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J. P. Gauyacq

Publications and source records attributed to J. P. Gauyacq.

4 recordsLinked to original sources

Extremely long-lived magnetic excitations in supported Fe chains

We report on a theoretical study of the lifetime of the first excited state of spin chains made of an odd number of Fe atoms on Cu2N/Cu(100). Yan et al (Nat. Nanotech. 10, 40 (2015)) recently observed very long lifetimes in the case of Fe3 chains. We consider the decay of the first excited state induced by electron-hole pair creation in the substrate. For a finite magnetic field, the two lowest-lying states in the chain have a quasi-Néel state structure. Decay from one state to the other strongly depends on the degree of entanglement of the local spins in the chain. The entanglement in the chain accounts for the long lifetimes that increase exponentially with chain length. Despite their apparently very different properties, the behaviour of odd and even chains is governed by the same kind of phenomena, in particular entanglement effects. The present results account quite well for the lifetimes recently measured by Yan et al on Fe3

cond-mat.mes-hall↗

Excitation of spin waves by tunnelling electrons in one-dimensional ferro and anti-ferromagnets

Excitation of finite chains of magnetic atoms adsorbed on a surface by tunnelling electrons from an STM (Scanning Tunnelling Microscope) tip is studied using a Heisenberg Hamiltonian description of the magnetic couplings along the chain and a strong coupling approach of inelastic tunnelling. The excitation probability of the magnetic levels is very high and the excitation spectra in chains of different lengths are very similar. The excitations in finite chains can be considered as spin waves quantized in the finite object. The energy and momentum spectra of the spin waves excited in the idealized infinite chain by tunnelling electrons are determined from the results on the finite chains. Both ferro- and antiferromagnetic couplings are considered, leading to very different results. In particular, in the anti-ferromagnetic case, excitations linked to the entanglement of the chain ground state are evidenced.

cond-mat.str-el↗

Optimization of a Langmuir-Taylor detector for lithium

This paper describes the construction and optimization of a Langmuir-Taylor detector for lithium, using a rhenium ribbon. The absolute detection probability of this very sensitive detector is measured and the dependence of this probability with oxygen pressure and surface temperature is studied. Sources of background signal and their minimization are also discussed in details. And a comparison between our data concerning the response time of the detector and literature values is given. A theoretical analysis has been made: this analysis supports the validity of the Saha-Langmuir law to relate the ionization probability to the work function. Finally, the rapid variations of the work function with oxygen pressure and temperature are explained by a chemical equilibrium model.

physics.ins-det↗

Wave packet propagation study of the charge transfer interaction in the F^- -Cu(111) and -Ag(111) systems

The electron transfer between an $F^{-}$ ion and $Cu(111)$ and $Ag(111)$ surfaces is studied by the wave packet propagation method in order to determine specifics of the charge transfer interaction between the negative ion and the metal surface due to the projected band gap. A new modeling of the $F^{-}$ ion is developed that allows one to take into account the six quasi-equivalent electrons of $F^{-}$ which are {\it a priori} active in the charge transfer process. The new model invokes methods of constrained quantum dynamics. The six-electron problem is transformed to two one-electron problems linked via a constraint. The projection method is used to develop a wave packet propagation subject to the modeling constraint. The characteristics (energy and width) of the ion $F^{-}$ ion level interacting with the two surfaces are determined and discussed in connection with the surface projected band gap.

physics.atom-ph↗