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J. Suhonen

Publications and source records attributed to J. Suhonen.

At least 19 recordsLinked to original sources

Electron spectral shape of the third-forbidden $\beta$-decay of $^{87}$Rb measured using a Rb$_2$ZrCl$_6$ crystal scintillator

In recent years, interest in experimental studies of $\beta$-decay electron spectra -- often referred to as $\beta$ spectra -- has been growing. This is particularly true for $\beta$ transitions where the electron spectra are sensitive to the effective value of the weak axial coupling, $g_{\rm A}$. Such measurements serve as important benchmarks for nuclear physics calculations and can also be used to characterize background in astroparticle physics experiments. In this work, a dedicated experiment has been carried out to investigate the spectral shape of the third-forbidden $^{87}$Rb $\beta$-decays, with the goal of estimating the effective $g_{\rm A}$ value for this transition and of deriving the T$_{1/2}$ value. This was done by comparing the experimental spectral shape with the estimates from various phenomenological models. The $^{87}$Rb source was embedded directly within the detector material of a new Rb$_2$ZrCl$_6$ crystal scintillator; the data taking was performed deep underground at Gran Sasso National Laboratory. The obtained experimental half-life value for the studied process is T$_{1/2} = 5.08(13) \times$ 10$^{10}$ yr; while a $g_{\rm A}$ value in the range 0.4 to 0.6 is obtained when accounting for uncertainties and depending on the model adopted as discussed in detail in the text.

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Determination of the Muon Lifetime in $^{76}$Se with the MONUMENT experiment

Ordinary muon capture provides a benchmark for the nuclear physics models of neutrinoless double beta decay under comparable momentum transfer conditions. The total capture strength defines the lifetime of the muonic atom. The muon lifetime in $^{76}$Se, the daughter nucleus of $^{76}$Ge, was determined with improved accuracy by the MONUMENT collaboration, using an array of high-purity germanium detectors and a set of scintillator counters at the $\pi$E1 muon beam line of the Paul Scherrer Institute. The new value of (135.1 $\pm$ 0.5) ns agrees with phenomenological calculations based on the quasiparticle random phase approximation with unquenched axial-vector coupling.

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Fabrication of thin planar radiopure foils with 82Se for the SuperNEMO Demonstrator

The SuperNEMO Demonstrator, designed to search for double beta decay using enriched 82Se, has been assembled in the Modane Underground Laboratory under the French Alps. Thin foils with radio - purified and enriched 82Se are installed centrally in the detector. A novel foil fabrication method has been developed, improving the radiopurity achieved in the previous generation experiment. It consists of wrapping standalone selenium pads in raw Mylar, combined with selenium purified by a new reverse-chromatography method. This paper describes the features of these foils, their fabrication process, the characterization results, and the integration of the foils into the SuperNEMO Demonstrator.

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The measurement of the $^{99}$Tc $\beta$-decay spectrum and its implications for the effective value of weak axial coupling

Measurements of $\beta$-spectral shapes is an important way to examine the effective value of the weak axial coupling $g_{\rm A}$. These stu\ dies focus specifically on forbidden non-unique $\beta^-$ transitions, as only in these cases is the spectral shape directly sensitive to th\ e ratio $g_{\rm A}/g_{\rm V}$. Here, the value of the weak vector coupling constant, $g_{\rm V}$, is fixed at 1.0 according to the Conserve\ d Vector Current (CVC) hypothesis. In previous studies for the fourth-forbidden non-unique $\beta^-$ decays of $^{113}$Cd [J.~Kostensalo \textit{et al.}, Phys. Lett. B 822, 136652 (2021)] and $^{115}$In [A.~F. Leder \textit{et al.}, Phys. Rev. Lett. 129, 232502 \ (2022) and L. Pagnanini \textit{et al.}, Phys. Rev. Lett. 133, 122501 (2024)] a quenched value was determined for the ratio $g_{\rm A}/g_{\rm V}$ using $g_{\rm V}=1.0$. A notable exception is the recent measurement and analysis of the second-forbidden non-unique $\ \beta$-decay transition in $^{99}$Tc, performed by M. Paulsen \textit{et al.}, Phys. Rev. C 110, 05503(2024). Where an enhanced ratio $g_{\\ rm A}/g_{\rm V}=1.526(92)$ was suggested. To resolve this apparently contradictory situation with the effective value of $g_{\rm A}$, we hav\ e performed calculations based on the nuclear shell model (NSM) Hamiltonians glekpn, jj45pnb, and the MQPM approach with a careful considera\ tion of the small relativistic vector nuclear matrix element (sNME). The theoretical spectra were compared to the $^{99}$Tc $\beta$-decay sp\ ectrum by using the 4$\pi$ gold absorber with a Metallic Magnetic Calorimeter (MMC). In all cases, we found that the data matches well with \ reduced $g_{\rm A}$/$g_{\rm V}$ values of 1.0--1.2. Our result contradicts the previously reported measurement for $^{99}$Tc and instead sup\ ports a quenched axial coupling as reported for other isotopes.

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The Impact of Helium Exposure on the PMTs of the SuperNEMO Experiment

The performance of Hamamatsu 8" photomultiplier tubes (PMTs) of the type used in the SuperNEMO neutrinoless double-beta decay experiment (R5912-MOD), is investigated as a function of exposure to helium (He) gas. Two PMTs were monitored for over a year, one exposed to varying concentrations of He, and the other kept in standard atmospheric conditions as a control. Both PMTs were exposed to light signals generated by a Bi-207 radioactive source that provided consistent large input PMT signals similar to those that are typical of the SuperNEMO experiment. The energy resolution of PMT signals corresponding to 1 MeV energy scale determined from the Bi-207 decay spectrum, shows a negligible degradation with He exposure; however the rate of after-pulsing shows a clear increase with He exposure, which is modelled and compared to diffusion theory. A method for reconstructing the partial pressure of He within the PMT and a method for determining the He breakdown point, are introduced. The implications for long-term SuperNEMO operations are briefly discussed.

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Calorimeter commissioning of the SuperNEMO Demonstrator

The SuperNEMO experiment is searching for neutrinoless double beta decay of \textsuperscript{82}Se, with the unique combination of a tracking detector and a segmented calorimeter. This feature allows to detect the two electrons emitted in the decay and measure their individual energy and angular distribution. The SuperNEMO calorimeter consists of 712 plastic scintillator blocks readout by large PMTs. After the construction of the demonstrator calorimeter underground, we have performed its first commissioning using $\gamma$-particles from calibration sources or from the ambient radioactive background. This article presents the quality assurance tests of the SuperNEMO demonstrator calorimeter and its first time and energy calibrations, with the associated methods.

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Precise $^{113}$Cd $\beta$ decay spectral shape measurement and interpretation in terms of possible $g_A$ quenching

Highly forbidden $\beta$ decays provide a sensitive test to nuclear models in a regime in which the decay goes through high spin-multipole states, similar to the neutrinoless double-$\beta$ decay process. There are only 3 nuclei ($^{50}$V, $^{113}$Cd, $^{115}$In) which undergo a $4^{\rm th}$ forbidden non-unique $\beta$ decay. In this work, we compare the experimental $^{113}$Cd spectrum to theoretical spectral shapes in the framework of the spectrum-shape method. We measured with high precision, with the lowest energy threshold and the best energy resolution ever, the $\beta$ spectrum of $^{113}$Cd embedded in a 0.43 kg CdWO$_4$ crystal, operated over 26 days as a bolometer at low temperature in the Canfranc underground laboratory (Spain). We performed a Bayesian fit of the experimental data to three nuclear models (IBFM-2, MQPM and NSM) allowing the reconstruction of the spectral shape as well as the half-life. The fit has two free parameters, one of which is the effective weak axial-vector coupling constant, $g_A^{\text{eff}}$, which resulted in $g_A^{\text{eff}}$ between 1.0 and 1.2, compatible with a possible quenching. Based on the fit, we measured the half-life of the $^{113}$Cd $\beta$ decay including systematic uncertainties as $7.73^{+0.60}_{-0.57} \times 10^{15}$ yr, in agreement with the previous experiments. These results represent a significant step towards a better understanding of low-energy nuclear processes.

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Ultra-low $Q_\beta$ value for the allowed decay of $^{110}$Ag$^m$ confirmed via mass measurements

The mass of the electron-antineutrino can be determined in dedicated measurements of the $\beta$ spectral shape near the $\beta$ endpoint of a $\beta^-$ transition, with a low $Q$ value enhancing the sensitivity of the measurement. One such low-$Q$-value candidate is the transition between the $6^+$ isomer of $^{110}$Ag and the $5^+_2$ state in $^{110}$Cd ($Q^{\ast}_{\beta,m}=-0.12(131)$ keV). To reduce the uncertainty of the $Q$ value, we have used the phase-imaging ion-cyclotron-resonance technique with the JYFLTRAP double Penning trap and performed a high-precision atomic-mass measurement of $^{109}$Ag with $^{110}$Cd as a reference. Combined with the known spectroscopic data, we obtain a re-evaluated value $Q^{\ast}_{\beta,m}=405(135)$ eV, for the $^{110}\text{Ag}(6^+_\text{m}) \rightarrow {^{110}\text{Cd}}(5^+_2)$ transition. This represents the lowest $Q_{\beta}$ value for any allowed transition observed to date. In order to estimate the partial half-life ($t_{1/2}$) and branching ratio (Br) of the transition, nuclear shell-model calculations were performed using the $jj45pnb$ Hamiltonian in combination with state-of-the-art atomic calculations. The computed values $t_{1/2} = 2.23^{+5.24}_{-1.28} \times 10^7$ years and $\textrm{Br} = 3.07^{+4.16}_{-2.15} \times 10^{-8}$, along with the thermal-neutron capture on stable $^{109}$Ag as a viable production method, make $^{110}\textrm{Ag}^m$ a promising candidate for future antineutrino-mass measurements.

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Direct high-precision measurement of the mass difference of $^{77}$As-$^{77}$Se related to neutrino mass determination

The first direct determination of the ground-state-to-ground-state ${β^{-}}$-decay $Q$-value of $^{77}$As to $^{77}$Se was performed by measuring their atomic mass difference utilizing the double Penning trap mass spectrometer, JYFLTRAP. The resulting $Q$-value is 684.463(70) keV, representing a remarkable 24-fold improvement in precision compared to the value reported in the most recent Atomic Mass Evaluation (AME2020). With the significant reduction of the uncertainty of the ground-state-to-ground-state $Q$-value and knowledge of the excitation energies in $^{77}$Se from $γ$-ray spectroscopy, the ground-state-to-excited-state $Q$-value of the transition $^{77}$As (3/2$^{-}$, ground state) $\rightarrow$ $^{77}$Se$^{*}$ (5/2$^{+}$, 680.1035(17) keV) was refined to be 4.360(70) keV. We confirm that this potential low $Q$-value ${β^{-}}$-decay transition for neutrino mass determination is energetically allowed at a confidence level of about 60$σ$. Nuclear shell-model calculations with two well-established effective Hamiltonians were used to estimate the partial half-life for the low $Q$-value transition. The half-life was found to be of the order of 10$^{9}$ years for this first-forbidden non-unique transition, which rules out this candidate a potential source for rare-event experiments searching for the electron antineutrino mass.

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Isomeric states of fission fragments explored via Penning trap mass spectrometry at IGISOL

The masses of $^{84}$Br, $^{105}$Mo, $^{115,119,121}$Pd, $^{122}$Ag, $^{127,129}$In, $^{132}$Sb and their respective isomeric states have been measured with the JYFLTRAP Penning trap mass spectrometer using the phase-imaging ion-cyclotron-resonance technique. The excitation energies of the isomeric states in $^{132}$Sb and $^{119}$Pd were experimentally determined for the first time, while for $^{84}$Br, $^{115}$Pd and $^{127,129}$In, the precision of the mass values was substantially improved. In $^{105}$Mo and $^{121}$Pd there were no signs of a long-lived isomeric state. The ground-state measurements of $^{119}$Pd and $^{122}$Ag indicated that both are significantly more bound than the literature values. For $^{122}$Ag, there was no indication of a proposed third long-lived state. The results for the $N=49$ nucleus $^{84}$Br and isomers close to doubly magic $^{132}$Sn have been compared to the shell-model and the microscopic quasiparticle-phonon model calculations.

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Simultaneous Measurement of Half-Life and Spectral Shape of $^{115}$In $\beta$-decay with an Indium Iodide Cryogenic Calorimeter

Current bounds on neutrino Majorana mass are affected by significant uncertainties in the nuclear calculations for neutrinoless double-beta decay. A key issue for a data-driven improvement of the nuclear theory is the actual value of the axial coupling constant $g_A$, which can be investigated through forbidden $\beta$-decays. We present the first measurement of 4$^{th}$-forbidden $\beta$-decay of $^{115}$In with a cryogenic calorimeter based on Indium Iodide. Exploiting the enhanced spectral shape method for the first time to this isotope, our study accurately determines simultaneously spectral shape, $g_A$, and half-life. The Interacting Shell Model, which best fits our data, indicates a half-life for this decay at $T_{1/2}=(5.26\pm0.06) \times 10^{14}$,yr.

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High-precision measurements of low-lying isomeric states in $^{120-124}$In with JYFLTRAP double Penning trap

Neutron-rich $^{120-124}$In isotopes have been studied utilizing the double Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. Using the phase-imaging ion-cyclotron-resonance technique, the isomeric states were resolved from ground states and their excitation energies measured with high precision in $^{121,123,124}$In. In $^{120,122}$In, the $1^+$ states were separated and their masses were measured while the energy difference between the unresolved $5^+$ and $8^-$ states, whose presence was confirmed by post-trap decay spectroscopy was determined to be $\leq15$ keV. In addition, the half-life of $^{122}$Cd, $T_{1/2} = 5.98(10)$ s, was extracted. Experimental results were compared with energy density functionals, density functional theory and shell-model calculations.

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Measurement of double-$β$ decay of $^{150}$Nd to the 0$^+_1$ excited state of $^{150}$Sm in NEMO-3

The NEMO-3 results for the double-$β$ decay of $^{150}$Nd to the 0$^+_1$ and 2$^+_1$ excited states of $^{150}$Sm are reported. The data recorded during 5.25 yr with 36.6 g of the isotope $^{150}$Nd are used in the analysis. For the first time, the signal of the $2νββ$ transition to the 0$^+_1$ excited state is detected with a statistical significance exceeding 5$σ$. The half-life is measured to be $T_{1/2}^{2νββ}(0^+_1) = \left[ 1.11 ^{+0.19}_{-0.14} \,\left(\mbox{stat}\right) ^{+0.17}_{-0.15}\, \left(\mbox{syst}\right) \right] \times10^{20}\,\mbox{yr}$. The limits are set on the $2νββ$ decay to the 2$^+_1$ level and on the $0νββ$ decay to the 0$^+_1$ and 2$^+_1$ levels of $^{150}$Sm.

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Rare $^{40}$K decay with implications for fundamental physics and geochronology

Potassium-40 is a widespread, naturally occurring isotope whose radioactivity impacts subatomic rare-event searches, nuclear structure theory, and estimated geological ages. A predicted electron-capture decay directly to the ground state of argon-40 has never been observed. The KDK (potassium decay) collaboration reports strong evidence of this rare decay mode. A blinded analysis reveals a non-zero ratio of intensities of ground-state electron-captures ($I_{\text{EC}^0}$) over excited-state ones ($I_\text{EC*}$) of $ I_{\text{EC}^0} / I_\text{EC*} = 0.0095 \stackrel{\text{stat}}{\pm} 0.0022 \stackrel{\text{sys}}{\pm} 0.0010 $ (68% C.L.), with the null hypothesis rejected at 4$σ$. In terms of branching ratio, this signal yields $I_{\text{EC}^0} = 0.098\% \stackrel{\text{stat}}{\pm} 0.023\% \stackrel{\text{sys}}{\pm} 0.010\% $, roughly half of the commonly used prediction, with consequences for various fields [L. Hariasz et al., companion paper, DOI: 10.1103/PhysRevC.108.014327].

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Evidence for ground-state electron capture of $^{40}$K

Potassium-40 is a widespread isotope whose radioactivity impacts estimated geological ages spanning billions of years, nuclear structure theory, and subatomic rare-event searches - including those for dark matter and neutrinoless double-beta decay. The decays of this long-lived isotope must be precisely known for its use as a geochronometer, and to account for its presence in low-background experiments. There are several known decay modes for $^{40}$K, but a predicted electron-capture decay directly to the ground state of argon-40 has never been observed, while theoretical predictions span an order of magnitude. The KDK Collaboration reports on the first observation of this rare decay, obtained using a novel combination of a low-threshold X-ray detector surrounded by a tonne-scale, high-efficiency $γ$-ray tagger at Oak Ridge National Laboratory. A blinded analysis reveals a distinctly nonzero ratio of intensities of ground-state electron-captures ($I_{\text{EC}^0}$) over excited-state ones ($I_{\text{EC}^*}$) of $I_{\text{EC}^0} / I_{\text{EC}^*}=0.0095\stackrel{\text{stat}}{\pm}0.0022\stackrel{\text{sys}}{\pm}0.0010$ (68% CL), with the null hypothesis rejected at 4$σ$ [Stukel et al., DOI:10.1103/PhysRevLett.131.052503]. This unambiguous signal yields a branching ratio of $I_{\text{EC}^0}=0.098\%\stackrel{\text{stat}}{\pm}0.023\%\stackrel{\text{sys}}{\pm}0.010$, roughly half of the commonly used prediction. This first observation of a third-forbidden unique electron capture improves understanding of low-energy backgrounds in dark-matter searches and has implications for nuclear-structure calculations. A shell-model based theoretical estimate for the $0νββ$ decay half-life of calcium-48 is increased by a factor of $7^{+3}_{-2}$. Our nonzero measurement shifts geochronological ages by up to a percent; implications are illustrated for Earth and solar system chronologies.

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$\beta^-$ decay $Q$-value measurement of $^{136}$Cs and its implications to neutrino studies

The $\beta^-$ decay $Q$-value of $^{136}$Cs ($J^\pi = 5^+$, $t_{1/2} \approx 13$~days) was measured with the JYFLTRAP Penning trap setup at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyv\"askyl\"a, Finland. The mono-isotopic samples required in the measurements were prepared with a new scheme utilised for the cleaning, based on the coupling of dipolar excitation with Ramsey's method of time-separated oscillatory fields and the phase-imaging ion-cyclotron-resonance (PI-ICR) technique. The $Q$ value is determined to be 2536.83(45) keV, which is $\sim$4 times more precise and 11.4(20) keV ($\sim$ 6$\sigma$) smaller than the adopted value in the most recent Atomic Mass Evaluation AME2020. The daughter, $^{136}$Ba, has a 4$^+$ state at 2544.481(24) keV and a $3^-$ state at 2532.653(23) keV, both of which can potentially be ultralow $Q$-value end-states for the $^{136}$Cs decay. With our new ground-to-ground state $Q$ value, the decay energies to these two states become -7.65(45) keV and 4.18(45) keV, respectively. The former is confirmed to be negative at the level of $\sim$ 17$\sigma$, which verifies that this transition is not a suitable candidate for neutrino mass determination. On the other hand, the slightly negative $Q$ value makes this transition an interesting candidate for the study of virtual $\beta$-$\gamma$ transitions. The decay to the 3$^{-}$ state is validated to have a positive low $Q$ value which makes it a viable candidate for neutrino mass determination. For this transition, we obtained a shell-model-based half-life estimate of $2.1_{-0.8}^{+1.6}\times10^{12}$ yr.

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Array of Cryogenic Calorimeters to Evaluate the Spectral Shape of forbidden $β$-decays: the ACCESS project

The ACCESS (Array of Cryogenic Calorimeters to Evaluate Spectral Shapes) project aims to establish a novel technique to perform precision measurements of forbidden \b{eta}-decays, which can serve as an important benchmark for nuclear physics calculations and represent a significant background in astroparticle physics experiments. ACCESS will operate a pilot array of cryogenic calorimeters based on natural and doped crystals containing \b{eta}-emitting radionuclides. In this way, natural (e.g. 113 Cd and 115In) and synthetic isotopes (e.g. 99Tc) will be simultaneously measured with a common experimental technique. The array will also include further crystals optimised to disentangle the different background sources, thus reducing the systematic uncertainty. In this paper, we give an overview of the ACCESS research program, discussing a detector design study and promising results of 115In.

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Ab initio calculation of muon capture on $^{24}$Mg

In this work we study ordinary muon capture (OMC) on $^{24}$Mg from a first principles perspective. Starting from a particular two- and three-nucleon interaction derived from chiral effective field theory, we use the valence-space in-medium similarity renormalization group (VS-IMSRG) framework to construct effective Hamiltonians and muon-capture operators which nonperturbatively account for many-body physics outside the valence space. The obtained nuclear matrix elements are compared against those from the phenomenological shell model. The impact of including the correlations from the nuclear shell model (NSM) as well as including the induced two-body part is studied in detail. Furthermore, the effects of realistic bound-muon wave function on the operators is studied. Finally, predictions for capture rates to the lowest excited states in $^{24}$Na are given and compared with available data. It is found that the spectroscopic properties of $^{24}$Mg and its OMC daughter $^{24}$Na are fairly well described by both the NSM and VS-IMSRG, and that the effect of the hadronic two-body currents significantly reduces the OMC rates. Both models have some difficulties in matching the measured OMC rates, especially for the $2^+$ final states. This calls for further studies in other light nuclei with available OMC data.

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