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Jacqueline Bloch

Publications and source records attributed to Jacqueline Bloch.

At least 19 recordsLinked to original sources

Accessing Chern Numbers From Bloch Eigenstates Singularities

We propose two methods to extract the Chern numbers of the Bloch bands of a two dimensional insulator, and apply them to a photonic lattice experiment. These two methods require the knowledge of the complex-valued components of the Bloch eigenvectors, or their ratios. Unlike other tomography methods relying on the approximate reconstruction of the Berry curvature and its integration over the Brillouin zone, our methods boil down to the observation of phase vorticities in the eigensates structure. Those measurements, robust to experimental noise, yield exactly quantized values. One of the two methods exploits the non-normalization of the eigenmodes, making it particularly relevant for classical wave systems.

cond-mat.mes-hall

Emission of time-ordered photon pairs from a coherently-driven Kerr microcavity

Weakly-interacting many-body systems possess remarkable quantum properties that are essential components of quantum technologies, and constitute a topic of fundamental interest. Here we show that in a solid-state nonlinear microcavity embedding discrete modes of exciton-dressed photons, we can isolate a single eigenmode of quantum fluctuations from the much brighter coherent fraction of the field. In this regime, we perform frequency- and time-resolved correlations measurements between photons on the red and blue side of the fluctuations spectrum. When the average number of fluctuation quanta is smaller than one, we observe the formation of large pairwise time-ordered correlations: red photon first and blue photon second. We show that this peculiar time-ordering correlation emerges spontaneously from the interplay between frequency-resolved detection, and the non-trivial internal quantum structure of the elementary fluctuations.

cond-mat.quant-gas

Line lasing in a two-dimensional lattice of orbital photonic resonators

The engineering of specialty lasers with unconventional mode structures is one of the modern challenges in the development of integrated coherent sources. Examples include the use of bound states in the continuum, microlasers with orbital angular momentum, Dirac-band lasers and topological lasers. In this work we engineer a two-dimensional lattice of coupled micropillars with lasing line modes. We use a convenient combination of orbital photonic modes to design photonic bands which are flat in one direction and dispersive in the perpendicular one giving rise to line lasing modes. Such an architecture opens the possibility of implementing densely packed lasing matrices in compact two dimensional lattices.

physics.optics

Measuring non-Abelian quantum geometry and topology in a multi-gap photonic lattice

Recent discoveries in semi-metallic multi-gap systems featuring band singularities have galvanized enormous interest in particular due to the emergence of non-Abelian braiding properties of band nodes. This previously uncharted set of topological phases necessitates novel approaches to probe them in laboratories, a pursuit that intricately relates to evaluating non-Abelian generalizations of the Abelian quantum geometric tensor (QGT) that characterizes geometric responses. Here, we pioneer the direct measurement of the non-Abelian QGT. We achieve this by implementing a novel orbital-resolved polarimetry technique to probe the full Bloch Hamiltonian of a six-band two-dimensional (2D) synthetic lattice, which grants direct experimental access to non-Abelian quaternion charges, the Euler curvature, and the non-Abelian quantum metric associated with all bands. Quantum geometry has been highlighted to play a key role on macroscopic phenomena ranging from superconductivity in flat-bands, to optical responses, transport, metrology, and quantum Hall physics. Therefore, our work unlocks the experimental probing of a wide phenomenology of multi-gap systems, at the confluence of topology, geometry and non-Abelian physics.

cond-mat.mes-hall

All-optical nonlinear phase modulation in open semiconductor microcavities

We report a significant advancement in ultra low power light-by-light phase modulation using open semiconductor microcavities in the strong light-matter coupling regime. We achieve cross-phase modulation of up to 247$\pm$17 mrad per particle between laser beams attenuated to single-photon average intensities. This breakthrough extends the potential for quantum information processing and nonlinear quantum optics in strongly coupled light-matter systems, setting a new benchmark in the field without relying on atom-like emitters. Our findings suggest promising new avenues for scalable quantum optical technologies.

physics.optics

Phase diagram and universal scaling regimes of two-dimensional exciton-polariton Bose-Einstein condensates

Many systems, classical or quantum, closed or open, exhibit universal statistical properties. Exciton-polariton condensates, being intrinsically driven-dissipative, offer a promising platform for observing non-equilibrium universal features. By conducting extensive numerical simulations of an incoherently pumped and interacting condensate coupled to an exciton reservoir we show that the effective nonlinearity of the condensate phase dynamics can be finely adjusted across a broad range, by varying the exciton-polariton interaction strength, allowing one to probe three main universal regimes with parameters accessible in current experiments: the weakly nonlinear Edwards-Wilkinson (EW) regime, where the phase fluctuations dominate, but the phase profile does not become rough, the strongly non-linear Kardar-Parisi-Zhang regime, where the condensate phase fluctuations grow in a superdiffusive manner leading to roughening of the phase, and a vortex-dominated phase emerging at stronger interactions, where both density and phase dynamics play significant roles. Our results provide a unified picture of the phase diagram of 2d exciton-polariton condensates under incoherent pumping, and shed light on recent experimental and numerical observations.

cond-mat.quant-gas

A sublattice Stokes polarimeter for bipartite photonic lattices

The concept of pseudo-spin provides a general framework for describing physical systems featuring two-component spinors, including light polarization, sublattice degrees of freedom in bipartite lattices, and valley polarization in 2D materials. In all cases, the pseudo-spin can be mapped to a Stokes vector on the Poincaré sphere. Stokes polarimeters for measuring the polarization of light are a powerful tool with a wide range of applications both in classical and quantum science. Generalizing Stokes polarimetry to other spinor degrees of freedom is thus a challenge of prime importance. Here, we introduce and demonstrate a Stokes polarimeter for the sublattice polarization in a bipartite photonic lattice. Our method relies on k-space photoluminescence intensity measurements under controlled phase shifts and attenuations applied independently to each sublattice. We implement our method using honeycomb arrays of coupled microcavities realizing photonic analogs of graphene and hexagonal boron nitride. Using our sublattice polarimeter, we reconstruct the Bloch modes in amplitude and phase across the Brillouin zone, achieving sub-linewidth precision in the determination of their eigenenergies, including near band touching points. This enables full access to the system Bloch Hamiltonian and quantum geometric tensor. Our approach can readily be extended to more complex systems with additional internal degrees of freedom, enabling experimental investigations of trigonal warping, Chern insulating phases, and Euler-class topology in multigap systems.

cond-mat.mes-hall

Directional transport and nonlinear localization of light in a one-dimensional driven-dissipative photonic lattice

Photonic lattices facilitate band structure engineering, supporting both localized and extended modes through their geometric design. However, greater control over these modes can be achieved by taking advantage of the interference effect between external drives with precisely tuned phases and photonic modes within the lattice. In this work, we build on this principle to demonstrate optical switching, directed light propagation and site-specific localization in a one-dimensional photonic lattice of coupled microresonators by resonantly driving the system with a coherent field of controlled phase. Importantly, our experimental results provide direct evidence that increased driving power acts as a tuning parameter enabling nonlinear localization at frequencies previously inaccessible in the linear regime. These findings open new avenues for controlling light propagation and localization in lattices with more elaborate band structures.

physics.optics

Excitonic oscillator-strength saturation dominates polariton-polariton interactions

Exciton-polaritons in semiconductor microcavities exhibit large two-body interactions that, thanks to ever refined nanotechnology techniques, are getting closer and closer to the quantum regime where single-photon nonlinearities start being relevant. To foster additional progress in this direction, in this work we experimentally investigate the microscopic mechanism driving polariton-polariton interactions. We measure the dispersion relation of the collective excitations that are thermally generated on top of a coherent fluid of interacting lower-polaritons. By comparing the measurements with the Bogoliubov theory over both the lower and upper polariton branches simultaneously, we find that polariton-polariton interactions stem dominantly from a mechanism of saturation of the exciton oscillator strength.

cond-mat.mes-hall

Bogoliubov excitations driven by thermal lattice phonons in a quantum fluid of light

The elementary excitations in weakly interacting quantum fluids have a non-trivial nature which is at the basis of defining quantum phenomena such as superfluidity. These excitations and the physics they lead to have been explored in closed quantum systems at thermal equilibrium both theoretically within the celebrated Bogoliubov framework, and experimentally in quantum fluids of ultracold atoms. Over the past decade, the relevance of Bogoliubov excitations has become essential to understand quantum fluids of interacting photons. Their driven-dissipative character leads to distinct properties with respect to their equilibrium counterparts. For instance, the condensate coupling to the photonic vacuum environment leads to a non-zero generation rate of elementary excitations with many striking implications. In this work, considering that quantum fluids of light are often hosted in solid-state systems, we show within a joint theory-experiment analysis that the vibrations of the crystal constitute another environment that the condensate is fundamentally coupled to. This coupling leads to a unique heat transfer mechanism, resulting in a large generation rate of elementary excitations in typical experimental conditions, and to a fundamental non-zero contribution at vanishing temperatures. Our work provides a complete framework for solid-embedded quantum fluids of light, which is invaluable in view of achieving a regime dominated by photon vacuum fluctuations.

cond-mat.quant-gas

Phase diagram of one-dimensional driven-dissipative exciton-polariton condensates

We consider a one-dimensional driven-dissipative exciton-polariton condensate under incoherent pump, described by the stochastic generalized Gross-Pitaevskii equation. It was shown that the condensate phase dynamics maps under some assumptions to the Kardar-Parisi-Zhang (KPZ) equation, and the temporal coherence of the condensate follows a stretched exponential decay characterized by KPZ universal exponents. In this work, we determine the main mechanisms which lead to the departure from the KPZ phase, and identify three possible other regimes: (i) a soliton-patterned regime at large interactions and weak noise, populated by localized structures analogue to dark solitons; (ii) a vortex-disordered regime at high noise and weak interactions, dominated by point-like phase defects in space-time; (iii) a defect-free reservoir-textured regime where the adiabatic approximation breaks down. We characterize each regime by the space-time maps, the first-order correlations, the momentum distribution and the density of topological defects. We thus obtain the phase diagram at varying noise, pump intensity and interaction strength. Our predictions are amenable to observation in state-of-art experiments with exciton-polaritons.

cond-mat.stat-mech

Strongly-Correlated Electron-Photon Systems

An important goal of modern condensed matter physics involves the search for states of matter with new emergent properties and desirable functionalities. Although the tools for material design remain relatively limited, notable advances have been recently achieved by controlling interactions at hetero-interfaces, precise alignment of low-dimensional materials and the use of extreme pressures . Here, we highlight a new paradigm, based on controlling light-matter interactions, which provides a new way to manipulate and synthesize strongly correlated quantum matter. We consider the case in which both electron-electron and electron-photon interactions are strong and give rise to a variety of novel phenomena. Photon-mediated superconductivity, cavity-fractional quantum Hall physics and optically driven topological phenomena in low dimensions are amongst the frontiers discussed in this perspective, which puts a spotlight on a new field that we term here "strongly-correlated electron-photon science."

cond-mat.str-el

Kardar-Parisi-Zhang universality in discrete two-dimensional driven-dissipative exciton polariton condensates

The statistics of the fluctuations of quantum many-body systems are highly revealing of their nature. In driven-dissipative systems displaying macroscopic quantum coherence, as exciton polariton condensates under incoherent pumping, the phase dynamics can be mapped to the stochastic Kardar-Parisi-Zhang (KPZ) equation. However, in two dimensions (2D), it was theoretically argued that the KPZ regime may be hindered by the presence of vortices, and a non-equilibrium BKT behavior was reported close to condensation threshold. We demonstrate here that, when a discretized 2D polariton system is considered, universal KPZ properties can emerge. We support our analysis by extensive numerical simulations of the discrete stochastic generalized Gross-Pitaevskii equation. We show that the first-order correlation function of the condensate exhibits stretched exponential behaviors in space and time with critical exponents characteristic of the 2D KPZ universality class, and find that the related scaling function accurately matches the KPZ theoretical one, stemming from functional Renormalization Group. We also obtain the distribution of the phase fluctuations and find that it is non-Gaussian, as expected for a KPZ stochastic process.

cond-mat.quant-gas

Probing many-body correlations using quantum-cascade correlation spectroscopy

The radiative quantum cascade, i.e. the consecutive emission of photons from a ladder of energy levels, is of fundamental importance in quantum optics. For example, the two-photon cascaded emission from calcium atoms was used in pioneering experiments to test Bell inequalities. In solid-state quantum optics, the radiative biexciton-exciton cascade has proven useful to generate entangled-photon pairs. More recently, correlations and entanglement of microwave photons emitted from a two-photon cascaded process were measured using superconducting circuits. All these experiments rely on the highly non-linear nature of the underlying energy ladder, enabling direct excitation and probing of specific single-photon transitions. Here, we use exciton polaritons to explore the cascaded emission of photons in the regime where individual transitions of the ladder are not resolved, a regime that has not been addressed so far. We excite a polariton quantum cascade by off-resonant laser excitation and probe the emitted luminescence using a combination of spectral filtering and correlation spectroscopy. Remarkably, the measured photon-photon correlations exhibit a strong dependence on the polariton energy, and therefore on the underlying polaritonic interaction strength, with clear signatures from two- and three-body Feshbach resonances. Our experiment establishes photon-cascade correlation spectroscopy as a highly sensitive tool to provide valuable information about the underlying quantum properties of novel semiconductor materials and we predict its usefulness in view of studying many-body quantum phenomena.

quant-ph

Enhanced Cavity Optomechanics with Quantum-well Exciton Polaritons

Semiconductor microresonators embedding quantum wells can host tightly confined and mutually interacting excitonic, optical and mechanical modes at once. We theoretically investigate the case where the system operates in the strong exciton-photon coupling regime, while the optical and excitonic resonances are parametrically modulated by the interaction with a mechanical mode. Owing to the large exciton-phonon coupling at play in semiconductors, we predict an enhancement of polariton-phonon interactions by two orders of magnitude with respect to mere optomechanical coupling: a near-unity single-polariton quantum cooperativity is within reach for current semiconductor resonator platforms. We further analyze how polariton nonlinearities affect dynamical back-action, modifying the capability to cool or amplify the mechanical motion.

quant-ph

Observation of KPZ universal scaling in a one-dimensional polariton condensate

Revealing universal behaviors is a hallmark of statistical physics. Phenomena such as the stochastic growth of crystalline surfaces, of interfaces in bacterial colonies, and spin transport in quantum magnets all belong to the same universality class, despite the great plurality of physical mechanisms they involve at the microscopic level. This universality stems from a common underlying effective dynamics governed by the non-linear stochastic Kardar-Parisi-Zhang (KPZ) equation. Recent theoretical works suggest that this dynamics also emerges in the phase of out-of-equilibrium systems displaying macroscopic spontaneous coherence. Here, we experimentally demonstrate that the evolution of the phase in a driven-dissipative one-dimensional polariton condensate falls in the KPZ universality class. Our demonstration relies on a direct measurement of KPZ space-time scaling laws, combined with a theoretical microscopic analysis that consistently reveals the other key signatures of this universality class, together with the possible resilience of KPZ dynamics to the presence of space-time vortices. Our results highlight fundamental physical differences between out-of-equilibrium condensates and their equilibrium counterparts, and open a new paradigm for exploring universal behaviors in open systems.

cond-mat.mes-hall

Few-photon all-optical phase rotation in a quantum-well micropillar cavity

Photonic platforms are an excellent setting for quantum technologies because weak photon-environment coupling ensures long coherence times. The second key ingredient for quantum photonics is interactions between photons, which can be provided by optical nonlinearities in the form of cross-phase-modulation (XPM). This approach underpins many proposed applications in quantum optics and information processing, but achieving its potential requires strong single-photon-level nonlinear phase shifts and also scalable nonlinear elements. In this work we show that the required nonlinearity can be provided by exciton-polaritons in micropillars with embedded quantum wells. These combine the strong interactions of excitons with the scalability of micrometer-sized emitters. We observe XPM up to $3 \pm 1$ mrad per particle using laser beams attenuated to below single photon average intensity. With our work serving as a first stepping stone, we lay down a route for quantum information processing in polaritonic lattices.

physics.optics

Spontaneous coherence in spatially extended photonic systems: Non-Equilibrium Bose-Einstein condensation

In this review, we give an interdisciplinary overview of Bose-Einstein condensation phenomena in photonic systems. We cover a wide range of systems, from lasers to photon condensates in dye-filled cavities, to excitons in semiconductor heterostructures, to microcavity polaritons, as well as emerging systems such as mode-locked lasers and classical light waves. Rather than diving into the specific properties of each system, our main focus will be to highlight those novel universal phenomena that stem from the driven-dissipative, non-equilibrium nature of these systems and affect the static, dynamic and coherence properties of the condensate. We conclude with our view on the future perspectives of this field for both fundamental science and technological applications.

physics.optics