arXiv subjects

J. Van de Vondel

Publications and source records attributed to J. Van de Vondel.

At least 19 recordsLinked to original sources

arXiv2026

Magnetic landscape of NbTiN superconducting resonators under radio-frequency excitation

Planar superconducting resonators are essential components in quantum circuits and highly sensitive sensors. However, their performance is often compromised by magnetic flux penetration, as the interaction of flux quanta and the induced radio-frequency (RF) currents in the superconducting thin film leads to significant energy dissipation. At low operating temperatures, this issue is aggravated as thermomagnetic instabilities can trigger the sudden propagation of magnetic flux avalanches. An important open question is whether the RF excitation itself stimulates the nucleation and propagation of magnetic flux avalanches in the superconducting thin film. The literature remains inconclusive on this point, partly due to the lack of compelling evidence for this phenomenon. In this work, we address this issue by unprecedented direct visualization of magnetic flux penetration through Faraday rotation imaging under simultaneous RF excitation. We demonstrate that the avalanche activity exhibits a weak dependence on the RF intensity for RF excitations within the linear Campbell regime. However, magnetic flux bursts clearly influence the RF transmission properties of the device. Furthermore, it is possible to unambiguously associate a particular avalanche event with a jump in resonance frequency. This enables us to identify the loci of most deleterious events and understand the distinct origins of upward and downward frequency shifts. These observations are supported by electromagnetic simulations in which local changes of the kinetic inductance mimic flux avalanches and confirm the invasive character of the MOI technique. The insights gained from this study aim to contribute to the broader understanding of the magnetic resilience of superconducting resonators, with the goal of improving their efficiency and stability.

cond-mat.supr-con↗

arXiv2025

Reversing Hydrogen-Related Loss in $α$-Ta Thin Films for Quantum Device Fabrication

$α$-Tantalum ($α$-Ta) is an emerging material for superconducting qubit fabrication due to the low microwave loss of its stable native oxide. However, hydrogen absorption during fabrication, particularly when removing the native oxide, can degrade performance by increasing microwave loss. In this work, we demonstrate that hydrogen can enter $α$-Ta thin films when exposed to 10 vol% hydrofluoric acid for 3 minutes or longer, leading to an increase in power-independent ohmic loss in high-Q resonators at millikelvin temperatures. Reduced resonator performance is likely caused by the formation of non-superconducting tantalum hydride (TaH$_x$) precipitates. We further show that annealing at 500°C in ultra-high vacuum (10$^{-8}$ Torr) for one hour fully removes hydrogen and restores the resonators' intrinsic quality factors to ~4 million at the single-photon level. These findings identify a previously unreported loss mechanism in $α$-Ta and offer a pathway to reverse hydrogen-induced degradation in quantum devices based on Ta and, by extension also Nb, enabling more robust fabrication processes for superconducting qubits.

quant-ph↗

arXiv2023

Argon milling induced decoherence mechanisms in superconducting quantum circuits

The fabrication of superconducting circuits requires multiple deposition, etch and cleaning steps, each possibly introducing material property changes and microscopic defects. In this work, we specifically investigate the process of argon milling, a potentially coherence limiting step, using niobium and aluminum superconducting resonators as a proxy for surface-limited behavior of qubits. We find that niobium microwave resonators exhibit an order of magnitude decrease in quality-factors after surface argon milling, while aluminum resonators are resilient to the same process. Extensive analysis of the niobium surface shows no change in the suboxide composition due to argon milling, while two-tone spectroscopy measurements reveal an increase in two-level system electrical dipole moments, indicating a structurally altered niobium oxide hosting larger two-level system defects. However, a short dry etch can fully recover the argon milling induced losses on niobium, offering a potential route towards state-of-the-art overlap Josephson junction qubits with niobium circuitry.

quant-ph↗

arXiv2022

Manufacturing high-Q superconducting α-tantalum resonators on silicon wafers

The performance of state-of-the-art superconducting quantum devices is currently limited by microwave dielectric losses at different surfaces and interfaces. α-tantalum is a superconductor that has proven effective in reducing dielectric loss and improving device performance due to its thin low-loss oxide. However, without the use of a seed layer, this tantalum phase has so far only been realised on sapphire substrates, which is incompatible with advanced processing in industry-scale fabrication facilities. Here, we demonstrate the fabrication of high-quality factor α-tantalum resonators directly on silicon wafers over a variety of metal deposition conditions and perform a comprehensive material and electrical characterization study. By comparing experiments with simulated resonator loss, we demonstrate that two-level-system loss is dominated by surface oxide contributions and not the substrate-metal interface. Our study paves the way to large scale manufacturing of low-loss superconducting circuits and to materials-driven advancements in superconducting circuit performance.

quant-ph↗

arXiv2022

Magnetic flux penetration in nanoscale wedge-shaped superconducting thin films

Thickness uniformity is regarded as an important parameter in designing thin film devices. However, some applications based on films with non-uniform thickness have recently emerged, such as gas sensors and optimized materials based on the gradual change of film composition. This work deals with superconducting Pb thin films with a thickness gradient prepared with the aid of a diffuse stencil mask. Atomic Force Microscopy and Energy-Dispersive X-ray Spectroscopy show variations ranging from 90~nm to 154~nm. Quantitative magneto-optical images reveal interesting features during both the abrupt and the smooth penetration regimes of magnetic flux, as well as the thickness-dependent critical current density ($J_c$). In addition, we observe a gradual superconducting transition as the upper critical field is progressively reached for certain thicknesses. Furthermore, the hysteresis observed for triggering flux avalanches when increasing and decreasing magnetic fields is also accounted for by the $J_c$ profile evolution along the thickness gradient. Numerical simulations based on the Thermomagnetic Model are in fair agreement with the experimental data. These findings demonstrate that wedge-shaped films are a viable approach to investigate, in a continuous fashion, thickness-dependent properties of a superconducting materials.

cond-mat.supr-con↗

arXiv2021

The impact of kinetic inductance on the critical current oscillations of nanobridge SQUIDs

In this work, we study the current phase relation ($CΦR$) of lithographically fabricated molybdenum germanium (MoGe) nanobridges, which is intimately linked to the nanobridge kinetic inductance. We do this by imbedding the nanobridges in a SQUID. We observe that for temperatures far below $T_c$, the $CΦR$ is linear as long as the condensate is not weakened by the presence of supercurrent. We demonstrate lithographic control over the nanobridge kinetic inductance, which scales with the nanobridge aspect ratio. This allows to tune the SQUID $I_c(B)$ characteristic. The SQUID properties that can be controlled in this way include the SQUID sensitivity and the positions of the critical current maxima. These observations can be of use for the design and operation of future superconducting devices such as magnetic memories or flux qubits.

cond-mat.supr-con↗

arXiv2018

Quantitative magneto-optical investigation of superconductor/ferromagnet hybrid structures

We present a detailed quantitative magneto-optical imaging study of several superconductor/ferromagnet hybrid structures, including Nb deposited on top of thermomagnetically patterned NdFeB, and permalloy/niobium with erasable and tailored magnetic landscapes imprinted in the permalloy layer. The magneto-optical imaging data is complemented with and compared to scanning Hall probe microscopy measurements. Comprehensive protocols have been developed for calibrating, testing, and converting Faraday rotation data to magnetic field maps. Applied to the acquired data, they reveal the comparatively weaker magnetic response of the superconductor from the background of larger fields and field gradients generated by the magnetic layer.

cond-mat.supr-con↗

arXiv2017

Tunable artificial vortex ice in nanostructured superconductors with frustrated kagome lattice of paired antidots

Theoretical proposals for spin ice analogs based on nanostructured superconductors have suggested larger flexibility for probing the effects of fluctuations and disorder than in the magnetic systems. In this work, we unveil the particularities of a vortex ice system by direct observation of the vortex distribution in a kagome lattice of paired antidots using scanning Hall probe microscopy. The theoretically suggested vortex ice distribution, lacking long range order, is observed at half matching field (H_{1}/2). Moreover, the vortex ice state formed by the pinned vortices is still preserved at 2H_{1}/3. This unexpected result is attributed to the introduction of interstitial vortices at these magnetic field values. Although the interstitial vortices increase the number of possible vortex configurations, it is clearly shown that the vortex ice state observed at 2H_{1}/3 is less prone to defects than at $H_{1}/2$. In addition, the non-monotonic variations of the vortex ice quality on the lattice spacing indicates that a highly ordered vortex ice state cannot be attained by simply reducing the lattice spacing. The optimal design to observe defect free vortex ice is discussed based on the experimental statistics. The direct observations of a tunable vortex ice state provides new opportunities to explore the order-disorder transition in artificial ice systems.

cond-mat.supr-con↗

arXiv2015

The onset, evolution and magnetic braking of vortex lattice instabilities in nanostructured superconducting films

In 1976 Larkin and Ovchinnikov [Sov. Phys. JETP 41, 960 (1976)] predicted that vortex matter in superconductors driven by an electrical current can undergo an abrupt dynamic transition from a flux-flow regime to a more dissipative state at sufficiently high vortex velocities. Typically this transition manifests itself as a large voltage jump at a particular current density, so-called instability current density $J^*$, which is smaller than the depairing current. By tuning the effective pinning strength in Al films, using an artificial periodic pinning array of triangular holes, we show that a unique and well defined instability current density exists if the pinning is strong, whereas a series of multiple voltage transitions appear in the relatively weaker pinning regime. This behavior is consistent with time-dependent Ginzburg-Landau simulations, where the multiple-step transition can be unambiguously attributed to the progressive development of vortex chains and subsequently phase-slip lines. In addition, we explore experimentally the magnetic braking effects, caused by a thick Cu layer deposited on top of the superconductor, on the instabilities and the vortex ratchet effect

cond-mat.supr-con↗

arXiv2014

Temperature dependence of lower critical field Hc1(T) shows nodeless superconductivity in FeSe

We investigate the temperature dependence of the lower critical field Hc1(T) of a high-quality FeSe single crystal under static magnetic fields H parallel to the c axis. The temperature dependence of the first vortex penetration field has been experimentally obtained by two independent methods and the corresponding Hc1(T) was deduced by taking into account demagnetization factors. A pronounced change in the Hc1(T) curvature is observed, which is attributed to anisotopic s-wave or multiband superconductivity. The London penetration depth λab(T) calculated from the lower critical field does not follow an exponential behavior at low temperatures, as it would be expected for a fully gapped clean s-wave superconductor. Using either a two-band model with s-wave-like gaps of magnitudes ?delta 1 = 0.41 meV and delta ?2 = 3.33 meV or a single anisotropic s-wave order parameter, the temperature dependence of the lower critical field Hc1(T) can be well described. These observations clearly show that the superconducting energy gap in FeSe is nodeless.

cond-mat.supr-con↗

arXiv2014

A closer look at the low frequency dynamics of vortex matter

Using scanning susceptibility microscopy, we shed new light on the dynamics of individual superconducting vortices and examine the hypotheses of the phenomenological models traditionally used to explain the macroscopic ac electromagnetic properties of superconductors. The measurements, carried out on a 2H-NbSe$_2$ single crystal at relatively high temperature $T=6.8$ K, show a linear amplitude dependence of the global ac-susceptibility for excitation amplitudes between 0.3 and 2.6 Oe. We observe that the low amplitude behavior, typically attributed to the shaking of vortices in a potential well defined by a single, relaxing, Labusch constant, corresponds actually to strongly non-uniform vortex shaking. This is particularly accentuated in the field-cooled disordered phase, which undergoes a dynamic reorganization above 0.8 Oe as evidenced by the healing of lattice defects and a more uniform oscillation of vortices. These observations are corroborated by molecular dynamics simulations when choosing the microscopic input parameters from the experiments. The theoretical simulations allow us to reconstruct the vortex trajectories providing deeper insight in the thermally induced hopping dynamics and the vortex lattice reordering.

cond-mat.supr-con↗

arXiv2013

Superconducting properties of corner-shaped Al microstrips

The electrical transport properties of corner-shaped Al superconducting microstrips have been investigated. We demonstrate that the sharp turns lead to asymmetric vortex dynamics, allowing for easier penetration from the inner concave angle than from the outer convex angle. This effect is evidenced by a strong rectification of the voltage signal otherwise absent in straight superconducting strips. At low magnetic fields, an enhancement of the critical current with increasing magnetic field is observed for a particular combination of field and current polarity, confirming a recently theoretically predicted competing interplay of superconducting screening currents and applied currents at the inner side of the turn.

cond-mat.supr-con↗

arXiv2012

Local mapping of dissipative vortex motion

We explore, with unprecedented single vortex resolution, the dissipation and motion of vortices in a superconducting ribbon under the influence of an external alternating magnetic field. This is achieved by combing the phase sensitive character of ac-susceptibility, allowing to distinguish between the inductive-and dissipative response, with the local power of scanning Hall probe microscopy. Whereas the induced reversible screening currents contribute only inductively, the vortices do leave a fingerprint in the out-of-phase component. The observed large phase-lag demonstrates the dissipation of vortices at timescales comparable to the period of the driving force (i.e. 13 ms). These results indicate the presence of slow microscopic loss mechanisms mediated by thermally activated hopping transport of vortices between metastable states.

cond-mat.supr-con↗

arXiv2012

Localization of superconductivity in superconductor-electromagnet hybrids

We investigate the nucleation of superconductivity in a superconducting Al strip under the influence of the magnetic field generated by a current-carrying Nb wire, perpendicularly oriented and located underneath the strip. The inhomogeneous magnetic field, induced by the Nb wire, produces a spatial modulation of the critical temperature T_c, leading to a controllable localization of the superconducting order parameter (OP) wave function. We demonstrate that close to the phase boundary T_c(B_ext) the localized OP solution can be displaced reversibly by either applying an external perpendicular magnetic field B_ext or by changing the amplitude of the inhomogeneous field.

cond-mat.supr-con↗

arXiv2011

Vortex core deformation and stepper motor behavior in a superconducting ratchet

We investigated experimentally the frequency dependence of a superconducting vortex ratchet effect by means of electrical transport measurements and modeled it theoretically using the time dependent Ginzburg-Landau formalism. We demonstrate that the high frequency vortex behavior can be described as a discrete motion of a particle in a periodic potential, i.e. the so called stepper motor behavior. Strikingly, in the more conventional low frequency response a transition takes place from an Abrikosov vortex rectifier to a phase slip line rectifier. This transition is characterized by a strong increase in the rectified voltage and the appearance of a pronounced hysteretic behavior.

cond-mat.supr-con↗

arXiv2011

Mesoscopic cross-film cryotrons: Vortex trapping and dc-Josephson-like oscillations of the critical current

We investigate theoretically and experimentally the transport properties of a plain Al superconducting strip in the presence of a single straight current-carrying wire, oriented perpendicular to the superconducting strip. It is well known that the critical current of the superconducting strip, Ic, in such cryotron--like system can be tuned by changing the current in the control wire, Iw. We demonstrated that the discrete change in the number of the pinned vortices/antivortices inside the narrow and long strip nearby the current-carrying wire results in a peculiar oscillatory dependence of Ic on Iw.

cond-mat.supr-con↗

arXiv2009

Tunable anisotropic nonlinearity in superconductors with asymmetric antidot array

The influence of the spatial asymmetry of the pinning potential on the spectral composition of the voltage, induced in perforated superconducting Al bridges by the injection of a sinusoidal bias current, was investigated. The loss of the mirror symmetry of the pinning potential leads to the appearance of even Fourier components in the induced voltage in the vicinity of the superconducting phase transition line on the H-T diagram (H is the external magnetic field, T is temperature). Artificially-introduced asymmetry for vortex motion makes it possible to create low-resistive materials, in which nonlinearity depends on the direction of injected electrical currents.

cond-mat.supr-con↗

arXiv2009

Symmetry-induced giant vortex state in a superconducting film with a Penrose array of magnetic pinning centers

A direct visualization of the flux distribution in a Pb film covering a five-fold Penrose array of Co dots is obtained by mapping the local field distribution with a scanning Hall probe microscope. We demonstrate that stable vortex configurations can be found for fields H~0.8H_1, H_1 and 1.6H_1, where H_1 corresponds to one flux quantum per pinning site. The vortex pattern at 0.8H_1 corresponds to one vacancy in one of the vertices of the thin tiles whereas at 1.6H_1 the vortex structure can be associated with one interstitial vortex inside each thick tile. Strikingly, for H=1.6H_1 interstitial and pinned vortices arrange themselves in ring-like structures ("vortex corrals") which favor the formation of a giant vortex state at their center.

cond-mat.supr-con↗