arXiv subjects

Jacek Szczytko

Publications and source records attributed to Jacek Szczytko.

At least 19 recordsLinked to original sources

arXiv2026

Discrete chiral ballistic polariton laser

Orbital angular momentum (OAM) of light appears when the phase of an electromagnetic wavefront winds around its direction of propagation, also known as optical vorticity. Contrary to the binary-valued photon spin, the integer-valued optical vortex charge is unbounded with many advantages in optical communication and trapping and enhancing the capacity of data encoding and multiplexing. Singular optoelectronic and chiroptic quantum technologies rely on the development of coherent and compact light sources of well-defined and reconfigurable OAM. We propose an optically tunable discrete chiral exciton-polariton microlaser that leverages strong spin-dependent polariton interactions, structured pumping, and inherent cavity photon spin-to-angular momentum conversion to emit coherent nonlinear light of variable OAM. By choosing pumping patterns with broken inversion symmetry in the microcavity plane we invoke geometric frustration between spinor ballistic condensates which spontaneously obtain a high-charge circulating current locked with the pump polarization. Our optically configurable system requires only a planar cavity thus avoiding the need for specialized irreversible cavity patterning or metasurfaces.

cond-mat.mes-hall↗

arXiv2026

Engineering Tunable Synthetic Su-Schrieffer-Heeger Chains in Liquid Crystal Microcavities

Optical microcavities have emerged as a powerful platform for emulating topological phases challenging to realize in conventional materials, offering precise control over dispersion, light confinement, and interactions. Among them, liquid crystal microcavities (LCMCs) offer exceptional tunability at room temperature, enabling voltage-controlled polarisation splitting, photonic spin-orbit coupling, and photonic potentials generated by self-assembled textures, such as cholesteric torons and uniform lying helix (ULH). Here, we design a LCMC hosting a dimerized ULH texture and show that the corresponding photonic potential describes two coupled Su-Schrieffer-Heeger chains with orthogonal linear polarisations, acting as an effective pseudospin degree of freedom. The applied voltage tunes the interchain coupling, enabling polarisation-dependent interactions. These results establish LCMCs as a versatile platform for tunable synthetic topological Hamiltonians.

physics.optics↗

arXiv2026

Electrically reconfigurable extended lasing state in an organic liquid-crystal microcavity

Small-footprint, low-power arrays of coupled coherent emitters with the capability of near- and far-field engineering and coherence control are highly sought after to meet modern nanophotonics evolving needs. Between existing solutions based on vertical-cavity surface-emitting lasers, phase masks in bulk traditional cavity-based systems, and lattices of exciton-polariton condensates, only the strongly light-matter coupled systems were shown to be capable of controlled on-chip interaction between the individual coherent states while often operating at cryogenic temperatures. Here we demonstrate electrically controlled in-plane interaction between optically reconfigurable spatially separated lasing states, operating at room temperature in the weak light-matter coupling regime. We show spatially extended coherent lasing state or "supermode" with wide-range micro-scale control of near-field, far-field and on-chip phase-locking tuning functionality. An extended lasing state appears due to near-field transverse coupling between distinct spatially pumped lasing states in the plane of an organic liquid crystal-filled microcavity. We realize electrical control over the interaction strength between lasing states and corresponding mutual coherence going beyond nearest neighbours through electrical tuning of the microcavity optical modes with external voltage, and a spin-selective directional coupling regime by using a photonic analogue of the Rashba-Dresselhaus spin-orbit interaction.

cond-mat.mes-hall↗

arXiv2025

Kibble-Zurek mechanism in a polariton supersolid

We study the formation of topological defects via the Kibble-Zurek mechanism in a polariton supersolid in a liquid crystal microcavity with tunable Rashba-Dresselhaus spin-orbit coupling. We predict analytically two different scalings in the slow- and fast-quench regimes, and confirm these predictions numerically. We also present experimental results for the slow-quench regime, demonstrating an original Kibble-Zurek scaling exponent $η_{KZM}=1.0\pm 0.2$

cond-mat.mes-hall↗

arXiv2025

Observation of a supersolid phase in a spin-orbit coupled exciton-polariton Bose-Einstein condensate at room temperature

In Bose-Einstein condensates (BEC), spin-orbit coupling (SOC) produces supersolidity. It is a peculiar state of matter, which, in addition to the superfluid behaviour shows periodic density modulation typical for crystals. Here, we report the fabrication of a new type of optical microcavity allowing to achieve room-temperature supersolidity for a quantum fluid of light. The microcavity is filled with a nematic liquid crystal (LC) and two layers of the organic polymer MeLPPP hosting exciton resonances. We demonstrate exciton-polariton condensation in the two distinct degenerate minima of the dispersion created by the LC induced Rashba-Dresselhaus (RD) SOC. The condensate real-space distribution shows density stripes located randomly from one condensate realization to another despite the presence of a random disorder potential. This demonstrates the immunity of stripes against disorder (that is, superfluidity) and the spontaneous breaking of translational invariance. We also report the random appearance of vortices via the Kibble-Zurek mechanism, another smoking gun of superfluidity.

cond-mat.mes-hall↗

arXiv2025

Multiplexed back focal plane imaging with on-chip integrated microlens array

On-chip optical architectures that enable angle-resolved spectroscopy are essential for advancing photonic platforms towards low-volume, scalable, and cryo-compatible devices. Here, we introduce spatially resolved momentum-space imaging using arrays of 3D-printed microlenses directly integrated onto semiconductor optical microcavities. Each microlens functions as an independent optical element with a high numerical aperture (approx. 0.95), enabling parallel back focal plane imaging across, in our implementation, 64 distinct locations. This approach eliminates the need for bulky microscope objectives while maintaining broad wavevector access, even under cryogenic conditions. We demonstrate its versatility across various cavity systems, including dielectric planar resonators, GaAs-based polariton microcavities, and CdTe platforms supporting nonequilibrium Bose-Einstein condensation of exciton-polaritons. The microlenses not only enhance collection efficiency but also enable tightly focused excitation, yielding an order of magnitude reduction in condensation thresholds compared with conventional setups. Our results establish 3D-printed microlens arrays as a compact, versatile, integrated platform for next-generation angle-resolved spectroscopy in nanophotonics and quantum materials.

physics.optics↗

arXiv2025

Electrically tunable momentum space polarization singularities in liquid crystal microcavities

Momentum space polarization singularities of light appear as vectorial twists in the scattered and radiated far field patterns of exotic photonic structures. They relate to important concepts such as bound states in the continuum, spatiotemporal light steering, polarization Möbius strips, Berry curvature and associated topological photonic phenomena. Polarization singularities, such as completely circularly polarized C-points, are readily designed in real space through interference of differently polarized beams. In momentum space, they require instead sophisticated patterning of photonic crystal slabs of reduced symmetries in order to appear in the corresponding band structure with scarce in-situ tunability. Here, we show that momentum space singularities can be generated and, importantly, electrically tuned in the band structure of a highly birefringent planar liquid crystal microcavity that retains many symmetries. Our results agree with theoretical predictions and offer exciting possibilities for integration of momentum space polarization singularities in spinoptronic technologies.

physics.optics↗

arXiv2024

Non-Hermitian polariton-photon coupling in a perovskite open microcavity

Exploring the non-Hermitian properties of semiconductor materials for optical applications is at the forefront of photonic research. However, the selection of appropriate systems to implement such photonic devices remains a topic of debate. In this work, we demonstrate that a perovskite crystal, characterized by its easy and low-cost manufacturing, when placed between two distributed Bragg reflectors with an air gap, can form a natural double microcavity. This construction shows promising properties for the realisation of novel, tunable non-Hermitian photonic devices through strong light-matter coupling. We reveal that such a system exhibits double-coupled polariton modes with dispersion including multiple inflection points. Owing to its non-Hermiticity, our system exhibits nonreciprocal properties and allows for the observation of exceptional points. Our experimental studies are in agreement with the theoretical analysis based on coupled mode theory and calculations based on transfer matrix method.

cond-mat.mes-hall↗

arXiv2024

In-situ tunneling control in photonic potentials by Rashba-Dresselhaus spin-orbit coupling

The tunability of individual coupling amplitudes in photonic lattices is highly desirable for photonic Hamiltonian engineering and for studying topological transitions in situ. In this work, we demonstrate the tunneling control between individual lattice sites patterned inside an optical microcavity. The tuning is achieved by applying a voltage to a liquid crystal microcavity possessing photonic Rashba-Dresselhaus spin-orbit coupling. This type of spin-orbit coupling emerges due to the high birefringence of the liquid crystal material and constitutes an artificial gauge field for photons. The proposed technique can be combined with strong-light matter coupling and non-Hermitian physics already established in liquid crystal microcavities.

physics.optics↗

arXiv2024

Magneto-optical induced supermode switching in quantum fluids of light

The insensitivity of photons towards external magnetic fields forms one of the hardest barriers against efficient magneto-optical control, aiming at modulating the polarization state of light. However, there is even scarcer evidence of magneto-optical effects that can spatially modulate light. Here, we demonstrate the latter by exploiting strongly coupled states of semimagnetic matter and light in planar semiconductor microcavities. We nonresonantly excite two spatially adjacent exciton-polariton condensates which, through inherent ballistic near field coupling mechanism, spontaneously synchronise into a dissipative quantum fluidic supermode of definite parity. Applying a magnetic field along the optical axis, we continuously adjust the light-matter composition of the condensate exciton-polaritons, inducing a supermode switch into a higher order mode of opposite parity. Our findings set the ground towards magnetic spatial modulation of nonlinear light.

cond-mat.mes-hall↗

arXiv2024

Direct Optical Probing of the Magnetic Properties of the Layered Antiferromagnet CrPS$_4$

Unusual magnetic properties of Van der Waals type antiferromagnetic semiconductors make them highly attractive for spintronics and optoelectronics. A link between the magnetic and optical properties of those materials, required for practical applications, has not been, however, established so far. Here, we report on a combined experimental and theoretical study of magnetic, optical, and structural properties of bulk CrPS$_{4}$ samples. We find that the magnetic-field-dependent circular polarization degree of the photoluminescence is a direct measure of the net magnetization of CrPS$_{4}$. Complementary, Raman scattering measured as a function of magnetic field and temperature enables the determination of the magnetic susceptibility curve of the material. Our experimental results are backed by Our experimental results are supported by density functional theory calculations that take as input the lattice parameters determined from temperature-dependent X-ray diffraction measurements. This allows us to explain the impact of spin ordering on the spectral position of Raman transitions in CrPS$_4$, as well as anomalous temperature shifts of selected of them. The presented method for all-optical determination of the magnetic properties is highly promising for studies of spin ordering and magnetic phase transitions in single- or a few-layer samples of magnetic layered materials, for which a poor signal-to-noise ratio precludes any reliable neutron scattering or magnetometry measurements.

cond-mat.mtrl-sci↗

arXiv2024

Electrically tunable spin-orbit coupled photonic lattice in a liquid crystal microcavity

We create a one-dimensional photonic crystal with strong polarization dependence and tunable by an applied electric field. We accomplish this in a planar microcavity by embedding a cholesteric liquid crystal (LC), which spontaneously forms a uniform lying helix (ULH). The applied voltage controls the orientation of the LC molecules and, consequently, the strength of a polarization-dependent periodic potential. It leads to opening or closing of photonic band gaps in the dispersion of the massive photons in the microcavity. In addition, when the ULH structure possesses a molecular tilt, it induces a spin-orbit coupling between the lattice bands of different parity. This interband spin-orbit coupling (ISOC) is analogous to optical activity and can be treated as a synthetic non-Abelian gauge potential. Finally, we show that doping the LC with dyes allows us to achieve lasing that inherits all the above-mentioned tunable properties of LC microcavity, including dual and circularly-polarized lasing.

physics.optics↗

arXiv2023

Erbium-based multifuncional compounds as molecular microkelvin-tunable driving-sensing units

We demonstrate the selective control of the magnetic response and photoluminescence properties of Er3+ centers with light, by associating them with a highly conjugated beta-diketonate (1,3-di(2-naphthyl)-1,3-propanedione) ligand. We demonstrate this system to be an optically-pumped molecular compound emittingin infra-red, which can be employed as a precise heat-driving and detecting unit for low temperatures

cond-mat.mtrl-sci↗

arXiv2023

Natural exceptional points in the excitation spectrum of a light-matter system

We observe natural exceptional points in the excitation spectrum of an exciton-polariton system by optically tuning the light-matter interactions. The observed exceptional points do not require any spatial or polarization degrees of freedom and result solely from the transition from weak to strong light-matter coupling. We demonstrate that they do not coincide with the threshold for photon lasing, confirming previous theoretical predictions [Phys. Rev. Lett. 122, 185301 (2019), Optica 7, 1015 (2020) ]. Using a technique where a strong coherent laser pump induces up-converted excitations, we encircle the exceptional point in the parameter space of coupling strength and particle momentum. Our method of local optical control of light-matter coupling paves the way to investigation of fundamental phenomena including dissipative phase transitions and non-Hermitian topological states.

physics.optics↗

arXiv2022

Training a neural network with exciton-polariton optical nonlinearity

In contrast to software simulations of neural networks, hardware implementations have often limited or no tunability. While such networks promise great improvements in terms of speed and energy efficiency, their performance is limited by the difficulty to apply efficient training. We propose and realize experimentally an optical system where highly efficient backpropagation training can be applied through an array of highly nonlinear, non-tunable nodes. The system includes exciton-polariton nodes realizing nonlinear activation functions. We demonstrate a high classification accuracy in the MNIST handwritten digit benchmark in a single hidden layer system.

cs.LG↗

arXiv2022

Control of dimer chain topology by Rashba-Dresselhaus spin-orbit coupling

We study theoretically a dimer chain in the presence of Rashba-Dresselhaus spin-orbit coupling (RDSOC) with equal strength. We show that the RDSOC can be described as a synthetic gauge field that controls not only the magnitude but also the sign of tunneling coefficients between sites. This allows to emulate not only a Su-Schrieffer-Heeger chain which is commonly implemented in various platforms, but also, all energy spectra of the transverse field Ising model with both ferromagnetic and antiferromagnetic coupling. We simulate a realistic implementation of these effective Hamiltonians based on liquid crystal microcavities. In that case, the RDSOC can be switched on and off by an applied voltage, which controls the band topology, the existence and characteristics of topological edge states, or the nature of the ground state. This setting is promising for topological photonics applications and from a quantum simulation perspective.

cond-mat.mes-hall↗

arXiv2022

Neural networks based on ultrafast time-delayed effects in exciton-polaritons

We demonstrate that time-delayed nonlinear effects in exciton-polaritons can be used to construct neural networks where information is coded in optical pulses arriving consecutively on the sample. The highly nonlinear effects are induced by time-dependent interactions with the excitonic reservoir. These nonlinearities allow to create a nonlinear XOR logic gate that can perform operations on the picosecond timescale. An optoelectronic neural network based on the constructed logic gate performs classification of spoken digits with a high accuracy rate.

physics.optics↗

arXiv2021

Lasing in the Rashba-Dresselhaus spin-orbit coupling regime in a dye-filled liquid crystal optical microcavity

In the presence of Rashba-Dresselhaus coupling, strong spin-orbit interactions in liquid crystal optical cavities result in a distinctive spin-split entangled dispersion. Spin coherence between such modes give rise to an optical persistent-spin-helix. In this letter, we introduce optical gain in such a system, by dispersing a molecular dye in a liquid-crystal microcavity. We demonstrate both lasing in the Rashba-Dresselhaus regime and the emergence of an optical persistent spin helix.

physics.optics↗