arXiv subjects

J. P. F. LeBlanc

Publications and source records attributed to J. P. F. LeBlanc.

48 records · Page 3Linked to original sources

arXiv2013

Equation of State of the Fermionic 2D Hubbard Model

We present results for the equation of state of the two-dimensional Hubbard model on an isotropic square lattice as obtained from a controlled and numerically exact large-cluster dynamical mean field simulation. Our results are obtained for large but finite systems and are extrapolated to infinite system size using a known finite size scaling relation. We present the energy, entropy, double occupancy and nearest-neighbour spin correlations extrapolated to the thermodynamic limit and discuss the implications of these calculations on pseudogap physics of the 2D-Hubbard model away from half filling. We find a strong behavioural shift in energy below a temperature $T^*$ which becomes more pronounced for larger clusters. Finally, we provide reference calculations and tables for the equation of state for values of doping away from half filling which are of interest to cold atom experiments.

cond-mat.str-el↗

arXiv2013

Effect of Dynamical Screening on Single Particle Spectral Features of Uniaxially Strained Graphene: Tuning the Plasmaron Ring

Electronic screening renormalizes the linear bands of graphene and in the vicinity of the Dirac point, creates a diamond shaped structure in the quasiparticle spectral density. This is a result of electron-plasmon scattering processes which produce a finite momentum feature referred to as the `plasmaron ring'. In this work we explore the effects of uniaxial strain on these spectral features with the aim of understanding how strain modifies correlations. We derive and calculate the spectral density to the G$_0$W-RPA level which allows us to identify the dispersive behaviour of the diamond geometry, and thus electron-plasmon scattering, for variation in electron-electron coupling strength and magnitude of applied strain. We find that the application of strain changes the geometry (in momentum) of the electron-plasmon scattering and that renormalizations beyond simple geometrical scalings further enhance this effect. These results suggest that the properties of the plasmaron ring can be tuned through the application of uniaxial strain, effectively producing a larger fine structure constant without the need to change the sample substrate.

cond-mat.mes-hall↗

arXiv2012

Impact of Electron-Phonon Coupling on Near-Field Optical Spectra

The finite momentum transfer ($\boldsymbol{q}$) longitudinal optical response $σ^L(\boldsymbol{q},ω)$ of graphene has a peak at an energy $ω=\hbar v_F q$. This corresponds directly to a quasiparticle peak in the spectral density at momentum relative to the Fermi momentum $k_F -q$. Inclusion of coupling to a phonon mode at $ω_E$ results, for $ω<|ω_E|$, in a constant electron-phonon renormalization of the bare bands by a mass enhancement factor $(1+λ)$ and this is followed by a phonon kink at $ω_E$ where additional broadening begins. Here we study the corresponding changes in the optical quasiparticle peaks which we find to continue to directly track the renormalized quasiparticle energies until $q$ is large enough that the optical transitions begin to sample the phonon kink region of the dispersion curves where linearity in momentum is lost in the renormalized Dirac Fermion dispersion curves and the correspondence to a single quasiparticle energy is lost. Nevertheless there remains in $σ^L(\boldsymbol{q},ω)$ features analogous to the phonon kinks of the dispersion curves which are observable through variation of $q$ and $ω$.

cond-mat.mes-hall↗

arXiv2012

Emergence of Plasmaronic Structure in the Near Field Optical Response of Graphene

The finite momentum optical response $σ({\boldsymbol{q}},ω)$ of graphene can be probed with the innovative technique of infrared nanoscopy where mid-infrared radiation is confined by an atomic force microscope cantilever tip. In contrast to conventional $q\sim 0$ optical absorption which primarily involves Dirac fermions with momentum near the Fermi momentum, $k\sim k_F$, for finite $q$, $σ({\boldsymbol{q}},ω)$ has the potential to provide information on many body renormalizations and collective phenomena which have been found at small $k< k_F$ near the Dirac point in electron-doped graphene. For electron-electron interactions, the low energy excitation spectrum characterizing the incoherent part of the quasiparticle spectral function of Dirac electrons with $k\sim k_F$ consists of a flat, small amplitude background which scales with chemical potential and Fermi momentum. However, probing of the states with $k$ near $k=0$ will reveal plasmarons, a collective state of a charge carrier and a plasmon. These collective modes in graphene have recently been seen in angle-resolved photoemission spectroscopy and here we describe how they manifest in near field optics.

cond-mat.mes-hall↗

arXiv2012

Optical Self Energy in Graphene due to Correlations

In highly correlated systems one can define an optical self energy in analogy to its quasiparticle (QP) self energy counterpart. This quantity provides useful information on the nature of the excitations involved in inelastic scattering processes. Here we calculate the self energy of the intraband optical transitions in graphene originating in the electron-electron interaction (EEI) as well as electron-phonon interaction (EPI). Although optics involves an average over all momenta ($k$) of the charge carriers, the structure in the optical self energy is nevertheless found to mirror mainly that of the corresponding quasiparticles for $k$ equal to or near the Fermi momentum $k_F$. Consequently plasmaronic structures which are associated with momenta near the Dirac point at $k=0$ are not important in the intraband optical response. While the structure of the electron-phonon interaction (EPI) reflects the sharp peaks of the phonon density of states, the excitation spectrum associated with the electron-electron interaction is in comparison structureless and flat and extends over an energy range which scales linearly with the value of the chemical potential. Modulations seen on the edge of the interband optical conductivity as it rises towards its universal background value are traced to structure in the quasiparticle self energies around $k_F$ of the lower Dirac cone associated with the occupied states.

cond-mat.str-el↗

arXiv2012

Distinguishing Coulomb and electron-phonon interactions for massless Dirac fermions

While many physical properties of graphene can be understood qualitatively on the basis of bare Dirac bands, there is specific evidence that electron-electron (EE) and electron-phonon (EP) interactions can also play an important role. We discuss strategies for extracting separate images of the EE and EP interactions as they present themselves in the electron spectral density and related self-energies. While for momentum, $k$, equal to its Fermi value, $k_F$, a composite structure is obtained which can be difficult to separate into its two constituent parts, at smaller values of $k$ the spectral function shows distinct incoherent sidebands on the left and right of the main quasiparticle line. These image respectively the EE and EP interactions, each being most prominent in its own energy window. We employ a maximum entropy inversion technique on the self energy to reveal the electron-phonon spectral density separate from the excitation spectrum due to coulomb correlations. Our calculations show that this technique can provide important new insights into inelastic scattering processes in graphene.

cond-mat.str-el↗

arXiv2011

Effect of electron-phonon coupling on energy and density of states renormalizations of dynamically screened graphene

Electronic screening strongly renormalizes the linear bands which occur near the Dirac crossing in graphene. The single bare Dirac crossing is split into two individual Dirac-like points, which are separated in energy but still at zero momentum relative to the K-point. A diamond-like structure occurs in between as a result of the formation of plasmarons. In this work we explore the combined effect of electron-electron and electron-phonon coupling on the renormalized energy dispersion, the spectral function and on the electronic density of states. We find that distinct signatures of the plasmaron structure are observable in the density of states with the split Dirac points presenting themselves as minima with quadratic dependence on energy about such points. By examining the slopes of both the density of states and the renormalized dispersion near the Fermi level, we illustrate how one can separate $k$-dependent and $ω$-dependent renormalizations and suggest how this might allow for the isolation of the renormalization due to the electron-phonon interaction from that of the electron-electron interaction.

cond-mat.mes-hall↗

arXiv2011

Electronic structure in underdoped cuprates due to the emergence of a pseudogap

The phenomenological Green's function developed in the works of Yang, Rice and Zhang has been very successful in understanding many of the anomalous superconducting properties of the deeply underdoped cuprates. It is based on considerations of the resonating valence bond spin liquid approximation and is designed to describe the underdoped regime of the cuprates. Here we emphasize the region of doping, $x$, just below the quantum critical point at which the pseudogap develops. In addition to Luttinger hole pockets centered around the nodal direction, there are electron pockets near the antinodes which are connected to the hole pockets by gapped bridging contours. We determine the contours of nearest approach as would be measured in angular resolved photoemission experiments and emphasize signatures of the Fermi surface reconstruction from the large Fermi contour of Fermi liquid theory (which contains $1+x$ hole states) to the Luttinger pocket (which contains $x$ hole states). We find that the quasiparticle effective mass renormalization increases strongly towards the edge of the Luttinger pockets beyond which it diverges.

cond-mat.supr-con↗

arXiv2010

Effects of a particle-hole asymmetric pseudogap on Bogoliubov quasiparticles

We show that in the presence of a pseudogap, the spectral function in the superconducting state of the underdoped cuprates exhibits additional Bogoliubov quasiparticle peaks at both positive and negative energy which are revealed by the particle-hole asymmetry of the pseudogapped energy bands. This provides direct information on the unoccupied band via measurement of the occupied states. When sufficiently close, these Bogoliubov peaks will appear to merge with existing peaks leading to the anomalous observation, seen in experiment, that the carrier spectral density broadens with reduced temperature in the superconducting state. Using the resonating valence bond (RVB) spin liquid model in conjunction with recent angle-resolved photoemission spectroscopy (ARPES) data allows for an empirical determination of the temperature dependence of the pseudogap suggesting that it opens only very gradually below the pseudogap onset temperature $T^*$.

cond-mat.supr-con↗

arXiv2009

Effect of pseudogap formation on the penetration depth of underdoped high $T_c$ cuprates

The penetration depth is calculated over the entire doping range of the cuprate phase diagram with emphasis on the underdoped regime. Pseudogap formation on approaching the Mott transition, for doping below a quantum critical point, is described within a model based on the resonating valence bond spin liquid which provides an ansatz for the coherent piece of the Green's function. Fermi surface reconstruction, which is an essential element of the model, has a strong effect on the superfluid density at T=0 producing a sharp drop in magnitude, but does not change the slope of the linear low temperature variation. Comparison with recent data on Bi-based cuprates provides validation of the theory and shows that the effects of correlations, captured by Gutzwiller factors, are essential for a qualitative understanding of the data. We find that the Ferrell-Glover-Tinkham sum rule still holds and we compare our results with those for the Fermi arc and the nodal liquid models.

cond-mat.supr-con↗

arXiv2009

Specific heat of underdoped cuprates: RVB versus Fermi arcs

A recent microscopic model of the pseudogap state, based on the resonating valence bond (RVB) spin liquid, has provided a simple ansatz for the electronic self energy in which a gap forms on the antiferromagnetic Brillouin zone as the limit of a Mott insulator is approached in the underdoped regime. Here, the ansatz is employed to calculate the electronic specific heat when a superconducting gap is also included. We find qualitative agreement with all experimental observations in the underdoped regime of the cuprates. We explore the relationship of the theory to two other purely phenomenological approaches, the nodal liquid and the Fermi arc model, and provide justification for their use on experimental data in light of this microscopic RVB theory.

cond-mat.supr-con↗

arXiv2008

Signatures of superconducting gap inhomogeneities in optical properties

Scanning tunneling spectroscopy applied to the high-$T_{c}$ cuprates has revealed significant spatial inhomogeneity on the nanoscale. Regions on the order of a coherence length in size show variations of the magnitude of the superconducting gap of order $\pm20%$ or more. An important unresolved question is whether or not these variations are also present in the bulk, and how they influence superconducting properties. As many theories and data analyses for high-$T_{c}$ superconductivity assume spatial homogeneity of the gap magnitude, this is a pressing question. We consider the far-infrared optical conductivity and evaluate, within an effective medium approximation, what signatures of spatial variations in gap magnitude are present in various optical quantities. In addition to the case of d-wave superconductivity, relevant to the high-$T_c$ cuprates, we have also considered s-wave gap symmetry in order to provide expected signatures of inhomogeneities for superconductors in general. While signatures of gap inhomogeneities can be strongly manifested in s-wave superconductors, we find that the far-infrared optical conductivity in d-wave is robust against such inhomogeneity.

cond-mat.supr-con↗