SearcharxivSearch

arXiv subjects

J. Nolen

Publications and source records attributed to J. Nolen.

3 recordsLinked to original sources

Photonuclear Cross Sections for the $^{197}$Au($\gamma$,pn)$^{195m}$Pt Reaction Near Threshold

Platinum radioisotopes are of growing interest for targeted cancer therapy and diagnostic imaging because their decay delivers highly localized radiation doses in tissue, herewith enabling precise DNA damage through Auger-electron emission. Developing production technologies that provide platinum isotopes with high specific activity is therefore essential, and photonuclear reactions on stable nuclei offer a viable accelerator-based route when supported by reliable cross-section data. We report photonuclear cross-section measurements for the $^{197}$Au($\gamma$,pn)$^{195m}$Pt reaction at incident $\gamma$-ray energies of 27, 29, and 31 MeV using the activation method. The measurements were performed by irradiating a stack of concentric-ring gold targets with a quasi-monoenergetic $\gamma$-ray beam provided by the High Intensity Gamma-ray Source (HI$\gamma$S). The induced $^{195m}$Pt activity was quantified using off-line $\gamma$-ray spectroscopy. These data provide the first experimental constraints on the $^{197}$Au($\gamma$,pn)$^{195m}$Pt cross section in the near-threshold region. The measured excitation function is compared with PHITS and TALYS calculations and indicates that the reaction becomes measurable only near 30 MeV, with substantially higher bremsstrahlung end-point energies required for practically meaningful production.

nucl-ex

Target Development Using the Method of High-Intensity Vibrational Powder Plating (HIVIPP) at the Center for Accelerator Target Science (CATS) at Argonne National Laboratory (ANL)

One of the primary goals of the Center for Accelerator Target Science (CATS) is to provide targets and foils in support of the ATLAS User Facility and the Low-Energy community at large. While a wide array of target production techniques are available at CATS, new methods that must be explored invariably arise. One such technique, the High-Intensity Vibrational Powder Plating (HIVIPP), was first reported in 1997 by Isao Sugai. It was developed to produce targets and stripper foils that were difficult to make by standard methods. At Argonne National Laboratory (ANL), we have successfully constructed and tested a simple system for this purpose. We have produced targets of carbon and titanium on various metal backings using the HIVIPP method. We are currently in the exciting phase of exploring the production of other elements, including isotopically enriched and radioactive material. This work is in progress and will be further detailed with specific examples.

physics.acc-ph

Multiscale Modelling and Inverse Problems

The need to blend observational data and mathematical models arises in many applications and leads naturally to inverse problems. Parameters appearing in the model, such as constitutive tensors, initial conditions, boundary conditions, and forcing can be estimated on the basis of observed data. The resulting inverse problems are often ill-posed and some form of regularization is required. These notes discuss parameter estimation in situations where the unknown parameters vary across multiple scales. We illustrate the main ideas using a simple model for groundwater flow. We will highlight various approaches to regularization for inverse problems, including Tikhonov and Bayesian methods. We illustrate three ideas that arise when considering inverse problems in the multiscale context. The first idea is that the choice of space or set in which to seek the solution to the inverse problem is intimately related to whether a homogenized or full multiscale solution is required. This is a choice of regularization. The second idea is that, if a homogenized solution to the inverse problem is what is desired, then this can be recovered from carefully designed observations of the full multiscale system. The third idea is that the theory of homogenization can be used to improve the estimation of homogenized coefficients from multiscale data.

math.ST