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J. L. Ullmann

Publications and source records attributed to J. L. Ullmann.

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Estimation of M1 scissors mode strength for deformed nuclei in the medium to heavy mass region by statistical Hauser-Feshbach model calculations

Radiative neutron capture is an important nuclear reaction whose accurate description is needed for many applications ranging from nuclear technology to nuclear astrophysics. The description of such a process relies on the Hauser-Feshbach theory which requires the nuclear optical potential, level density and $γ$-strength function as model inputs. It has recently been suggested that the M1 scissors mode may explain discrepancies between theoretical calculations and evaluated data. We explore statistical model calculations with the strength of the M1 scissors mode estimated to be dependent on the nuclear deformation of the compound system. We show that the form of the M1 scissors mode improves the theoretical description of evaluated data and the match to experiment in both the fission product and actinide regions. Since the scissors mode occurs in the range of a few keV $\sim$ a few MeV, it may also impact the neutron capture cross sections of neutron-rich nuclei that participate in the rapid neutron capture process of nucleosynthesis. We comment on the possible impact to nucleosynthesis by evaluating neutron capture rates for neutron-rich nuclei with the M1 scissors mode active.

nucl-th

The $^{63}$Ni(n,$γ$) cross section measured with DANCE

The neutron capture cross section of the s-process branch nucleus $^{63}$Ni affects the abundances of other nuclei in its region, especially $^{63}$Cu and $^{64}$Zn. In order to determine the energy dependent neutron capture cross section in the astrophysical energy region, an experiment at the Los Alamos National Laboratory has been performed using the calorimetric 4$π$ BaF$_2$ array DANCE. The (n,$γ$) cross section of $^{63}$Ni has been determined relative to the well known $^{197}$Au standard with uncertainties below 15%. Various $^{63}$Ni resonances have been identified based on the Q-value. Furthermore, the s-process sensitivity of the new values was analyzed with the new network calculation tool NETZ.

nucl-ex

A 4p BaF2 detector for (n,g) cross section measurements at a spallation neutron source

The quest for improved neutron capture cross sections for advanced reactor concepts, transmutation of radioactive wastes as well as for astrophysical scenarios of neutron capture nucleosynthesis has motivated new experimental efforts based on modern techniques. Recent measurements in the keV region have shown that a 4p BaF2 detector represents an accurate and versatile instrument for such studies. The present work deals with the potential of such a 4p BaF2 detector in combination with spallation neutron sources, which offer large neutron fluxes over a wide energy range. Detailed Monte Carlo simulations with the GEANT package have been performed to investigate the critical backgrounds at a spallation facility, to optimize the detector design, and to discuss alternative solutions.

physics.ins-det

Background identification and suppression for the measurement of (n,g) reactions with the DANCE array at LANSCE

In the commissioning phase of the DANCE project (Detector for Advanced Neutron Capture Experiments) measurements have been performed with special emphasis on the identification and suppression of possible backgrounds for the planned (n,g) experiments. This report describes several background sources, observed in the experiment or anticipated from simulations, which will need to be suppressed in this and in similar detectors that are planned at other facilities. First successes are documented in the suppression of background from scattered neutrons captured in the detector as well as from the internal radiation. Experimental results and simulations using the GEANT code are compared.

nucl-ex

Cross Sections from 800 MeV Proton Irradiation of Terbium

A single terbium foil was irradiated with 800 MeV protons to ascertain the potential for production of lanthanide isotopes of interest in medical, astrophysical, and basic science research and to contribute to nuclear data repositories. Isotopes produced in the foil were quantified by gamma spectroscopy. Cross sections for 36 isotopes produced in the irradiation are reported and compared with predictions by the MCNP6 transport code using the CEM03.03, Bertini, and INCL+ABLA event generators. Our results indicate the need to accurately consider fission and fragmentation of relatively light target nuclei like terbium in the modeling of nuclear reactions at 800 MeV. The predictive power of the code was found to be different for each event generator tested but was satisfactory for most of the product yields in the mass region where spallation reactions dominate. However, none of the event generators' results are in complete agreement with measured data.

nucl-ex

Proton-induced cross sections relevant to production of 225Ac and 223Ra in natural thorium targets below 200 MeV

Cross sections for 223,225Ra, 225Ac and 227Th production by the proton bombardment of natural thorium targets were measured at proton energies below 200 MeV. Our measurements are in good agreement with previously published data and offer a complete excitation function for 223,225Ra in the energy range above 90 MeV. Comparison of theoretical predictions with the experimental data shows reasonable-to-good agreement. Results indicate that accelerator-based production of 225Ac and 223Ra below 200 MeV is a viable production method.

nucl-ex

225-Ac and 223-Ra Production via 800 MeV Proton Irradiation of Natural Thorium Target

Cross sections for the formation of 225,227-Ac, 223,225-Ra, and 227-Th via the proton bombardment of natural thorium targets were measured at a nominal proton energy of 800 MeV. No earlier experimental cross section data for the production of 223,225-Ra, 227-Ac and 227-Th by this method were found in the literature. A comparison of theoretical predictions with the experimental data shows agreement within a factor of two. Results indicate that accelerator-based production of 225-Ac and 223-Ra is a viable production method.

nucl-ex

Neutron Resonance Data Exclude Random Matrix Theory

Almost since the time it was formulated, the overwhelming consensus has been that random matrix theory (RMT) is in excellent agreement with neutron resonance data. However, over the past few years, we have obtained new neutron-width data at Oak Ridge and Los Alamos National Laboratories that are in stark disagreement with this theory. We also have reanalyzed neutron widths in the most famous data set, the nuclear data ensemble (NDE), and found that it is seriously flawed, and, when analyzed carefully, excludes RMT with high confidence. More recently, we carefully examined energy spacings for these same resonances in the NDE using the $Δ_{3}$ statistic. We conclude that the data can be found to either confirm or refute the theory depending on which nuclides and whether known or suspected p-wave resonances are included in the analysis, in essence confirming results of our neutron-width analysis of the NDE. We also have examined radiation widths resulting from our Oak Ridge and Los Alamos measurements, and find that in some cases they do not agree with RMT. Although these disagreements presently are not understood, they could have broad impact on basic and applied nuclear physics, from nuclear astrophysics to nuclear criticality safety.

nucl-ex

Abrupt Change in Radiation-Width Distribution for 147Sm Neutron Resonances

We obtained total radiation widths of s-wave resonances through R-matrix analysis of 147Sm(n,gamma) cross-sections. Distributions of these widths differ markedly for resonances below and above 300 eV, in stark contrast to long-established theory. We show that this change, as well as a similar change in the neutron-width distribution reported previously, are reflected in abrupt increases in both the average 147Sm(n,gamma) cross section and fluctuations about the average near 300 eV. Such effects could have important consequences for applications such as nuclear astrophysics and nuclear criticality safety.

nucl-ex

Non-Statistical Effects in Neutron Capture

There have been many reports of non-statistical effects in neutron-capture measurements. However, reports of deviations of reduced-neutron-width distributions from the expected Porter-Thomas (PT) shape largely have been ignored. Most of these deviations have been reported for odd-A nuclides. Because reliable spin (J) assignments have been absent for most resonances for such nuclides, it is possible that reported deviations from PT might be due to incorrect J assignments. We recently developed a new method for measuring spins of neutron resonances by using the DANCE detector at LANSCE. Measurements made with a 147Sm sample allowed us to determine spins of almost all known resonances below 1 keV. Furthermore, analysis of these data revealed that the reduced-neutron-width distribution was in good agreement with PT for resonances below 350 eV, but in disagreement with PT for resonances between 350 and 700 eV. Our previous (n,alpha) measurements had revealed that the alpha strength function also changes abruptly at this energy. There currently is no known explanation for these two non-statistical effects. Recently, we have developed another new method for determining the spins of neutron resonances. To implement this technique required a small change (to record pulse-height information for coincidence events) to a much simpler apparatus: A pair of C6D6 gamma-ray detectors which we have employed for many years to measure neutron-capture cross sections at ORELA. Measurements with a 95Mo sample revealed that not only does the method work very well for determining spins, but it also makes possible parity assignments. Taken together, these new techniques at LANSCE and ORELA could be very useful for further elucidation of non-statistical effects.

nucl-ex

Spin measurements for 147Sm+n resonances: Further evidence for non-statistical effects

We have determined the spins J of resonances in the 147Sm(n,gamma) reaction by measuring multiplicities of gamma-ray cascades following neutron capture. Using this technique, we were able to determine J values for all but 14 of the 140 known resonances below En = 1 keV, including 41 firm J assignments for resonances whose spins previously were either unknown or tentative. These new spin assignments, together with previously determined resonance parameters, allowed us to extract separate level spacings and neutron strength functions for J = 3 and 4 resonances. Furthermore, several statistical test of the data indicate that very few resonances of either spin have been missed below En = 700eV. Because a non-statistical effect recently was reported near En = 350 eV from an analysis of 147Sm(n,alpha) data, we divided the data into two regions; 0 < En < 350 eV and 350 < En < 700 eV. Using neutron widths from a previous measurement and published techniques for correcting for missed resonances and for testing whether data are consistent with a Porter-Thomas distribution, we found that the reduced-neutron-width distribution for resonances below 350 eV is consistent with the expected Porter-Thomas distribution. On the other hand, we found that reduced-neutron-width data in the 350 < En < 700 eV region are inconsistent with a Porter-Thomas distribution, but in good agreement with a chi-squared distribution having two or more degrees of freedom. We discuss possible explanations for these observed non-statistical effects and their possible relation to similar effects previously observed in other nuclides.

nucl-ex

GEANT simulations of neutron capture experiments with a 4p BaF2 detector

The goal of this research project is to give quantitative information useful for the design of a g-ray detector to investigate neutron capture (n, g) reactions on radioactive nuclei at the Manuel Lujan Jr. Neutron Scattering Center (MLNSC) moderated neutron source at LANSCE. Data for neutron energies from thermal up to approximately 500 keV are desired. The radioactive nuclei can have half-lives as short as a few months. With the sample sizes foreseen, typically 1 mg, the radioactive decay rate can exceed tens of Curies (Ci).

nucl-ex

Pinning Action of Correlated Disorder against Equilibrium Properties of HgBa$_2$Ca$_2$Cu$_3$O$_x$: a Delicate Balance

We report significant alteration of the equilibrium properties of the superconductor HgBa$_2$Ca$_2$Cu$_3$O$_x$ when correlated disorder in the form of randomly oriented columnar tracks is introduced via induced fission of Hg-nuclei. From studies of the equilibrium magnetization $M_{eq}$ and the persistent current density over a wide range of temperatures, applied magnetic fields, and track densities up to a ``matching field'' of 3.4 Tesla, we observe that the addition of more columnar tracks acting as pinning centers is progressively offset by reductions in the magnitude of $M_{eq}$. Invoking anisotropy induced ``refocusing'' of the random track array and incorporating vortex-defect interactions, we find that this corresponds to increases in the London penetration depth $λ$; this reduces the vortex line energy and consequently reduces the pinning effectiveness of the tracks.

cond-mat.supr-con

Current density and reversible magnetization of HgBa(2)Ca(2)Cu(3)O(x) superconductors containing randomly oriented columnar defects

Bulk polycrystalline HgBa(2)Ca(2)Cu(3)O(x) materials were irradiated with 0.8 GeV protons to form randomly oriented columnar defects, by induced fission of Hg-nuclei. Proton fluences from 0 to 35 times 10^{16} cm^{-2} were used to install defects with area densities up to a "matching field" of 3.4 Tesla. Studies were conducted on the dependence of the equilibrium magnetization and the intragrain persistent current density on temperature and applied magnetic field, at various defect densities. The magnetization was modeled using London theory with the addition of vortex-defect interactions.

cond-mat.supr-con

Vortex pinning in high-Tc materials via randomly oriented columnar defects, created by GeV proton-induced fission fragments

Extensive work has shown that irradiation with 0.8 GeV protons can produce randomly oriented columnar defects (CD's) in a large number of HTS materials, specifically those cuprates containing Hg, Tl, Pb, Bi, and similar heavy elements. Absorbing the incident proton causes the nucleus of these species to fission, and the recoiling fission fragments create amorphous tracks, i.e., CD's. The superconductive transition temperature Tc decreases linearly with proton fluence and we analyze how the rate depends on the family of superconductors. In a study of Tl-2212 materials, adding defects decreases the equilibrium magnetization Meq(H) significantly in magnitude and changes its field dependence; this result is modeled in terms of vortex pinning. Analysis of the irreversible magnetization and its time dependence shows marked increases in the persistent current density and effective pinning energy, and leads to an estimate for the elementary attempt time for vortex hopping, tau ~ 4x10^(-9) s.

cond-mat.supr-con