arXiv subjects

J. Marganiec

Publications and source records attributed to J. Marganiec.

30 records · Page 2Linked to original sources

arXiv2014

Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN

Background:The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Reduce the $^{243}$Am(n,$γ$) cross section uncertainty. Method: The $^{243}$Am(n,$γ$) cross section has been measured at the n_TOF facility at CERN with a BaF$_{2}$ Total Absorption Calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The $^{243}$Am(n,$γ$) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature has been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the $^{243}$Am(n,$γ$) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries.

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arXiv2014

High accuracy determination of the $^{238}$U/$^{235}$U fission cross section ratio up to $\sim$1 GeV at n_TOF (CERN)

The $^{238}$U to $^{235}$U fission cross section ratio has been determined at n_TOF up to $\sim$1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets have been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at n_TOF have been suitably combined to yield a unique fission cross section ratio as a function of the neutron energy. The result confirms current evaluations up to 200 MeV. A good agreement is also observed with theoretical calculations based on the INCL++/Gemini++ combination up to the highest measured energy. The n_TOF results may help solving a long-standing discrepancy between the two most important experimental dataset available so far above 20 MeV, while extending the neutron energy range for the first time up to $\sim$1 GeV.

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arXiv2014

Measurement of the $^{12}$C($n,p$)$^{12}$B cross section at n_TOF (CERN) by in-beam activation analysis

The integral cross section of the $^{12}$C($n,p$)$^{12}$B reaction has been determined for the first time in the neutron energy range from threshold to several GeV at the n_TOF facility at CERN. The measurement relies on the activation technique, with the $β$-decay of $^{12}$B measured over a period of four half-lives within the same neutron bunch in which the reaction occurs. The results indicate that model predictions, used in a variety of applications, are mostly inadequate. The value of the integral cross section reported here can be used as a benchmark for verifying or tuning model calculations.

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arXiv2014

GEANT4 simulation of the neutron background of the C$_6$D$_6$ set-up for capture studies at n_TOF

The neutron sensitivity of the C$_6$D$_6$ detector setup used at n_TOF for capture measurements has been studied by means of detailed GEANT4 simulations. A realistic software replica of the entire n_TOF experimental hall, including the neutron beam line, sample, detector supports and the walls of the experimental area has been implemented in the simulations. The simulations have been analyzed in the same manner as experimental data, in particular by applying the Pulse Height Weighting Technique. The simulations have been validated against a measurement of the neutron background performed with a $^\mathrm{nat}$C sample, showing an excellent agreement above 1 keV. At lower energies, an additional component in the measured $^\mathrm{nat}$C yield has been discovered, which prevents the use of $^\mathrm{nat}$C data for neutron background estimates at neutron energies below a few hundred eV. The origin and time structure of the neutron background have been derived from the simulations. Examples of the neutron background for two different samples are demonstrating the important role of accurate simulations of the neutron background in capture cross section measurements.

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arXiv2014

$^{62}$Ni($n,γ$) and $^{63}$Ni($n,γ$) cross sections measured at n_TOF/CERN

The cross section of the $^{62}$Ni($n,γ$) reaction was measured with the time-of-flight technique at the neutron time-of-flight facility n_TOF at CERN. Capture kernels of 42 resonances were analyzed up to 200~keV neutron energy and Maxwellian averaged cross sections (MACS) from $kT=5-100$ keV were calculated. With a total uncertainty of 4.5%, the stellar cross section is in excellent agreement with the the KADoNiS compilation at $kT=30$ keV, while being systematically lower up to a factor of 1.6 at higher stellar temperatures. The cross section of the $^{63}$Ni($n,γ$) reaction was measured for the first time at n_TOF. We determined unresolved cross sections from 10 to 270 keV with a systematic uncertainty of 17%. These results provide fundamental constraints on $s$-process production of heavier species, especially the production of Cu in massive stars, which serve as the dominant source of Cu in the solar system.

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arXiv2014

Experimental neutron capture data of $^{58}$Ni from the CERN n_TOF facility

The $^{58}$Ni $(n,γ)$ cross section has been measured at the neutron time of flight facility n_TOF at CERN, in the energy range from 27 meV up to 400 keV. In total, 51 resonances have been analyzed up to 122 keV. Maxwellian averaged cross sections (MACS) have been calculated for stellar temperatures of kT$=$5-100 keV with uncertainties of less than 6%, showing fair agreement with recent experimental and evaluated data up to kT = 50 keV. The MACS extracted in the present work at 30 keV is 34.2$\pm$0.6$_\mathrm{stat}\pm$1.8$_\mathrm{sys}$ mb, in agreement with latest results and evaluations, but 12% lower relative to the recent KADoNIS compilation of astrophysical cross sections. When included in models of the s-process nucleosynthesis in massive stars, this change results in a 60% increase of the abundance of $^{58}$Ni, with a negligible propagation on heavier isotopes. The reason is that, using both the old or the new MACS, 58Ni is efficiently depleted by neutron captures.

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arXiv2013

Beyond the Neutron Drip-Line: The Unbound Oxygen Isotopes 25O and 26O

The very neutron-rich oxygen isotopes 25O and 26O are investigated experimentally and theoret- ically. In this first R3B-LAND experiment, the unbound states are populated at GSI via proton- knockout reactions from 26F and 27F at relativistic energies around 450 MeV/nucleon. From the kinematically complete measurement of the decay into 24O plus one or two neutrons, the 25O ground- state energy and lifetime are determined, and upper limits for the 26O ground state are extracted. In addition, the results provide evidence for an excited state in 26O at around 4 MeV. The ex- perimental findings are compared to theoretical shell-model calculations based on chiral two- and three-nucleon (3N) forces, including for the first time residual 3N forces, which are shown to be amplified as valence neutrons are added.

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arXiv2013

Approaching the precursor nuclei of the third r-process peak with RIBs

The rapid neutron nucleosynthesis process involves an enormous amount of very exotic neutron-rich nuclei, which represent a theoretical and experimental challenge. Two of the main decay properties that affect the final abundance distribution the most are half-lives and neutron branching ratios. Using fragmentation of a primary $^{238}$U beam at GSI we were able to measure such properties for several neutron-rich nuclei from $^{208}$Hg to $^{218}$Pb. This contribution provides a short update on the status of the data analysis of this experiment, together with a compilation of the latest results published in this mass region, both experimental and theoretical. The impact of the uncertainties connected with the beta-decay rates and with beta-delayed neutron emission is illustrated on the basis of $r$-process network calculations. In order to obtain a reasonable reproduction of the third $r$-process peak, it is expected that both half-lives and neutron branching ratios are substantially smaller, than those based on FRDM+QRPA, commonly used in $r$-process model calculations. Further measurements around $N\sim126$ are required for a reliable modelling of the underlying nuclear structure, and for performing more realistic $r$-process abundance calculations.

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arXiv2013

Neutron capture cross section of unstable 63Ni: implications for stellar nucleosynthesis

The $^{63}$Ni($n, γ$) cross section has been measured for the first time at the neutron time-of-flight facility n\_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian Averaged Cross Sections were calculated for thermal energies from kT = 5 keV to 100 keV with uncertainties around 20%. Stellar model calculations for a 25 M$_\odot$ star show that the new data have a significant effect on the $s$-process production of $^{63}$Cu, $^{64}$Ni, and $^{64}$Zn in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.

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arXiv2012

Neutron-skin thickness from the study of the anti-analog giant dipole resonance

The gamma-decay of the anti-analog of the giant dipole resonance (AGDR) has been measured to the isobaric analog state excited in the p(124Sn,n) reaction at a beam energy of 600 MeV/nucleon. The energy of the transition was also calculated with state-of-the-art self-consistent random-phase approximation (RPA) and turned out to be very sensitive to the neutron-skin thickness (\DeltaR_(pn)). By comparing the theoretical results with the measured one, the \DeltaR_(pn) value for 124Sn was deduced to be 0.175 \pm 0.048 fm, which agrees well with the previous results. The energy of the AGDR measured previously for ^(208)Pb was also used to determine the \DeltaR_(pn) for ^(208)Pb. In this way a very precise \DeltaR_(pn) = 0.181 \pm 0.031 neutron-skin thickness has been obtained for 208Pb. The present method offers new possibilities for measuring the neutron-skin thicknesses of very exotic isotopes.

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arXiv2011

Cross sections for proton-induced reactions on Pd isotopes at energies relevant for the gamma process

Proton-activation reactions on natural and enriched palladium samples were investigated via the activation technique in the energy range of E_p=2.75 MeV to 9 MeV, close to the upper end of the respective Gamow window of the gamma process. We have determined cross sections for 102Pd(p,gamma)103Ag, 104Pd(p,gamma)105Ag, and 105Pd(p,n)105Ag, as well as partial cross sections of 104Pd(p,n)104Ag^g, 105Pd(p,gamma)106Ag^m, 106Pd(p,n)106Ag^m, and 110Pd(p,n)110Ag^m with uncertainties between 3% and 15% for constraining theoretical Hauser-Feshbach rates and for direct use in gamma-process calculations.

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arXiv2002

A new method for nuclear-reaction network analysis, element production in S-Cl region during the He and C burning in 25 Ms stars

This paper presents the results of calculation of element overproduction in the S-Cl region during helium and carbon burning in massive stars (25 Ms). Calculations for a given set of differential equations were performed using integrated mathematical systems. The authors think that this method may be successfully adopted for other physical problems in which solving nuclear-reaction network play an important role, in particular for the problem of transmutation of heavy elements and chemical kinetics.

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