arXiv subjects

J. Michalicka

Publications and source records attributed to J. Michalicka.

3 recordsLinked to original sources

arXiv2026

Superconductivity in epitaxial PtSb(0001) thin films

We report superconductivity in epitaxial PtSb(0001) thin films grown on SrF2(111). Electrical transport measurements reveal a superconducting transition at $T_{\mathrm c}=1.72$ K. The field-induced broadening of the transition and the presence of finite upper critical fields are consistent with type-II superconductivity. We determine the resistively defined upper critical fields for magnetic fields applied perpendicular and parallel to the film plane and parameterize their temperature dependence using an anisotropic Ginzburg-Landau approach. For the thickest film ($d=50$ nm), this yields coherence lengths of $\xi_{ab}\approx 55$ nm and $\xi_c\approx 14$ nm. Current-voltage characteristics show sizeable critical currents, with a critical current density reaching $J_{\mathrm c}\approx 6e4$ A/cm$^2$ at 0.5 K. These results establish epitaxial PtSb as a superconducting thin-film platform compatible with lattice-matched heterostructures in the NiAs-type materials family.

cond-mat.supr-con↗

arXiv2024

E-Beam Induced Micropattern Generation and Amorphization of L-Cysteine-Functionalized Graphene Oxide Nano-composites

The evolution of dynamic processes in graphene-family materials are of great interest for both scientific purposes and technical applications. Scanning electron microscopy and transmission electron microscopy outstand among the techniques that allow both observing and controlling such dynamic processes in real time. On the other hand, functionalized graphene oxide emerges as a favorable candidate from graphene-family materials for such an investigation due to its distinctive properties, that encompass a large surface area, robust thermal stability, and noteworthy electrical and mechanical properties after its reduction. Here, we report on studies of surface structure and adsorption dynamics of L-Cysteine on electrochemically exfoliated graphene oxides basal plane. We show that electron beam irradiation prompts an amorphization of functionalized graphene oxide along with the formation of micropatterns of controlled geometry composed of L-Cysteine-Graphene oxide nanostructures. The controlled growth and predetermined arrangement of micropatterns as well as controlled structure disorder induced by e beam amorphization, in its turn potentially offering tailored properties and functionalities paving the way for potential applications in nanotechnology, sensor development, and surface engineering. Our findings demonstrate that graphene oxide can cover L-Cysteine in such a way to provide a control on the positioning of emerging microstructures about 10-20 um in diameter. Besides, Raman and SAED measurement analyses yield above 50% amorphization in a material. The results of our studies demonstrate that such a technique enables the direct creation of micropatterns of L-Cysteine-Graphene oxide eliminating the need for complicated mask patterning procedures.

cond-mat.mtrl-sci↗

arXiv2020

Mn-rich MnSb2Te4: A topological insulator with magnetic gap closing at high Curie temperatures of 45-50 K

Ferromagnetic topological insulators exhibit the quantum anomalous Hall effect that might be used for high precision metrology and edge channel spintronics. In conjunction with superconductors, they could host chiral Majorana zero modes which are among the contenders for the realization of topological qubits. Recently, it was discovered that the stable 2+ state of Mn enables the formation of intrinsic magnetic topological insulators with A1B2C4 stoichiometry. However, the first representative, MnBi2Te4, is antiferromagnetic with 25 K N\'eel temperature and strongly n-doped. Here, we show that p-type MnSb2Te4, previously considered topologically trivial, is a ferromagnetic topological insulator in the case of a few percent of Mn excess. It shows (i) a ferromagnetic hysteresis with record high Curie temperature of 45-50 K, (ii) out-of-plane magnetic anisotropy and (iii) a two-dimensional Dirac cone with the Dirac point close to the Fermi level which features (iv) out-of-plane spin polarization as revealed by photoelectron spectroscopy and (v) a magnetically induced band gap that closes at the Curie temperature as demonstrated by scanning tunneling spectroscopy. Moreover, it displays (vi) a critical exponent of magnetization beta~1, indicating the vicinity of a quantum critical point. Ab initio band structure calculations reveal that the slight excess of Mn that substitutionally replaces Sb atoms provides the ferromagnetic interlayer coupling. Remaining deviations from the ferromagnetic order, likely related to this substitution, open the inverted bulk band gap and render MnSb2Te4 a robust topological insulator and new benchmark for magnetic topological insulators.

cond-mat.mtrl-sci↗