arXiv subjects

J. M. Allmond

Publications and source records attributed to J. M. Allmond.

At least 19 recordsLinked to original sources

arXiv2026

Commissioning the Resonance Ionization Spectroscopy Experiment at FRIB

This manuscript reports on the commissioning of the Resonance Ionization Spectroscopy Experiment (RISE) at the BECOLA facility at FRIB. The new instrument implements the collinear resonance ionization spectroscopy technique for sensitive measurements of isotope shifts and hyperfine structure of short-lived isotopes produced at FRIB. The existing BECOLA beamline was extended to integrate an electrostatic ion-beam bender and an ion detector at ultra-high vacuum. An injection-seeded Ti:Sapphire laser and a multi-harmonic pulsed Nd:YAG laser were installed to perform resonant excitation and selective ionization. Commissioning tests were performed to demonstrate the capabilities of the new instrument by measuring the hyperfine structure of stable $^{27}$Al produced in an offline ion source. The RISE instrument is ready and operational for future studies of short-lived isotopes at FRIB.

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arXiv2025

Beta-decay Half Lives beyond $^{54}$Ca: A Systematic Survey of Decay Properties approaching the Neutron Dripline

In an experiment performed at the Facility for Rare Isotope Beams (FRIB) using the FRIB Decay Station initiator (FDSi), 15 new half lives of isotopes near $^{54}$Ca were measured. A new method of extracting lifetimes from experimental data, taking into account the unknown $β$-delayed neutron emission branches of very neutron-rich nuclei, was developed to enable systematic uncertainty analysis. The experiment observed a dramatic change in the half-life systematics for the isotopes with neutron number N =34. Beyond N =34, the decline of nuclear lifetime is much slower, leading to longer than anticipated lifetimes for near-dripline nuclei. State-of-the-art shell-model calculations can explain the experimental results for Z$>$19 nuclei, revealing the imprint of shell effects and the need for modification of single-particle neutron states. The results from a newly developed QRPA model with potential for making global predictions were also tested against the experimental results and good agreement was found.

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arXiv2025

Triaxiality and shape dynamics in $^{70}$Ge

The electromagnetic properties of low-lying states in $^{70}$Ge were investigated via multi-step Coulomb excitation of a $^{70}$Ge beam impinging on a $^{208}$Pb target at the ATLAS facility of the Argonne National Laboratory. A total of 27 transitional elements and six diagonal matrix elements coupling 11 low-lying states, were extracted from the measured cross sections. These were used to calculate reduced transition probabilities, spectroscopic quadrupole moments, and rotational invariant shape parameters, providing enhanced precision and expanding on previous studies. The experimental data were compared within several theoretical frameworks, including the generalized triaxial rotor model, configuration interaction shell-model calculations, and computations within the combined frameworks of relativistic density functional theory and the five-dimensional collective Hamiltonian. The results demonstrate a good agreement with the experimental data and, in conjunction with calculations using a two-state mixing model, support significant triaxiality and strong mixing between the $0^+_1$ and $0^+_2$ states. This results in the magnitudes of their respective quadrupole deformations $[β_\text{rms}(0^+_1) = 0.228\,(3),\,β_\text{rms}(0^+_2) = 0.273\,(1)]$ being more similar than previously observed. The implications of these results for understanding the complex shape coexistence phenomena, the role of triaxiality, and shape evolution along the Ge isotopic chain are discussed.

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arXiv2025

Modeling of Light Production in Inorganic Scintillators

In recent experiments, inorganic scintillators have been used to study the decays of exotic nuclei, providing an alternative to silicon detectors and enabling measurements that were previously impossible. However, proper use of these materials requires us to understand and quantify the scintillation process. In this work, we propose a framework based on that of Birks [Proc. Phys. Soc. A 64, 874] and Meyer and Murray [Phys. Rev. 128, 98] to model the light output of inorganic scintillators in response to beams of energetic heavy ions over a broad range of energies. Our model suggests that, for sufficiently heavy ions at high energies, the majority of the light output is associated with the creation of delta electrons, which are induced by the passage of the beam through the material. These delta electrons dramatically impact the response of detection systems when subject to ions with velocities typical of beams in modern fragmentation facilities. We test the accuracy of our model with data from Lutetium Yttrium Orthosilicate (LYSO:Ce), a common inorganic scintillator. We compare calculated light production and quenching factors with experimental data for heavy ions of varying mass and energy as well as make a quantitative estimate of the effects of delta rays on overall light output. The model presented herein will serve as a basic framework for further studies of scintillator response to heavy ions. Our results are crucial in planning future experiments where relativistic exotic nuclei are interacting with scintillator detectors.

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arXiv2025

Universal Effective Charges in the $sd$ and $fp$ Shells

The 247-keV state in $^{54}$Sc, populated in the $β$ decay of $^{54}$Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the $1^+$ member of the $πf_{7/2}\otimesνf_{5/2}$ spin-coupled multiplet, which decays to the $3^+,πf_{7/2} \otimes νp_{1/2}$ ground state. The new half-life corresponds to a pure $E2$ transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous $B(E2)$ value in the neutron-rich $fp$ region to date for a nucleus with valence protons above $Z=20$. Notably, it is roughly four times larger than the $B(E2; 1/2^{-} \rightarrow 5/2^{-})$ value in $^{55}$Ca. The results, as compared to semi-empirical and ab initio shell-model calculations, indicate (1) a weak $N=34$ sub-shell gap relative to $N = 32$, (2) a large $E2$ enhancement in Sc as compared to Ca due to $1p-1h$ proton excitations across $Z=28$, and (3) empirical effective proton and neutron charges, $e_π$ = 1.30(8)$e$ and $e_ν$ = 0.452(7)$e$, respectively, that are in contrast to reports of $e_π\approx 1.1-1.15e$ and $e_ν\approx 0.6-0.8e$ for $fp$-shell nuclei near $N = Z$. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the $sd$ and $fp$ shells.

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arXiv2025

Object Detection with Deep Learning for Rare Event Search in the GADGET II TPC

In the pursuit of identifying rare two-particle events within the GADGET II Time Projection Chamber (TPC), this paper presents a comprehensive approach for leveraging Convolutional Neural Networks (CNNs) and various data processing methods. To address the inherent complexities of 3D TPC track reconstructions, the data is expressed in 2D projections and 1D quantities. This approach capitalizes on the diverse data modalities of the TPC, allowing for the efficient representation of the distinct features of the 3D events, with no loss in topology uniqueness. Additionally, it leverages the computational efficiency of 2D CNNs and benefits from the extensive availability of pre-trained models. Given the scarcity of real training data for the rare events of interest, simulated events are used to train the models to detect real events. To account for potential distribution shifts when predominantly depending on simulations, significant perturbations are embedded within the simulations. This produces a broad parameter space that works to account for potential physics parameter and detector response variations and uncertainties. These parameter-varied simulations are used to train sensitive 2D CNN object detectors. When combined with 1D histogram peak detection algorithms, this multi-modal detection framework is highly adept at identifying rare, two-particle events in data taken during experiment 21072 at the Facility for Rare Isotope Beams (FRIB), demonstrating a 100% recall for events of interest. We present the methods and outcomes of our investigation and discuss the potential future applications of these techniques.

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arXiv2024

The evidence of $N=16$ shell closure and $β$-delayed neutron emission from $^{25}$F

We measured the $β$-delayed neutron emission from $^{25}$F for the first time at the Facility for Rare Isotope Beams (FRIB). Using combined neutron and $γ$-ray detector systems of the FRIB Decay Station Initiator (FDSi), we observed $β$-decay transitions populating neutron unbound states between 4.2 and 8 MeV in $^{25}$Ne. The experimental results led to the revision of the $β$-decay half-life and $β$-delayed neutron-emission probability of $^{25}$F. The $β$-decay strength distribution of $^{25}$F extracted from the data agrees with the shell-model predictions using the USDB and SDPF-M effective interactions. This result indicates that the spherical neutron $N = 16$ shell gap persists in $^{25}$F and $^{25}$Ne.

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arXiv2024

Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $γγ$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $γγ$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $γγ$-coincidence and $γ$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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arXiv2024

Suppressed Electric Quadrupole Collectivity in $^{49}$Ti

Single-step Coulomb excitation of $^{46,48,49,50}$Ti is presented. A complete set of $E2$ matrix elements for the quintuplet of states in $^{49}$Ti, centered on the $2^+$ core excitation, was measured for the first time. A total of nine $E2$ matrix elements are reported, four of which were previously unknown. $^{49}_{22}$Ti$_{27}$ shows a $20\%$ quenching in electric quadrupole transition strength as compared to its semi-magic $^{50}_{22}$Ti$_{28}$ neighbour. This $20\%$ quenching, while empirically unprecedented, can be explained with a remarkably simple two-state mixing model, which is also consistent with other ground-state properties such as the magnetic dipole moment and electric quadrupole moment. A connection to nucleon transfer data and the quenching of single-particle strength is also demonstrated. The simplicity of the $^{49}$Ti-$^{50}$Ti pair (i.e., approximate single-$j$ $0f_{7/2}$ valence space and isolation of yrast states from non-yrast states) provides a unique opportunity to disentangle otherwise competing effects in the ground-state properties of atomic nuclei, the emergence of collectivity, and the role of proton-neutron interactions.

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arXiv2024

New isomeric transition in $^{36}$Mg: Bridging the N=20 and N=28 islands of inversion

We observed a new isomeric gamma transition at 168 keV in $^{36}$Mg, with a half-life of T$_{1/2}$=[130-500]$(\pm40)(^{+800}_{-20})_{sys}$ ns. We propose that the observed transition de-excites a new 0$^+$ isomeric state and populates the previously known first 2$^+$ state. The existence of this isomer is consistent with the predictions of the large-scale shell model calculations of $^{36}$Mg using the sdpf-u-mix interaction. The observed excitation energy of the second 0$^+$ state is caused by the small energy separation between two prolate-deformed configurations where the intruder configuration corresponds to two neutron excitations from the {\it sd} to the {\it pf} shell. Within this interpretation, $^{36}$Mg becomes the crossing point between nuclei in which ground state deformed/superdeformed configurations are caused by the dominance of N=20 intruders ($^{32,34}$Mg) and nuclei where deformed configurations are associated with N=28 intruders ($^{38}$Mg and beyond). We found the lack of three-body monopole corrections in other effective interactions results in a predominance of N=20 intruder configurations past $^{38}$Mg incompatible with our observation. We conclude that $^{36}$Mg bridges the N=20 and N=28 islands of inversion, forming the so-called Big Island of Deformation.

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arXiv2023

Understanding Excitations in $^{59,61}$Co, $^{59}$Ni

High spin states in $^{59}$Co ($Z=27$), $^{59}$Ni ($Z=28$) and $^{61}$Co have been populated by the fusion evaporation reactions, $^{48}$Ti($^{14}$C, p2n)$^{59}$Co, $^{48}$Ti($^{14}$C, 3n)$^{59}$Ni, and $^{50}$Ti($^{14}$C, p2n)$^{61}$Co. The 9 MV tandem accelerator at the John D Fox Laboratory, Florida State University (FSU) was used to accelerate the $^{14}$C beam and the de-exciting $γ$ rays were detected by the FSU detector array consisting of six High Purity Germanium (HPGe) clover detectors, and three single crystals. Directional correlation of the $γ$ rays de-exciting oriented states (DCO ratios) and polarization asymmetry measurements helped to establish spin and parities of the excited states whenever possible. The level scheme of $^{59}$Co has been expanded with the inclusion of positive parity states up to 31/2$^+$ at around 11 MeV. The $^{59}$Ni positive parity states known from previous study were verified with modifications to some of the spins and parities. On the other hand, the negative parity states were extended to 31/2 at an excitation energy of 12 MeV. No new transition was observed for $^{61}$Co, but one of the major bands has been reassigned as consisting of positive parity states by reason of this study which is a candidate for magnetic rotation band. Cross shell excitations were observed in the three nuclei studied and the prominent role of excitation to g$_{9/2}$ orbital crossing the $N=40$ shell gap was established in relation to collective excitation in these nuclei by comparison with large-scale shell model calculations.

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arXiv2023

Microsecond Isomer at the N=20 Island of Shape Inversion Observed at FRIB

Excited-state spectroscopy from the first Facility for Rare Isotope Beams (FRIB) experiment is reported. A 24(2)-$μ$s isomer was observed with the FRIB Decay Station initiator (FDSi) through a cascade of 224- and 401-keV $γ$ rays in coincidence with $^{32}\textrm{Na}$ nuclei. This is the only known microsecond isomer ($1{\text{ }μ\text{s}}\leq T_{1/2} < 1\text{ ms}$) in the region. This nucleus is at the heart of the $N=20$ island of shape inversion and is at the crossroads of spherical shell-model, deformed shell-model, and ab initio theories. It can be represented as the coupling of a proton hole and neutron particle to $^{32}\textrm{Mg}$, $^{32}\textrm{Mg}+π^{-1} + ν^{+1}$. This odd-odd coupling and isomer formation provides a sensitive measure of the underlying shape degrees of freedom of $^{32}\textrm{Mg}$, where the onset of spherical-to-deformed shape inversion begins with a low-lying deformed $2^+$ state at 885 keV and a low-lying shape-coexisting $0_2^+$ state at 1058 keV. We suggest two possible explanations for the 625-keV isomer in $^{32}$Na: a $6^-$ spherical shape isomer that decays by $E2$ or a $0^+$ deformed spin isomer that decays by $M2$. The present results and calculations are most consistent with the latter, indicating that the low-lying states are dominated by deformation.

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arXiv2022

E2 Rotational Invariants of $0^+_1$ and $2^+_1$ states for $^{106}$Cd: the Emergence of Collective Rotation

The collective structure of $^{106}$Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/$A$ beam of $^{106}$Cd on a 1.1 mg/cm$^2$ $^{208}$Pb target using GRETINA-CHICO2 at ATLAS. Fourteen $E2$ matrix elements were obtained. The nucleus $^{106}$Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of $E2$ matrix elements. The ${\langle 0_2^+ ||E2||2_1^+ \rangle}$ matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, $\langle Q^2 \rangle$, of the first-excited $2_1^+$ level relative to the $0_1^+$ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in $^{114}$Cd by C. Fahlander et al., Nucl. Phys. A485, 327 (1988), which is complicated by low-lying shape coexistence near midshell.

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arXiv2022

CLARION2-TRINITY: a Compton-suppressed HPGe and GAGG:Ce-Si-Si array for absolute cross-section measurements with heavy ions

The design and performance of a new Compton-suppressed HPGe and charged-particle array, CLARION2-TRINITY, are described. The TRINITY charged-particle array is comprised of 64 Cerium-doped Gadolinium Aluminium Gallium Garnet (GAGG:Ce) crystals configured into five rings spanning 7-54 degrees, and two annular silicon detectors that can shadow or extend the angular coverage to backward angles with minimal $γ$-ray attenuation. GAGG:Ce is a non-hygroscopic, bright, and relatively fast scintillator with a light distribution well matched to SiPMs. Count rates up to 40 kHz per crystal are sustainable. Fundamental characteristics of GAGG:Ce are measured and presented, including light- and heavy-ion particle identification (PID) capability, pulse-height defects, radiation hardness, and emission spectra. The CLARION2 array consists of up to 16 Compton-suppressed HPGe Clover detectors ($\approx4\%$ efficiency at 1 MeV) configured into four rings (eight HPGe crystal rings) using a non-Archimedean geometry that suppresses back-to-back coincident 511-keV gamma rays. The entire array is instrumented with 100- and 500-MHz (14 bit) waveform digitizers which enable triggerless operation, pulse-shape discrimination, fast timing, and pileup correction. Finally, two examples of experimental data taken during the commissioning of the CLARION2-TRINITY system are given: a PID spectrum from $^{16}$O + $^{18}$O fusion-evaporation, and PID and Doppler-corrected $γ$-ray spectra from $^{48}$Ti + $^{12}$C Coulomb excitation.

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arXiv2022

Neutron transfer reactions on the ground state and isomeric state of a 130Sn beam

The structure of nuclei around the neutron-rich nucleus 132Sn is of particular interest due to the vicinity of the Z = 50 and N = 82 shell closures and the r-process nucleosynthetic path. Four states in 131Sn with a strong single-particle-like component have previously been studied via the (d,p) reaction, with limited excitation energy resolution. The 130Sn(9Be,8Be)131Sn and 130Sn(13C,12C)131Sn single-neutron transfer reactions were performed in inverse kinematics at the Holifield Radioactive Ion Beam Facility using particle-gamma coincidence spectroscopy. The uncertainties in the energies of the single-particle-like states have been reduced by more than an order of magnitude using the energies of gamma rays. The previous tentative Jpi values have been confirmed. Decays from high-spin states in 131Sn have been observed following transfer on the isomeric component of the 130Sn beam. The improved energies and confirmed spin-parities of the p-wave states important to the r-process lead to direct-semidirect cross-sections for neutron capture on the ground state of 130Sn at 30 keV that are in agreement with previous analyses. A similar assessment of the impact of neutron-transfer on the isomer would require significant nuclear structure and reaction theory input. There are few measurements of transfer reaction on isomers, and this is the first on an isomer in the 132Sn region.

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arXiv2021

ADC Nonlinearity Correction for the MAJORANA DEMONSTRATOR

Imperfections in analog-to-digital conversion (ADC) cannot be ignored when signal digitization requirements demand both wide dynamic range and high resolution, as is the case for the Majorana Demonstrator 76Ge neutrinoless double beta decay search. Enabling the experiment's high-resolution spectral analysis and efficient pulse shape discrimination required careful measurement and correction of ADC nonlinearites. A simple measurement protocol was developed that did not require sophisticated equipment or lengthy data taking campaigns. A slope-dependent hysteresis was observed and characterized. A correction applied to digitized waveforms prior to signal processing reduced the differential and integral nonlinearites by an order of magnitude, eliminating these as dominant contributions to the systematic energy uncertainty at the double-beta decay Q value.

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arXiv2021

Ground-state and decay properties of neutron-rich 106Nb

The ground-state properties of neutron-rich 106Nb and its beta decay into 106Mo have been studied using the CARIBU radioactive-ion-beam facility at Argonne National Laboratory. Niobium-106 ions were extracted from a 252Cf fission source and mass separated before being delivered as low-energy beams to the Canadian Penning Trap, as well as the X-Array and SATURN beta-decay-spectroscopy station. The measured 106Nb ground-state mass excess of -66202.0(13) keV is consistent with a recent measurement but has three times better precision; this work also rules out the existence of a second long-lived, beta-decaying state in 106Nb above 5 keV in excitation energy. The decay half-life of 106Nb was measured to be 1.097(21) s, which is 8% longer than the adopted value. The level scheme of the decay progeny, 106Mo, has been expanded up to approximately 4 MeV. The distribution of decay strength and considerable population of excited states in 106Mo of J >= 3 emphasises the need to revise the adopted Jpi = 1- ground-state spin-parity assignment of 106Nb; it is more likely to be J => 3.

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arXiv2020

First candidates for γ vibrational bands built on the [505]11/2- neutron orbital in odd-A Dy isotopes

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd(α,2n)157Dy and 148Nd(12C, 5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ= 2+ γ vibrational band, built on the [505]11/2- neutron orbital, in both odd-A 155, 157Dy isotopes. The coupling of the first excited K=0+ states or the so-called \b{eta} vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2- orbital, to produce a Kπ=11/2- band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the core nuclei 154Dy and 156Dy are also discussed.

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