arXiv subjects

J. M. Maxson

Publications and source records attributed to J. M. Maxson.

12 recordsLinked to original sources

arXiv2025

Multi-Objective Optimizations of High Gradient C-band Photoinjector for High Bunch Charge Applications

The high gradients potentially achievable in distributed-coupling C-band photoinjectors make them attractive for many high brightness applications. Here we discuss optimization results for a 1.6 cell C-band photoinjector with a 240 MV/m peak field at the cathode that delivers a 250 pC electron bunch charge. We use a Multi-Objective Genetic Algorithm (MOGA), obtaining a Pareto front of emittance vs. bunch length. We also perform MOGA optimizations including an aperture to retain only a bright beam core. We find this reduces the emittance of the final beam by more than factor of 2 in some cases. For example, we find that at a root mean square bunch length of 1.6 ps, the use of an aperture improves the transverse emittance from 120 nm to 58 nm assuming negligible photocathode intrinsic emittance. The sacrificial charge at the periphery of the electron beam removed by the aperture linearizes the final slice phase space inside of the remaining beam core. The results obtained surpass the experimental state-of-the-art for beamlines with similar bunch charge.

physics.acc-ph↗

arXiv2025

Photoinduced twist and untwist of moir\'e superlattices in TMDC heterobilayers

Two-dimensional moir\'e materials are formed by artificially stacking atomically thin monolayers. A wealth of correlated and topological quantum phases can be engineered via precise choice of stacking geometry. These designer electronic properties depend crucially on interlayer coupling and atomic registry. An important open question is how atomic registry responds on ultrafast timescales to optical excitation and whether the moir\'e geometry can be dynamically reconfigured to tune emergent phenomena in real time. Here we show that femtosecond photoexcitation drives a coherent twist-untwist motion of the moir\'e superlattice in $2^\circ$ and $57^\circ$ twisted WSe$_2$/MoSe$_2$ heterobilayers, resolved directly by ultrafast electron diffraction. Upon above-band-gap photoexcitation, the moir\'e superlattice diffraction features are enhanced within 1 ps and subsequently suppressed several picoseconds after, deviating markedly from typical photoinduced lattice heating. Kinetic diffraction analysis, supported by simulations of the sample dynamics, indicates a peak-to-trough local twist angle modulation of $0.6^\circ$, correlated with a sub-THz frequency moir\'e phonon. This motion is driven by ultrafast charge transfer that transiently increases interlayer attraction. Our results could lead to ultrafast control of moir\'e periodic lattice distortions and, by extension, the local moir\'e potential that shapes excitons, polarons, and correlation-driven behaviors

cond-mat.mtrl-sci↗

arXiv2024

Measurement of Spin-Polarized Photoemission from Wurtzite and Zinc-Blende Gallium Nitride Photocathodes

Spin-polarized photoemission from wurtzite and zinc-blende gallium nitride (GaN) photocathodes has been observed and measured for the first time. The p-doped GaN photocathodes were epitaxially grown and activated to negative electron affinity (NEA) with a cesium monolayer deposited on their surfaces. A field-retarding Mott polarimeter was used to measure the spin-polarization of electrons photoemitted from the top of the valence band. A spectral scan with a tunable optical parametric amplifier (OPA) constructed to provide low-bandwidth light revealed peak spin polarizations of 17% and 29% in the wurtzite and zinc-blende photocathodes, respectively. Zinc-blende GaN results are analyzed with a spin-polarization model accounting for experimental parameters used in the measurements, while possible mechanisms influencing the obtained spin polarization values of wurtzite GaN are discussed.

physics.acc-ph↗

arXiv2024

Compensating slice emittance growth in high brightness photoinjectors using sacrificial charge

Achieving maximum electron beam brightness in photoinjectors requires detailed control of the 3D bunch shape and precise tuning of the beam focusing. Even in state-of-the-art designs, slice emittance growth due to nonlinear space charge forces and partial nonlaminarity often remains non-negligible. In this work we introduce a new means to linearize the transverse slice phase space: a sacrificial portion of the bunch's own charge distribution, formed into a wavebroken shock front by highly nonlinear space charge forces within the gun, whose downstream purpose is to dynamically linearize the desired bunch core. We show that linearization of an appropriately prepared bunch can be achieved via strongly nonlaminar focusing of the sacrificial shock front, while the inner core focuses laminarly. This leads to a natural spatial separation of the two distributions: a dense core surrounded by a diffuse halo of sacrificial charge that can be collimated. Multi-objective genetic algorithm optimizations of the ultra-compact x-ray free electron laser (UCXFEL) injector employ this concept, and we interpret it with an analytic model that agrees well with the simulations. In simulation we demonstrate a final bunch charge of 100 pC, peak current $\sim 30$ A, and a sacrificial charge of 150 pC (250 pC total emitted from cathode) with normalized emittance growth of $<20$ nm-rad due to space charge. This implies a maximum achievable brightness approximately an order of magnitude greater than existing FEL injector designs.

physics.acc-ph↗

arXiv2023

Multi-scale time-resolved electron diffraction: A case study in moiré materials

Ultrafast-optical-pump -- structural-probe measurements, including ultrafast electron and x-ray scattering, provide direct experimental access to the fundamental timescales of atomic motion, and are thus foundational techniques for studying matter out of equilibrium. High-performance detectors are needed in scattering experiments to obtain maximum scientific value from every probe particle. We deploy a hybrid pixel array direct electron detector to perform ultrafast electron diffraction experiments on a WSe$_2$/MoSe$_2$ 2D heterobilayer, resolving the weak features of diffuse scattering and moiré superlattice structure without saturating the zero order peak. Enabled by the detector's high frame rate, we show that a chopping technique provides diffraction difference images with signal-to-noise at the shot noise limit. Finally, we demonstrate that a fast detector frame rate coupled with a high repetition rate probe can provide continuous time resolution from femtoseconds to seconds, enabling us to perform a scanning ultrafast electron diffraction experiment that maps thermal transport in WSe$_2$/MoSe$_2$ and resolves distinct diffusion mechanisms in space and time.

physics.ins-det↗

arXiv2023

Atomically smooth films of CsSb: a chemically robust visible light photocathode

Alkali antimonide semiconductor photocathodes provide a promising platform for the generation of high brightness electron beams, which are necessary for the development of cutting-edge probes including x-ray free electron lasers and ultrafast electron diffraction. However, to harness the intrinsic brightness limits in these compounds, extrinsic degrading factors, including surface roughness and contamination, must be overcome. By exploring the growth of CsxSb thin films monitored by in situ electron diffraction, the conditions to reproducibly synthesize atomically smooth films of CsSb on 3C-SiC (100) and graphene coated TiO2 (110) substrates are identified, and detailed structural, morphological, and electronic characterization is presented. These films combine high quantum efficiency in the visible (up to 1.2% at 400 nm), an easily accessible photoemission threshold of 550 nm, low surface roughness (down to 600 pm on a 1 um scale), and a robustness against oxidation up to 15 times greater then Cs3Sb. These properties suggest that CsSb has the potential to operate as an alternative to Cs$_3$Sb in electron source applications where the demands of the vacuum environment might otherwise preclude the use of traditional alkali antimonides.

physics.acc-ph↗

arXiv2022

Four-Dimensional Emittance Measurements of Ultrafast Electron Diffraction Optics Corrected Up to Sextupole Order

Ultrafast electron diffraction (UED) is a technique in which short-pulse electron beams can probe the femtosecond-scale evolution of atomic structure in matter driven far from equilibrium. As an accelerator physics challenge, UED imposes stringent constraints on the brightness of the probe electron beam. The low normalized emittance employed in UED, often at the 10 nm scale and below, is particularly sensitive to both applied field aberrations and space charge effects. The role of aberrations is increasingly important in small probe systems that often feature multiple orders of magnitude variations in beam size during transport. In this work, we report the correction of normal quadrupole, skew quadrupole, and sextupole aberrations via dedicated corrector elements in an ultrafast electron micro-diffraction beamline. To do this, we generate precise 4-dimensional phase space maps of rf-compressed electron beams, and find excellent agreement with aberration-free space charge simulations. Finally, we discuss the role a probe-forming aperture can play in improving the brightness of bunches with appreciable space charge effects.

physics.acc-ph↗

arXiv2022

Ab initio study of the crystal and electronic structure of mono- and bi-alkali antimonides: Stability, Goldschmidt-like tolerance factors, and optical properties

Mono- and bi-alkali antimonides, X$_2$YSb (X and Y from Group I), are promising for next-generation electron emitters due to their capability of producing high-quality electron beams. However, these materials are not yet well understood, in part due to the technical challenges in growing pure, ordered alkali antimonides. For example, in the current literature there is a lack of complete understanding of the mechanically stable crystal structures of these materials. As a first step towards understanding this issue, this paper presents an ab initio study of stability of single-crystal mono- and bi-alkali antimonides in the $D0_3$ structure, the structure generally assumed in the literature for these materials. Finding that many of these materials actually are unstable in the $D0_3$ structure, we formulate a new set of Goldschmidt-like tolerance factors that accurately predict $D0_3$ stability using a procedure analogous to machine-learning perceptron-based analysis. Next, we consider possible stable structures for materials that we predict to be unstable in the $D0_3$ structure. Taking as examples the mono- and bi-alkali antimonides Cs$_3$Sb and Cs$_2$KSb, which also are technologically interesting for photoemission and photoabsorption applications, respectively, we note that the most unstable phonon displacements are consistent with the cubic structure, and we therefore perform extensive ab initio searches to identify potential ground-state structures in a cubic lattice. Our X-ray diffraction experiments confirm that indeed these two materials are not stable in the $D0_3$ structure and show scattering that is consistent with our new, proposed stable structures. Finally, we explore ab initio the implications of the breaking of the $D0_3$ symmetry on the electronic structure, showing significant impact on the location of the optical absorption edge.

cond-mat.mtrl-sci↗

arXiv2022

A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes

We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micron probe size, long coherence length, and $200$ fs rms time resolution. We measure the 5d (peak) beam brightness at the sample location in micro-diffraction mode to be $7 \times 10^{13} \ \mathrm{A}/\text{m}^2\text{-rad}^2$. To generate high brightness electron bunches, the system employs high efficiency, low emittance semiconductor photocathodes driven with a wavelength near the photoemission threshold at a repetition rate up to 250 kHz. We characterize spatial, temporal, and reciprocal space resolution of the apparatus. We perform proof-of-principle measurements of ultrafast heating in single crystal Au samples and compare experimental results with simulations that account for the effects of multiple-scattering.

physics.acc-ph↗

arXiv2021

A single-crystal alkali antimonide photocathode: high efficiency in the ultra-thin limit

The properties of photoemission electron sources determine the ultimate performance of a wide class of electron accelerators and photon detectors. To date, all high-efficiency visible-light photocathode materials are either polycrystalline or exhibit intrinsic surface disorder, both of which limit emitted electron beam brightness. In this letter we demonstrate the synthesis of epitaxial thin films of Cs$_3$Sb on 3C-SiC (001) using molecular-beam epitaxy. Films as thin as 4 nm have quantum efficiencies exceeding 2\% at 532 nm. We also find that epitaxial films have an order of magnitude larger quantum efficiency at 650 nm than comparable polycrystalline films on Si. Additionally, these films permit angle-resolved photoemission spectroscopy measurements of the electronic structure, which are found to be in good agreement with theory. Epitaxial films open the door to dramatic brightness enhancements via increased efficiency near threshold, reduced surface disorder, and the possibility of engineering new photoemission functionality at the level of single atomic layers.

physics.acc-ph↗

arXiv2021

Simulation of the transit-time optical stochastic cooling process in the Cornell Electron Storage Ring

In preparation for a demonstration of optical stochastic cooling in the Cornell Electron Storage Ring (CESR) we have developed a particle tracking simulation to study the relevant beam dynamics. Optical radiation emitted in the pickup undulator gives a momentum kick to that same particle in the kicker undulator. The optics of the electron bypass from pickup to kicker couples betatron amplitude and momentum offset to path length so that the momentum kick reduces emittance and momentum spread. Nearby electrons contribute an incoherent noise. Layout of the bypass line is presented that accommodates optics with a range of transverse and longitudinal cooling parameters. The simulation is used to determine cooling rates and their dependence on bunch and lattice parameters for bypass optics with distinct emittance and momentum acceptance.

physics.acc-ph↗

arXiv2020

Optical Stochastic Cooling with an Arc-Bypass in CESR

A proposed experiment to demonstrate Optical Stochastic Cooling (OSC) in the Cornell Electron Storage Ring (CESR) based on an arc-bypass design is presented. This arc-bypass provides significantly longer optical delay than the dog-leg style chicane, opening up the possibility of a multi-pass or staged optical amplifier that can achieve the gains required for effective cooling of hadron or heavy-ions. Beyond introducing the arc-bypass, in this paper we study the stability requirements for the dipoles comprising it and investigate the use of an optical feedback system to relax the dipole and light-path stability tolerances.

physics.acc-ph↗