arXiv subjects

J. P. Carbotte

Publications and source records attributed to J. P. Carbotte.

At least 55 records · Page 3Linked to original sources

arXiv2014

Dielectric screening of surface states in a topological insulator

Hexagonal warping provides an anisotropy to the dispersion curves of the helical Dirac fermions that exist at the surface of a topological insulator. A sub-dominant quadratic in momentum term leads to an asymmetry between conduction and valence band. A gap can also be opened through magnetic doping. We show how these various modifications to the Dirac spectrum change the polarization function of the surface states and employ our results to discuss their effect on the plasmons. In the long wavelength limit, the plasmon dispersion retains its square root dependence on its momentum, $\boldsymbol{q}$, but its slope is modified and it can acquire a weak dependence on the direction of $\boldsymbol{q}$. Further, we find the existence of several plasmon branches, one which is damped for all values of $\boldsymbol{q}$, and extract the plasmon scattering rate for a representative case.

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arXiv2013

Conductivity of Dirac fermions with phonon induced topological crossover

We study the Hall conductivity in single layer gapped Dirac fermion materials including coupling to a phonon field, which not only modifies the quasi-particle dynamics through the usual self-energy term but also renormalizes directly the gap. Consequently the Berry curvature is modified. As the temperature is increased the sign of the renormalized gap can change and the material can cross over from a band insulator to a topological insulator at higher temperature (T). The effective Chern numbers defined for valley and spin Hall conductivity show a rich phase diagram with increasing temperature. While the spin and valley DC Hall conductivity is no longer quantized at elevated temperature a change in sign with increasing T is a clear indication of a topological crossover. The chirality of the circularly polarized light which is dominantly absorbed by a particular valley can change with temperature as a result of a topological crossover.

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arXiv2013

Vanishing of interband light absorption in a persistent spin helix state

Spin-orbit coupling plays an important role in various properties of very different materials. Moreover efforts are underway to control the degree and quality of spin-orbit coupling in materials with a concomitant control of transport properties. We calculate the frequency dependent optical conductivity in systems with both Rashba and Dresselhaus spin-orbit coupling. We find that when the linear Dresselhaus spin-orbit coupling is tuned to be equal to the Rashba spin-orbit coupling, the interband optical conductivity disappears. This is taken to be the signature of the recovery of SU(2) symmetry. The presence of the cubic Dresselhaus spin-orbit coupling modifies the dispersion relation of the charge carriers and the velocity operator. Thus the conductivity is modified, but the interband contribution remains suppressed at most but not all photon energies for a cubic coupling of reasonable magnitude. Hence, such a measurement can serve as a diagnostic probe of engineered spin-orbit coupling.

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arXiv2013

Evolution of electron-boson spectral density in the underdoped region of Bi_2Sr_{2-x}La_xCuO_6

We use a maximum entropy technique to obtain the electron-boson spectral density from optical scattering rate data across the underdoped region of the Bi_2Sr_{2-x}La_xCuO_6 (Bi-2201) phase diagram. Our method involves a generalization of previous work which explicitly include finite temperature and the opening of a pseudogap which modifies the electronic structure. We find that the mass enhancement factor λassociated with the electron-boson spectral density increases monotonically with reduced doping and closer proximity to the Mott antiferromagnetic insulating state. This observation is consistent with increased coupling to the spin fluctuations. At the same time the system has reduced metallicity because of increased pseudogap effects which we model with a reduced effective density of states around the Fermi energy with the range of the modifications in energy set by the pseudogap scale.

cond-mat.supr-con↗

arXiv2013

Determination of boson spectrum from optical data in pseudogap phase of underdoped cuprates

Information on the nature of the dominant inelastic processes operative in correlated metallic systems can be obtained from an analysis of their AC optical response. An electron-boson spectral density can usefully be extracted. This density is closely related to the optical scattering rate. However, in the underdoped region of the high Tc cuprate phase diagram a new energy scale (the pseudogap) emerges, which alters the optical scattering and needs to be taken into account in any fit to data. This can influence the shape and strength of the recovered boson spectral function. Including a pseudogap in an extended maximum entropy inversion for optimally doped Bi-2212 is more consistent with existing data than when it is left out as done previously.

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arXiv2013

Phonon structure in dispersion curves and density of states of massive Dirac Fermions

Dirac fermions exist in many solid state systems including graphene, silicene and other two dimensional membranes such as are found in group VI dichalcogenides, as well as on the surface of some insulators where such states are protected by topology. Coupling of those fermions to phonons introduces new structures in their dispersion curves and, in the case of massive Dirac fermions, can shift and modify the gap. We show how these changes present in angular-resolved photoemission spectroscopy of the dressed charge carrier dispersion curves and scanning tunneling microscopy measurements of their density of states. In particular we focus on the region around the band gap. In this region the charge carrier spectral density no longer consists of a dominant quasiparticle peak and a smaller incoherent phonon related background. The quasiparticle picture has broken down and this leads to important modification in both dispersion curves and density of states.

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arXiv2013

Magneto-optical conductivity in a topological insulator

Adding a small subdominant quadratic in momentum term to a dominant linear Dirac dispersion curve affects conduction and valence band differently and leads to an hourglass-like structure for energy as a function of momentum. This applies to the protected surface states in topological insulators. The energies of the conduction and valence band Landau levels are also different and this leads to the splitting of optical absorption lines produced by the magnetic field, which acquire a two peak structure. It also changes the peaks in the imaginary part of the Hall conductivity into two distinct contributions of opposite signs. The real part of the circularly polarized optical conductivity however retains its single peak structure but the peaks in right and left handedness case are shifted in energy with respect to each other in contrast to the pure Dirac case. The magnitude of the semiclassical cyclotron frequency is significantly modified by the presence of a mass term as is its variation with value of the chemical potential $μ$. Its optical spectral weight is found to decrease with increasing $μ$ rather than increase as it does in the pure Dirac limit.

cond-mat.mes-hall↗

arXiv2013

Magneto-optical conductivity of Weyl semimetals

Weyl semimetals are a topological phase of matter that have drawn recent interest and have been suggested as a possible phase of the pyrochlore irridates, among other materials. Here, we compute the magneto-optical response of an isolated Weyl point. We find that the conductivity is a series of asymmetric peaks lying on top of a linear background. We find additional features in the conductivity that are explained by the underlying Landau level structure. We show that weak disorder tends to blur out the peaks, but they still show up as measurable oscillations on a linear background.

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arXiv2013

Three-dimensional Dirac fermions in quasicrystals as seen via optical conductivity

The optical conductivity of quasicrystals is characterized by two features not seen in ordinary metallic systems. There is an absence of the Drude peak and the interband conductivity rises linearly from a very low value up to normal metallic levels over a wide range of frequencies. The absence of a Drude peak has been attributed to a pseudogap at the Fermi surface but a detailed explanation of the linear behavior has not been found. Here we show that the linear conductivity, which seems to be universal in all Al based icosahedral quasicrystal families, as well as their periodic approximants, follows from a simple model that assumes that the entire Fermi surface is gapped except at a finite set of Dirac points. There is no evidence of a semiconducting gap in any of the materials suggesting that the Dirac spectrum is massless, protected by topology leading to a Weyl semimetal. This model gives rise to a linear conductivity with only one parameter, the Fermi velocity. This picture suggests that decagonal quasicrystals should, like graphene, have a frequency independent conductivity, without a Drude peak. This is in accord with the experimental data as well.

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arXiv2013

C-axis optical conductivity from the Yang-Rice-Zhang model of the underdoped cuprates

The c-axis optical response of the underdoped cuprates is qualitatively different from its in-plane counterpart. The features of the pseudogap show themselves more prominently in the c-axis than in-plane. We compute both the c-axis and in-plane optical conductivity using the Yang-Rice-Zhang model of the underdoped cuprates. This model combined with coherent interlayer tunnelling is enough to explain the qualitative differences between the in-plane and c-axis data. We show how pseudogap features manifest themselves in the infrared and microwave conductivity within this model.

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arXiv2013

Effect of Dynamical Screening on Single Particle Spectral Features of Uniaxially Strained Graphene: Tuning the Plasmaron Ring

Electronic screening renormalizes the linear bands of graphene and in the vicinity of the Dirac point, creates a diamond shaped structure in the quasiparticle spectral density. This is a result of electron-plasmon scattering processes which produce a finite momentum feature referred to as the `plasmaron ring'. In this work we explore the effects of uniaxial strain on these spectral features with the aim of understanding how strain modifies correlations. We derive and calculate the spectral density to the G$_0$W-RPA level which allows us to identify the dispersive behaviour of the diamond geometry, and thus electron-plasmon scattering, for variation in electron-electron coupling strength and magnitude of applied strain. We find that the application of strain changes the geometry (in momentum) of the electron-plasmon scattering and that renormalizations beyond simple geometrical scalings further enhance this effect. These results suggest that the properties of the plasmaron ring can be tuned through the application of uniaxial strain, effectively producing a larger fine structure constant without the need to change the sample substrate.

cond-mat.mes-hall↗

arXiv2012

Impact of Electron-Phonon Coupling on Near-Field Optical Spectra

The finite momentum transfer ($\boldsymbol{q}$) longitudinal optical response $σ^L(\boldsymbol{q},ω)$ of graphene has a peak at an energy $ω=\hbar v_F q$. This corresponds directly to a quasiparticle peak in the spectral density at momentum relative to the Fermi momentum $k_F -q$. Inclusion of coupling to a phonon mode at $ω_E$ results, for $ω<|ω_E|$, in a constant electron-phonon renormalization of the bare bands by a mass enhancement factor $(1+λ)$ and this is followed by a phonon kink at $ω_E$ where additional broadening begins. Here we study the corresponding changes in the optical quasiparticle peaks which we find to continue to directly track the renormalized quasiparticle energies until $q$ is large enough that the optical transitions begin to sample the phonon kink region of the dispersion curves where linearity in momentum is lost in the renormalized Dirac Fermion dispersion curves and the correspondence to a single quasiparticle energy is lost. Nevertheless there remains in $σ^L(\boldsymbol{q},ω)$ features analogous to the phonon kinks of the dispersion curves which are observable through variation of $q$ and $ω$.

cond-mat.mes-hall↗

arXiv2012

Resonating valence bonds and Fermi surface reconstruction: The resistivity in the underdoped cuprates

The pseudogap phase of the underdoped cuprates is the host to a variety of novel electronic phenomenon. An example is the dc-resistivity which shows metallic behaviour in the ab-plane, while the c-axis response is insulating. We apply a model, originally formulated by Yang, Rice, and Zhang, to study the resistivity in the pseudogap phase. This model is able to reproduce the qualitative features of the resistivity, including the systematic deviations from linear behaviour for the in-plane conductivity, and the insulating behaviour along the c-axis. We compare this to the predictions of the arc model and find similar qualitative behaviour. We find that the most important element in understanding the resistivity is the reconstruction of the Fermi surface, which puts strong restrictions on the number of quasiparticles allowed to participate in dc-transport.

cond-mat.supr-con↗

arXiv2012

Tracking Quasiparticle Energies in Graphene with Near Field Optics

Advances in infrared nanoscopy have enabled access to the finite momentum optical conductivity $σ(\vec{q},ω)$. The finite momentum optical conductivity in graphene has a peak at the Dirac fermion quasiparticle energy $ε(k_F-q)$, i.e. at the Fermi momentum minus the incident photon momentum. We find that the peak remains robust even at finite temperature as well as with residual scattering. It can be used to trace out the fermion dispersion curves. However, this effect depends strongly on the linearity of the Dirac dispersion. Should the Dirac fermions acquire a mass, the peak in $σ(q,w)$ shifts to lower energies and broadens as optical spectral weight is redistributed over an energy range of the order of the mass gap energy. Even in this case structures remain in the conductivity which can be used to describe the excitation spectrum. By contrast, in graphene strained along the armchair direction, the peak remains intact, but shifts to a lower value of $q$ determined by the anisotropy induced by the deformation.

cond-mat.mes-hall↗

arXiv2012

Emergence of Plasmaronic Structure in the Near Field Optical Response of Graphene

The finite momentum optical response $σ({\boldsymbol{q}},ω)$ of graphene can be probed with the innovative technique of infrared nanoscopy where mid-infrared radiation is confined by an atomic force microscope cantilever tip. In contrast to conventional $q\sim 0$ optical absorption which primarily involves Dirac fermions with momentum near the Fermi momentum, $k\sim k_F$, for finite $q$, $σ({\boldsymbol{q}},ω)$ has the potential to provide information on many body renormalizations and collective phenomena which have been found at small $k< k_F$ near the Dirac point in electron-doped graphene. For electron-electron interactions, the low energy excitation spectrum characterizing the incoherent part of the quasiparticle spectral function of Dirac electrons with $k\sim k_F$ consists of a flat, small amplitude background which scales with chemical potential and Fermi momentum. However, probing of the states with $k$ near $k=0$ will reveal plasmarons, a collective state of a charge carrier and a plasmon. These collective modes in graphene have recently been seen in angle-resolved photoemission spectroscopy and here we describe how they manifest in near field optics.

cond-mat.mes-hall↗

arXiv2012

Magneto-optical conductivity in graphene including electron-phonon coupling

We show how coupling to an Einstein phonon $ω_E$ affects the absorption peaks seen in the optical conductivity of graphene under a magnetic field $B$. The energies and widths of the various lines are shifted, and additional peaks arise in the spectrum. Some of these peaks are Holstein sidebands, resulting from the transfer of spectral weight in each Landau level (LL) into phonon-assisted peaks in the spectral function. Other additional absorption peaks result from transitions involving split LLs, which occur when a LL falls sufficiently close to a peak in the self-energy. We establish the selection rules for the additional transitions and characterize the additional absorption peaks. For finite chemical potential, spectral weight is asymmetrically distributed about the Dirac point; we discuss how this causes an asymmetry in the transitions due to left- and right-handed circularly polarized light and therefore oscillatory behavior in the imaginary part of the off-diagonal Hall conductivity. We also find that the semiclassical cyclotron resonance region is renormalized by an effective-mass factor but is not directly affected by the additional transitions. Last, we discuss how the additional transitions can manifest in broadened, rather than split, absorption peaks due to large scattering rates seen in experiment.

cond-mat.mes-hall↗

arXiv2012

Optical Self Energy in Graphene due to Correlations

In highly correlated systems one can define an optical self energy in analogy to its quasiparticle (QP) self energy counterpart. This quantity provides useful information on the nature of the excitations involved in inelastic scattering processes. Here we calculate the self energy of the intraband optical transitions in graphene originating in the electron-electron interaction (EEI) as well as electron-phonon interaction (EPI). Although optics involves an average over all momenta ($k$) of the charge carriers, the structure in the optical self energy is nevertheless found to mirror mainly that of the corresponding quasiparticles for $k$ equal to or near the Fermi momentum $k_F$. Consequently plasmaronic structures which are associated with momenta near the Dirac point at $k=0$ are not important in the intraband optical response. While the structure of the electron-phonon interaction (EPI) reflects the sharp peaks of the phonon density of states, the excitation spectrum associated with the electron-electron interaction is in comparison structureless and flat and extends over an energy range which scales linearly with the value of the chemical potential. Modulations seen on the edge of the interband optical conductivity as it rises towards its universal background value are traced to structure in the quasiparticle self energies around $k_F$ of the lower Dirac cone associated with the occupied states.

cond-mat.str-el↗

arXiv2012

Distinguishing Coulomb and electron-phonon interactions for massless Dirac fermions

While many physical properties of graphene can be understood qualitatively on the basis of bare Dirac bands, there is specific evidence that electron-electron (EE) and electron-phonon (EP) interactions can also play an important role. We discuss strategies for extracting separate images of the EE and EP interactions as they present themselves in the electron spectral density and related self-energies. While for momentum, $k$, equal to its Fermi value, $k_F$, a composite structure is obtained which can be difficult to separate into its two constituent parts, at smaller values of $k$ the spectral function shows distinct incoherent sidebands on the left and right of the main quasiparticle line. These image respectively the EE and EP interactions, each being most prominent in its own energy window. We employ a maximum entropy inversion technique on the self energy to reveal the electron-phonon spectral density separate from the excitation spectrum due to coulomb correlations. Our calculations show that this technique can provide important new insights into inelastic scattering processes in graphene.

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