arXiv subjects

J. P. Carbotte

Publications and source records attributed to J. P. Carbotte.

At least 91 records · Page 5Linked to original sources

arXiv2009

Characteristics of oxygen isotope substitutions in the quasiparticle spectrum of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$

There is an ongoing debate about the nature of the bosonic excitations responsible for the quasiparticle self energy in high temperature superconductors -- are they phonons or spin fluctuations? We present a careful analysis of the bosonic excitations as revealed by the `kink' feature at 70 meV in angle resolved photoemission data using Eliashberg theory for a d-wave superconductor. Starting from the assumption that nodal quasiparticles are not coupled to the $(π,π)$ magnetic resonance, the sharp structure at $70 $meV can be assigned to phonons. We find that not only can we account for the shifts of the kink energy seen on oxygen isotope substitution but also get a quantitative estimate of the fraction of the area under the electron-boson spectral density which is due to phonons. We conclude that for optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ phonons contribute $\sim 10$% and non-phononic excitations $\sim 90$%.

cond-mat.supr-con↗

arXiv2009

Phonon spectroscopy through the electronic density of states in graphene

We study how phonon structure manifests itself in the electronic density of states of graphene. A procedure for extracting the value of the electron-phonon renormalization $λ$ is developed. In addition, we identify direct phonon structures. With increasing doping, these structures, along with $λ$, grow in amplitude and no longer display particle-hole symmetry.

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arXiv2009

Specific heat of underdoped cuprates: RVB versus Fermi arcs

A recent microscopic model of the pseudogap state, based on the resonating valence bond (RVB) spin liquid, has provided a simple ansatz for the electronic self energy in which a gap forms on the antiferromagnetic Brillouin zone as the limit of a Mott insulator is approached in the underdoped regime. Here, the ansatz is employed to calculate the electronic specific heat when a superconducting gap is also included. We find qualitative agreement with all experimental observations in the underdoped regime of the cuprates. We explore the relationship of the theory to two other purely phenomenological approaches, the nodal liquid and the Fermi arc model, and provide justification for their use on experimental data in light of this microscopic RVB theory.

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arXiv2009

Non-BCS behavior of optical properties across the cuprate phase diagram

The finite-frequency optical properties of the underdoped cuprates, in both the normal and superconducting state, display features which go beyond a Fermi liquid and a BCS description. We provide an understanding of these properties within a simplified analytical model, which has been evolved out of the Hubbard model and ideas based on a resonating valence bond spin liquid. We find that: 1) in underdoped samples, the missing area integrals reveal a second energy scale due to the pseudogap, not present at optimum or overdoping; 2) the real part of the optical self-energy shows a large sharp peak, that emerges with the opening of the pseudogap which exists within the superconducting state and persists in the normal state; and 3) the amount of optical spectral weight which is transferred to the condensate is greatly reduced by the presence of the pseudogap as compared to the Fermi liquid case. These non-BCS features of the superconducting state are in good qualitative agreement with a body of experimental work on different cuprate systems and provide strong evidence from optical conductivity that they are all a manifestation of the pseudogap energy scale.

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arXiv2009

Spin Dynamics in Cuprates: Optical Conductivity of HgBa2CuO4

The electron-boson spectral density function I^2ChiOmega responsible for carrier scattering of the high temperature superconductor HgBa2CuO4 (Tc = 90 K) is calculated from new data on the optical scattering rate. A maximum entropy technique is used. Published data on HgBa2Ca2Cu3O8 (Tc = 130 K) are also inverted and these new results are put in the context of other known cases. All spectra (with two notable exceptions) show a peak at an energy (Omega_r) proportional to the superconducting transition temperature Omega_r ~= 6.3 kB.Tc. This charge channel relationship follows closely the magnetic resonance seen by polarized neutron scattering, Omega_r^{neutron} ~= 5.4 kB.Tc. The amplitudes of both peaks decrease strongly with increasing temperature. In some cases, the peak at Omega_r is weak and the spectrum can have additional maxima and a background extending up to several hundred meV.

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arXiv2008

Multiple bosonic mode coupling in the charge dynamics of the electron-doped superconductor (Pr$_{2-x}$Ce$_x$)CuO$_4$

We analyze optical spectroscopy data of the electron-doped superconductor (Pr$_{2-x}$Ce$_x$)CuO$_4$ (PCCO) to investigate the coupling of the charge carriers to bosonic modes. The method of analysis is the inversion of the optical scattering rate $τ^{-1}_{\rm op}(ω,T)$ at different temperatures $T$ by means of maximum entropy technique combined with Eliashberg theory. We find that in the superconducting state the charge carriers couple to two dominant modes one at $\sim 10 $meV and a second one at $\sim 45 $meV. The low energy mode shows a strong temperature dependence and disappears at or slightly above the critical temperature $T_c$. The high energy mode exists above $T_c$ and moves towards higher energies with increasing temperatures. It also becomes less prominent at temperatures $> 100 $K above which it evolves into a typical spin-fluctuation background. In contrast to the hole-doped High-$T_c$ superconductors PCCO proves to be a superconductor close to the dirty limit.

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arXiv2008

Optical spectroscopy of superconducting Ba{0.55}K{0.45}Fe2As2: evidence for strong coupling to low energy bosons

Optical spectroscopy on single crystals of the new iron arsenide superconductor Ba{0.55}K{0.45}Fe2As2 shows that the infrared spectrum consists of two major components: a strong metallic Drude band and a well separated mid infrared absorption centered at 0.7 eV. It is difficult to separate the two components unambiguously but several fits of Lorentzian peaks suggest a model with a Drude peak having a plasma frequency of 1.8 to 2.1 eV and a midinfrared peak with a plasma frequency of 2.5 eV. In contrast to the cuprate superconductors the scattering rate obtained from the extended Drude model saturates at 150 meV as compared to 500 meV for a typical cuprate. Detailed analysis of the frequency dependent scattering rate shows that the charge carriers interact with broad bosonic spectrum with a peak at 25 meV and a coupling constant lambda =approx 2 at low temperature. As the temperature increases this coupling weakens to lambda=0.6 at ambient temperature. This suggests a bosonic spectrum that is similar to what is seen in the lower Tc cuprates.

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arXiv2008

Signatures of superconducting gap inhomogeneities in optical properties

Scanning tunneling spectroscopy applied to the high-$T_{c}$ cuprates has revealed significant spatial inhomogeneity on the nanoscale. Regions on the order of a coherence length in size show variations of the magnitude of the superconducting gap of order $\pm20%$ or more. An important unresolved question is whether or not these variations are also present in the bulk, and how they influence superconducting properties. As many theories and data analyses for high-$T_{c}$ superconductivity assume spatial homogeneity of the gap magnitude, this is a pressing question. We consider the far-infrared optical conductivity and evaluate, within an effective medium approximation, what signatures of spatial variations in gap magnitude are present in various optical quantities. In addition to the case of d-wave superconductivity, relevant to the high-$T_c$ cuprates, we have also considered s-wave gap symmetry in order to provide expected signatures of inhomogeneities for superconductors in general. While signatures of gap inhomogeneities can be strongly manifested in s-wave superconductors, we find that the far-infrared optical conductivity in d-wave is robust against such inhomogeneity.

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arXiv2008

Manifestation of pseudogap in ab-plane optical characteristics

A model in which a gap forms in the renormalized electronic density of state (DOS) with missing states recovered just above the pseudogap $Δ_{pg}$, is able to give a robust description of the striking, triangular like, peak seen in the real part of the optical self-energy of underdoped cuprates. We use this model to explore the effect of the pseudogap on the real part of the optical conductivity and on the partial sum rule associated with it. An important result is that the optical spectral weight redistributes over a much larger frequency window than it does in the DOS.

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arXiv2008

Fermi surface arcs and the infrared conductivity of underdoped YBa$_{2}$Cu$_{3}$O$_{6.50}$

We reanalyze the data on the in-plane far infrared conductivity of underdoped orthoII YBa$_{2}$Cu$_{3}$O$_{6.50}$ (YBCO$_{6.50}$) in terms of a model in which a pseudogap opens on part of the Fermi surface with the remaining ungaped piece proportional to the temperature. The motivation for our model comes from recent angle-resolved photoemission spectroscopy data in underdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi-2212), which have revealed the existence of arcs on the Fermi surface. We find the optical data to be consistent with arc formation. In addition we find some evidence that the electronic states lost below the pseudogap energy $Δ_{pg}$ are recovered in the energy region immediately above it at least for temperatures near $T_c$.

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arXiv2008

Evidence for a pseudogap in underdoped $Bi_2Sr_2CaCu_2O_{8+δ}$ and $YBa_2Cu_3O_{6.50}$ from in-plane optical conductivity measurements

The real part of the in-plane optical self-energy data in underdoped Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ (Bi-2212) and ortho II YBa$_{2}$Cu$_{3}$O$_{6.5}$ contains new and important information on the pseudogap. Using a theoretical model approach we find that the density of state lost below the pseudogap $Δ_{pg}$ is accompanied with a pileup just above this energy. The pileup along with a sharp mode in the bosonic spectral function leads to an unusually rapid increase in the optical scattering rate and a characteristically sloped peak in the real part of the optical self-energy. These features are not found in optimally doped and overdoped samples and represent a clearest signature so far of the opening of a pseudogap in the in-plane optical conductivity.

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arXiv2008

Bosonic spectral density of epitaxial thin-film La1.83Sr0.17CuO4 superconductors from infrared conductivity measurements

We use optical spectroscopy to investigate the excitations responsible for the structure in the optical self-energy of thin epitaxial films of La1.83Sr0.17CuO4. Using Eliashberg formalism to invert the optical spectra we extract the electron-boson spectral function and find that at low temperature it has a two component structure closely matching the spin excitation spectrum recently measured by magnetic neutron scattering. We contrast the temperature evolution of the spectral density and the two-peak behavior in La2-xSrxCuO4 with another high temperature superconductor Bi2Sr2CaCu2O8+d. The bosonic spectral functions of the two materials account for the low Tc of LSCO as compared to Bi-2212.

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arXiv2008

Robustness of the optical-conductivity sum rule in Bilayer Graphene

We calculate the optical sum associated with the in-plane conductivity of a graphene bilayer. A bilayer asymmetry gap generated in a field-effect device can split apart valence and conduction bands, which otherwise would meet at two K points in the Brillouin zone. In this way one can go from a compensated semimetal to a semiconductor with a tunable gap. However, the sum rule turns out to be 'protected' against the opening of this semiconducting gap, in contrast to the large variations observed in other systems where the gap is induced by strong correlation effects.

cond-mat.mes-hall↗

arXiv2008

Optical conductivity of bilayer graphene with and without an asymmetry gap

When a bilayer of graphene is placed in a suitably configured field effect device, an asymmetry gap can be generated and the carrier concentration made different in each layer. This provides a tunable semiconducting gap, and the valence and the conductance band no longer meet at the two Dirac points of the graphene Brillouin zone. We calculate the optical conductivity of such a semiconductor with particular emphasis on the optical spectral weight redistribution brought about by changes in gap and chemical potential due to charging. We derive an algebraic formula for arbitrary value of the chemical potential for the case of the bilayer conductivity without a gap.

cond-mat.mes-hall↗

arXiv2008

The unusual thickness dependence of superconductivity in $α$-MoGe thin films

Thin films of $α$-MoGe show progressively reduced $T_{c}$'s as the thickness is decreased below 30 nm and the sheet resistance exceeds 100 $Ω/\Box$. We have performed far-infrared transmission and reflection measurements for a set of $α$-MoGe films to characterize this weakened superconducting state. Our results show the presence of an energy gap with ratio $2Δ_0/k_BT_{c} = 3.8 \pm 0.1$ in all films studied, slightly higher than the BCS value, even though the transition temperatures decrease significantly as film thickness is reduced. The material properties follow BCS-Eliashberg theory with a large residual scattering rate except that the coherence peak seen in the optical scattering rate is found to be strongly smeared out in the thinner superconducting samples. A peak in the optical mass renormalization at $2Δ_0$ is predicted and observed for the first time.

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arXiv2008

Optical self-energy of superconducting Pb in the THz region

New THz data on the optical conductivity of Pb are presented as well as a detailed Eliashberg analysis with particular emphasis on phonon-assisted processes not included in a BCS approach. Consideration of the optical self-energy instead of the conductivity itself helps highlight the differences with BCS predictions. Predicted coherence peaks are observed in the optical scattering rates. Impurities enhance the optical effective mass at zero frequency by an order of magnitude and induce a large peak at twice the gap in agreement with theory. This work illustrates the usefulness of the optical self-energy for the analysis of data.

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arXiv2008

Finite band inversion of ARPES in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ in comparison with optics

Using a maximum entropy technique within a finite band Eliashberg formalism we extract from recent high accuracy nodal direction angular resolved photo-emission spectroscopy (ARPES) data in optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi2212) a quasiparticle electron-boson spectral density. Both normal and superconducting state with d-wave gap symmetry are treated. Finite and infinite band results are considered and contrasted. We compare with results obtained for the related transport spectral density which follows from a similar inversion of optical data. We discuss the implication of our results for quasiparticle renormalizations in the antinodal direction.

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arXiv2007

AC conductivity of graphene: from tight-binding model to 2+1-dimensional quantum electrodynamics

We consider the relationship between the tight-binding Hamiltonian of the two-dimensional honeycomb lattice of carbon atoms with nearest neighbor hopping only and the 2+1 dimensional Hamiltonian of quantum electrodynamics which follows in the continuum limit. We pay particular attention to the symmetries of the free Dirac fermions including spatial inversion, time reversal, charge conjugation and chirality. We illustrate the power of such a mapping by considering the effect of the possible symmetry breaking which corresponds to the creation of a finite Dirac mass, on various optical properties. In particular, we consider the diagonal AC conductivity with emphasis on how the finite Dirac mass might manifest itself in experiment. The optical sum rules for the diagonal and Hall conductivities are discussed.

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