arXiv subjects

Jack Clarke

Publications and source records attributed to Jack Clarke.

11 recordsLinked to original sources

arXiv2026

Bell Test of Photons from Electron-Positron Annihilation via POVM-based Compton Polarimetry

Quantum entanglement between gamma-ray photons emitted following electron-positron annihilation is expected to be maximal and may be characterized via non-classical polarization correlations. However, this is difficult to verify experimentally because there are no established schemes that approach ideal projective-polarization measurements for high-energy photons. Hence, polarization entanglement between MeV-scale annihilation photons has not yet been conclusively demonstrated. We develop here a framework that models polarization measurements of high-energy photons via Compton polarimetry, employing the formalism of positive operator-valued measures (POVMs). We extend the POVM description to sequences of repeated interactions and show that the measurement converges toward an ideal projective measurement of linear polarization as the number of interactions increases. We demonstrate that this progressive improvement in measurement sharpness can enable the experimental violation of CHSH inequalities.

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arXiv2025

Deterministic Mechanical Wigner Negativity via Nonlinear Cavity Quantum Optomechanics in the Unresolved-Sideband Regime

Non-Gaussian quantum states of mechanical motion exhibiting Wigner negativity offer promising capabilities for quantum technologies and tests of fundamental physics. Within the field of cavity quantum optomechanics, deterministic preparation of nonclassical mechanical states with such Wigner negativity is a highly sought goal but is challenging as the intracavity interaction Hamiltonian is linear in mechanical position. Here, we show that, despite this form of interaction, by utilizing the nonlinearity of the cavity response with mechanical position, mechanical Wigner negativity can be prepared deterministically in the unresolved-sideband regime, without additional nonlinearities, nonclassical drives, or conditional measurements. In particular, we find that Wigner negativity can be prepared with an optical pulse, even without single-photon strong coupling, and the negativity persists in the steady state of a continuously driven system. Our results deepen our understanding of cavity-enhanced radiation pressure and establish a pathway for deterministic preparation of nonclassical mechanical states in the unresolved sideband regime.

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arXiv2025

Optimizing confidence in negative-partial-transpose-based entanglement criteria

A key requirement of any separable quantum state is that its density matrix has a positive partial transpose. For continuous bipartite quantum states, violation of this condition may be tested via the hierarchy of negative-partial-transpose (NPT) based entanglement criteria introduced by Shchukin and Vogel [Phys. Rev. Lett. 95, 230502 (2005)]. However, a procedure for selecting the optimal NPT-based criterion is currently lacking. Here, we develop a framework to select the optimal criterion by determining the level of confidence of criteria within the Shchukin and Vogel hierarchy for finite measurement number, environmental noise, and the optimal allocation of measurement resources. To demonstrate the utility of our approach, we apply our statistical framework to prominent example Gaussian and non-Gaussian states, including the two-mode squeezed vacuum state, the quanta-subtracted two-mode squeezed vacuum state, and the two-mode Schr\"odinger-cat state. Beyond bipartite inseparability tests, our framework can be applied to any Hermitian matrix constructed of observable moments and thus can be utilized for a wide variety of other nonclassicality criteria and multi-mode entanglement tests.

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arXiv2024

Theoretical framework for enhancing or enabling cooling of a mechanical resonator via the anti-Stokes or Stokes interaction and zero-photon detection

We develop a theoretical framework to describe how zero-photon detection may be utilized to enhance laser cooling via the anti-Stokes interaction and, somewhat surprisingly, enable cooling via the Stokes interaction commonly associated with heating. Our description includes both pulsed and continuous measurements as well as optical detection efficiency and open-system dynamics. For both cases, we discuss how the cooling depends on the system parameters such as detection efficiency and optomechanical cooperativity, and we study the continuous-measurement-induced dynamics, contrasting to single-photon detection events. For the Stokes case, we explore the interplay between cooling and heating via optomechanical parametric amplification, and we find the efficiency required to cool a mechanical oscillator via zero-photon detection. This work serves as a companion article to the recent experiment [E. A. Cryer-Jenkins, K. D. Major, et al., arXiv:2408.01734 (2024)], which demonstrated enhanced laser cooling of a mechanical oscillator via zero-photon detection on the anti-Stokes signal. The framework developed here provides new approaches for cooling mechanical resonators that can be applied to a wide range of areas including nonclassical state preparation, quantum thermodynamics, and avoiding the often unwanted heating effects of parametric amplification.

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arXiv2024

Enhanced Laser Cooling of a Mechanical Resonator via Zero-Photon Detection

Throughout quantum science and technology, measurement is used as a powerful resource for nonlinear operations and quantum state engineering. In particular, single-photon detection is commonly employed for quantum-information applications and tests of fundamental physics. By contrast, and perhaps counter-intuitively, measurement of the absence of photons also provides useful information, and offers significant potential for a wide range of new experimental directions. Here, we propose and experimentally demonstrate cooling of a mechanical resonator below its laser-cooled mechanical occupation via zero-photon detection on the anti-Stokes scattered optical field and verify this cooling through heterodyne measurements. Our measurements are well captured by a stochastic master equation and the techniques introduced here open new avenues for cooling, quantum thermodynamics, quantum state engineering, and quantum measurement and control.

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arXiv2022

Cavity quantum optomechanical nonlinearities and position measurement beyond the breakdown of the linearized approximation

Several optomechanics experiments are now entering the highly sought nonlinear regime where optomechanical interactions are large even for low light levels. Within this regime, new quantum phenomena and improved performance may be achieved, however, a corresponding theoretical formalism of cavity quantum optomechanics that captures the nonlinearities of both the radiation-pressure interaction and the cavity response is needed to unlock these capabilities. Here, we develop such a nonlinear cavity quantum optomechanical framework, which we then utilize to propose how position measurement can be performed beyond the breakdown of the linearized approximation. Our proposal utilizes optical general-dyne detection, ranging from single to dual homodyne, to obtain mechanical position information imprinted onto both the optical amplitude and phase quadratures and enables both pulsed and continuous modes of operation. These cavity optomechanical nonlinearities are now being confronted in a growing number of experiments, and our framework will allow a range of advances to be made in e.g. quantum metrology, explorations of the standard quantum limit, and quantum measurement and control.

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arXiv2022

Two-mode Schrödinger-cat states with nonlinear optomechanics: generation and verification of non-Gaussian mechanical entanglement

Cavity quantum optomechanics has emerged as a new platform for quantum science and technology with applications ranging from quantum-information processing to tests of the foundations of physics. Of crucial importance for optomechanics is the generation and verification of non-Gaussian states of motion and a key outstanding challenge is the observation of a canonical two-mode Schrödinger-cat state in the displacement of two mechanical oscillators. In this work, we introduce a pulsed approach that utilizes the nonlinearity of the radiation-pressure interaction combined with photon-counting measurements to generate this entangled non-Gaussian mechanical state, and, importantly, describe a protocol using subsequent pulsed interactions to verify the non-Gaussian entanglement generated. Our pulsed verification protocol allows quadrature moments of the two mechanical oscillators to be measured up to any finite order providing a toolset for experimental characterisation of bipartite mechanical quantum states and allowing a broad range of inseparability criteria to be evaluated. Key experimental factors, such as optical loss and open-system dynamics, are carefully analyzed and we show that the scheme is feasible with only minor improvements to current experiments that operate outside the resolved-sideband regime. Our scheme provides a new avenue for quantum experiments with entangled mechanical oscillators and offers significant potential for further research and development that utilizes such non-Gaussian states for quantum-information and sensing applications, and for studying the quantum-to-classical transition.

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arXiv2021

Can the displacemon device test objective collapse models?

Testing the limits of the applicability of quantum mechanics will deepen our understanding of the universe and may shed light on the interplay between quantum mechanics and gravity. At present there is a wide range of approaches for such macroscopic tests spanning from matter-wave interferometry of large molecules to precision measurements of heating rates in the motion of micro-scale cantilevers. The "displacemon" is a proposed electromechanical device consisting of a mechanical resonator flux-coupled to a superconducting qubit enabling generation and readout of mechanical quantum states. In the original proposal, the mechanical resonator was a carbon nanotube, containing $10^6$ nucleons. Here, in order to probe quantum mechanics at a more macroscopic scale, we propose using an aluminium mechanical resonator on two larger mass scales, one inspired by the Marshall-Simon-Penrose-Bouwmeester moving-mirror proposal, and one set by the Planck mass. For such a device, we examine the experimental requirements needed to perform a more macroscopic quantum test and thus feasibly detect the decoherence effects predicted by two objective collapse models: Diósi-Penrose and continuous spontaneous localization. Our protocol for testing these two theories takes advantage of the displacemon architecture to create non-Gaussian mechanical states out of equilibrium with their environment and then analyzing the measurement statistics of a superconducting qubit. We find that with improvements to the fabrication and vibration sensitivities of these electromechanical devices, the displacemon device provides a new route to feasibly test decoherence mechanisms beyond standard quantum theory.

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arXiv2021

Non-Gaussian mechanical motion via single and multi-phonon subtraction from a thermal state

Quantum optical measurement techniques offer a rich avenue for quantum control of mechanical oscillators via cavity optomechanics. In particular, a powerful yet little explored combination utilizes optical measurements to perform heralded non-Gaussian mechanical state preparation followed by tomography to determine the mechanical phase-space distribution. Here, we experimentally perform heralded single- and multi-phonon subtraction via photon counting to a laser-cooled mechanical thermal state with a Brillouin optomechanical system at room temperature, and use optical heterodyne detection to measure the $s$-parameterized Wigner distribution of the non-Gaussian mechanical states generated. The techniques developed here advance the state-of-the-art for optics-based tomography of mechanical states and will be useful for a broad range of applied and fundamental studies that utilize mechanical quantum-state engineering and tomography.

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arXiv2021

Preparation and Verification of Two-Mode Mechanical Entanglement Through Pulsed Optomechanical Measurements

We propose a protocol how to generate and verify bipartite Gaussian entanglement between two mechanical modes coupled to a single optical cavity, by means of short optical pulses and measurement. Our protocol requires neither the resolved sideband regime, nor low thermal phonon occupancy, and allows the generation and verification of quantum entanglement in less than a mechanical period of motion. Entanglement is generated via effective two-mode mechanical squeezing through conditioning position measurements. We study the robustness of entanglement to experimental deviations in mechanical frequencies and optomechanical coupling rates.

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arXiv2018

Growing macroscopic superposition states via cavity quantum optomechanics

The investigation of macroscopic quantum phenomena is a current active area of research that offers significant promise to advance the forefronts of both fundamental and applied quantum science. Utilizing the exquisite precision and control of quantum optics provides a powerful toolset for generating such quantum states where the types and 'size' of the states that can be generated are set by the resourcefulness of the protocol applied. In this work we present a new scheme for 'growing' macroscopic superposition states of motion of a mechanical oscillator via cavity quantum optomechanics. The scheme consists of a series of optical pulses interacting with a mechanical mode via radiation-pressure followed by photon-counting measurements. The multistep nature of our protocol allows macroscopic superposition states to be prepared with a relaxed requirement for the single-photon optomechanical coupling strength. To demonstrate the feasibility of our scheme, we quantify how initial mechanical thermal occupation and decoherence affects the non-classicality and macroscopicity of the states generated. We show that under realistic experimental conditions, mechanical quantum states can exhibit significant non-classicality and can be grown to a macroscopic scale.

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