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J. Zaanen

Publications and source records attributed to J. Zaanen.

At least 19 recordsLinked to original sources

Incoherent transport across the strange metal regime of highly overdoped cuprates

Strange metals possess highly unconventional transport characteristics, such as a linear-in-temperature ($T$) resistivity, an inverse Hall angle that varies as $T^2$ and a linear-in-field ($H$) magnetoresistance. Identifying the origin of these collective anomalies has proved profoundly challenging, even in materials such as the hole-doped cuprates that possess a simple band structure. The prevailing dogma is that strange metallicity in the cuprates is tied to a quantum critical point at a doping $p*$ inside the superconducting dome. Here, we study the high-field in-plane magnetoresistance of two superconducting cuprate families at doping levels beyond $p*$. At all dopings, the magnetoresistance exhibits quadrature scaling and becomes linear at high $H/T$ ratios. Moreover, its magnitude is found to be much larger than predicted by conventional theory and insensitive to both impurity scattering and magnetic field orientation. These observations, coupled with analysis of the zero-field and Hall resistivities, suggest that despite having a single band, the cuprate strange metal phase hosts two charge sectors, one containing coherent quasiparticles, the other scale-invariant `Planckian' dissipators.

cond-mat.str-el

Magnetic excitations in infinite-layer nickelates

The discovery of superconductivity in infinite-layer nickelates brings us tantalizingly close to a new material class that mirrors the cuprate superconductors. Here, we report on magnetic excitations in these nickelates, measured using resonant inelastic x-ray scattering (RIXS) at the Ni L3-edge, to shed light on the material complexity and microscopic physics. Undoped NdNiO2 possesses a branch of dispersive excitations with a bandwidth of approximately 200 meV, reminiscent of strongly-coupled, antiferromagnetically aligned spins on a square lattice, despite a lack of evidence for long range magnetic order. The significant damping of these modes indicates the importance of coupling to rare-earth itinerant electrons. Upon doping, the spectral weight and energy decrease slightly, while the modes become overdamped. Our results highlight the role of Mottness in infinite-layer nickelates.

cond-mat.supr-con

Propagation of shear stress in strongly interacting metallic Fermi liquids enhances transmission of terahertz radiation

A highlight of Fermi-liquid phenomenology, as explored in neutral $^3$He, is the observation that in the collisionless regime shear stress propagates as if one is dealing with the transverse phonon of a solid. The existence of this $"$transverse zero sound$"$ requires that the quasiparticle mass enhancement exceeds a critical value. Could such a propagating shear stress also exist in strongly correlated electron systems? Despite some noticeable differences with the neutral case in the Galilean continuum, we arrive at the verdict that transverse zero sound should be generic. We present an experimental setup that should be exquisitely sensitive in this regard: the transmission of terahertz radiation through a thin slab of heavy-fermion material will be strongly enhanced at low temperature and accompanied by giant oscillations, which reflect the interference between light itself and the $"$material photon$"$ being the actual manifestation of transverse zero sound in the charged Fermi liquid.

cond-mat.str-el

Spectroscopic Evidence for Charge Order Melting via Quantum Fluctuations in a Cuprate

Copper-oxide high TC superconductors possess a number of exotic orders co-existing with or proximal to superconductivity, whose quantum fluctuations may account for the unusual behaviors of the normal state, even affecting superconductivity. Yet, spectroscopic evidence about such quantum fluctuations remains elusive. Here, we reveal spectroscopic fingerprints for such fluctuations associated with a charge order (CO) in nearly optimally-doped Bi2Sr2CaCu2O8+d, using resonant inelastic x-ray scattering (RIXS). In the superconducting state, while the quasi-elastic CO signal decreases with temperature, the interplay between CO fluctuations and bond-stretching phonons in the form of a Fano-like interference paradoxically increases, incompatible with expectations for competing orders. Invoking general principles, we argue that this behavior reflects the properties of a dissipative system near an order-disorder quantum critical point, where the dissipation varies with the opening of the pseudogap and superconducting gap at low temperatures, leading to the proliferation of quantum critical fluctuations which melt CO.

cond-mat.supr-con

Electronic structure of the parent compound of superconducting infinite-layer nickelates

The search for oxide materials with physical properties similar to the cuprate high Tc superconductors, but based on alternative transition metals such as nickel, has grown and evolved over time. The recent discovery of superconductivity in doped infinite-layer nickelates RNiO2 (R = rare-earth element) further strengthens these efforts.With a crystal structure similar to the infinite-layer cuprates - transition metal oxide layers separated by a rare-earth spacer layer - formal valence counting suggests that these materials have monovalent Ni1+ cations with the same 3d electron count as Cu2+ in the cuprates. Here, we use x-ray spectroscopy in concert with density functional theory to show that the electronic structure of RNiO2 (R = La, Nd), while similar to the cuprates, includes significant distinctions. Unlike cuprates with insulating spacer layers between the CuO2 planes, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly-interacting three-dimensional 5d metallic state. This three-dimensional metallic state hybridizes with a quasi-two-dimensional, strongly correlated state with 3dx2-y2 symmetry in the NiO2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare earth intermetallics, well-known for heavy Fermion behavior, where the NiO2 correlated layers play an analogous role to the 4f states in rare-earth heavy Fermion compounds. This unique Kondo- or Anderson-lattice-like "oxide-intermetallic" replaces the Mott insulator as the reference state from which superconductivity emerges upon doping.

cond-mat.supr-con

Charge trapping and super-Poissonian noise centers in a cuprate high-temperature superconductor

The electronic properties of cuprate high temperature superconductors in their normal state are very two-dimensional: while transport in the ab plane is perfectly metallic, it is insulating along the c-axis, with ratios between the two exceeding 10^4. This anisotropy has been identified as one of the mysteries of the cuprates early on, and while widely different proposals exist for its microscopic origin, little is known empirically on the microscopic scale. Here, we elucidate the properties of the insulating layers with a newly developed scanning noise spectroscopy technique that can spatially map not only the current but also the current fluctuations in time. We discover atomic-scale noise centers that exhibit MHz current fluctuations 40 times the expectation from Poissonian noise, more than what has been observed in mesoscopic systems. Such behaviour can only happen in highly polarizable insulators and represents strong evidence for trapping of charge in the charge reservoir layers. Our measurements suggest a picture of metallic layers separated by polarizable insulators within a three-dimensional superconducting state.

cond-mat.str-el

Holographic pump probe spectroscopy

We study the non-linear response of a 2+1 dimensional holographic model with weak momentum relaxation and finite charge density to an oscillatory electric field pump pulse. Following the time evolution of one point functions after the pumping has ended, we find that deviations from thermality are well captured within the linear response theory. For electric pulses with a negligible zero frequency component the response approaches the instantaneously thermalizing form typical of holographic Vaidya models. We link this to the suppression of the amplitude of the quasinormal mode that governs the approach to equilibrium. In the large frequency limit, we are also able to show analytically that the holographic geometry takes the Vaidya form. A simple toy model captures these features of our holographic setup. Computing the out-of-equilibrium probe optical conductivity after the pump pulse, we similarly find that for high-frequency pulses the optical conductivity reaches its final equilibrium value effectively instantaneously. Pulses with significant DC components show exponential relaxation governed by twice the frequency of the vector quasinormal mode that governs the approach to equilibrium for the background solution. We explain this numerical factor in terms of a simple symmetry argument.

hep-th

Holography and thermalization in optical pump-probe spectroscopy

Using holography, we model experiments in which a 2+1D strange metal is pumped by a laser pulse into a highly excited state, after which the time evolution of the optical conductivity is probed. We consider a finite-density state with mildly broken translation invariance and excite it by oscillating electric field pulses. At zero density, the optical conductivity would assume its thermalized value immediately after the pumping has ended. At finite density, pulses with significant DC components give rise to slow exponential relaxation, governed by a vector quasinormal mode. In contrast, for high-frequency pulses the amplitude of the quasinormal mode is strongly suppressed, so that the optical conductivity assumes its thermalized value effectively instantaneously. This surprising prediction may provide a stimulus for taking up the challenge to realize these experiments in the laboratory. Such experiments would test a crucial open question faced by applied holography: Are its predictions artefacts of the large $N$ limit or do they enjoy sufficient UV independence to hold at least qualitatively in real-world systems?

hep-th

Entanglement entropies and fermion signs of critical metals

The fermion sign problem is often viewed as a sheer inconvenience that plagues numerical studies of strongly interacting electron systems. Only recently, it has been suggested that fermion signs are fundamental for the universal behavior of critical metallic systems and crucially enhance their degree of quantum entanglement. In this work we explore potential connections between emergent scale invariance of fermion sign structures and scaling properties of bipartite entanglement entropies. Our analysis is based on a wavefunction ansatz that incorporates collective, long-range backflow correlations into fermionic Slater determinants. Such wavefunctions mimic the collapse of a Fermi liquid at a quantum critical point. Their nodal surfaces -- a representation of the fermion sign structure in many-particle configurations space -- show fractal behavior up to a length scale $ξ$ that diverges at a critical backflow strength. We show that the Hausdorff dimension of the fractal nodal surface depends on $ξ$, the number of fermions and the exponent of the backflow. For the same wavefunctions we numerically calculate the second Rényi entanglement entropy $S_2$. Our results show a cross-over from volume scaling, $S_2\sim \ell^θ$ ($θ=2$ in $d=2$ dimensions), to the characteristic Fermi-liquid behavior $S_2\sim \ell\ln \ell$ on scales larger than $ξ$. We find that volume scaling of the entanglement entropy is a robust feature of critical backflow fermions, independent of the backflow exponent and hence the fractal dimension of the scale invariant sign structure.

cond-mat.str-el

Holographic fermions at strong translational symmetry breaking: a Bianchi-VII case study

It is presently unknown how strong lattice potentials influence the fermion spectral function of the holographic strange metals predicted by the AdS/CFT correspondence. This embodies a crucial test for the application of holography to condensed matter experiments. We show that for one particular momentum direction this spectrum can be computed for arbitrary strength of the effective translational symmetry breaking potential of the so-called Bianchi-VII geometry employing ordinary differential equations. Deep in the strange metal regime we find rather small changes to the single-fermion response computed by the emergent quantum critical IR, even when the potential becomes relevant in the infra-red. However, in the regime where holographic quasi-particles occur, defining a Fermi surface in the continuum, they acquire a finite lifetime at any finite potential strength. At the transition from irrelevancy to relevancy of the Bianchi potential in the deep infra-red the quasi-particle remnants disappear completely and the fermion spectrum exhibits a purely relaxational behaviour.

hep-th

Probing the Nuclear Spin-Lattice Relaxation Time at the Nanoscale

Nuclear spin-lattice relaxation times are measured on copper using magnetic resonance force microscopy performed at temperatures down to 42 mK. The low temperature is verified by comparison with the Korringa relation. Measuring spin-lattice relaxation times locally at very low temperatures opens up the possibility to measure the magnetic properties of inhomogeneous electron systems realized in oxide interfaces, topological insulators and other strongly correlated electron systems such as high-Tc superconductors.

cond-mat.mes-hall

Exciton-driven quantum phase transitions in holography

We study phase transitions driven by fermionic double-trace deformations in gauge-gravity duality. Both the strength of the double trace deformation and the infrared conformal dimension/self-energy scaling of the quasiparticle can be used to decrease the critical temperature to zero, leading to a line of quantum critical points. The self-energy scaling is controlled indirectly through an applied magnetic field and the quantum phase transition naturally involves the condensation of a fermion bilinear which models the spin density wave in an antiferromagnetic state. The nature of the quantum critical points depends on the parameters and we find either a Berezinskii-Kosterlitz-Thouless-type transition or one of two distinct second order transitions with non-mean field exponents. One of these is an anomalous branch where the order parameter of constituent non-Fermi liquid quasiparticles is enhanced by the magnetic field. Stabilization of ordered non-Fermi liquids by a strong magnetic field is observed in experiments with highly oriented pyrolytic graphite.

hep-th

High Temperature Superconductivity in the Cuprates

The discovery of high temperature superconductivity in the cuprates in 1986 triggered a spectacular outpouring of creative and innovative scientific inquiry. Much has been learned over the ensuing 28 years about the novel forms of quantum matter that are exhibited in this strongly correlated electron system. This progress has been made possible by improvements in sample quality, coupled with the development and refinement of advanced experimental techniques. In part, avenues of inquiry have been motivated by theoretical developments, and in part new theoretical frameworks have been conceived to account for unanticipated experimental observations. An overall qualitative understanding of the nature of the superconducting state itself has been achieved, while profound unresolved issues have come into increasingly sharp focus concerning the astonishing complexity of the phase diagram, the unprecedented prominence of various forms of collective fluctuations, and the simplicity and insensitivity to material details of the "normal" state at elevated temperatures. New conceptual approaches, drawing from string theory, quantum information theory, and various numerically implemented approximate approaches to problems of strong correlations are being explored as ways to come to grips with this rich tableaux of interrelated phenomena.

cond-mat.supr-con

Holographic description of strongly correlated electrons in external magnetic fields

We study the Fermi level structure of (2+1)-dimensional strongly interacting electron systems in external magnetic field using the AdS/CFT correspondence. The gravity dual of a finite density fermion system is a Dirac field in the background of the dyonic AdS-Reissner-Nordstrom black hole. In the probe limit the magnetic system can be reduced to the non-magnetic one, with Landau-quantized momenta and rescaled thermodynamical variables. We find that at strong enough magnetic fields, the Fermi surface vanishes and the quasiparticle is lost either through a crossover to conformal regime or through a phase transition to an unstable Fermi surface. In the latter case, the vanishing Fermi velocity at the critical magnetic field triggers the non-Fermi liquid regime with unstable quasiparticles and a change in transport properties of the system. We associate it with a metal-"strange metal" phase transition. We compute the DC Hall and longitudinal conductivities using the gravity-dressed fermion propagators. As expected, the Hall conductivity is quantized according to integer Quantum Hall Effect (QHE) at weak magnetic fields. At strong magnetic fields, new plateaus typical for the fractional QHE appear. Our pattern closely resembles the experimental results on graphite which are described using the fractional filling factor proposed by Halperin.

hep-th

Type-II Bose-Mott insulators

The Mott insulating state formed from bosons is ubiquitous in solid He-4, cold atom systems, Josephson junction networks and perhaps underdoped high-Tc superconductors. We predict that close to the quantum phase transition to the superconducting state the Mott insulator is not at all as featureless as is commonly believed. In three dimensions there is a phase transition to a low temperature state where, under influence of an external current, a superconducting state consisting of a regular array of 'wires' that each carry a quantized flux of supercurrent is realized. This prediction of the "type-II Mott insulator" follows from a field theoretical weak-strong duality, showing that this 'current lattice' is the dual of the famous Abrikosov lattice of magnetic fluxes in normal superconductors. We argue that this can be exploited to investigate experimentally whether preformed Cooper pairs exist in high-Tc superconductors.

cond-mat.str-el

Holographic fermions in external magnetic fields

We study the Fermi level structure of 2+1-dimensional strongly interacting electron systems in external magnetic field using the AdS/CFT correspondence. The gravity dual of a finite density fermion system is a Dirac field in the background of the dyonic AdS-Reissner-Nordstrom black hole. In the probe limit the magnetic system can be reduced to the non-magnetic one, with Landau-quantized momenta and rescaled thermodynamical variables. We find that at strong enough magnetic fields, the Fermi surface vanishes and the quasiparticle is lost either through a crossover to conformal regime or through a phase transition to an unstable Fermi surface. In the latter case, the vanishing Fermi velocity at the critical magnetic field triggers the non-Fermi liquid regime with unstable quasiparticles and a change in transport properties of the system. We associate it with a metal-"strange metal" phase transition. Next we compute the DC Hall and longitudinal conductivities using the gravity-dressed fermion propagators. For dual fermions with a large charge, many different Fermi surfaces contribute and the Hall conductivity is quantized as expected for integer Quantum Hall Effect (QHE). At strong magnetic fields, as additional Fermi surfaces open up, new plateaus typical for the fractional QHE appear. The somewhat irregular pattern in the length of fractional QHE plateaus resemble the outcomes of experiments on thin graphite in a strong magnetic field. Finally, motivated by the absence of the sign problem in holography, we suggest a lattice approach to the AdS calculations of finite density systems.

hep-th

The emergence of gauge invariance: the stay-at-home gauge versus local-global duality

In condensed matter physics gauge symmetries other than the U(1) of electromagnetism are of an emergent nature. Two emergence mechanisms for gauge symmetry are well established: the way these arise in Kramers-Wannier type local-global dualities, and as a way to encode local constraints encountered in (doped) Mott insulators. We demonstrate that these gauge structures are closely related, and appear as counterparts in either the canonical or field-theoretical language. The restoration of symmetry in a disorder phase transition is due to having the original local variables subjected to a coherent superposition of all possible topological defect configurations, with the effect that correlation functions are no longer well-defined. This is completely equivalent to assigning gauge freedom to those variables. Two cases are considered explicitly: the well-known vortex duality in bosonic Mott insulators serves to illustrate the principle. The acquired wisdoms are then applied to the less familiar context of dualities in quantum elasticity, where we elucidate the relation between the quantum nematic and linearized gravity. We reflect on some deeper implications for the emergence of gauge symmetry in general.

cond-mat.str-el