arXiv subjects

J. N. Eckstein

Publications and source records attributed to J. N. Eckstein.

At least 19 recordsLinked to original sources

arXiv2016

Temperature-dependent ellipsometry measurements of partial Coulomb energy in superconducting cuprates

We performed an experimental study of the temperature and doping dependence of the energy-loss function of the bilayer and trilayer Bi-cuprate family. The primary aim is to obtain information on the energy stored in the Coulomb interaction between the conduction electrons, on the temperature dependence thereof, and on the change of Coulomb interaction when Cooper-pairs are formed. We performed temperature-dependent ellipsometry measurements on several Bi$_2$Sr$_2$CaCu$_2$O$_{8-x}$ single crystals: under-doped with $T_c=60, 70$ and 83K, optimally doped with $T_c=91$K, overdoped with $T_c=84, 81, 70$ and $58$K, as well as optimally doped Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+x}$ with $T_c=110$K. Our first observation is that, as the temperature drops through $T_c$, the loss function in the range up to 2~eV displays a change of temperature dependence as compared to the temperature dependence in the normal state. This effect at - or close to - $T_c$ depends strongly on doping, with a sign-change for weak overdoping. The size of the observed change in Coulomb energy, using an extrapolation with reasonable assumptions about its $q$-dependence, is about the same size as the condensation energy that has been measured in these compounds. Our results therefore lend support to the notion that the Coulomb energy is an important factor for stabilizing the superconducting phase. Due to the restriction to small momentum, our observations do not exclude a possible significant contribution to the condensation energy of the Coulomb energy associated to the region of $q$ around $(π,π)$.

cond-mat.supr-con↗

arXiv2013

LaAlO3 stoichiometry found key to electron liquid formation at LaAlO3/SrTiO3 interfaces

Emergent phenomena, including superconductivity and magnetism, found in the two-dimensional electron liquid (2-DEL) at the interface between the insulators LaAlO3 and SrTiO3 distinguish this rich system from conventional two-dimensional electron gases at compound semiconductor interfaces. The origin of this 2-DEL, however, is highly debated with focus on the role of defects in the SrTiO3 while the LaAlO3 has been assumed perfect. Our experiments and first principles calculations show that the cation stoichiometry of the nominal LaAlO3 layer is key to 2-DEL formation: only Al-rich LaAlO3 results in a 2-DEL. While extrinsic defects including oxygen deficiency are known to render LaAlO3/SrTiO3 samples conducting, our results show that in the absence of such extrinsic defects, an interface 2-DEL can form. Its origin is consistent with an intrinsic electronic reconstruction occurring to counteract a polarization catastrophe. This work provides a roadmap for identifying other interfaces where emergent behaviors await discovery.

cond-mat.mtrl-sci↗

arXiv2011

Resonant soft x-ray scattering from La(1-x)Sr(x)MnO(3) quantum wire arrays

We describe a strategy for using resonant soft x-ray scattering (RSXS) to study the electronic structure of transition metal oxide quantum wires. Using electron beam lithography and ion milling, we have produced periodic, patterned arrays of colossal magnetoresistance (CMR) phase La(1-x)Sr(x)MnO(3) consisting of ~ 5000 wires, each of which is 80 nm in width. The scattered intensity exhibits a series of peaks that can be interpreted as Bragg reflections from the periodic structure or, equivalently, diffraction orders from the grating-like structure. RSXS measurements at the Mn L(2,3) edge, which has a large magnetic cross section, show clear evidence for a magnetic superstructure with a commensurate period of five wires, which we interpret as commensurately modulated antiferromagnetism. This superstructure, which is accompanied by non-trivial reorganization of the magnetization within each wire, likely results from classical dipole interactions among the wires. We introduce a simple, exactly soluble, analytic model of the scattering that captures, semi-quantitatively, the primary features in the RSXS data; this model will act as a foundation for forthcoming, detailed studies of the magnetic structure in these systems.

cond-mat.str-el↗

arXiv2008

Magnetically asymmetric interfaces in a (LaMnO$_3$)/(SrMnO$_3$) superlattice due to structural asymmetries

Polarized neutron reflectivity measurements of a ferromagnetic [(LaMnO$_3$)$_{11.8}$/(SrMnO$_3$)$_{4.4}$]$_6$ superlattice reveal a modulated magnetic structure with an enhanced magnetization at the interfaces where LaMnO$_3$ was deposited on SrMnO$_3$ (LMO/SMO). However, the opposite interfaces (SMO/LMO) are found to have a reduced ferromagnetic moment. The magnetic asymmetry arises from the difference in lateral structural roughness of the two interfaces observed via electron microscopy, with strong ferromagnetism present at the interfaces that are atomically smooth over tens of nanometers. This result demonstrates that atomic-scale roughness can destabilize interfacial phases in complex oxide heterostructures.

cond-mat.mtrl-sci↗

arXiv2007

The metal-insulator transition and its relation to magnetic structure in (LaMnO3)2n/(SrMnO3)n superlattices

Superlattices of (LaMnO3)2n/(SrMnO3)n (n=1 to 5), composed of the insulators LaMnO3 and SrMnO3, undergo a metal-insulator transition as a function of n, being metallic for n<=2 and insulating for n>=3. Measurements of transport, magnetization and polarized neutron reflectivity reveal that the ferromagnetism is relatively uniform in the metallic state, and is strongly modulated in the insulating state, being high in LaMnO3 and suppressed in SrMnO3. The modulation is consistent with a Mott transition driven by the proximity between the (LaMnO3)/(SrMnO3) interfaces. Disorder localizes states at the Fermi level at the interfaces for n>=3. We suggest that this disorder is due to magnetic frustration at the interfaces.

cond-mat.str-el↗

arXiv2007

Viscous spin exchange torque on precessional magnetization in $(\mathrm{LaMnO}_3)_{2n}/(\mathrm{SrMnO}_3)_{n}$ superlattices

Photoinduced magnetization dynamics is investigated in chemically ordered $(\mathrm{LaMnO}_3)_{2n}/(\mathrm{SrMnO}_3)_n$ superlattices using the time-resolved magneto-optic Kerr effect. A monotonic frequency-field dependence is observed for the $n=1$ superlattice, indicating a single spin population consistent with a homogeneous hole distribution. In contrast, for $n\geq2$ superlattices, a large precession frequency is observed at low fields indicating the presence of an exchange torque in the dynamic regime. We propose a model that ascribes the emergence of exchange torque to the coupling between two spin populations -- viscous and fast spins.

cond-mat.mtrl-sci↗

arXiv2007

Nanoscale Suppression of Magnetization at Atomically Assembled Manganite Interfaces

Using polarized X-rays, we compare the electronic and magnetic properties of a La(2/3)Sr(1/3)MnO(3)(LSMO)/SrTiO(3)(STO) and a modified LSMO/LaMnO(3)(LMO)/STO interface. Using the technique of X-ray resonant magnetic scattering (XRMS), we can probe the interfaces of complicated layered structures and quantitatively model depth-dependent magnetic profiles as a function of distance from the interface. Comparisons of the average electronic and magnetic properties at the interface are made independently using X-ray absorption spectroscopy (XAS) and X-ray magnetic circular dichroism (XMCD). The XAS and the XMCD demonstrate that the electronic and magnetic structure of the LMO layer at the modified interface is qualitatively equivalent to the underlying LSMO film. From the temperature dependence of the XMCD, it is found that the near surface magnetization for both interfaces falls off faster than the bulk. For all temperatures in the range of 50K - 300K, the magnetic profiles for both systems always show a ferromagnetic component at the interface with a significantly suppressed magnetization that evolves to the bulk value over a length scale of ~1.6 - 2.4 nm. The LSMO/LMO/STO interface shows a larger ferromagnetic (FM) moment than the LSMO/STO interface, however the difference is only substantial at low temperature.

cond-mat.str-el↗

arXiv2006

Suppressed Magnetization at the Surfaces and Interfaces of Ferromagnetic Metallic Manganites

What happens to ferromagnetism at the surfaces and interfaces of manganites? With the competition between charge, spin, and orbital degrees of freedom, it is not surprising that the surface behavior may be profoundly different than that of the bulk. Using a powerful combination of two surface probes, tunneling and polarized x-ray interactions, this paper reviews our work on the nature of the electronic and magnetic states at manganite surfaces and interfaces. The general observation is that ferromagnetism is not the lowest energy state at the surface or interface, which results in a suppression or even loss of ferromagnetic order at the surface. Two cases will be discussed ranging from the surface of the quasi-2D bilayer manganite (La$_{2-2x}$Sr$_{1+2x}$Mn$_2$O$_7$) to the 3D Perovskite (La$_{2/3}$Sr$_{1/3}$MnO$_3$)/SrTiO$_3$ interface. For the bilayer manganite, that is, ferromagnetic and conducting in the bulk, these probes present clear evidence for an intrinsic insulating non-ferromagnetic surface layer atop adjacent subsurface layers that display the full bulk magnetization. This abrupt intrinsic magnetic interface is attributed to the weak inter-bilayer coupling native to these quasi-two-dimensional materials. This is in marked contrast to the non-layered manganite system (La$_{2/3}$Sr$_{1/3}$MnO$_3$/SrTiO$_3$), whose magnetization near the interface is less than half the bulk value at low temperatures and decreases with increasing temperature at a faster rate than the bulk.

cond-mat.str-el↗

arXiv2006

Doping Controlled Superconductor-Insulator Transition in Bi2Sr2-xLaxCaCu2O8+delta

We show that the doping-controlled superconductor-insulator transition (SIT) in a high critical temperature cuprate system (Bi2Sr2-xLaxCaCu2O8+delta) exhibits a fundamentally different behavior than is expected from conventional SIT. At the critical doping, the sheet resistance seems to diverge in the zero temperature limit. Above the critical doping, the transport is universally scaled by a two-component conductance model. Below, it continuously evolves from weakly to strongly insulating behavior. The two-component conductance model suggests that a collective electronic phase separation mechanism may be responsible for this unconventional SIT behavior.

cond-mat.supr-con↗

arXiv2005

Spatially Selective and Reversible Doping Control in Cuprate Films

We describe a reversible, spatially-controlled doping method for cuprate films. The technique has been used to create superconductor-antiferromagnetic insulator-superconductor (S-AFI-S) junctions and optimally doped superconductor-underdoped superconductor-optimally doped superconductor (OS-US-OS) cuprate structures. We demonstrate how the S-AFI-S structure can be employed to reliably measure the transport properties of the antiferromagnetic insulator region at cryogenic temperatures using the superconductors as seamless electrical leads. We also discuss applied and fundamental issues which may be addressed with the structures created with this doping method. Although it is implemented on a cuprate film (YBa2Cu3O7-delta) in this work, the method can also be applied to any mixed-valence transition metal oxide whose physical properties are determined by oxygen content.

cond-mat.supr-con↗

arXiv2003

Critical dynamics of superconducting BSCCO films

We report on a systematic investigation of the critical fluctuations in the complex conductivity of epitaxially-grown Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ films for ${T \lesssim T_c}$ using a two-coil inductive technique at zero applied field. We observe the static 3D-XY critical exponent in the superfluid density near $T_{c}$. Linear scaling analysis close to the critical temperature yields a dynamic critical exponent of $z = 2.0$ for small drive currents, but non-linear effects are seen to be important. At $T_{c}$, a non-linear scaling analysis also yields a 3D dynamic exponent of $z = 2.0$.

cond-mat.supr-con↗

arXiv2002

Atomic Scale Imaging and Spectroscopy of a CuO_2 Plane at the Surface of Bi_2Sr_2CaCu_2O_{8+delta}

We have used a scanning tunneling microscope to demonstrate that a single CuO_2 plane can form a stable and atomically ordered layer at the surface of Bi_2Sr_2CaCu_2O_{8+delta}. In contrast to previous studies on high-T_c surfaces, the CuO_2-terminated surface exhibits a strongly suppressed tunneling conductance at low voltages. We consider a number of different explanations for this phenomena and propose that it may be caused by how the orbital symmetry of the CuO_2 plane's electronic states affects the tunneling process.

cond-mat.supr-con↗

arXiv2000

Measurement of Transport Lifetime in a Cuprate Superconductor

We report measurements of the phase of the conductivity, $ϕ_σ\equiv arg(σ)$, in the normal state of a $Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}$ (BSCCO) thin film from 0.2-1.0 THz. From $ϕ_σ$ we obtain the time delay of the current response, $τ_σ\equivϕ_σ/ω$. After discovering a systematic error in the data analysis, the extracted $τ_σ$ has changed from that reported earlier. The revised data is shown in the sole figure below. Analysis and discussion of these data will follow.

cond-mat.supr-con↗

arXiv2000

Signature of Superfluid Density in the Single-Particle Excitation Spectrum of Bi2Sr2CaCu2O8+delta

We report that the doping and temperature dependence of photoemission spectra near the Brillouin zone boundary of Bi2Sr2CaCu2O8+delta exhibit unexpected sensitivity to the superfluid density. In the superconducting state, the photoemission peak intensity as a function of doping scales with the superfluid density and the condensation energy. As a function of temperature, the peak intensity shows an abrupt behavior near the superconducting phase transition temperature where phase coherence sets in, rather than near the temperature where the gap opens. This anomalous manifestation of collective effects in single-particle spectroscopy raises important questions concerning the mechanism of high-temperature superconductivity.

cond-mat.supr-con↗

arXiv2000

Nonlinear I-V, High Flux-Flow Velocity Instability and Evidence for Quantum Fluctuations in BSCCO Superconducting Films

The large flux-flow velocity behavior of the high temperature superconductor BSCCO in the mixed state is studied by measurement of the current-voltage characteristic as a function of temperature and magnetic field direction. We find strong evidence for vortex-antivortex pairs that are excited by quantum fluctuations and contribute to the dissipation when dissociated by a large current.

cond-mat.supr-con↗

arXiv2000

Nodal Quasiparticle Lifetime in the Superconducting State of BSCCO(2212)

We have measured the complex conductivity of a BSCCO(2212) thin film between 0.2 and 1.0 THz. We find the conductivity in the superconducting state to be well described as the sum of contributions from quasiparticles, the condensate, and order parameter fluctuations which draw 30% of the spectral weight from the condensate. An analysis based on this decomposition yields a quasiparticle scattering rate on the order of k_(B)*T/(hbar) for temperatures below Tc.

cond-mat.supr-con↗

arXiv2000

Low Temperature AC Conductivity in BSCCO (2212)

We report measurements of anamolously large dissipative conductivities in BiSrCaCuO(2212) at low temperatures. We have measured the complex conductivity of BSCCO thin films at 100-600 GHz as a function of doping from the underdoped to the overdoped state. At low temperatures there exists a residual dissipative conductivity which scales with the T=0 superfluid density as the doping is varied. This residual dissipative conductivity is larger than the possible contribution from a thermal population of quasiparticles at the d-wave gap nodes.

cond-mat.supr-con↗

arXiv1999

Vanishing of phase coherence in underdoped Bi_2Sr_2CaCu_2O_8+d

Coherent time-domain spectroscopy is used to measure the screening and dissipation of high-frequency electromagnetic fields in a set of underdoped Bi_2Sr_2CaCu_2O_8+d thin films. The measurements provide direct evidence for a phase-fluctuation driven transition from the superconductor to normal state, with dynamics described well by the Berezinskii-Kosterlitz-Thouless theory of vortex-pair unbinding.

cond-mat.supr-con↗