arXiv subjects

J. L. Sarrao

Publications and source records attributed to J. L. Sarrao.

At least 127 records · Page 7Linked to original sources

arXiv2002

First order superconducting phase transition in CeCoIn$_5$

We investigated the magnetic field dependence of the superconducting phase transition in heavy fermion CeCoIn_5 (T_c = 2.3 K) using specific heat, magneto-caloric effect, and thermal expansion measurements. The superconducting transition becomes first order when the magnetic field is oriented along the 001 crystallographic direction with a strength greater that 4.7 T, and transition temperature below T_0 ~ 0.31 T_c. The change from second order at lower fields is reflected in strong sharpening of both specific heat and thermal expansion anomalies associated with the phase transition, a strong magnetocaloric effect, and a step-like change in the sample volume. The first order superconducting phase transition in CeCoIn_5 is caused by Pauli limiting in type-II superconductors, and was predicted theoretically in the mid 1960s. We do not see evidence for the inhomogeneous Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting state (predicted by an alternative theory also dating back to mid-60's) in CeCoIn_5 with field H || [001].

cond-mat.supr-con↗

arXiv2002

Low-temperature electrical transport in bilayer manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$

The temperature $T$ and magnetic field $H$ dependence of anisotropic in-plane $ρ_{ab}$ and out-of-plane $ρ_{c}$ resistivities have been investigated in single crystals of the bilayer manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$. Below the Curie transition temperature $T_c=$ 125 K, $ρ_{ab}$ and $ρ_{c}$ display almost the same temperature dependence with an up-turn around 50 K. In the metallic regime (50 K $\leq T \leq$ 110 K), both $ρ_{ab}(T)$ and $ρ_{c}(T)$ follow a $T^{9/2}$ dependence, consistent with the two-magnon scattering. We found that the value of the proportionality coefficient $B_{ab}^{fit}$ and the ratio of the exchange interaction $J_{ab}/J_c$ obtained by fitting the data are in excellent agreement with the calculated $B_{ab}$ based on the two-magnon model and $J_{ab}/J_c$ deduced from neutron scattering, respectively. This provides further support for this scattering mechanism. At even lower $T$, in the non-metallic regime ($T<$ 50 K), {\it both} the in-plane $σ_{ab}$ and out-of-plane $σ_{c}$ conductivities obey a $T^{1/2}$ dependence, consistent with weak localization effects. Hence, this demonstrates the three-dimensional metallic nature of the bilayer manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$ at $T<T_c$.

cond-mat.mtrl-sci↗

arXiv2002

Comparison of the Crystal Structure of the Heavy-Fermion Materials CeCoIn5, CeRhIn5 and CeIrIn5

The crystal structure of the recently discovered heavy-fermion (HF) superconductor CeCoIn5 (Tc = 2.3 K) has been determined by high-resolution neutron powder diffraction. It is tetragonal (space group P4/mmm), with lattice parameters a = 4.61292(9) A and c = 7.5513(2) A at ambient conditions. Whereas CeCoIn5 is isostructural with the HF aniferromagnet CeRhIn5 and the HF superconductor CeIrIn5, its cell constants and its only variable positional parameter, zIn2, differ significantly from the corresponding ones of CeRhIn5 and CeIrIn5. As a result, the distortions of the cuboctahedron [CeIn3], which is the key structural unit in all three materials, are different in CeCoIn5 from the ones in CeRhIn5 and CeIrIn5. The compounds CeCoIn5 and CeIrIn5, which contain the most distorted (in one or another way) [CeIn3] cuboctahedra exhibit superconductivity at ambient pressure below 2.3 K and 0.4 K respectively. On the other hand, CeRhIn5, in which [CeIn3] cuboctahedra are the less distorted, and the parent compound of the materials CeTIn5 i.e. the cubic HF CeIn3 are antiferromagnets at ambient pressure with TN = 3.8 K and 10 K correspondingly.

cond-mat.str-el↗

arXiv2002

Neutron-diffraction study of field-induced transitions in the heavy-fermion compound Ce2RhIn8

We present neutron diffraction measurements in high magnetic fields (0 to 14.5 T) and at low temperatures (2.5, 2.3, 0.77 and 0.068 K) on single crystals of the tetragonal heavy fermion antiferromagnet Ce2RhIn8. For B//[110] the field dependence of selected magnetic and nuclear reflections reveals that the material undergoes several transitions, the temperature dependence of which suggests a complex B-T phase diagram. We present the detailed evolution of the integrated intensities of selected reflections and discuss the associated field-induced transitions.

cond-mat.str-el↗

arXiv2002

Effect of pressure on magnetic structure in heavy fermion CeRhIn5

The effect of hydrostatic pressure on the incommensurate antiferromagnetic structure of CeRhIn5 is investigated with neutron diffraction using a He pressure cell. At 3.8 kbar, the staggered magnetic moment is 0.37(4) Bohr magneton per Ce at 1.6 K, which is the same as the ambient-pressure value. The Neel temperature T_N=3.8(1) K is also the same as the ambient-pressure one, although the curve of order parameter has changed by pressure. The incommensurability "delta" of the magnetic wave vector q_M=(1/2,1/2,"delta") has reduced from "delta"=0.297 at ambient pressure to "delta"=0.294(1) at 3.8 kbar.

cond-mat.str-el↗

arXiv2002

Magnetic Properties of Heavy Fermion Superconductors CeRhIn5 and Ce2RhIn8

Some recent neutron scattering works on CeRhIn5 and Ce2RhIn8, together with related resistivity and specific heat measurements, are summarized. In spite of its layered crystal structure, CeRhIn5 is shown to be 3-dimensional both magnetically and in transport. We also find that the Fisher-Langer behavior is closely followed in CeRhIn5. This may circumvent the Kondo lattice model and support applying established Fermi-liquid superconductivity theory to heavy fermion superconductors.

cond-mat.str-el↗

arXiv2002

Magnetocrystalline Anisotropy in a Single Crystal of CeNiGe2

We report measurements on single crystals of orthorhombic CeNiGe2, which is found to exhibit highly anisotropic magnetic and transport properties. The magnetization ratio M(H//b)/M(H^b) at 2 K is observed to be about 18 at 4 T and the electrical resistivity ratio r//b/r^b is about 70 at room temperature. It is confirmed that CeNiGe2 undergoes two-step antiferromagnetic transition at 4 and 3 K, as reported for polycrystalline samples. The application of magnetic field along the b axis (the easy magnetization axis) stabilizes a ferromagnetic correlation between the Ce ions and enhances the hopping of carriers. This results in large negative magnetoresistance along the b axis.

cond-mat.str-el↗

arXiv2002

Carrier relaxation dynamics in heavy fermion compounds

The first femtosecond carrier relaxation dynamics studies in heavy fermion compounds are presented. The carrier relaxation time shows a dramatic hundred-fold increase below the Kondo temperature revealing a dramatic sensitivity to the electronic density of states near the Fermi level.

cond-mat.str-el↗

arXiv2002

Low Temperature Thermal Transport in High Temperature Superconducting BSCCO via Y-doped Insulating Analogue

In order to separate electronic and phonon mechanisms of thermal transport in high temperature superconducting Bi2212, we measured thermal conductivity of single crystals of Y-doped Bi2212, an insulating analogue of pure Bi2212, in the temperature range between 40 mK and 2 K. Temperature dependence of the thermal conductivity of insulating samples changes from T$^{1.7}$ between 1 and 2 K to $T^{2.6}$ below 200 mK, indicating saturation of the phonon mean free path with decreasing temperature. Overall, thermal conductivity of the insulating samples (which is due entirely to phonons) is strongly suppressed in comparison to that of the superconducting samples. Therefore, a large (and at the lowest temperatures, predominant) part of the total thermal transport in superconducting Bi2212 is due to electrons.

cond-mat.supr-con↗

arXiv2001

Response of the Heavy-Fermion Superconductor CeCoIn$_5$ to Pressure: Roles of Dimensionality and Proximity to a Quantum-Critical Point

We report measurements of the pressure-dependent superconducting transition temperature $T_c$ and electrical resistivity of the heavy-fermion compound CeCoIn$_5$. Pressure moves CeCoIn$_5$ away from its proximity to a quantum-critical point at atmospheric pressure. Experimental results are qualitatively consistent with theoretical predictions for strong-coupled, d-wave superconductivity in an anisotropic 3D superconductor.

cond-mat.str-el↗

arXiv2001

Effect of La doping on magnetic structure in heavy fermion CeRhIn5

The magnetic structure of Ce0.9La0.1RhIn5 is measured using neutron diffraction. It is identical to the incommensurate transverse spiral for CeRhIn5, with a magnetic wave vector q_M=(1/2,1/2,0.297), a staggered moment of 0.38(2)Bohr magneton per Ce at 1.4K and a reduced Neel temperature of 2.7 K.

cond-mat.str-el↗

arXiv2001

Specific Heat of CeRhIn5: Pressure-Driven Evolution of the Ground State from Antiferromagnetism to Superconductivity

Measurements of the specific heat of antiferromagnetic CeRhIn5, to 21 kbar, and for 21 kbar to 70 kOe, show a discontinuous change from an antiferromagnetic ground state below 15 kbar to a superconducting ground state above, and suggest that it is accompanied by a weak thermodynamic first-order transition. Bulk superconductivity appears, apparently with d-wave electron pairing, at the critical pressure, 15 kbar; with further increase in pressure a residual temperature-proportional term in the specific heat disappears.

cond-mat.str-el↗

arXiv2001

Anomalous Superconducting Properties and Field Induced Magnetism in CeCoIn5

In the heavy fermion superconductor CeCoIn5 (Tc=2.3K) the critical field is large, anisotropic and displays hysteresis. The magnitude of the critical-field anisotropy in the a-c plane can be as large as 70 kOe and depends on orientation. Critical field measurements in the (110) plane suggest 2D superconductivity, whereas conventional effective mass anisotropy is observed in the (100) plane. Two distinct field-induced magnetic phases are observed: Ha appears deep in the superconducting phase, while Hb intersects Hc2 at T=1.4 K and extends well above Tc. These observations suggest the possible realization of a direct transition from ferromagnetism to Fulde-Ferrel-Larkin-Ovchinnikov superconductivity in CeCoIn5.

cond-mat.str-el↗

arXiv2001

Unusual kondo behavior in the indium-rich heavy fermion antiferromagnet Ce3Pt4In13

We report the thermodynamic, magnetic, and electronic transport properties of the new ternary intermetallic system (Ce,La)3Pt4In13. Ce3Pt4In13 orders antiferromagnetically at 0.95 K while the non-magnetic compound La3Pt4In13 is a conventional 3.3 K superconductor. Kondo lattice effects appear to limit the entropy associated with the Neel transition to (1/4)Rln2 as an electronic contribution to the specific heat of gamma = 1 J/mole-Ce K2 is observed at TN; roughly 35% of this gamma survives the ordering transition. Hall effect, thermoelectric power, and ambient-pressure resistivity measurements confirm this interpretation. These results suggest that RKKY and Kondo interactions are closely balanced in this compound (TN = TK). Contrary to expectations based on the Doniach Kondo necklace model, applied hydrostatic pressure modestly enhances the magnetic ordering temperature with dTN/dP = +23 mK/kbar. As such Ce3Pt4In13 provides a counterexample to Kondo systems with similar Kondo and RKKY energy scales wherein applied pressure enhances TK at the expense of the ordered magnetic state.

cond-mat.str-el↗

arXiv2001

Magnetotransport of CeRhIn5

We report measurements of the temperature-dependent anisotropic resistivity and in-plane magnetoresistance on single crystals of the tetragonal heavy-fermion antiferromagnet (TN = 3.8 K) CeRhIn5. The measurements are reported in the temperature range 1.4 K to 300 K and in magnetic fields to 18 tesla. The resistivity is moderately anisotropic, with a room-temperature c-axis to in-plane resistivity ratio rho_c/rho_a(300 K) = 1.7. rho(T) measurements on the non-magnetic analog LaRhIn5 indicate that the anisotropy in the CeRhIn5 resistivity stems predominately from anisotropy in Kondo-derived magnetic scattering. In the magnetically ordered regime an applied field H reduces TN only slightly due to the small ordered moment (0.37mu_B) and magnetic anisotropy. The magnetoresistance (MR) below TN is positive and varies linearly with H. In the paramagnetic state a positive MR is present below 7.5 K, while a high-field negative contribution is evident at higher temperatures. The positive contribution decreases in magnitude with increasing temperature. Above 40 K the positive contribution is no longer observable, and the MR is negative. The low-T positive MR results from interactions with the Kondo-coherent state, while the high-T negative MR stems from single-impurity effects. The H and T-dependent magnetotransport reflects the magnetic anisotropy and Kondo interactions at play in CeRhIn5.

cond-mat.str-el↗

arXiv2001

On the origin of the zero-resistance anomaly in heavy fermion superconducting Ir: a clue from magnetic field and Rh-doping studies

We present the results of the specific heat and AC magnetic susceptibility measurements of $CeIr_{1-x}Rh_xIn_5$ for x from 0 to 0.5. As x is increased from 0 both quantities reflect the competition between two effects. The first is a suppression of superconductivity below the bulk transition temperature of T$_c = 0.4$ K, which is due to the pair breaking effect of Rh impurities. The second is an increase in the volume fraction of the superconducting regions above T$_c$, which we attribute to defect-induced strain. Analysis of the H-T phase diagram for CeIrIn$_5$obtained from the bulk probes and resistance measurements points to the filamentary origin of the inhomogeneous superconductivity at T$_ρ\approx 1.2$ K, where the resistance drops to zero. The identical anisotropies in the magnetic field dependence of the specific heat and the resistance anomalies in CeIrIn$_5$ indicate that the filamentary superconductivity is intrinsic, involving electrons from the part of the Fermi surface responsible for bulk superconductivity.

cond-mat.str-el↗

arXiv2001

Two energy scales and slow crossover in YbAl3

Experimental results for the susceptibility, specific heat, 4f occupation number, Hall effect and magnetoresistance for single crystals of YbAl$_{3}$ show that, in addition to the Kondo energy scale $k_{B}T_{K}$ $% \sim $ 670K, there is a low temperature scale $T_{coh}<50$K for the onset of coherence. Furthermore the crossover from the low temperature Fermi liquid regime to the high temperature local moment regime is slower than predicted by the Anderson impurity model. These effects may reflect the behavior of the Anderson Lattice in the limit of low conduction electron density.

cond-mat.str-el↗

arXiv2001

Temperature Dependent 5f-states in URu_2Si_2

A dramatic temperature dependent enhancement of U 5f spectral weight at $E_F$ is observed in angle-resolved photoemission measurements of $URu_2Si_2$ at the center of an X-point hole-pocket. Comparison of this temperature dependent behavior for excitation both at and below the U $5d \to 5f$ resonant threshold is presented.

cond-mat.str-el↗