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J. Sperling

Publications and source records attributed to J. Sperling.

At least 19 recordsLinked to original sources

Quantum optical coherence: From linear to nonlinear interferometers

Interferometers provide a highly sensitive means to investigate and exploit the coherence properties of light in metrology applications. However, interferometers come in various forms and exploit different properties of the optical states within. In this paper, we introduce a classification scheme that characterizes any interferometer based on the number of involved nonlinear elements by studying their influence on single-photon and photon-pair states. Several examples of specific interferometers from these more general classes are discussed, and the theory describing the expected first-order and second-order coherence measurements for single-photon and single-photon-pair input states is summarized and compared. These theoretical predictions are then tested in an innovative experimental setup that is easily able to switch between implementing an interferometer consisting of only one or two nonlinear elements. The resulting singles and coincidence rates are measured in both configurations and the results are seen to fit well with the presented theory. The measured results of coherence are tied back to the presented classification scheme, revealing that our experimental design can be useful in gaining insight into the properties of the various interferometeric setups containing different degrees of nonlinearity.

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Climbing the Fock ladder: Advancing multiphoton state generation

A scheme for the enhanced generation of higher photon-number states is realized, using an optical time-multiplexing setting that exploits a parametric down-conversion source for an iterative state generation. We use a quantum feedback mechanism for already generated photons to induce self-seeding of the consecutive nonlinear process, enabling us to coherently add photons to the light that propagates in the feedback loop. The addition can be carried out for any chosen number of round trips, resulting in a successive buildup of multiphoton states. Our system is only limited by loop losses. The looped design is rendered possible by a carefully engineered waveguide source that is compatible with and preserves the shape of the propagating mode. We compare the fidelities and success probabilities of our protocol with the common direct heralding of photon-number states. This comparison reveals that, for same the fidelity, our feedback-based setup significantly enhances success probabilities, being vital for an efficient utilization in quantum technologies. Moreover, quantum characteristics of the produced states are analyzed, and the flexibility of producing higher photon-number states with our setup beyond the common direct heralding is demonstrated.

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Quantum Correlations beyond Entanglement and Discord

Dissimilar notions of quantum correlations have been established, each being motivated through particular applications in quantum information science and each competing for being recognized as the most relevant measure of quantumness. In this contribution, we experimentally realize a form of quantum correlation that exists even in the absence of entanglement and discord. We certify the presence of such quantum correlations via negativities in the regularized two-mode Glauber-Sudarshan function. Our data show compatibility with an incoherent mixture of orthonormal photon-number states, ruling out quantum coherence and other kinds of quantum resources. By construction, the quantumness of our state is robust against dephasing, thus requiring fewer experimental resources to ensure stability. In addition, we theoretically show how multimode entanglement can be activated based on the generated, nonentangled state. Therefore, we implement a robust kind of nonclassical photon-photon correlated state with useful applications in quantum information processing.

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Quantum photonics with active feedback loops

We develop a unified theoretical framework for the efficient description of multiphoton states generated and propagating in loop-based optical networks which contain nonlinear elements. These active optical components are modeled as nonlinear media, resembling a two-mode squeezer. First, such nonlinear components can be seeded to manipulate quantum states of light, as such enabling photon addition protocols. And, second, they can function as an amplifying medium for quantum light. To prove the practical importance of our approach, the impact of multiple round trips is analyzed for states propagating in experimentally relevant loop configurations of networks, such as time-multiplexed driven quantum walks and iterative photon-number state generation protocols. Our method not only enables us to model such complex systems but also allows us to propose alternative setups that overcome previous limitations. To characterize the systems under study, we provide exact expressions for fidelities with target states, success probabilities of heralding-type measurements, and correlations between optical modes, including many realistic imperfections. Moreover, we provide an easily implementable numerical approach by devising a vector-type representation of photonic states, measurement operators, and passive and active processes.

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Classical evolution in quantum systems

We investigate quantum effects in the evolution of general systems. For studying such temporal quantum phenomena, it is paramount to have a rigorous concept and profound understanding of the classical dynamics in such a system in the first place. For this reason, we derive from first principles equations of motions that describe the classical propagation in quantum systems. A comparison of this classical model with the actual temporal quantum behavior enables us to identify quantum phenomena in the system's dynamics and distinguish them from static quantum features at individual points in time. For instance, we show how Newton's second law emerges as a special case of our general treatment, connecting it to a Schrödinger-type equation. As applications of our universal technique, we analyze nonlinear optical processes, semiclassical models, and the multipartite entanglement dynamics of macroscopic ensembles.

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Quasiprobability distributions for quantum-optical coherence and beyond

We study the quasiprobability representation of quantum light, as introduced by Glauber and Sudarshan, for the unified characterization of quantum phenomena. We begin with reviewing the past and current impact of this technique. Regularization and convolution methods are specifically considered since they are accessible in experiments. We further discuss more general quantum systems for which the concept of negative probabilities can be generalized, being highly relevant for quantum information science. For analyzing quantum superpositions, we apply recently developed approaches to visualize quantum coherence of states via negative quasiprobability representations, including regularized quasiprobabilities for light and more general quantum correlated systems.

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Detector-Agnostic Phase-Space Distributions

The representation of quantum states via phase-space functions constitutes an intuitive technique to characterize light. However, the reconstruction of such distributions is challenging as it demands specific types of detectors and detailed models thereof to account for their particular properties and imperfections. To overcome these obstacles, we derive and implement a measurement scheme that enables a reconstruction of phase-space distributions for arbitrary states whose functionality does not depend on the knowledge of the detectors, thus defining the notion of detector-agnostic phase-space distributions. Our theory presents a generalization of well-known phase-space quasiprobability distributions, such as the Wigner function. We implement our measurement protocol, using state-of-the-art transition-edge sensors without performing a detector characterization. Based on our approach, we reveal the characteristic features of heralded single- and two-photon states in phase space and certify their nonclassicality with high statistical significance.

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Benchmarking of Gaussian boson sampling using two-point correlators

Gaussian boson sampling is a promising scheme for demonstrating a quantum computational advantage using photonic states that are accessible in a laboratory and, thus, offer scalable sources of quantum light. In this contribution, we study two-point photon-number correlation functions to gain insight into the interference of Gaussian states in optical networks. We investigate the characteristic features of statistical signatures which enable us to distinguish classical from quantum interference. In contrast to the typical implementation of boson sampling, we find additional contributions to the correlators under study which stem from the phase dependence of Gaussian states and which are not observable when Fock states interfere. Using the first three moments, we formulate the tools required to experimentally observe signatures of quantum interference of Gaussian states using two outputs only. By considering the current architectural limitations in realistic experiments, we further show that a statistically significant discrimination between quantum and classical interference is possible even in the presence of loss, noise, and a finite photon-number resolution. Therefore, we formulate and apply a theoretical framework to benchmark the quantum features of Gaussian boson sampling under realistic conditions.

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Experimental Reconstruction of Entanglement Quasiprobabilities

We report on the first experimental reconstruction of an entanglement quasiprobability. In contrast to related techniques, the negativities in our distributions are a necessary and sufficient identifier of separability and entanglement and enable a full characterization of the quantum state. A reconstruction algorithm is developed, a polarization Bell state is prepared, and its entanglement is certified based on the reconstructed entanglement quasiprobabilities, with a high significance and without correcting for imperfections.

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Quasistates and quasiprobabilities

The quasiprobability representation of quantum states addresses two main concerns, the identification of nonclassical features and the decomposition of the density operator. While the former aspect is a main focus of current research, the latter decomposition property has been studied less frequently. In this contribution, we introduce a method for the generalized expansion of quantum states in terms of so-called quasistates. In contrast to the quasiprobability decomposition through nonclassical distributions and pure-state operators, our technique results in classical probabilities and nonpositive semidefinite operators, defining the notion of quasistates, that carry the information about the nonclassical characteristics of the system. Therefore, our method presents a complementary approach to prominent quasiprobability representations. We explore the usefulness of our technique with several examples, including applications for quantum state reconstruction and the representation of nonclassical light. In addition, using our framework, we also demonstrate that inseparable quantum correlations can be described in terms of classical joint probabilities and tensor-product quasistates for an unambiguous identification of quantum entanglement.

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Quasiprobability representation of quantum coherence

We introduce a general method for the construction of quasiprobability representations for arbitrary notions of quantum coherence. Our technique yields a nonnegative probability distribution for the decomposition of any classical state. Conversely, quantum phenomena are certified in terms of signed distributions, i.e., quasiprobabilities, and a residual component unaccessible via classical states. Our unifying method combines well-established concepts, such as phase-space distributions in quantum optics, with resources of quantumness relevant for quantum technologies. We apply our approach to analyze various forms of quantum coherence in different physical systems. Moreover, our framework renders it possible to uncover complex quantum correlations between systems, for example, via quasiprobability representations of multipartite entanglement.

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Continuity of measurement outcomes

It is demonstrated that the collapse of the wave function is equivalent to the continuity of measurement outcomes. The latter states that a second measurement has to result in the same outcome as the first measurement of the same observable for a vanishing time between both observations. In contrast to the exclusively quantum-physical collapse description, the equivalent continuity requirement also applies in classical physics, allowing for a comparison of both domains. In particular, it is found that quantum coherences are the single cause for measurable deviations in statistical properties due to the collapse. Therefore, the introduced approach renders it possible to characterize and quantify the unique features of the quantum-physical measurement problem within the framework of modern quantum resource theories and compare them to classical physics.

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Geometrical picture of photocounting measurements

We revisit the representation of generalized quantum observables by establishing a geometric picture in terms of their positive operator-valued measures (POVMs). This leads to a clear geometric interpretation of Born's rule by introducing the concept of contravariant operator-valued measures. Our approach is applied to the theory of array detectors, which is a challenging task as the finite dimensionality of the POVM substantially restricts the available information about quantum states. Our geometric technique allows for a direct estimation of expectation values of different observables, which are typically not accessible with such detection schemes. In addition, we also demonstrate the applicability of our method to quantum-state reconstruction with unbalanced homodyne detection.

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Incomplete Detection of Nonclassical Phase-Space Distributions

We implement the direct sampling of negative phase-space functions via unbalanced homodyne measurement using click-counting detectors. The negativities significantly certify nonclassical light in the high-loss regime using a small number of detectors which cannot resolve individual photons. We apply our method to heralded single-photon states and experimentally demonstrate the most significant certification of nonclassicality for only two detection bins. By contrast, the frequently applied Wigner function fails to indicate such quantum characteristics for the quantum efficiencies present in our setup. In addition, it would require ideal photon-number resolution. Hence, we realize a robust, reliable, and resource-efficient approach to characterize nonclassical light in phase space under realistic conditions.

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Separable and Inseparable Quantum Trajectories

The dynamical behavior of interacting systems plays a fundamental role for determining quantum correlations, such as entanglement. In this Letter, we describe temporal quantum effects of the inseparable evolution of composite quantum states by comparing the trajectories to their classically correlated counterparts. For this reason, we introduce equations of motions describing the separable propagation of any interacting quantum system, which are derived by requiring separability for all times. The resulting Schroedinger-type equations allow for comparing the trajectories in a separable configuration with the actual behavior of the system and, thereby, identifying inseparable and time-dependent quantum properties. As an example, we study bipartite discrete- and continuous-variable interacting systems. The generalization of our developed technique to multipartite scenarios is also provided.

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Conditional Hybrid Nonclassicality

We derive and implement a general method to characterize the nonclassicality in compound discrete- and continuous-variable systems. For this purpose, we introduce the operational notion of conditional hybrid nonclassicality which relates to the ability to produce a nonclassical continuous-variable state by projecting onto a general superposition of discrete-variable subsystem. We discuss the importance of this form of quantumness in connection with interfaces for quantum communication. To verify the conditional hybrid nonclassicality, a matrix version of a nonclassicality quasiprobability is derived and its sampling approach is formulated. We experimentally generate an entangled, hybrid Schrödinger cat state, using a coherent photon-addition process acting on two temporal modes, and we directly sample its nonclassicality quasiprobability matrix. The introduced conditional quantum effects are certified with high statistical significance.

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Displaced photon-number entanglement tests

Based on correlations of coherently displaced photon-numbers, we derive entanglement criteria for the purpose to verify non-Gaussian entanglement. Our construction method enables us to verify bipartite and multipartite entanglement of complex states of light. An important advantage of our technique is that the certified entanglement even persists in the presence of arbitrarily high, constant losses. We exploit experimental correlation schemes for the two-mode and multimode scenarios, which allow us to directly measure the desired observables. To detect entanglement of a given state, a genetic algorithm is applied to optimize over the infinite set of our constructed witnesses. In particular, we provide suitable witnesses for several distinct two-mode states. Moreover, a mixed non-Gaussian four-mode state is shown to be entangled in all possible non-trivial partitions.

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Identification of nonclassical properties of light with multiplexing layouts

In a recent contribution, we introduced and applied a detector-independent method to uncover nonclassicality. Here, we extend those techniques and give more details on the performed analysis. We derive a general theory of the positive-operator-valued measure that describes multiplexing layouts with arbitrary detectors. From the resulting quantum version of a multinomial statistics, we infer nonclassicality probes based on a matrix of normally ordered moments. We discuss these criteria and apply the theory to our data which are measured with superconducting transition-edge sensors. Our experiment produces heralded multi-photon states from a parametric down-conversion light source. We show that the known notions of sub-Poisson and sub-binomial light can be deduced from our general approach, and we establish the concept of sub-multinomial light, which is shown to outperform the former two concepts of nonclassicality for our data.

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