arXiv subjects

J. P. Araujo

Publications and source records attributed to J. P. Araujo.

13 recordsLinked to original sources

arXiv2026

Independent Tuning of Surface Acoustic-Waves and Spin-Waves via Buffer-Layer Engineering in Co2FeGe Heusler Thin Films

Understanding and controlling acoustic and spin-wave excitations in magnetic thin films is critical for the development of magnonic and spin-acoustic devices. We report on the use of Cr and W buffer layers to independently modify the acoustic and magnetic excitations in Co2FeGe full-Heusler thin films grown on MgO(001). Using Brillouin light scattering (BLS) spectroscopy and ferromagnetic resonance (FMR), we probed Rayleigh and Sezawa surface acoustic waves (SAWs) alongside Damon-Eshbach and perpendicular standing spin-wave (PSSW) modes. Our results show that acoustic dispersion depends strongly on the buffer material; W-buffered films exhibit a pronounced 16% reduction in Rayleigh SAW frequency compared to buffer-free films, primarily due to mass loading and acoustic impedance shifts. While the buffer layers significantly shift acoustic frequencies, they simultaneously modify the dynamic magnetic response (increasing spin-wave group velocity by ~34%) through different physical mechanisms. Finite-element simulations show excellent agreement with the experimental acoustic data. These findings demonstrate that buffer-layer engineering is an effective strategy for the independent tailoring of elastic and magnetic excitations, providing a versatile platform for hybrid spin-acoustic technologies.

cond-mat.mtrl-sci↗

arXiv2026

AI Application Gives Users Real-Time Feedback on the Level of Peace in the Social Media Videos They Watch

Most people now get their news from videos on social media, such as YouTube and Facebook, rather than through curated journalism. "We become what we behold." The content and tone of language plays an essential role in starting or ending conflicts. "Hate Speech" can enhance conflict, "Peace Speech" can enhance peace. We developed an application that measures, in real time, these aspects of speech from YouTube videos, which can give users helpful feedback on their own media diet. We used two approaches: 1) supervised machine learning. Language in the text of online news media text was tagged by surveys that measure the level of peace in those countries. One fully connected feedforward and 2 convolutional neural networks trained on that data were $\sim 97\%$ accurate in predicting levels of peace in the test set and $\sim 70\%$ accurate in another distinct news text data set, but did not generalize to YouTube videos, suggesting that written text is different than transcribed spoken language. 2) social science dimensions. There is no similar external data to tag the text in the YouTube video transcripts. We therefore used 2 word-level sentiment analysis (SA) and 6 context-level large language models (LLMs) to measure 5 social dimensions in peace identified by 59 social science studies: compassion-contempt, news-opinion, promotion-prevention, creativity-order, nuance-simplification. LLMs more closely matched the values by 3 human coders on 52 videos, $r^2\sim0.60$ than SA, at $r^2\sim0.03$. Results: LLMs successfully measured social dimensions important in peace in YouTube videos, compared to human coders. These results serve as the basis of an analysis engine that can give users and content creators feedback on their own media diet and creations.

cs.CL↗

arXiv2025

Spin waves in Co$_2$FeGe films

The dynamic magnetic properties of Full Heusler alloy thin films of Co$_2$FeGe, grown on MgO (001) substrates under different thermal conditions, were investigated. Brillouin light scattering and ferromagnetic resonance measurements revealed that depositing at room temperature followed by annealing at 300 deg C for 1 hour produces the best results for maximizing magnetization, exchange stiffness, and minimizing spin-dynamic dissipation in the films, which are desirable characteristics for high-speed spintronic devices. Additionally, strong hybridization of spin waves in the Damon-Eshbach geometry was observed, which is attractive for applications in magnonic signal processing circuits.

cond-mat.mtrl-sci↗

arXiv2018

An Electromagnet-Based Magnetically-Activated Thermal Switch Without Moving Parts

With the ever increasing power dissipation in electrical devices, new thermal management solutions are in high demand to maintain an optimal operating temperature and efficient performance. In particular, recently developed magnetically-activated thermal switches (MATSs) provide an alternative to existing devices, using the magnetic and thermal properties of superparamagnetic nanofluids to dissipate heat in a controlled manner. However, the presence of moving parts is a major drawback in those systems that must still be addressed. Herein, we present a compact and automatized MATS composed by an encapsulated superparamagnetic nanofluid and an electromagnet allowing to activate the MATS without any moving part. We investigate the effect of different temperature gradients (40, 26 and 10 C) and powers applied to the coil (6.5, 15, 25 and 39 W) on the performance of this novel MATS. The results show that the highest (44.4$) and fastest (0.6 C/s) temperature variation occur for the highest studied temperature gradient. On the other hand, with increasing power, there is also an increase in the efficiency of the heat exchange process between the two surfaces. These results remove one of the main barriers preventing the actual application of magnetic thermal switches and opens new venues for the design of efficient thermal management devices.

physics.app-ph↗

arXiv2016

Electrical Switching of Magnetization in Films of alpha-Iron with Naturally Hydroxidized Surface

Control of the magnetization vector in ferromagnetic films and heterostructures by using electric tools instead of external magnetic fields can lead to low-power memory devices. We observe the robust changes in magnetization states of a thin (about 30 nm) film of alpha-Fe covered by the naturally formed layer ( about 6 nm in thickness) of iron ohyhydroxides (FeOOH) under discharging a capacitor through the film. Strikingly, the magnetization vector is switchable by the discharge even with no any biasing field at room temperatures. In this electrically induced magnetization switching (EIMS) we reveal the key role of the FeOOH layer. We demonstrate experimental evidences that not the discharge current itself but the electric field (of the order of 10 kV/m) generated by this current is responsible for EIMS. The results reported here provide a plausible explanation of the observed phenomenon in terms of electric-field-induced weak ferromagnetism in the FeOOH layer and its coupling with the underlying alpha-Fe.

cond-mat.mtrl-sci↗

arXiv2008

New phase transition in $Pr_{1-x}Ca_xMnO_3$ system: evidence for electrical polarization in charge ordered manganites

A detailed study of the electric field gradient (EFG) across the Pr1-xCaxMnO3 phase diagram and its temperature dependence is given. Clearly, distinct EFG behaviours for samples outside/inside the charge order (CO) region are observed. The EFG temperature dependence evidences a new phase transition occurring over the broad CO region of the phase diagram. This transition is discontinuous and occurs at temperatures between the charge ordering and the Neel temperatures. The features observed in the EFG are associated with polar atomic vibrations which eventually lead to a spontaneous local electric polarization below CO transition.

cond-mat.str-el↗

arXiv2006

Short-range effects and magnetization reversal in Co$_{80}$Fe$_{20}$ thin films: a MOKE magnetometry/domain imaging and AMR study

A MOKE magnetometry unit simultaneously sensitive to both in-plane magnetization components, based on an intensity differential detection method, allows us to observe the uniaxial anisotropy impressed during CoFe-deposition and to discriminate the magnetization processes under a magnetic field parallel and perpendicular to such axes. Our MOKE imaging unit, using a CCD camera for Kerr effect domain visualization provides direct evidence on the dominant M-processes, namely domain wall motion and moment rotation. Further magnetic information was obtained by AMR measurements due to the dependence of the electrical resistivity on the short-range spin disorder and also on the angle between the electrical current direction (I) and the spontaneous magnetization ($\emph{\textbf{M}}_{S}$).

cond-mat.mtrl-sci↗

arXiv2006

Nanoscopic processes of Current Induced Switching in thin tunnel junctions

In magnetic nanostructures one usually uses a magnetic field to commute between two resistance (R) states. A less common but technologically more interesting alternative to achieve R-switching is to use an electrical current, preferably of low intensity. Such Current Induced Switching (CIS) was recently observed in thin magnetic tunnel junctions, and attributed to electromigration of atoms into/out of the insulator. Here we study the Current Induced Switching, electrical resistance, and magnetoresistance of thin MnIr/CoFe/AlO$_x$/CoFe tunnel junctions. The CIS effect at room temperature amounts to 6.9% R-change between the high and low states and is attributed to nanostructural rearrangements of metallic ions in the electrode/barrier interfaces. After switching to the low R-state some electro-migrated ions return to their initial sites through two different energy channels. A low (high) energy barrier of $\sim$0.13 eV ($\sim$0.85 eV) was estimated. Ionic electromigration then occurs through two microscopic processes associated with different types of ions sites/defects. Measurements under an external magnetic field showed an additional intermediate R-state due to the simultaneous conjugation of the MR (magnetic) and CIS (structural) effects.

cond-mat.mtrl-sci↗

arXiv2006

Domain imaging, MOKE and magnetoresistance studies of CoFeB films for MRAM applications

We present a detailed study on domain imaging, Kerr effect magnetometry (MOKE) and magnetoresistance (MR), for a series of 20 nm Co$_{73.8}$Fe$_{16.2}$B$_{10}$ thin films, both as-deposited (amorphous) and annealed (crystalline). By considering the two different (orthogonal) in-plane magnetization components, obtained by MOKE measurements, we were able to study the uniaxial anisotropy induced during CoFeB-deposition and to discriminate the magnetization processes under a magnetic field parallel and perpendicular to such axis. MOKE magnetic imaging enabled us to observe the dominant magnetization processes, namely domain wall motion and moment rotation. These processes were correlated with the behavior of the magnetoresistance, which depends both on short-range spin disorder electron scattering and on the angle between the electrical current and the spontaneous magnetization ($\emph{\textbf{M}}_{S}$). A simple numerical treatment based on Stoner-Wolfarth model enables us to satisfactorily predict the magnetization behaviour observed in these films. A comparison between the results in Co$_{73.8}$Fe$_{16.2}$B$_{10}$ films and the previous ones obtained in annealed Co$_{80}$Fe$_{20}$ films, show that the introduction of boron in CoFe reduces significatively the coercive and saturation fields along the easy axis (e.g. $H_{c}$ from $\sim$ 2 down to $\sim$ 0.5 kAm$^{-1}$). Also, the magnetization along the hard axis saturates at lower fields. We conclude that amorphous and nanocrystalline CoFeB films show low coercive fields and abrupt switching, as well as absence of short range spin disorder effects after switching when compared with Co$_{80}$Fe$_{20}$.

cond-mat.mtrl-sci↗

arXiv2005

Percolative phase transition on ferromagnetic insulator manganites: uncorrelated to correlated polaron clusters

In this work, we report an atomic scale study on the ferromagnetic insulator manganite LaMnO$_{3.12}$ using $γ-γ$ PAC spectroscopy. Data analysis reveals a nanoscopic transition from an undistorted to a Jahn-Teller-distorted local environment upon cooling. The percolation thresholds of the two local environments enclose a macroscopic structural transition (Rhombohedric-Orthorhombic). Two distinct regimes of JT-distortions were found: a high temperature regime where uncorrelated polaron clusters with severe distortions of the Mn$^{3+}$O$_{6}$ octahedra survive up to $T \approx 800 K$ and a low temperature regime where correlated regions have a weaker JT-distorted symmetry.

cond-mat.str-el↗

arXiv2003

Influence of charge ordering on the magnetocaloric effect of (Pr,Ca)MnO$_3$ manganites

In the present work we analyze the influence of the charge-ordering on the magnetocaloric effect of Pr$_{1-x}$Ca$_x$MnO$_3$ manganites. The results for the samples with $x<$0.30 present the usual ferromagnetic behavior, peaking at the Curie temperature T$_C$. In contrast, for the samples above the onset concentration for the charge-ordering ($x\sim$0.30), an anomalous magnetic entropy change was observed below the charge-ordering temperature $T_{CO}$, persisting for lower temperatures. This effect is associated to a positive contribution to the magnetic entropy change due to charge-ordering, which is superimposed to the negative contribution from the spin ordering. We found that the charge-ordering component peaks at $T_N$ and is negligible above $T_{CO}$. Moreover, around T$^\star$ (temperature below which the insulator-metal transition induced by magnetic field becomes completely irreversible, where the system remains in such state even after the external magnetic field has been removed), we found extremely large values for the magnetic entropy change, establishing a `colossal' magnetocaloric effect on CMR manganites.

cond-mat.mtrl-sci↗

arXiv2003

Magnetic phase diagram for a non-extensive system: Experimental connection with manganites

In the present paper we make a thorough analysis of a classical spin system, within the framework of Tsallis nonextensive statistics. From the analysis of the generalized Gibbs free energy, within the mean-field approximation, a para-ferromagnetic phase diagram, which exhibits first and second order phase transitions, is built. The features of the generalized, and classical, magnetic moment are mainly determined by the values of $q$, the non-extensive parameter. The model is successfully applied to the case of La$_{0.60}$Y$_{0.07}$Ca$_{0.33}$MnO$_3$ manganite. The temperature and magnetic field dependence of the experimental magnetization on this manganite are faithfully reproduced. The agreement between rather "exotic" magnetic properties of manganites and the predictions of the $q$-statistics, comes to support our early claim that these materials are magnetically nonextensive objects.

cond-mat.stat-mech↗

arXiv2002

Magnetic behavior of a non-extensive S-spin system: possible connections to manganites

We analyzed the magnetic behavior of a S-spin system within framework of the Tsallis nonextensive statistics, employing the normalized approach. Unusual properties on magnetization, entropy and susceptibility emerge, as a consequence of nonextensivity. We further show that the nonextensive approach can be relevant to the field of manganites, materials which exhibit long-range interactions and fractality, two basic ingredients for nonextensivity. Our results are in qualitative agreement to experimental data in La$_{0.67}$Ca$_{0.33}$MnO$_3$ and Pr$_{0.5}$Ca$_{0.5}$Mn$_{0.95}$Ga$_{0.05}$O$_3$ manganites.

cond-mat.stat-mech↗