternated with deterministic depinning-like avalanches, occur below the depinning threshold. We rationalize the spatiotemporal patterns by making an analogy of the present model in the near-threshold creep regime with some well-known models with extremal dynamics, particularly the Bak-Sneppen model.

cond-mat.dis-nn↗

arXiv2016

Universal behavior for single-file diffusion on a disordered fractal

We study single-file diffusion on a one-dimensional lattice with a random fractal distribution of hopping rates. For finite lattices, this problem shows three clearly different regimes, namely, nearly independent particles, highly interacting particles, and saturation. The mean-square displacement of a tagged particle as a function of time follows a power law in each regime. The first crossover time $t_s$, between the first and the second regime, depends on the particle density. The other crossover time $t_l$, between the second and the third regime, depends on the lattice length. We find analytic expressions for these dependencies and show how the general behavior can be characterized by an universal form. We also show that the mean-square displacement of the center of mass presents two regimes; anomalous diffusion for times shorter than $t_l$, and normal diffusion for times longer than $t_l$. We study single-file diffusion on a one-dimensional lattice with a random fractal distribution of hopping rates. For finite lattices, this problem shows three clearly different regimes, namely, nearly independent particles, highly interacting particles, and saturation. The mean-square displacement of a tagged particle as a function of time follows a power law in each regime. The first crossover time $t_s$, between the first and the second regime, depends on the particle density. The other crossover time $t_l$, between the second and the third regime, depends on the lattice length. We find analytic expressions for these dependencies and show how the general behavior can be characterized by an universal form. We also show that the mean-square displacement of the center of mass presents two regimes; anomalous diffusion for times shorter than $t_l$, and normal diffusion for times longer than $t_l$.

cond-mat.stat-mech↗

arXiv2015

Low-coverage heteroepitaxial growth with interfacial mixing

We investigate the influence of intermixing on heteroepitaxial growth dynamics, using a two-dimensional point island model, expected to be a good approximation in the early stages of epitaxy. In this model, which we explore both analytically and numerically, every deposited B atom diffuses on the surface with diffusion constant $D_{\rm B}$, and can exchange with any A atom of the substrate at constant rate. There is no exchange back, and emerging atoms diffuse on the surface with diffusion constant $D_{\rm A}$. When any two diffusing atoms meet, they nucleate a point island. The islands neither diffuse nor break, and grow by capturing other diffusing atoms. The model leads to an island density governed by the diffusion of one of the species at low temperature, and by the diffusion of the other at high temperature. We show that these limit behaviors, as well as intermediate ones, all belong to the same universality class, described by a scaling law. We also show that the island-size distribution is self-similarly described by a dynamic scaling law in the limits where only one diffusion constant is relevant to the dynamics, and that this law is affected when both $D_{\rm A}$ and $D_{\rm B}$ play a role.

cond-mat.stat-mech↗

arXiv2014

Single-file diffusion on self-similar substrates

We study the single file diffusion problem on a one-dimensional lattice with a self-similar distribution of hopping rates. We find that the time dependence of the mean-square displacement of both a tagged particle and the center of mass of the system present anomalous power laws modulated by logarithmic periodic oscillations. The anomalous exponent of a tagged particle is one half of the exponent of the center of mass, and always smaller than 1/4. Using heuristic arguments, the exponents and the periods of oscillation are analytically obtained and confirmed by Monte Carlo simulations.

cond-mat.stat-mech↗

arXiv2012

Intermediate Range Structure in Ion-Conducting Tellurite Glasses

We present ac conductivity spectra of tellurite glasses at several temperatures. For the first time, we report oscillatory modulations at frequencies around MHz. This effect is more pronounced the lower the temperature, and washes out when approaching the glass transition temperature $T_g$. We show, by using a minimal model, how this modulation may be attributed to the fractal structure of the glass at intermediate mesoscopic length scales.

cond-mat.dis-nn↗

arXiv2012

Anisotropic anomalous diffusion modulated by log-periodic oscillations

We introduce finite ramified self-affine substrates in two dimensions with a set of appropriate hopping rates between nearest-neighbor sites, where the diffusion of a single random walk presents an anomalous {\it anisotropic} behavior modulated by log-periodic oscillations. The anisotropy is revealed by two different random walk exponents, $ν_x$ and $ν_y$, in the {\it x} and {\it y} direction, respectively. The values of these exponents, as well as the period of the oscillation, are analytically obtained and confirmed by Monte Carlo simulations.

cond-mat.stat-mech↗

arXiv2010

Anomalous diffusion with log-periodic modulation in a selected time interval

On certain self-similar substrates the time behavior of a random walk is modulated by logarithmic periodic oscillations on all time scales. We show that if disorder is introduced in a way that self-similarity holds only in average, the modulating oscillations are washed out but subdiffusion remains as in the perfect self-similar case. Also, if disorder distribution is appropriately chosen the oscillations are localized in a selected time interval. Both the overall random walk exponent and the period of the oscillations are analytically obtained and confirmed by Monte Carlo simulations.

cond-mat.stat-mech↗

arXiv2010

Log-periodic oscillations for diffusion on self-similar finitely ramified structures

Under certain circumstances, the time behavior of a random walk is modulated by logarithmic periodic oscillations. The goal of this paper is to present a simple and pedagogical explanation of the origin of this modulation for diffusion on a substrate with two properties: self-similarity and finite ramification order. On these media, the time dependence of the mean-square displacement shows log-periodic modulations around a leading power law, which can be understood on the base of a hierarchical set of diffusion constants. Both the random walk exponent and the period of oscillations are analytically obtained for a pair of examples, one fractal, the other non-fractal, and confirmed by Monte Carlo simulations.

cond-mat.stat-mech↗

arXiv2008

Log-periodic modulation in one-dimensional random walks

We have studied the diffusion of a single particle on a one-dimensional lattice. It is shown that, for a self-similar distribution of hopping rates, the time dependence of the mean-square displacement follows an anomalous power law modulated by logarithmic periodic oscillations. The origin of this modulation is traced to the dependence on the length of the diffusion coefficient. Both the random walk exponent and the period of the modulation are analytically calculated and confirmed by Monte Carlo simulations.

cond-mat.stat-mech↗

arXiv2003

Putting hydrodynamic interactions to work: tagged particle separation

Separation of magnetically tagged cells is performed by attaching markers to a subset of cells in suspension and applying fields to pull from them in a variety of ways. The magnetic force is proportional to the field gradient, and the hydrodynamic interactions play only a passive, adverse role. Here we propose using a homogeneous rotating magnetic field only to make tagged particles rotate, and then performing the actual separation by means of hydrodynamic interactions, which thus play an active role. The method, which we explore here theoretically and by means of numerical simulations, lends itself naturally to sorting on large scales.

cond-mat.soft↗