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J. Qi

Publications and source records attributed to J. Qi.

At least 19 recordsLinked to original sources
arXiv2026

Globular Clusters in the Time of the JWST. I. Survey Design and First Results on Multiple Populations and Beyond

Globular clusters (GCs) host multiple stellar populations with distinct chemical compositions, but their properties among very low-mass stars remain poorly constrained. The James Webb Space Telescope (JWST) enables precise infrared studies that are highly sensitive to abundance variations in cool stars. We initiate a homogeneous survey of Galactic GCs, based primarily on deep JWST GO-8960 observations and complemented by archival JWST and Hubble Space Telescope data, to characterize multiple populations across a wide range of cluster properties. In this first paper, we present the survey and initial NIRCam results. We analyze eleven GCs, deriving high-precision photometry and astrometry to measure proper motions. Multiple populations are detected among low-mass stars in all clusters, with diverse behaviors. We find discrete main sequences in NGC 288, NGC 6723, and NGC 2808, and more continuous distributions in NGC 104 and the Type II clusters NGC 1851 and NGC 6656. The bulge clusters NGC 6528, NGC 6553, and NGC 6440 show patterns consistent with varying helium and oxygen abundances that do not scale simply with cluster mass. In Terzan 5 and Liller 1, we identify populations spanning different ages and helium variations within the old population of Terzan 5. We also detect an M-dwarf gap in NGC 104 around 0.35 solar masses, consistent with the Jao Gap of field stars and open clusters. This work establishes the foundation for a homogeneous JWST survey of Galactic GCs and provides a valuable dataset for studies of cluster evolution, Galactic stellar populations, and background extragalactic sources.

astro-ph.GA↗
arXiv2025

Competing Lattice and Defect Dynamics Govern Terahertz-Induced Ferroelectricity in Quantum Paraelectric SrTiO$_3$

Intense terahertz (THz) pulses induce transient inversion-symmetry breaking in quantum paraelectric SrTiO$_3$, yet the underlying mechanism remains controversial. Using fields up to $\sim$1.1 MV/cm, we reveal spatially inhomogeneous THz-field-induced second harmonic generation (TFISH) governed by competing lattice and defect dynamics. Short-lived coherent antiferrodistortive (AFD) modes suppress dipole correlations within $\sim$5 ps, while heavily damped soft/AFD modes and a defect-induced low-frequency mode ($\sim$0.1-0.3 THz) jointly prevent long-range ferroelectric coherence in oxygen-vacancy-rich regions. Collective modes manifested by oscillatory TFISH components exhibit softening followed by hardening below a critical temperature $T^*\simeq$28 K, confirming transient ferroelectric order where defects are sparse. These results reconcile conflicting interpretations, establish defect-mediated competition as a central regulator of light-induced ferroelectricity, and open routes to ultrafast control of quantum materials.

cond-mat.mtrl-sci↗
arXiv2024

Exploring Simple-Population and Multiple-Population Globular Clusters in the Outer Galactic Halo using the Hubble Space Telescope

The pseudo two-color diagram, known as chromosome map (ChM), is a valuable tool for identifying globular clusters (GCs) that consist of single or multiple stellar populations (MPs). Recent surveys of Galactic GCs using the ChM have provided stringent observational constraints on the formation of GCs and their stellar populations. However, these surveys have primarily focused on GCs at moderate distances from the Galactic center and composed of MPs. In this paper, we present the first detailed study of the stellar composition of four GCs in the outer halo of the Milky Way: Arp 2, Ruprecht 106, Terzan 7, and Terzan 8. Our analysis is based on high-precision photometry obtained from images collected with the Hubble Space Telescope in the F275W, F336W, F438W, F606W, and F814W bands. We find that Ruprecht 106 and Terzan 7 are composed solely of a single stellar population, whereas Arp 2 and Terzan 8 host both first- and second-population stars. In these clusters, the second population comprises about half and one-third of the total number of GC stars, respectively. The results from this paper and the literature suggest that the threshold in the initial GC mass, if present, should be smaller than approximately 10^5 M$_{\odot}$. The first-population stars of Arp 2 and Terzan 8, along with the stars of the simple-population GCs Ruprecht 106 and Terzan 7, exhibit intrinsic F275W - F814W color spreads, likely indicative of [Fe/H] variations of approximately 0.05 -- 0.30 dex. This suggests that star-to-star metallicity variations are a common feature of star clusters, regardless of the presence of MPs.

astro-ph.GA↗
arXiv2024

The pervasiveness of shape coexistence in nuclear pair condensates

We investigate nuclear shape coexistence for a wide range of even-even nuclides. By varying general pair condensates, which include Slater determinants as a limit but also allow for arbitrary pairing channels, we frequently find multiple coexisting mimina, and often more than two. This is consistent with recent experimental results. In order to measure general pairwise correlations beyond a simple Slater determinant, we introduce a novel entropy-like measure, which is smallest mid-shell and largest near shell closures; this is consistent with a picture of pairing-like behavior dominating near closed shells and deformation mid-shell. After surveying nuclides spanning from the $sd$ shell to nuclides between magic numbers 50 and 82, we focus on the six lightest nuclei with shape coexistence. Angular-momentum projected variational pair condensate (PVPC) calculations identify band structures, including two newly proposed coexisting bands in $^{26}$Si/Mg and $^{24}$Si/Ne. The PVPC results agree well with data, providing robust experimental support for the pervasiveness of coexistence in these light nuclei.

nucl-th↗
arXiv2021

Extremely low-energy collective modes in a quasi-one-dimensional system

We have investigated the quasiparticle dynamics and collective excitations in the quasi-one-dimensional material ZrTe$_5$ using ultrafast optical pump-probe spectroscopy. Our time-domain results reveal two coherent oscillations having extremely low energies of $\hbar\omega_1\sim$0.33 meV (0.08 THz) and $\hbar\omega_2\sim$1.9 meV (0.45 THz), which are softened as the temperature approaches two different critical temperatures ($\sim$54 K and $\sim$135 K). We attribute these two collective excitations to the amplitude mode of charge density wave instabilities in ZrTe$_5$ with tremendously small nesting wave vectors. Furthermore, scattering with the $\hbar\omega_2$ mode may result in a peculiar quasiparticle decay process with a timescale of $\sim$1-2 ps below the transition temperature $T^*$ ($\sim$135 K). Our findings provide pivotal information for studying the fluctuating order parameters and their associated quasiparticle dynamics in various low-dimensional topological systems and other materials.

cond-mat.mtrl-sci↗
arXiv2021

Search for Coherent Elastic Scattering of Solar $^8$B Neutrinos in the XENON1T Dark Matter Experiment

We report on a search for nuclear recoil signals from solar $^8$B neutrinos elastically scattering off xenon nuclei in XENON1T data, lowering the energy threshold from 2.6 keV to 1.6 keV. We develop a variety of novel techniques to limit the resulting increase in backgrounds near the threshold. No significant $^8$B neutrino-like excess is found in an exposure of 0.6 t $\times$ y. For the first time, we use the non-detection of solar neutrinos to constrain the light yield from 1-2 keV nuclear recoils in liquid xenon, as well as non-standard neutrino-quark interactions. Finally, we improve upon world-leading constraints on dark matter-nucleus interactions for dark matter masses between 3 GeV/c$^2$ and 11 GeV/c$^2$ by as much as an order of magnitude.

hep-ex↗
arXiv2021

Search for inelastic scattering of WIMP dark matter in XENON1T

We report the results of a search for the inelastic scattering of weakly interacting massive particles (WIMPs) in the XENON1T dark matter experiment. Scattering off $^{129}$Xe is the most sensitive probe of inelastic WIMP interactions, with a signature of a 39.6 keV de-excitation photon detected simultaneously with the nuclear recoil. Using an exposure of 0.89 tonne-years, we find no evidence of inelastic WIMP scattering with a significance of more than 2$σ$. A profile-likelihood ratio analysis is used to set upper limits on the cross-section of WIMP-nucleus interactions. We exclude new parameter space for WIMPs heavier than 100 GeV/c${}^2$, with the strongest upper limit of $3.3 \times 10^{-39}$ cm${}^2$ for 130 GeV/c${}^2$ WIMPs at 90\% confidence level.

hep-ex↗
arXiv2021

Unveiling the Hybridization Process in a Quantum Critical Ferromagnet by Ultrafast Optical Spectroscopy

We report the ultrafast optical pump-probe spectroscopy measurements on the recently discovered quantum critical ferromagnet CeRh$_6$Ge$_4$. Our experimental results reveal the two-stage development of the hybridization between localized $f$ moments and conduction electrons with lowering temperature, as evidenced by (1) the presence of hybridization fluctuation for temperatures from $\sim$85 K ($T^*$) to $\sim$140 K ($T^\dagger$), and (2) the emergence of collective hybridization below the coherence temperature, $T^*$, marked by the opening of an indirect gap of 2$Δ$ $\approx$12 meV. We also observe three coherent phonon modes being softened anomalously below $T^*$, reflecting directly their coupling with the emergent coherent heavy electrons. Our findings establish the universal nature of the hybridization process in different heavy fermion systems.

cond-mat.str-el↗
arXiv2020

Hybridization dynamics in CeCoIn5 revealed by ultrafast optical spectroscopy

We investigate the quasiparticle dynamics in the prototype heavy fermion CeCoIn$_5$ using ultrafast optical pump-probe spectroscopy. Our results indicate that this material system undergoes hybridization fluctuations before full establishment of the heavy electron coherence, as the temperature decreases from $\sim$120 K ($T^\dagger$) to $\sim$55 K ($T^*$ ). We reveal that the observed anomalous phonon softening and damping reduction below $T^*$ are directly associated with opening of an indirect hybridization gap. We also discover a distinct collective mode with an energy of $\sim$8 meV, which may be the experimental evidence of the predicted unconventional density wave. Our observations provide critical informations for understanding the hybridization dynamics in heavy fermion materials.

cond-mat.str-el↗
arXiv2020

LBECA: A Low Background Electron Counting Apparatus for Sub-GeV Dark Matter Detection

Two-phase noble liquid detectors, with large target masses and effective background reduction, are currently leading the dark matter direct detection for WIMP masses above a few GeV. Due to their sensitivity to single ionized electron signals, these detectors were shown to also have strong constraints for sub-GeV dark matter via their scattering on electrons. In fact, the most stringent direct detection constraints for sub-GeV dark matter down to as low as ~5 MeV come from noble liquid detectors, namely XENON10, DarkSide-50, XENON100 and XENON1T, although these experiments still suffer from high background at single or a few electron level. LBECA is a planned 100-kg scale liquid xenon detector with significant reduction of the single and a few electron background. The experiment will improve the sensitivity to sub-GeV dark matter by three orders of magnitude compared to the current best constraints.

physics.ins-det↗
arXiv2019

Chiral terahertz wave emission from the Weyl semimetal TaAs

As a fascinating topological phase of matter, Weyl semimetals host chiral fermions with distinct chiralities and spin textures. Optical excitations involving those chiral fermions can induce exotic carrier responses, and in turn lead to novel optical phenomena. Here, we discover strong coherent chiral terahertz emission from the Weyl semimetal TaAs and demonstrate unprecedented manipulation over its polarization on a femtosecond timescale. Such polarization control is achieved via the colossal ultrafast photocurrents in TaAs arising from the circular or linear photogalvanic effect. We unravel that the chiral ultrafast photocurrents are attributed to the large band velocity changes when the Weyl fermions are excited from the Weyl bands to the high-lying bands. The photocurrent generation is maximized at near-IR frequency range close to 1.5 eV. Our findings provide an entirely new design concept for creating chiral photon sources using quantum materials and open up new opportunities for developing ultrafast opto-electronics using Weyl physics.

cond-mat.mtrl-sci↗
arXiv2019

Measurement of Two Low-Temperature Energy Gaps in the Electronic Structure of Antiferromagnetic USb2 Using Ultrafast Optical Spectroscopy

Ultrafast optical spectroscopy is used to study the antiferromagnetic f-electron system USb2. We observe the opening of two charge gaps at low temperatures (<45 K), arising from renormalization of the electronic structure. Analysis of our data indicates that one gap is due to hybridization between localized f-electron and conduction electron bands, while band renormalization involving magnons leads to the emergence of the second gap. These experiments thus enable us to shed light on the complex electronic structure emerging at the Fermi surface in f-electron systems.

cond-mat.str-el↗
arXiv2018

Broadband terahertz generation via the interface inverse Rashba-Edelstein effect

Novel mechanisms for electromagnetic wave emission in the terahertz (THz) frequency regime emerging at the nanometer scale have recently attracted intense attention for the purpose of searching next-generation broadband THz emitters. Here, we report a new mechanism for broadband THz emission, utilizing the interface inverse Rashba-Edelstein effect. By engineering the symmetry of the Ag/Bi Rashba interface, we demonstrate a controllable THz radiation (~0.1-5 THz) waveform emitted from metallic Fe/Ag/Bi heterostructures following photo-excitation. We further reveal that this type of THz radiation can be selectively superimposed on the emission discovered recently due to the inverse Spin Hall effect, yielding a unique film thickness dependent emission pattern. Our results thus offer new opportunities for versatile broadband THz radiation using the interface quantum effects.

cond-mat.mtrl-sci↗
arXiv2017

Bosonic excitations and electron pairing in an electron-doped cuprate superconductor

Superconductivity originates from the coupling between charge carriers and bosonic excitations of either phononic or electronic origin. Identifying the most relevant pairing glue is a key step towards a clear understanding of the unconventional superconductivity. Here, by applying the ultrafast optical spectroscopy on the electron-doped cuprates La$_{1.9}$Ce$_{0.1}$CuO$_{4\pmδ}$, we discern a bosonic mode of electronic origin that has the strongest coupling with the charge carriers near $T_c$. We argue that this mode is associated with the two-dimensional antiferromagnetic spin fluctuations, and can fully account for the superconducting pairing. Our work may help to establish a quantitative relation between bosonic excitations and superconducting pairing in electron-doped cuprates, and pave the way for systematic exploration of superconductivity and other collective phenomena in all correlated materials.

cond-mat.str-el↗
arXiv2017

Nested Dissection Solver for Transport in 3D Nano-Electronic Devices

The Hierarchical Schur Complement method (HSC), and the HSC-extension, have significantly accelerated the evaluation of the retarded Green's function, particularly the lesser Green's function, for two-dimensional nanoscale devices. In this work, the HSC-extension is applied to determine the solution of non-equilibrium Green's functions (NEGF) on three-dimensional nanoscale devices. The operation count for the HSC-extension is analyzed for a cuboid device. When a cubic device is discretized with $N \times N \times N$ grid points, the state-of-the-art Recursive Green Function (RGF) algorithm takes $\mathcal{O}(N^7)$ operations, whereas the HSC-extension only requires $\mathcal{O}(N^6)$ operations. %Realistic operation counts also depend on the system dimensions in $xyz$-directions and the form of contact self-energy matrix. Operation counts and runtimes are also studied for three-dimensional nanoscale devices of practical interest: a graphene-boron\- nitride-graphene multilayer system, a silicon nanowire, and a DNA molecule. The numerical experiments indicate that the cost for the HSC-extension is proportional to the solution of one linear system (or one LU-factorization) and that the runtime speed-ups over RGF exceed three orders of magnitude when simulating realistic devices, such as a graphene-boron nitride-graphene multilayer system with 40,000 atoms.

physics.comp-ph↗
arXiv2016

Probing and controlling terahertz-driven structural dynamics with surface sensitivity

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of how they couple to other degrees of freedom in the material (e.g., ferroelectricity, conductivity and magnetism) while enabling coherent control of lattice vibrations and the symmetry changes associated with them. However, an ultrafast method for observing the resulting structural changes at the atomic scale is essential for studying phonon dynamics. A simple approach for doing this is optical second harmonic generation (SHG), a technique with remarkable sensitivity to crystalline symmetry in the bulk of a material as well as at surfaces and interfaces. This makes SHG an ideal method for probing phonon dynamics in topological insulators (TI), materials with unique surface transport properties. Here, we resonantly excite a polar phonon mode in the canonical TI Bi$_2$Se$_3$ with intense THz pulses and probe the subsequent response with SHG. This enables us to separate the photoinduced lattice dynamics at the surface from transient inversion symmetry breaking in the bulk. Furthermore, we coherently control the phonon oscillations by varying the time delay between a pair of driving THz pulses. Our work thus demonstrates a versatile, table-top tool for probing and controlling ultrafast phonon dynamics in materials, particularly at surfaces and interfaces, such as that between a TI and a magnetic material, where exotic new states of matter are predicted to exist.

cond-mat.str-el↗
arXiv2016

Unraveling photoinduced spin dynamics in topological insulator Bi2Se3

We report on time-resolved ultrafast optical spectroscopy study of the topological insulator (TI) Bi$_2$Se$_3$. We unravel that a net spin polarization can not only be generated using circularly polarized light via interband transitions between topological surface states (SSs), but also via transitions between SSs and bulk states. Our experiment demonstrates that tuning photon energy or temperature can essentially allow for photoexcitation of spin-polarized electrons to unoccupied topological SSs with two distinct spin relaxation times ($\sim$25 fs and $\sim$300 fs), depending on the coupling between SSs and bulk states. The intrinsic mechanism leading to such distinctive spin dynamics is the scattering in SSs and bulk states which is dominated by $E_g^2$ and $A_{1g}^1$ phonon modes, respectively. These findings are suggestive of novel ways to manipulate the photoinduced coherent spins in TIs.

cond-mat.mtrl-sci↗