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J. Schwarzkopf

Publications and source records attributed to J. Schwarzkopf.

2 recordsLinked to original sources

Linear dichroic soft X-ray microscopy of ferroelectric stripe domains in epitaxial K$_\mathbf{0.6}$Na$_\mathbf{0.4}$NbO$_\mathbf{3}$

Functional properties of ferroelectric thin films are governed by domains that can be engineered by epitaxial strain. Soft X-ray microscopy can image domain structures with elemental and electronic sensitivity, but hitherto its application to strain-stabilized domains has been hindered by the absorption of soft X-rays in epitaxial substrates. Here, it is demonstrated how this limitation can be overcome by locally back-thinning the (110) TbScO$_3$ substrate of epitaxial K$_{0.6}$Na$_{0.4}$NbO$_3$ ferroelectric thin films to achieve soft X-ray transparency at the O K-edge around 530 eV. Strain-induced ferroelectric stripe domains with periods down to 44 nm were resolved by scanning transmission X-ray microscopy and coherent diffractive imaging by exploiting the X-ray linear dichroism of hybridized O 2p-Nb 4d states, providing sensitivity to in-plane polarization components under normal incidence. The results establish soft X-ray microscopy for nanoscale imaging of epitaxial ferroelectric domains structures and open perspectives for time-resolved studies thereof.

cond-mat.mtrl-sci

Demonstration of a picosecond Bragg switch for hard x-rays in a synchrotron-based pump-probe experiment

We report a benchmark experiment that demonstrates shortening of hard x-ray pulses in a synchrotron-based optical pump - x-ray probe experiment. The pulse shortening device, a picosecond Bragg switch, reduces the temporal resolution of an incident x-ray pulse to 7.5 ps. We employ the Bragg switch to monitor propagating sound waves in nanometer-thin epitaxial films. With the experimental data we infer pulse duration, diffraction efficiency and switching contrast of the device. A detailed efficiency analysis shows, that the switch can deliver up to 1010 photons/sec in high-repetition rate synchrotron experiments.

cond-mat.mtrl-sci