arXiv subjects

J. Valenta

Publications and source records attributed to J. Valenta.

5 recordsLinked to original sources

arXiv2025

Suppression of ferromagnetism in van der Waals insulator due to pressure-induced layer stacking variation

Ferromagnetism in van der Waals insulators like CrBr3 is highly sensitive to structural modifications. We explore the pressure-driven structural and magnetic transformations of the van der Waals magnet CrBr3, establishing it as a model platform for phenomena emerging in layered vdW systems. Single-crystal X-ray diffraction revealed intrinsic trimorphism with two known phases (monoclinic and rhombohedral) and a so-far unreported trigonal phase. The paracrystal model well captures the coexistence of the rhombohedral and trigonal phases at ambient conditions. Increasing pressure drives the growth of the AA-stacked trigonal phase at the expense of the rhombohedral phase, which becomes undetectable above 8.4 GPa. Magnetization measurements provided the first direct evidence of a collapse of ferromagnetism above 5.8 GPa. This behavior is attributed to the increasing number of AFM-coupled Cr moments in AA stackings. Ab initio DFT calculations of electronic structure and atomistic simulations of finite-temperature magnetism corroborate the scenario.

cond-mat.mtrl-sci↗

arXiv2022

Unusually strong electronic correlation and field-induced ordered phase in YbCo$_2$

We report the first study of electrical resistivity, magnetization, and specific heat on YbCo$_2$. The measurements on a single-phased sample of YbCo$_2$ bring no evidence of magnetic ordering down to 0.3 K in a zero magnetic field. The manifestations of low Kondo temperature are observed. The specific heat value divided by temperature, C/T, keeps increasing logarithmically beyond 7 J/mol.K2 with decreasing temperature down to 0.3 K without no sign of magnetic ordering, suggesting a very large electronic specific heat. Analysis of the magnetic specific heat indicates that the large portion of the low-temperature specific heat is not explained simply by the low Kondo temperature but is due to the strong intersite magnetic correlation in both the 3d and 4f electrons. Temperature-dependent measurements under static magnetic fields up to 7 T are carried out, which show the evolution of field-induced transition above 2 T. The transition temperature increases with increasing field, pointing to a ferromagnetic character. The extrapolation of the transition temperature to zero field suggests that YbCo$_2$ is in the very proximity of the quantum critical point. These results indicate that in the unique case of YbCo$_2$, the itinerant electron magnetism of Co 3d-electrons and the Kondo effect within the vicinity of quantum criticality of Yb 4f-local moments can both play a role.

cond-mat.str-el↗

arXiv2020

Pressure-induced huge increase of Curie temperature of the van der Waals ferromagnet VI3

Evolution of magnetism in single crystals of the van der Waals compound VI3 in external pressure up to 7.3 GPa studied by measuring magnetization and ac magnetic susceptibility is reported. Four magnetic phase transitions, at T1 = 54.5 K, T2 = 53 K, TC = 49.5 K, and TFM = 26 K, respectively have been observed at ambient pressure. The first two have been attributed to the onset of ferromagnetism in specific crystal-surface layers. The bulk ferromagnetism is characterized by the magnetic ordering transition at Curie temperature TC and the transition between two different ferromagnetic phases TFM, accompanied by a structure transition from monoclinic to triclinic symmetry upon cooling. The pressure effects on magnetic parameters were studied with three independent techniques. TC was found to be almost unaffected by pressures up to 0.6 GPa whereas TFM increases rapidly with increasing pressure and reaches TC at a triple point at ~ 0.85 GPa. At higher pressures, only one magnetic phase transition is observed moving to higher temperatures with increasing pressure to reach 99 K at 7.3 GPa. In contrast, the low-temperature bulk magnetization is dramatically reduced by applying pressure (by more than 50% at 2.5 GPa) suggesting a possible pressure-induced reduction of vanadium magnetic moment. We discussed these results in light of recent theoretical studies to analyze exchange interactions and provide how to increase the Curie temperature of VI3.

cond-mat.mtrl-sci↗

arXiv2018

Magnetoelastic phenomena in antiferromagnetic uranium intermetallics: the $\mathrm{UAu_{2}Si_{2}}$ case

Thermal expansion, magnetostriction and magnetization measurements under magnetic field and hydrostatic pressure were performed on a $\mathrm{UAu_{2}Si_{2}}$ single crystal. They revealed a large anisotropy of magnetoelastic properties manifested by prominent length changes leading to a collapse of the unit-cell volume accompanied by breaking the fourfold symmetry (similar to that in $\mathrm{URu_{2}Si_{2}}$ in the hidden-order state) in the antiferromagnetic state as consequences of strong magnetoelastic coupling. The magnetostriction curves measured at higher temperatures confirm a bulk character of the 50 K weak ferromagnetic phase. The large positive pressure change of the ordering temperature predicted from Ehrenfest relation contradicts the more than an order of magnitude smaller pressure dependence observed by the magnetization and specific heat measured under hydrostatic pressure. A comprehensive magnetic phase diagram of $\mathrm{UAu_{2}Si_{2}}$ in magnetic field applied along the $c$ axis is presented. The ground-state antiferromagnetic phase is suppressed by a field-induced metamagnetic transition that changes its character from the second to the first order at the tricritical point.

cond-mat.str-el↗

arXiv2004

Investigation of top mass measurements with the ATLAS detector at LHC

Several methods for the determination of the mass of the top quark with the ATLAS detector at the LHC are presented. All dominant decay channels of the top quark can be explored. The measurements are in most cases dominated by systematic uncertainties. New methods have been developed to control those related to the detector. The results indicate that a total error on the top mass at the level of 1 GeV should be achievable.

hep-ex↗