arXiv subjects

J. Samuel Jiang

Publications and source records attributed to J. Samuel Jiang.

8 recordsLinked to original sources

arXiv2026

Gate-tunable electronic properties of epitaxial Bi (111) films using a printable hexagonal boron nitride ionogel

Achieving effective electrostatic control of carrier transport in semimetals remains challenging due to strong screening and multiband effects. We report efficient low voltage top gated control of electronic transport in epitaxial Bi (111) thin films grown on GaAs (111) substrates using a printable hexagonal boron nitride ionogel. Magnetotransport measurements reveal pronounced nonlinear Hall conductivities arising from multiband electron and hole contributions. Remarkably, the application of a small gate voltage (less than 0.4 V in magnitude) leads to a systematic evolution of the low field Hall conductivity slope and the electron-hole compensation point. The response to gate voltage depends upon thickness and temperature. The observed behavior cannot be explained by a conventional Fermi level shift with rigid bands and instead indicates a non rigid band response associated with multiband effects and a gat tunable Rashba spin orbit coupling. Our results establish printable ionogel gating as a powerful approach to tune multiband transport in topological semimetals.

cond-mat.mtrl-sci↗

arXiv2024

Tunable Anomalous Hall Effect in a Kagome Ferromagnetic Weyl Semimetal

Emerging from the intricate interplay of topology and magnetism, the giant anomalous Hall effect (AHE) is the most known topological property of the recently discovered kagome ferromagnetic Weyl semimetal Co_3Sn_2S_2 with the magnetic Co atoms arranged on a kagome lattice. Here we report that the AHE in Co_3Sn_2S_2 can be fine-tuned by an applied magnetic field orientated within ~2 degrees of the kagome plane, while beyond this regime, it stays unchanged. Particularly, it can vanish in magnetic fields parallel to the kagome plane and even decrease in magnetic fields collinear with the spin direction. This tunable AHE can be attributed to local spin switching enabled by the geometrical frustration of the magnetic kagome lattice, revealing that spins in a kagome ferromagnet change their switching behavior as the magnetic field approaches the kagome plane. Our results also suggest a versatile way to tune the properties of a kagome magnet.

cond-mat.mtrl-sci↗

arXiv2023

Field Orientation Dependent Magnetic Phases In Weyl Semimetal Co3Sn2S2

Magnetism plays a key role in the emergence of topological phenomena in the Weyl semimetal Co3Sn2S2, which exhibits a ferromagnetic (FM) interactions along the c-axis of the crystal and an antiferromagnetic (AFM) interactions within the ab plane. Extensive studies on the temperature dependence of the magnetism with the magnetic field along the c-axis have uncovered a number of magnetic phases. Currently, the nature and origins of the reported magnetic phases are under debate. Here we report on magnetic field orientation effects on the magnetism in Co3Sn2S2. The shape of the hysteresis loop of the Hall resistance at a fixed temperature is found to change from rectangular to bow-tie-like as the magnetic field is tilted from the c-axis towards the ab plane, resembling that reported for magnetic fields along the c-axis as the temperature approaches the Curie temperature from below. Unlike their temperature-dependent counterparts, the newly observed bow-tie-like hysteresis loops show exchange bias. Our results showcase the contribution of the in-plane AFM interactions to the magnetism in Co3Sn2S2 and demonstrate a new way to tune its magnetic phases. They also shed light on the temperature-dependent magnetic phases occurring in the magnetic field along the c-axis of the crystal.

cond-mat.mtrl-sci↗

arXiv2020

Voltage control of magnon spin currents in antiferromagnetic Cr2O3

Voltage-controlled spintronic devices utilizing the spin degree of freedom are desirable for future applications, and may allow energy-efficient information processing. Pure spin current can be created by thermal excitations in magnetic systems via the spin Seebeck effect (SSE). However, controlling such spin currents, only by electrical means, has been a fundamental challenge. Here, we investigate voltage control of the SSE in the antiferromagnetic insulator Cr2O3. We demonstrate that the SSE response generated in this material can be effectively controlled by applying a bias voltage, owing to the sensitivity of the SSE to the orientation of the magnetic sublattices as well as the existence of magnetoelectric couplings in Cr2O3. Our experimental results are explained using a model based on the magnetoelectric effect in Cr2O3.

cond-mat.mtrl-sci↗

arXiv2020

Discovery of two-dimensional anisotropic superconductivity at KTaO$_3$ (111) interfaces

The unique electronic structure found at interfaces between materials can allow unconventional quantum states to emerge. Here we observe superconductivity in electron gases formed at interfaces between (111) oriented KTaO$_3$ and insulating overlayers of either EuO or LaAlO$_3$. The superconducting transition temperature, approaching 2.2 K, is about one order of magnitude higher than that of the LaAlO$_3$/SrTiO$_3$ system. Strikingly, similar electron gases at (001) KTaO$_3$ interfaces remain normal down to 25 mK. The critical field and current-voltage measurements indicate that the superconductivity is two dimensional. Higher mobility EuO/KTaO$_3$ (111) samples show a large in-plane anisotropy in transport properties at low temperatures prior to onset of superconductivity, suggesting the emergence of a stripe like phase where the superconductivity is nearly homogeneous in one direction, but strongly modulated in the other.

cond-mat.supr-con↗

arXiv2018

Probing short-range magnetic order in a geometrically frustrated magnet by spin Seebeck effect

Competing magnetic interactions in geometrically frustrated magnets give rise to new forms of correlated matter, such as spin liquids and spin ices. Characterizing the magnetic structure of these states has been difficult due to the absence of long-range order. Here, we demonstrate that the spin Seebeck effect (SSE) is a sensitive probe of magnetic short-range order (SRO) in geometrically frustrated magnets. In low temperature (2 - 5 K) SSE measurements on a model frustrated magnet \mathrm{Gd_{3}Ga_{5}O_{12}}, we observe modulations in the spin current on top of a smooth background. By comparing to existing neutron diffraction data, we find that these modulations arise from field-induced magnetic ordering that is short-range in nature. The observed SRO is anisotropic with the direction of applied field, which is verified by theoretical calculation.

cond-mat.mtrl-sci↗

arXiv2016

Antiferromagnetic spin Seebeck Effect

We report on the observation of the spin Seebeck effect in antiferromagnetic MnF$_2$. A device scale on-chip heater is deposited on a bilayer of Pt (4 nm)/MnF$_2$ (110) (30 nm) grown by molecular beam epitaxy on a MgF$_2$ (110) substrate. Using Pt as a spin detector layer it is possible to measure thermally generated spin current from MnF$_2$ through the inverse spin Hall effect. The low temperature (2 - 80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (>9 T) are applied parallel the easy axis of the MnF$_2$ thin film. When magnetic field is applied perpendicular to the easy axis, the spin flop transition is absent, as expected.

cond-mat.mtrl-sci↗

arXiv2001

Hysteresis in layered spring magnets

This article addresses a problem of micromagnetics: the reversal of magnetic moments in layered spring magnets. A one-dimensional model is used of a film consisting of several atomic layers of a soft material on top of several atomic layers of a hard material. Each atomic layer is taken to be uniformly magnetized, and spatial inhomogeneities within an atomic layer are neglected. The state of such a system is described by a chain of magnetic spin vectors. Each spin vector behaves like a spinning top driven locally by the effective magnetic field and subject to damping (Landau-Lifshitz-Gilbert equation). A numerical integration scheme for the LLG equation is presented that is unconditionally stable and preserves the magnitude of the magnetization vector at all times. The results of numerical investigations for a bilayer in a rotating in-plane magnetic field show hysteresis with a basic period of $2π$ at moderate fields and hysteresis with a basic period of $π$ at strong fields.

math.DS↗