arXiv subjects

J. Van de Walle

Publications and source records attributed to J. Van de Walle.

12 recordsLinked to original sources

arXiv2020

Signature of a possible $α$-cluster state in $N=Z$ doubly-magic $^{56}$Ni

An inelastic $α$-scattering experiment on the unstable $N=Z$, doubly-magic $^{56}$Ni nucleus was performed in inverse kinematics at an incident energy of 50 A.MeV at GANIL. High multiplicity for $α$-particle emission was observed within the limited phase-space of the experimental setup. This observation cannot be explained by means of the statistical-decay model. The ideal classical gas model at $kT$ = 0.4 MeV reproduces fairly well the experimental momentum distribution and the observed multiplicity of $α$ particles corresponds to an excitation energy around 96 MeV. The method of distributed $mα$-decay ensembles is in agreement with the experimental results if we assume that the $α$-gas state in $^{56}$Ni exists at around $113^{+15}_{-17}$ MeV. These results suggest that there may exist an exotic state consisting of many $α$ particles at the excitation energy of $113^{+15}_{-17}$ MeV.

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arXiv2015

Low-energy Coulomb excitation of $^{62}$Fe and $^{62}$Mn following in-beam decay of $^{62}$Mn

Sub-barrier Coulomb-excitation was performed on a mixed beam of $^{62}$Mn and $^{62}$Fe, following in-trap $β^{-}$ decay of $^{62}$Mn at REX-ISOLDE, CERN. The trapping and charge breeding times were varied in order to alter the composition of the beam, which was measured by means of an ionisation chamber at the zero-angle position of the Miniball array. A new transition was observed at 418~keV, which has been tentatively associated to a $(2^{+},3^{+})\rightarrow1^{+}_{g.s.}$ transition. This fixes the relative positions of the $β$-decaying $4^{+}$ and $1^{+}$ states in $^{62}$Mn for the first time. Population of the $2^{+}_{1}$ state was observed in $^{62}$Fe and the cross-section determined by normalisation to the $^{109}$Ag target excitation, confirming the $B(E2)$ value measured in recoil-distance lifetime experiments.

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arXiv2015

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around $Z=82$ and the neutron mid-shell at $N=104$. Purpose: Evidence for shape coexistence has been inferred from $α$-decay measurements, laser spectroscopy and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of $^{202}$Rn and $^{204}$Rn were studied by means of low-energy Coulomb excitation at the REX-ISOLDE facility in CERN. Results: The electric-quadrupole ($E2$) matrix element connecting the ground state and first-excited $2^{+}_{1}$ state was extracted for both $^{202}$Rn and $^{204}$Rn, corresponding to ${B(E2;2^{+}_{1} \to 2^{+}_{1})=29^{+8}_{-8}}$ W.u. and $43^{+17}_{-12}$ W.u., respectively. Additionally, $E2$ matrix elements connecting the $2^{+}_{1}$ state with the $4^{+}_{1}$ and $2^{+}_{2}$ states were determined in $^{202}$Rn. No excited $0^{+}$ states were observed in the current data set, possibly due to a limited population of second-order processes at the currently-available beam energies. Conclusions: The results are discussed in terms of collectivity and the deformation of both nuclei studied is deduced to be weak, as expected from the low-lying level-energy schemes. Comparisons are also made to state-of-the-art beyond-mean-field model calculations and the magnitude of the transitional quadrupole moments are well reproduced.

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arXiv2014

Sizeable beta-strength in 31Ar(beta-3p) decay

We present for the first time precise spectroscopic information on the recently discovered decay mode beta-delayed 3p-emission. The detection of the 3p events gives an increased sensitivity to the high energy part of the Gamow-Teller strength distribution from the decay of 31Ar revealing that as much as 30% of the strength resides in the beta-3p decay mode. A simplified description of how the main decay modes evolve as the excitation energy increases in 31Cl is provided.

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arXiv2014

Multi-particle emission in the decay of 31Ar

A multi-hit capacity setup was used to study the decay of the dripline nucleus 31Ar, produced at the ISOLDE facility at CERN. A spectroscopic analysis of the beta-delayed three-proton decay of 31Ar is presented for the first time together with a quantitative analysis of the beta-delayed two-proton-gamma-decay. A new method for determination of the spin of low-lying levels in the beta-proton-daughter 30S using proton-proton angular correlations is presented and used for the level at 5.2 MeV, which is found to be either a 3+ or 4+ level, with the data pointing towards the 3+. The half-life of 31Ar is found to be 15.1(3) ms. An improved analysis of the Fermi beta-strength gives a total measured branching for the beta-3p-decay of 3.60(44) %, which is lower than the theoretical value found to be 4.24(43) %. Finally the strongest gamma-transitions in the decay of 33Ar are shown including a line at 4734(3) keV associated to the decay of the IAS, which has not previously been identified.

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arXiv2013

Relative proton and gamma widths of astrophysically important states in 30S studied in the beta-decay of 31Ar

Resonances just above the proton threshold in 30S affect the 29P(p,gamma)30S reaction under astrophysical conditions. The (p,gamma)-reaction rate is currently determined indirectly and depends on the properties of the relevant resonances. We present here a method for finding the ratio between the proton and gamma partial widths of resonances in 30S. The widths are determined from the beta-2p and beta-p-gamma decay of 31Ar, which is produced at the ISOLDE facility at the European research organization CERN. Experimental limits on the ratio between the proton and gamma partial widths for astrophysical relevant levels in 30S have been found for the first time. A level at 4688(5) keV is identified in the gamma spectrum, and an upper limit on the proton to gamma width of 0.26 (95 % C.L.) is found. In the two-proton spectrum two levels at 5227(3) keV and 5847(4) keV are identified. These levels are previously seen to gamma decay and upper limits on the gamma to proton width of 0.5 and 9, respectively, (95 % C.L.) are found, where the latter differs from previous calculations.

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arXiv2010

Coulomb excitation of 73Ga

The B(E2; Ii -> If) values for transitions in 71Ga and 73Ga were deduced from a Coulomb excitation experiment at the safe energy of 2.95 MeV/nucleon using post-accelerated beams of 71,73Ga at the REX-ISOLDE on-line isotope mass separator facility. The emitted gamma rays were detected by the MINIBALL-detector array and B(E2; Ii->If) values were obtained from the yields normalized to the known strength of the 2+ -> 0+ transition in the 120Sn target. The comparison of these new results with the data of less neutron-rich gallium isotopes shows a shift of the E2 collectivity towards lower excitation energy when adding neutrons beyond N = 40. This supports conclusions from previous studies of the gallium isotopes which indicated a structural change in this isotopical chain between N = 40 and N = 42. Combined with recent measurements from collinear laser spectroscopy showing a 1/2- spin and parity for the ground state, the extracted results revealed evidence for a 1/2-; 3/2- doublet near the ground state in 73 31Ga42 differing by at most 0.8 keV in energy.

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arXiv2010

Discovery of the shape coexisting 0+ state in 32Mg by a two neutron transfer reaction

The Island of Inversion nucleus 32Mg has been studied by a (t,p) two neutron transfer reaction in inverse kinematics at REX-ISOLDE. The shape coexistent excited 0+ state in 32Mg has been identified by the characteristic angular distribution of the protons of the DeltaL = 0 transfer. The excitation energy of 1058 keV is much lower than predicted by any theoretical model. The low gamma-ray intensity observed for the decay of this 0+ state indicates a lifetime of more than 10 ns. Deduced spectroscopic amplitudes are compared with occupation numbers from shell model calculations.

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arXiv2010

Early onset of ground-state deformation in the neutron-deficient polonium isotopes

In-source resonant ionization laser spectroscopy of the even-$A$ polonium isotopes $^{192-210,216,218}$Po has been performed using the $6p^37s$ $^5S_2$ to $6p^37p$ $^5P_2$ ($λ=843.38$ nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in $^{200-210}$Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.

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arXiv2009

Structure of 65,67Co studied through the beta decay of 65,67Fe and a deep-inelastic reaction

The neutron-rich isotopes 65,67Fe and 65Co have been produced at the LISOL facility, Louvain-La-Neuve, in the proton-induced fission of 238U. Beams of these isotopes have been extracted with high selectivity by means of resonant laser ionization combined with mass separation. Yrast and near-yrast levels of 65Co have also been populated in the 64Ni+238U reaction at Argonne National Laboratory. The level structure of 65Co could be investigated by combining all the information from both the 65Fe and 65Co beta decay and the deep-inelastic reaction. The 65Fe, 65Co and 67Fe decay schemes and the 65Co yrast structure are fully established. The 65,67Co level structures can be interpreted as resulting from the coexistence of core-coupled states with levels based on a low-energy proton-intruder configuration.

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arXiv2008

Coulomb excitation of $^{68}$Ni at safe energies

The $B(E2;0^+\to2^+)$ value in $^{68}$Ni has been measured using Coulomb excitation at safe energies. The $^{68}$Ni radioactive beam was post-accelerated at the ISOLDE facility (CERN) to 2.9 MeV/u. The emitted $γ$ rays were detected by the MINIBALL detector array. A kinematic particle reconstruction was performed in order to increase the measured c.m. angular range of the excitation cross section. The obtained value of 2.8$^{+1.2}_{-1.0}$ 10$^2$ e$^2$fm$^4$ is in good agreement with the value measured at intermediate energy Coulomb excitation, confirming the low $0^+\to2^+$ transition probability.

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arXiv2008

Shape Isomerism at N = 40: Discovery of a Proton Intruder in 67Co

The nuclear structure of 67Co has been investigated through 67Fe beta-decay. The 67Fe isotopes were produced at the LISOL facility in proton-induced fission of 238U and selected using resonant laser ionization combined with mass separation. The application of a new correlation technique unambiguously revealed a 496(33) ms isomeric state in 67Co at an unexpected low energy of 492 keV. A 67Co level scheme has been deduced. Proposed spin and parities suggest a spherical (7/2-) 67Co ground state and a deformed first excited (1/2-) state at 492 keV, interpreted as a proton 1p-2h prolate intruder state.

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