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J. van Tilborg

Publications and source records attributed to J. van Tilborg.

At least 19 recordsLinked to original sources
arXiv2026

Experimental demonstration of Flying-Focus enhanced Thomson scattering

We report the experimental demonstration of a spatiotemporally engineered "Flying-Focus" laser pulse for enhanced x-ray generation in relativistic Thomson scattering. A combination of longitudinal chromatic aberration, angular dispersion, and group delay dispersion was applied to an ultrashort relativistically intense laser pulse to control the motion of its focal point. Precise tuning of the group delay dispersion was used to match the velocity of the focus to the trajectory of a counterpropagating electron bunch, produced by a laser wakefield accelerator. This prolonged the Thomson scattering interaction while reducing nonlinear effects, leading to an enhanced x-ray yield. The approach has the potential to increase the spectral density and brightness of the x-ray beam by orders of magnitude compared to equivalent focusing without spatiotemporal control. This experiment establishes a new technique for structured-light control at high intensity, demonstrating the realization of dynamic intensity structures that enhance light-matter interactions and for the generation of ultra-bright radiation sources.

physics.optics↗
arXiv2026

Revealing Laser and Electron Beam Evolution in 10-GeV-class Laser-Plasma Accelerators

Guiding relativistically intense laser pulses in low-density plasmas enables extended acceleration lengths in laser-plasma accelerators (LPAs), allowing for the production of multi-GeV electron beams. Quantitative interpretation of such experiments is often limited by substantial uncertainties in key plasma parameters, particularly the transverse density profile of hydrodynamic optically field-ionized channels. Distinct plasma density distributions can produce similar terminal beam energies, complicating efforts to infer the underlying interaction physics from measurements at the accelerator exit alone. By combining longitudinally resolved electron beam diagnostics with independent measurements of laser spectral evolution in a 10 GeV LPA, we establish a multi-observable constraint on plasma density profiles. Once plasma downramps are taken into account, excellent agreement is observed with simulation over the entire accelerator length for two plasma channel sizes. The validated simulations indicate that extending the accelerator length to 65 cm would increase the electron beam energy to 15 GeV. They also point the way to achieving $\sim$20 GeV electron beams in $\sim$70 cm via linear matching using the same 24 J laser energy.

physics.acc-ph↗
arXiv2025

Bayesian Optimization of Laser-Wakefield Acceleration via Spectral Pulse Shaping

In this paper, we investigate the effect of spectral pulse shaping of the laser driver on the performance of channel-guided, laser-plasma accelerators. The study was carried out with the assistance of Bayesian optimization using particle-in-cell simulations. We used a realistic plasma profile based on a novel optical-field-ionized channel technique with ionization injection and low on-axis plasma densities to maximize the energy gain of the electron bunch trailing the laser. Spectral shaping allows us to modify the temporal profile of the laser driver while keeping the laser energy constant, affecting the acceleration and injection processes. Given the complexity and breadth of the parameter space in question, we used numerical optimization to identify high performers. In particular, we found laser profiles with additional spectral content that, when used with optimal plasma channel parameters, result in charge content an order of magnitude higher than the baseline Gaussian case while also increasing the mean energy of the electron bunch.

physics.plasm-ph↗
arXiv2025

Stability and optical quality of "windmill"-formed 8CB liquid crystal films for replenishable plasma mirrors

Liquid crystal (LC) film plasma mirrors (PMs) based on 4-octyl-4'-cyanobiphenyl (8CB) are an enabling technology for reflecting high-fluence laser pulses. These freestanding LC films can achieve high optical quality and are well-suited for rep-rated applications, as motorized devices continuously replenish films over an aperture following each destructive laser shot. However, a systematic characterization of film quality as a function of seminal operating conditions had not yet been performed for the LC "windmill" version of the device, which aims to match the repetition rate of an existing "spinning disk" (SDI) version and the angular stability of the "linear slider" (LSTI) version. We determined the 8CB film quality using low-power wavefront measurements, and studied the film-to-film wavefront stability and formation reliability. The film-formation reliability of 8CB LC films demonstrated >97% formation success at 2.7 mm/s film-forming speeds, but decreased to 45% at 10.8 mm/s. These reliability numbers will inform future designs to reach Hz-level repetition rates and beyond. Depending on area-of-interest within the 10 mm diameter film, the added wavefront root-mean-squared (RMS) variation was as small as 12 nm for a 2 mm diameter region, and <50 nm for a 3 mm diameter region. Within the optimal 21-22 degrees C operating regime, pointing fluctuations remained at or below 0.5 mrad. With a maximum effective film formation frequency of approximately 0.25 Hz, these results establish windmill-formed 8CB films as promising candidates to pursue next-iteration improvements towards rep-rated plasma-mirror operation.

physics.optics↗
arXiv2024

Longitudinal tapering in meter-scale gas jets for increased efficiency of laser plasma accelerators

Modern laser plasma accelerators (LPAs) often require plasma waveguides tens of cm long to propagate a high-intensity drive laser pulse. Tapering the longitudinal gas density profile in 10 cm scale gas jets could allow for single stage laser plasma acceleration well beyond 10 GeV with current petawatt-class laser systems. Via simulation and interferometry measurements, we show density control by longitudinally adjusting the throat width and jet angle. Density profiles appropriate for tapering were calculated analytically and via particle-in-cell (PIC) simulations, and were matched experimentally. These simulations show that tapering can increase electron beam energy using 19 J laser energy from ~9 GeV to >12 GeV in a 30 cm plasma, and the accelerated charge by an order of magnitude. This paper was published in Review of Scientific Instruments on April 11, 2025 DOI: https://doi.org/10.1063/5.0250698

physics.acc-ph↗
arXiv2024

Modeling and Design of Compact, Permanent-Magnet Transport Systems for Highly Divergent, Broad Energy Spread Laser-Driven Proton Beams

Laser-driven (LD) ion acceleration has been explored in a newly constructed short focal length beamline at the BELLA petawatt facility (interaction point 2, iP2). For applications utilizing such LD ion beams, a beam transport system is required, which for reasons of compactness be ideally contained within 3 m. While they are generated from a micron-scale source, large divergence and energy spread of LD ion beams present a unique challenge to transporting them compared to beams from conventional accelerators. This study gives an overview of proposed compact transport designs using permanent magnets satisfying different requirements depending on the application for the iP2 proton beamline such as radiation biology, material science, and high energy density science. These designs are optimized for different parameters such as energy spread and peak proton density according to the application's need. The various designs consist solely of permanent magnet elements, which can provide high magnetic field gradients on a small footprint. While the field strengths are fixed, we have shown that the beam size is able to be tuned effectively by varying the placement of the magnets. The performance of each design was evaluated based on high order particle tracking simulations of typical LD proton beams. We also examine the ability of certain configurations to tune and select beam energies, critical for specific applications. A more detailed investigation was carried out for a design to deliver 10 MeV LD accelerated ions for radiation biology applications. With these transport system designs, the iP2 beamline is ready to house various application experiments.

physics.acc-ph↗
arXiv2024

Matched Guiding and Controlled Injection in Dark-Current-Free, 10-GeV-Class, Channel-Guided Laser Plasma Accelerators

We measure the high intensity laser propagation throughout meter-scale, channel-guided LPAs by adjusting the length of the plasma channel on a shot-by-shot basis, showing high quality guiding of 500 TW laser pulses over 30 cm in a hydrogen plasma of density $n_0 \approx 1 \times 10^{17} \, \mathrm{cm^{-3}}$. We observed transverse energy transport of higher-order modes in the first $\approx 12 \, \mathrm{cm}$ of the plasma channel, followed by quasi-matched propagation, and the gradual, dark-current-free depletion of laser energy to the wakefield. We quantify the laser-to-wake transfer efficiency limitations of currently available PW-class laser systems, and demonstrate via simulation how control over the laser mode can significantly improve accelerated beam parameters. Using just 21.3 J of laser energy, and triggering localized electron injection into the accelerator, we observed electron bunches with single, quasimonoenergetic peaks, relative energy spreads as low as 3 % and energy up to 9.2 GeV with charge extending beyond 10 GeV.

physics.plasm-ph↗
arXiv2024

The Next Generation of MeV Energy X-ray Sources for use in the Inspection of Additively Manufactured Parts for Industry

For the first time, we demonstrate the application of an inverse Compton scattering X-ray Source, driven by a laser-plasma accelerator, to image an additively manufactured component. X-rays with a mean energy of 380 keV were produced and used to image an additively manufactured part made of an Inconel (Nickel 718) alloy. Because inverse Compton scattering driven by laser-plasma acceleration produces high-energy X-rays while maintaining a focal spot size on the order of a micron, the source can provide several benefits over conventional X-ray production methods, particularly when imaging superalloy parts, with the potential to revolutionise what can be inspected.

physics.acc-ph↗
arXiv2022

Strong-Field QED Experiments using the BELLA PW Laser Dual Beamlines

The Petawatt (PW) laser facility of the Berkeley Lab Laser Accelerator (BELLA) Center has recently commissioned its second laser pulse transport line. This new beamline can be operated in parallel with the first beamline and enables strong-field quantum electrodynamics (SF-QED) experiments at BELLA. In this paper, we present an overview of the upgraded BELLA PW facility with a SF-QED experimental layout in which intense laser pulses collide with GeV-class laser-wakefield-accelerated electron beams. We present simulation results showing that experiments will allow the study of laser-particle interactions from the classical to the SF-QED regime with a nonlinear quantum parameter of up to $χ\sim$2. In addition, we show that experiments will enable the study and production of GeV-class, mrad-divergence positron beams via the Breit-Wheeler process.

physics.acc-ph↗
arXiv2022

Carbon nanotube substrates enhance SARS-CoV-2 spike protein ion yields in matrix assisted laser desorption-ionization mass spectrometry

Nanostructured surfaces enhance ion yields in matrix assisted laser desorption-ionization mass spectrometry (MALDI-MS). The spike protein complex, S1, is one fingerprint signature of Sars-CoV-2 with a mass of 75 kDa. Here, we show that MALDI-MS yields of Sars-CoV-2 spike protein ions in the 100 kDa range are enhanced 50-fold when the matrix-analyte solution is placed on substrates that are coated with a dense forest of multi-walled carbon nanotubes, compared to yields from uncoated substrates. Nanostructured substrates can support the development of mass spectrometry techniques for sensitive pathogen detection and environmental monitoring.

physics.bio-ph↗
arXiv2022

Whitepaper submitted to Snowmass21: Advanced accelerator linear collider demonstration facility at intermediate energy

It is widely accepted that the next lepton collider beyond a Higgs factory would require center-of-mass energy of the order of up to 15 TeV. Since, given reasonable space and cost restrictions, conventional accelerator technology reaches its limits near this energy, high-gradient advanced acceleration concepts are attractive. Advanced and novel accelerators (ANAs) are leading candidates due to their ability to produce acceleration gradients on the order of 1--100~GV/m, leading to compact acceleration structures. Over the last 10-15 years significant progress has been achieved in accelerating electron beams by ANAs. For example, the demonstration of several-GeV electron beams from laser-powered capillary discharge waveguides, as well as the proof-of-principle coupling of two accelerating structures powered by different laser pulses, has increased interest in ANAs as a viable technology to be considered for a compact, TeV-class, lepton linear collider. However, intermediate facilities are required to test the technology and demonstrate key subsystems. A 20-100 GeV center-of-mass energy ANA-based lepton collider can be a possible candidate for an intermediate facility. Apart from being a test beam facility for accelerator and detector studies, this collider will provide opportunities to study muon and proton beam acceleration, investigate charged particle interactions with extreme electromagnetic fields (relevant for beam delivery system designs and to study the physics at the interaction point), as well as precision Quantum Chromodynamics and Beyond the Standard Model physics measurements. Possible applications of this collider include the studies of $γγ$ and $e$-ion collider designs.

physics.acc-ph↗
arXiv2021

Radial Density Profile and Stability of Capillary Discharge Plasma Waveguides of Lengths up to 40 Centimeters

We measured the parameter reproducibility and radial electron density profile of capillary discharge waveguides with diameters of 650 um to 2 mm and lengths of 9 to 40 cm. To our knowledge, 40 cm is the longest discharge capillary plasma waveguide to date. This length is important for >= 10 GeV electron energy gain in a single laser driven plasma wakefield acceleration (LPA) stage. Evaluation of waveguide parameter variations showed that their focusing strength was stable and reproducible to <0.2% and their average on-axis plasma electron density to <1%. These variations explain only a small fraction of LPA electron bunch variations observed in experiments to date. Measurements of laser pulse centroid oscillations revealed that the radial channel profile rises faster than parabolic and are in excellent agreement with magneto-hydro-dynamic simulation results. We show that the effects of non-parabolic contributions on Gaussian pulse propagation were negligible when the pulse was approximately matched to the channel. However, they affected pulse propagation for a non-matched configuration in which the waveguide was used as a plasma telescope to change the focused laser pulse spot size.

physics.plasm-ph↗
arXiv2018

Direct Measurement of Focusing Fields in Active Plasma Lenses

Active plasma lenses have the potential to enable broad-ranging applications of plasma-based accelerators owing to their compact design and radially symmetric kT/m-level focusing fields, facilitating beam-quality preservation and compact beam transport. We report on the direct measurement of magnetic field gradients in active plasma lenses and demonstrate their impact on the emittance of a charged particle beam. This is made possible by the use of a well-characterized electron beam with 1.4 mm mrad normalized emittance from a conventional accelerator. Field gradients of up to 823 T/m are investigated. The observed emittance evolution is supported by numerical simulations, which suggest the potential for conservation of the core beam emittance in such a plasma lens setup.

physics.acc-ph↗
arXiv2017

On production and asymmetric focusing of flat electron beams using rectangular capillary discharge plasmas

A method for the asymmetric focusing of electron bunches, based on the active plasma lensing technique is proposed. This method takes advantage of the strong inhomogeneous magnetic field generated inside the capillary discharge plasma to focus the ultrarelativistic electrons. The plasma and magnetic field parameters inside the capillary discharge are described theoretically and modeled with dissipative magnetohydrodynamic computer simulations enabling analysis of the capillaries of rectangle cross-sections. Large aspect ratio rectangular capillaries might be used to transport electron beams with high emittance asymmetries, as well as assist in forming spatially flat electron bunches for final focusing before the interaction point.

physics.plasm-ph↗
arXiv2014

Watching the acetylene vinylidene intramolecular reaction in real time

It is a long-standing dream of scientists to capture the ultra-fast dynamics of molecular or chemical reactions in real time and to make a molecular movie. With free-electron lasers delivering extreme ultraviolet (XUV) light at unprecedented intensities, in combination with pump-probe schemes, it is now possible to visualize structural changes on the femtosecond time scale in photo-excited molecules. In hydrocarbons the absorption of a single photon may trigger the migration of a hydrogen atom within the molecule. Here, such a reaction was filmed in acetylene molecules (C2H2) showing a partial migration of one of the protons along the carbon backbone which is consistent with dynamics calculations on ab initio potential energy surfaces. Our approach opens attractive perspectives and potential applications for a large variety of XUV-induced ultra-fast phenomena in molecules relevant to physics, chemistry, and biology.

physics.atm-clus↗
arXiv2011

Ultrafast Internal Conversion in Ethylene I. The Excited State Lifetime

Using a combined theoretical and experimental approach, we investigate the non-adiabatic dynamics of the prototypical ethylene (C2H4) molecule upon π \to π* excitation. In this first part of a two part series, we focus on the lifetime of the excited electronic state. The femtosecond Time-Resolved Photoelectron Spectrum (TRPES) of ethylene is simulated based on our recent molecular dynamics simulation using the ab initio multiple spawning method (AIMS) with Multi-State Second Order Perturbation Theory (Tao, et al. J. Phys. Chem. A 113 13656 2009). We find excellent agreement between the TRPES calculation and the photoion signal observed in a pump-probe experiment using femtosecond vacuum ultraviolet (hν = 7.7 eV) pulses for both pump and probe. These results explain the apparent discrepancy over the excited state lifetime between theory and experiment that has existed for ten years, with experiments (e.g., Farmanara, et al. Chem. Phys. Lett. 288 518 1998 and Kosma, et al. J. Phys. Chem. A 112 7514 2008) reporting much shorter lifetimes than predicted by theory. Investigation of the TRPES indicates that the fast decay of the photoion yield originates from both energetic and electronic factors, with the energetic factor playing a larger role in shaping the signal.

physics.chem-ph↗
arXiv2011

Ultrafast Internal Conversion in Ethylene. II. Mechanisms and Pathways for Quenching and Hydrogen Elimination

Through a combined experimental and theoretical approach, we study the nonadiabatic dynamics of the prototypical ethylene (C$_2$H$_4$) molecule upon $π\rightarrow π^*$ excitation with 161 nm light. Using a novel experimental apparatus, we combine femtosecond pulses of vacuum ultraviolet (VUV) and extreme ultraviolet (XUV) radiation with variable delay to perform time resolved photo-ion fragment spectroscopy. In this second part of a two part series, the extreme ultraviolet (17 eV$ < h ν< 23$ eV) probe pulses are sufficiently energetic to break the C-C bond in photoionization, or photoionize the dissociation products of the vibrationally hot ground state. The experimental data is directly compared to ab initio molecular dynamics simulations accounting for both the pump and probe steps. Enhancements of the CH$_2^+$ and CH$_3^+$ photoion fragment yields, corresponding to molecules photoionized in ethylene (CH$_2$CH$_2$) and ethylidene (CH$_3$CH) like geometries are observed within 100 fs after $π\rightarrow π^*$ excitation. Quantitative agreement between theory and experiment on the relative CH$_2^+$ and CH$_3^+$ yields provides experimental confirmation of the theoretical prediction of two distinct transition states and their branching ratio (Tao, et al. J. Phys. Chem. A. 113, 13656 (2009)). Fast, non-statistical, elimination of H$_2$ molecules and H atoms is observed in the time resolved H$_2^+$ and H$^+$ signals.

physics.chem-ph↗