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J. Z. Han

Publications and source records attributed to J. Z. Han.

12 recordsLinked to original sources

Learning Unified Control of Intrinsic Nonlinear Spin Dynamics in Atomic Qudits for Magnetometry

Generating and preserving metrologically useful quantum states is a central challenge in quantum-enhanced metrology. In low-field atomic magnetometry with multilevel atoms, the nonlinear Zeeman (NLZ) effect is both a resource and a limitation. It can generate internal spin squeezing within a single atomic qudit, but under fixed readout it also rotates and distorts the measurement-relevant quadrature, limiting the usable metrological gain. The problem is further complicated by the time dependence of both the squeezing axis and the nonlinear evolution itself. Here we show that reinforcement learning can transform NLZ dynamics from a source of readout degradation into a sustained metrological resource. Using only experimentally accessible low-order spin moments, a trained agent identifies a unified control policy for this class of intrinsically nonlinear sensing dynamics. We illustrate the approach in the $f=21/2$ manifold of $^{161}\mathrm{Dy}$, where the learned policy rapidly prepares strongly squeezed internal states and stabilizes more than $4\,\mathrm{dB}$ of fixed-axis spin squeezing under continuous NLZ evolution. Including state-preparation overhead, the learned protocol yields a single-atom magnetic-field sensitivity of $13.9\,\mathrm{pT}/\sqrt{\mathrm{Hz}}$, approximately $3\,\mathrm{dB}$ beyond the standard quantum limit. Our results establish learning-based control as an experimentally feasible route for converting unavoidable intrinsic nonlinear dynamics in multilevel atomic sensors into operational metrological advantage.

quant-ph

Nuclear charge radii of germanium isotopes around $N$ = 40

Collinear laser spectroscopy measurements were performed on $^{68-74}$Ge isotopes ($Z = 32$) at ISOLDE-CERN, by probing the $4s^2 4p^2 \, ^3\!P_1 \rightarrow 4s^2 4p 5s \, ^3\!P_1^o$ atomic transition (269~nm) of germanium. Nuclear charge radii are determined via the measured isotope shifts, revealing a larger local variation than the neighboring isotopic chains. Nuclear density functional theory with the Fayans functionals Fy($\Delta r$,HFB) and Fy(IVP), and the SV-min Skyrme describes the experimental data for the differential charge radii $\delta\langle r^{2} \rangle$ and charge radii $R_{\rm c}$ within the theoretical uncertainties. The observed large variation in the charge radii of germanium isotopes is better accounted for by theoretical models incorporating ground state quadrupole correlations. This suggests that the polarization effects due to pairing and deformation contribute to the observed large odd-even staggering in the charge radii of the Ge isotopic chain.

nucl-ex

Precise determination of ground-state hyperfine splitting and calculation of Zeeman coefficients for 171Yb+ microwave frequency standard

We report precise measurement of the hyperfine splitting and calculation of the Zeeman coefficients of the $^{171}$Yb$^+$ ground state. The absolute hyperfine splitting frequency is measured using high-resolution laser-microwave double-resonance spectroscopy at 0.1 mHz level, and evaluated using more accurate Zeeman coefficients. These Zeeman coefficients are derived using Landé $g_J$ factors calculated by two atomic-structure methods, multiconfiguration Dirac-Hartree-Fock, and multireference configuration interaction. The cross-check of the two calculations ensures an accuracy of the Zeeman coefficients at $10^{-2}$ Hz/G$^2$ level. The results provided in this paper improve the accuracy and reliability of the second-order Zeeman shift correction, thus further improving the accuracy of the microwave frequency standards based on $^{171}$Yb$^+$. The high-precision hyperfine splitting and Zeeman coefficients could also support could also support further experiments to improve the constraints of fundamental constants through clock frequency comparison of the Yb$^+$ system.

physics.atom-ph

$^{174}\mathrm{Yb}^+$-$^{113}\mathrm{Cd}^+$ sympathetic-cooling bi-species Coulomb crystal applied to microwave frequency standard

We reported the realization of a $^{174}\mathrm{Yb}^+$-$^{113}\mathrm{Cd}^+$ bi-species Coulomb crystal comprising $^{174}\mathrm{Yb}^+$ ions as coolant and verified its potential for application as a $^{113}\mathrm{Cd}^+$ microwave frequency standard employing sympathetic cooling.The two species of massive ions stably trapped in a Paul trap make up this large two-component crystal. The $^{113}\mathrm{Cd}^+$ ions are trapped in the center, which reduces considerably RF heating and excess micromotion to which the $^{113}\mathrm{Cd}^+$ ions are subjected. Under this scheme, the uncertainty due to the second-order Doppler effect is reduced to $5\times10^{-16}$, which represents an order of magnitude improvement over sympathetic cooled $^{40}\mathrm{Ca}^+$-$^{113}\mathrm{Cd}^+$ crystal. The uncertainty from the second-order Zeeman effect, which contributes the largest uncertainty to the microwave-ion frequency standard, is reduced to $4\times10^{-16}$. The relevant AC Stark shift uncertainty is estimated to be $4\times10^{-19}$. These results indicate using $^{174}\mathrm{Yb}^+$ as coolant ions for $^{113}\mathrm{Cd}^+$ is far superior and confirm the feasibility of a sympathetic-cooled cadmium-ion microwave clock system employing a $^{174}\mathrm{Yb}^+$-$^{113}\mathrm{Cd}^+$ two-component crystal.

physics.atom-ph

Second-order Doppler frequency shifts of trapped ions in a linear Paul trap

The accurate evaluation of the second-order Doppler frequency shift (SODFS) of trapped ions in a linear Paul trap has been studied with experiments and molecular dynamics (MD) simulations. The motion of trapped ions in the trap has three contributions, and we focus on the ion excess micromotion, which is rarely discussed when evaluating the SODFS. Based on the hypothesis that the ion density is uniformly distributed in the radial direction, we propose a new model to accurately evaluate the total SODFS for ion microwave clocks. The effectiveness of the model has been verified both in simulation and experiment, especially for ion ensemble with temperature less than 100 mK. We believe that our new model offers advantages in accurately evaluating the SODFS for the ion trap, especially those of laser-cooled ion microwave clocks based on large ion clouds.

physics.atom-ph

Determination of hyperfine splittings and Landé $g_J$ factors of $5s~^2S_{1/2}$ and $5p~^2P_{1/2,3/2}$ states of $^{111,113}$Cd$^+$ for a microwave frequency standard

Regarding trapped-ion microwave-frequency standards, we report on the determination of hyperfine splittings and Landé $g_J$ factors of $^{111,113}$Cd$^+$. The hyperfine splittings of the $5p~^2P_{3/2}$ state of $^{111,113}$Cd$^+$ ions were measured using laser-induced fluorescence spectroscopy. The Cd$^+$ ions were confined in a linear Paul trap and sympathetically cooled by Ca$^+$ ions. Furthermore, the hyperfine splittings and Landé $g_J$ factors of the $5s~^2S_{1/2}$ and $5p~^2P_{1/2,3/2}$ levels of $^{111,113}$Cd$^+$ were calculated with greater accuracy using the multiconfiguration Dirac--Hartree--Fock scheme. The measured hyperfine splittings and the Dirac--Hartree--Fock calculation values were cross-checked, thereby further guaranteeing the reliability of our results. The results provided in this work can improve the signal-to-noise ratio of the clock transition and the accuracy of the second-order Zeeman shift correction, and subsequently the stability and accuracy of the microwave frequency standard based on trapped Cd$^+$ ions.

physics.atom-ph

Progress toward a microwave frequency standard based on laser-cooled large scale 171Yb+ ion crystal

We report on progress towards a microwave frequency standard based on a laser-cooled 171Yb+ ion trap system. The electronics, lasers, and magnetic shields are integrated into a single physical package. With over 1E5 ions are stably trapped, the system offers a high signal-to-noise ratio Ramsey line-shape. In comparison with previous work, the frequency instability of a 171Yb+ microwave clock was further improved to $8.5 \times {10^{ - 13}}/\sqrt τ$ for averaging times between 10 and 1000 s.

physics.atom-ph

Multidimensional King-plot analysis for accurate extraction of Cd nuclear charge radii: a challenge for nuclear structure theory

High-accuracy determination of isotope shift factors, which plays a crucial role in accurate extraction of nuclear charge radius, is well-known to be challenging experimentally and theoretically. Nonetheless, based on an accurate measurement of the isotope shifts for the Cd$^+$ $5s~^2S_{1/2}-5p~^2P_{3/2}$ and the Cd $5s^2~^1S_0-5s5p~^1P_1$ transition, a multidimensional King-plot analysis is performed to extract the atomic field shift and mass shift factors accurately. The results are further cross-checked against results from atomic structure calculations using a high-accuracy configuration interaction and many-body perturbation theory. Combined with previous isotope shifts, nuclear charge radii for $^{100-130}$Cd of the highest accuracy are reported. For the neutron-rich region, accuracies for the charge radii are improved by nearly one order of magnitude. This work provides a coherent and systematic extraction of Cd nuclear charge radii from isotope shifts. The results offer stringent testing and possible challenges to the latest advances in nuclear theory and excellent benchmarking to the atomic structure calculations.

physics.atom-ph

Precision determination of the ground-state hyperfine splitting of trapped ${}^{113}$Cd${}^{+}$ ions

We measured the ground-state hyperfine splitting of trapped ${}^{113}$Cd${}^{+}$ ions to be 15199862855.02799(27) Hz with a fractional uncertainty of $1.8\times10^{-14}$. The ions were trapped and laser-cooled in a linear quadrupole Paul trap. The fractional frequency stability was measured to be ${4.2} \times 10^{-13}/\sqrtτ $, obtained from Ramsey fringes of high signal-to-noise ratio and taken over a measurement time of nearly 5 hours, which is close to the short-term stability limit estimated from the Dick effect. Our result is consistent with previous reported values, but the measurement precision is four times better than the best result obtained to date.

physics.atom-ph

Sympathetic cooling of $^{113}$Cd$^+$ by laser-cooled $^{40}$Ca$^+$ in a linear Paul trap for Microwave Ion Clocks

We report sympathetic cooling of $^{113}$Cd$^+$ by laser-cooled $^{40}$Ca$^+$ in a linear Paul trap for microwave clocks. Long-term low-temperature confinement of $^{113}$Cd$^+$ ions was achieved. The temperature of these ions was measured at $90(10)$ mK, and the corresponding uncertainty arising from the second-order Doppler shifts was estimated to a level of $2\times10^{-17}$. Up to $4.2\times10^5$ Cd$^+$ ions were confined in the trap, and the confinement time constant was measured to be 84 hours. After three hours of confinement, there were still $10^5$ Cd$^+$ ions present, indicating that this Ca$^+$--Cd$^+$ dual ion system is surprisingly stable. The ac Stark shift was induced by the Ca$^+$ lasers and fluorescence, which was carefully estimated to an accuracy of $5.4(0.5)\times10^{-17}$ using a high-accuracy \textit{ab initio} approach. The Dick-effect-limited Allan deviation was also deduced because deadtimes were shorter. These results indicate that a microwave clock based on this sympathetic cooling scheme holds promise in providing ultra-high frequency accuracy and stability.

physics.atom-ph

Roles of electron correlation effects for accurate determination of $g_j$ factors of low-lying states of $^{113}$Cd$^+$ and their applications to atomic clock

We investigate roles of electron correlation effects in the determination of $g_j$ factors of the $ns~^2S_{1/2}$ ($n$=5,6,7), $np~^2P_{1/2,3/2}$ ($n$=5,6), $5d~^2D_{3/2,5/2}$, and $4f~^2F_{5/2,7/2}$ states of the singly ionized cadmium (Cd$^+$) ion. Single and double excited configurations along with important valence triple excited configurations through relativistic coupled-cluster (RCC) theory are taken into account for incorporating electron correlation effects in our calculations. We find significant contributions from the triples to the lower $S$ and $P$ states for attaining high accuracy results. The contributions of Breit interaction and lower-order quantum electrodynamics effects, such as vacuum polarization and self-energy corrections, are also estimated using the RCC theory and are quoted explicitly. In addition, we present energies of the aforementioned states from our calculations and compare them with the experimental results to validate $g_j$ values. Using the $g_j$ factor of the ground state, systematical shift due to the Zeeman effect in the microwave clock frequency of the $|5s~^2S_{1/2}, F=0,m_F=0 \rangle \leftrightarrow |5s~^2S_{1/2}, F=1,m_F=0 \rangle$ transition in $^{113}$Cd$^+$ ion has been estimated.

physics.atom-ph

Direct temperature determination of a sympathetically cooled large 113Cd+ ion crystal for a microwave clock

This paper reports the direct temperature determination of sympathetically cooled 113Cd+ ions with laser-cooled 24Mg+ in a linear Paul trap. The sympathetically cooled ion species distribute in the outer shell of the large ensembles, which contain up to 3.3E5 ions. With optimized parameters, the minimum temperature of the sympathetically cooled 113Cd+ ions was measured to be tens of mK. These results indicate promising performance for microwave atomic clocks. The second order Doppler frequency shift is two orders of magnitudes lower and the Dick effect is suppressed.

physics.atom-ph