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Jacques Hawecker

Publications and source records attributed to Jacques Hawecker.

3 recordsLinked to original sources

Incoherent dark excitons extend Floquet-like physics across time and momentum

Floquet phenomena - where a coherent, time-periodic drive hybridizes the conduction band with energy-replicated copies of the valence band - have been demonstrated with intense optical fields and, more recently, other bosonic excitations. However, within mean-field approximations and the current understanding of Floquet phenomena, these effects survive only for the coherence time of the drive, limiting practical use and current demonstrations to the sub-picosecond regime. Here, consistent with recent theoretical predictions beyond the mean-field picture, using time- and angle-resolved photoemission spectroscopy in WSe$_2$/MoS$_2$ heterostructures, we show that incoherent, dense populations of dark interlayer excitons hybridize the conduction band with energy-replicated copies of the valence band, mimicking Floquet-like phenomena - now persisting for nearly a nanosecond. With increasing interlayer exciton density, the valence band and its replica evolve from an inverted-parabolic to a Mexican-hat dispersion, a signature of the predicted non-zero static coupling that hybridizes the bands and scales linearly with the exciton density. By tuning twist angle, we further show that dark excitons with net momentum create replicas that hybridize with bands offset not just in energy but also in momentum, providing another powerful degree of freedom beyond conventional Floquet engineering. These results establish a robust, long-lived route to engineering electronic states, beyond a coherent, zero-momentum drive.

cond-mat.mes-hall↗

Quasiparticle phono-conversion: filming carriers coalescing into excitons

Condensed matter physics is replete with phenomena involving high-energy free particles coalescing into low-energy bound few-particle states. While the cooling of the individual particles is well understood, the crucial step by which cold free carriers form a bound state remains elusive, involving complex energy and momentum relaxation pathways. Here, by combining ultrafast time- and momentum-resolved photoemission spectroscopy on a monolayer WSe$_2$ with the first-principles excitonic-Bloch equations, we resolve the conversion of initially free electrons and holes at the bandedges into bound excitons. With unprecedented energy resolution, we observe the transient \textit{coexistence} of free-carrier and excitonic bands, accompanied by a transfer of spectral weight between the two. We establish the phononic origin of exciton formation and ascribe this coexistence to a sequential relaxation cascade toward the lowest-energy excitonic states, wherein intermediate states remain weakly populated. The efficiency of this process is controlled by valley multiplicity, large-momentum phonon emission and spin-flip processes. By elucidating how bound states emerge from their elementary constituents, our results point to strategies for engineering exciton formation, with direct implications for optical materials and devices that operate with excitons or free carriers.

cond-mat.mtrl-sci↗

Spin injection efficiency at metallic interfaces probed by THz emission spectroscopy

Terahertz (THz) spin-to-charge conversion has become an increasingly important process for THz pulse generation and as a tool to probe ultrafast spin interactions at magnetic interfaces. However, its relation to traditional, steady state, ferromagnetic resonance techniques is poorly understood. Here we investigate nanometric trilayers of Co/X/Pt (X=Ti, Au or Au0:85W0:15) as a function of the 'X' layer thickness, where THz emission generated by the inverse spin Hall effect is compared to the Gilbert damping of the ferromagnetic resonance. Through the insertion of the 'X' layer we show that the ultrafast spin current injected in the non-magnetic layer defines a direct spin conductance, whereas the Gilbert damping leads to an effective spin mixing-conductance of the trilayer. Importantly, we show that these two parameters are connected to each other and that spin-memory losses can be modeled via an effective Hamiltonian with Rashba fields. This work highlights that magneto-circuits concepts can be successfully extended to ultrafast spintronic devices, as well as enhancing the understanding of spin-to-charge conversion processes through the complementarity between ultrafast THz spectroscopy and steady state techniques.

cond-mat.mes-hall↗