arXiv subjects

J. Rosen

Publications and source records attributed to J. Rosen.

6 recordsLinked to original sources

arXiv2022

Correlation strength, orbital-selective incoherence, and local moments formation in the magnetic MAX-phase Mn$_2$GaC

We perform a theoretical study of the electronic structure and magnetic properties of the prototypical magnetic MAX-phase Mn$_2$GaC with the main focus given to the origin of magnetic interactions in this system. Using the density functional theory+dynamical mean-field theory (DFT+DMFT) method we explore the effects of electron-electron interactions and magnetic correlations on the electronic properties, magnetic state, and spectral weight coherence of paramagnetic and magnetically-ordered phases of Mn$_2$GaC. We also benchmark the DFT-based disordered local moment approach for this system by comparing the obtained electronic and magnetic properties with that of the DFT+DMFT method. Our results reveal a complex magnetic behavior characterized by a near degeneracy of the ferro- and antiferromagnetic configurations of Mn$_2$GaC, implying a high sensitivity of its magnetic state to fine details of the crystal structure and unit-cell volume, consistent with experimental observations. We observe robust local-moment behavior and orbital-selective incoherence of the spectral properties of Mn$_2$GaC, implying the importance of orbital-dependent localization of the Mn $3d$ states. We find that Mn$_2$GaC can be described in terms of local magnetic moments, which may be modeled by DFT with disordered local moments. However, the magnetic properties are dictated by the proximity to the regime of formation of local magnetic moments, in which the localization is in fact driven by the Hund's exchange interaction, and not the Coulomb interaction.

cond-mat.str-el↗

arXiv2019

Tin+1Cn MXene with fully saturated and thermally stable Cl terminations

MXenes are a rapidly growing family of 2D materials that exhibit a highly versatile structure and composition, allowing for significant tuning of the material properties. These properties are, however, ultimately limited by the surface terminations, which are typically a mixture of species, including F and O that are inherent to the MXene processing. Other and robust terminations are lacking. Here, we apply high-resolution scanning transmission electron microscopy (STEM), corresponding image simulations and first-principles calculations to investigate the surface terminations on MXenes synthesized from MAX phases through Lewis acidic melts. The results show that atomic Cl terminates the synthesized MXenes, with mere residual presence of other termination species. Furthermore, in situ STEM-electron energy loss spectroscopy (EELS) heating experiments show that the Cl terminations are stable up to 750 °C. Thus, we present an attractive new termination that widely expands the MXenes functionalization space and enable new applications.

cond-mat.mtrl-sci↗

arXiv2019

Optimal Needle Diameter, Shape, and Path in Autonomous Suturing

Needle shape, diameter, and path are critical parameters that directly affect suture depth and tissue trauma in autonomous suturing. This paper presents an optimization-based approach to specify these parameters. Given clinical suturing guidelines, a kinematic model of needle-tissue interaction was developed to quantify suture parameters and constraints. The model was further used to formulate constant curvature needle path planning as a nonlinear optimization problem. The optimization results were confirmed experimentally with the Raven II surgical system. The proposed needle path planning algorithm guarantees minimal tissue trauma and complies with a wide range of suturing requirements.

cs.RO↗

arXiv2007

Large Deviations for Riesz Potentials of Additive Processes

We study functionals of the form \[ζ_{t}=\int_0^{t}...\int_0^{t} | X_1(s_1)+...+ X_p(s_p)|^{-σ}ds_1... ds_p\] where $X_1(t),..., X_p(t)$ are i.i.d. $d$-dimensional symmetric stable processes of index $0<\bb\le 2$. We obtain results about the large deviations and laws of the iterated logarithm for $ζ_{t}$.

math.PR↗

arXiv2007

Precision measurements of the total and partial widths of the psi(2S) charmonium meson with a new complementary-scan technique in antiproton-proton annihilations

We present new precision measurements of the psi(2S) total and partial widths from excitation curves obtained in antiproton-proton annihilations by Fermilab experiment E835 at the Antiproton Accumulator in the year 2000. A new technique of complementary scans was developed to study narrow resonances with stochastically cooled antiproton beams. The technique relies on precise revolution-frequency and orbit-length measurements, while making the analysis of the excitation curve almost independent of machine lattice parameters. We study the psi(2S) meson through the processes pbar p -> e+ e- and pbar p -> J/psi + X -> e+ e- + X. We measure the width to be Gamma = 290 +- 25(sta) +- 4(sys) keV and the combination of partial widths Gamma_e+e- * Gamma_pbarp / Gamma = 579 +- 38(sta) +- 36(sys) meV, which represent the most precise measurements to date.

hep-ex↗

arXiv2006

Universal Mixing of Quantum Walk on Graphs

We study the set of probability distributions visited by a continuous-time quantum walk on graphs. An edge-weighted graph G is universal mixing if the instantaneous or average probability distribution of the quantum walk on G ranges over all probability distributions on the vertices as the weights are varied over non-negative reals. The graph is uniform mixing if it visits the uniform distribution. Our results include the following: (a) All weighted complete multipartite graphs are instantaneous universal mixing. This is in contrast to the fact that no unweighted complete multipartite graphs are uniform mixing (except for the four-cycle). (b) The weighted claw or star graph is a minimally connected instantaneous universal mixing graph. In fact, as a corollary, the unweighted claw is instantaneous uniform mixing. This adds a new family of uniform mixing graphs to a list that so far contains only the hypercubes. (c) Any weighted graph is average almost-uniform mixing unless its spectral type is sublinear in the size of the graph. This provides a nearly tight characterization for average uniform mixing on circulant graphs. (d) No weighted graphs are average universal mixing. This shows that weights do not help to achieve average universal mixing, unlike the instantaneous case. Our proofs exploit the spectra of the underlying weighted graphs and path collapsing arguments.

quant-ph↗