arXiv subjects

Jacques Tempere

Publications and source records attributed to Jacques Tempere.

At least 37 records · Page 2Linked to original sources

arXiv2022

Polaron with Quadratic Electron-phonon Interaction

We present the first numerically exact study of a polaron with quadratic coupling to the oscillator displacement, using two alternative methodological developments. Our results cover both anti-adiabatic and adiabatic regimes and the entire range of electron-phonon coupling $g_2$, from the system's stability threshold at attractive $g_2=-1$ to arbitrary strong repulsion at $g_2 \gg 1$. Key properties of quadratic polarons prove dramatically different from their linear counterparts. They (i) are insensitive even to large quadratic coupling except in the anti-adiabatic limit near the threshold of instability at attraction; (ii) depend only on the adiabatic ratio but are insensitive to the electron dispersion and dimension of space; (iii) feature weak lattice deformations even at the instability point. Our results are of direct relevance to properties of electrons at low densities in polar materials, including recent proposals for their superconducting states.

cond-mat.str-el↗

arXiv2022

Stability conditions for a large anharmonic bipolaron

A large polaron is a quasiparticle that consists of a nearly free electron interacting with the phonons of a material, whose lattice parameters are much smaller than the polaron scale. The electron-phonon interaction also leads to an attractive interaction between electrons, which can allow two polarons to pair up and form a bipolaron. It has been shown that large bipolarons can form in theory due to strong 1-electron-1-phonon coupling, but they have not been seen in real materials because the critical value of the required electron-phonon interaction is too large. Here, we investigate the effect of 1-electron-2-phonon coupling on the large bipolaron problem. Starting from a generalization of the Fröhlich Hamiltonian that includes both the standard 1-electron-1-phonon interaction as well as an anharmonic 1-electron-2-phonon interaction, we use the path integral method to find a semi-analytical upper bound for the bipolaron energy that is valid at all values of the Fröhlich coupling strength $α$. We find the bipolaron phase diagram and conditions for the bipolaron stability by comparing the bipolaron energy to the energy of two free polarons. The critical value of the Fröhlich coupling strength $α_{\text{crit}}$ is calculated as a function of the strength of the 1-electron-2-phonon interaction. The results suggest that large bipolaron formation is more likely in materials with significant 1-electron-2-phonon interaction as well as strong 1-electron-1-phonon interaction, such as strontium titanate.

cond-mat.supr-con↗

arXiv2022

Josephson effect as signature of electron-hole superfluidity in bilayers of van der Waals heterostructures

We investigate a Josephson junction in an electron-hole superfluid in a double layer TMD heterostructure. Observation of a critical tunneling current is a clear signature of superfluidity. In addition, we find the BCS-BEC crossover physics in the narrow barrier region controls the critical current across the entire system. The corresponding critical velocity, which is measurable in this system, has a maximum when the excitations pass from bosonic to fermionic. Remarkably, this occurs for the density at the boundary of the BEC to BCS-BEC crossover regime determined from the condensate fraction. This provides, for the first time in a semiconductor system, an experimental way to determine the position of this boundary.

cond-mat.supr-con↗

arXiv2022

Quantum effective action for the bosonic Josephson junction

We investigate a bosonic Josephson junction by using the path-integral formalism with relative phase and population imbalance as dynamical variables. We derive an effective only-phase action performing functional integration over the population imbalance. We then analyze the quantum effective only-phase action, which formally contains all the quantum corrections. To the second order in the derivative expansion and to the lowest order in $\hbar$, we obtain the quantum correction to the Josephson frequency of oscillation. Finally, the same quantum correction is found by adopting an alternative approach. Our predictions are a useful theoretical tool for experiments with atomic or superconducting Josephson junctions.

cond-mat.quant-gas↗

arXiv2022

General memory kernels and further corrections to the variational path integral approach for the Bogoliubov-Fröhlich Hamiltonian

The celebrated variational path integral approach to the polaron problem shows remarkable discrepancies with diagrammatic Monte Carlo for the Bogoliubov-Fröhlich Hamiltonian which describes an impurity weakly coupled to a Bose condensed atomic gas. It has been shown both via a renormalization group approach and by the method of correlated Gaussian wavefunctions that the model has a subtle UV divergence caused by quantum fluctuations, which are not captured within Feynman's approach. In this work we address the issues with Feynman's approach and show that by extending the model action to a more general form, and by considering higher order corrections beyond the Jensen-Feynman inequality, a good agreement with diagrammatic Monte Carlo can be obtained.

cond-mat.quant-gas↗

arXiv2022

Quasiparticle disintegration in fermionic superfluids

We study the fermionic quasiparticle spectrum in a zero-temperature superfluid Fermi gas, and in particular how it is modified by different disintegration processes. On top of the disintegration by emission of a collective boson ($1\to2$, subject of a previous study, PRL 124, 073404), we consider here disintegration events where three quasiparticles are emitted ($1\to3$). We show that both disintegration processes are described by a $t$-matrix self-energy (as well as some highly off-resonant vacuum processes), and we characterize the associated disintegration continua. At strong coupling, we show that the quasiparticle spectrum is heavily distorted near the $1\to3$ disintegration threshold. Near the dispersion minimum, where the quasiparticles remain well-defined, the main effect of the off-shell disintegration processes is to shift the location of the minimum by a value that corresponds to the Hartree shift in the BCS limit. With our approximation of the self-energy, the correction to the energy gap with respect to the mean-field result however remains small, in contrast with experimental measurements.

cond-mat.quant-gas↗

arXiv2021

Gaussian trajectory description of fragmentation in an isolated spinor condensate

Spin-1 Bose gases quenched to spin degeneracy exhibit fragmentation: the appearance of a condensate in more than one single-particle state. Due to its highly entangled nature, the dynamics leading to this collective state are beyond the scope of a Gaussian variational approximation of the many-body wave function. Here, we improve the performance of the Gaussian variational Ansatz by considering dissipation into a fictitious environment, effectively suppressing entanglement within individual quantum trajectories at the expense of introducing a classical mixture of states. We find that this quantum trajectory approach captures the dynamical formation of a fragmented condensate, and analyze how much dissipation should be added to the experiment in order to keep a single realization in a non-fragmented state.

cond-mat.quant-gas↗

arXiv2021

Revisiting the Maxwell multipoles for vectorized angular functions

Across many areas of physics, multipole expansions are used to simplify problems, solve differential equations, calculate integrals, and process experimental data. Spherical harmonics are the commonly used basis functions for a multipole expansion. However, they are not the preferred basis when the expression to be expanded is written as an explicit function of the unit vector on the sphere. Here, we revisit a different set of basis functions that are well-suited for multipole expansions of such vectorized angular functions. These basis functions are known in the literature by a variety of different names, including Maxwell multipoles, harmonic tensors, symmetric trace-free (STF) tensors, and Sachs-Pirani harmonics, but they do not seem be well-known among physicists. We provide a novel derivation of the Maxwell multipoles that highlights their analogy with the Legendre polynomials. We also rederive their key properties, and compile a list of further properties for pratical use, since this list seems to be missing in the current literature. We show the equivalence between the Maxwell multipoles and the spherical harmonics, derive conversion formulas between the two, and motivate when it is preferable to use either formalism. Since vectorized functions occur naturally in many physical problems, we expect that the method presented in this article can simplify calculations for physicists in many different fields.

math-ph↗

arXiv2021

Path-integral approach to the thermodynamics of bosons with memory: Partition function and specific heat

For a system of bosons that interact through a class of general memory kernels, a recurrence relation for the partition function is derived within the path-integral formalism. This approach provides a generalization to previously known treatments in the literature of harmonically coupled systems of identical particles. As an example the result is applied to the specific heat of a simplified model of an open quantum system of bosons, harmonically coupled to a reservoir of distinguishable fictitious masses.

cond-mat.quant-gas↗

arXiv2021

Path-integral approach to the thermodynamics of bosons with memory: Density and correlation functions

Expanding upon previous work, using the path-integral formalism we derive expressions for the one-particle reduced density matrix and the two-point correlation function for a quadratic system of bosons that interact through a general class of memory kernels. The results are applied to study the density, condensate fraction and pair correlation function of trapped bosons harmonically coupled to external distinguishable masses.

cond-mat.quant-gas↗

arXiv2021

Beyond the Fröhlich Hamiltonian: Path integral treatment of large polarons in anharmonic solids

The properties of an electron in a typical solid are modified by the interaction with the crystal ions, leading to the formation of a quasiparticle: the polaron. Such polarons are often described using the Fröhlich Hamiltonian, which assumes the underlying lattice phonons to be harmonic. However, this approximation is invalid in several interesting materials, including the recently discovered high-pressure hydrides which superconduct at temperatures above $200$K. In this paper, we show that Fröhlich theory can be extended to eliminate this problem. We derive four additional terms in the Fröhlich Hamiltonian to account for anharmonicity up to third order. We calculate the energy and effective mass of the new polaron, using both perturbation theory and Feynman's path integral formalism. It is shown that the anharmonic terms lead to significant additional trapping of the electron. The derived Hamiltonian is well-suited for analytical calculations, due to its simplicity and since the number of model parameters is low. Since it is a direct extension of the Fröhlich Hamiltonian, it can readily be used to investigate the effect of anharmonicity on other polaron properties, such as the optical conductivity and the formation of bipolarons.

cond-mat.supr-con↗

arXiv2020

Absorption and emission of a collective excitation by a fermionic quasiparticle in a Fermi superfluid

We study the process of absorption or emission of a bosonic collective excitation by a fermionic quasiparticle in a superfluid of paired fermions. From the RPA equation of motion of the bosonic excitation annihilation operator, we obtain an expression of the coupling amplitude of this process which is limited neither to resonant processes nor to the long wavelength limit. We confirm our result by independently deriving it in the functional integral approach using the gaussian fluctuation approximation, and by comparing it in the long wavelength limit to the quantum hydrodynamic result. Last, we give a straightforward application of the coupling amplitude we obtain by calculating the lifetime of the bosonic excitations of arbitrary wave number. We find a mode quality factor that decreases from its maximum at low wave numbers and vanishes when the bosonic branch hits the pair-breaking continuum.

physics.atm-clus↗

arXiv2020

Vortices in Fermi gases with spin-dependent rotation potentials

The rotation of two-component Fermi gases and the subsequent appearance of vortices have been the subject of numerous experimental and theoretical studies. Recent experimental advances in hyperfine state-dependent potentials and highly degenerate heteronuclear Fermi gases suggest that it would be feasible to create component-dependent rotation potentials in future experiments. In this study we use an effective field theory for Fermi gases to consider the effects of rotating only one component of the Fermi gas. We find that the superfluid band gap in bulk exists up to higher rotation frequencies because the superfluid at rest, far away from the vortex, has to resist only half of the rotational effects. The vortex remains the energetically favorable state above a critical frequency but exhibits a larger core size.

cond-mat.quant-gas↗

arXiv2020

Effect of segregation on inequality in kinetic models of wealth exchange

Empirical distributions of wealth and income can be reproduced using simplified agent-based models of economic interactions, analogous to microscopic collisions of gas particles. Building upon these models of freely interacting agents, we explore the effect of a segregated economic network in which interactions are restricted to those between agents of similar wealth. Agents on a 2D lattice undergo kinetic exchanges with their nearest neighbours, while continuously switching places to minimize local wealth differences. A spatial concentration of wealth leads to a steady state with increased global inequality and a magnified distinction between local and global measures of combatting poverty. Individual saving propensity proves ineffective in the segregated economy, while redistributive taxation transcends the spatial inhomogeneity and greatly reduces inequality. Adding fluctuations to the segregation dynamics, we observe a sharp phase transition to lower inequality at a critical temperature, accompanied by a sudden change in the distribution of the wealthy elite.

physics.soc-ph↗

arXiv2020

Beyond mean-field corrections to the quasiparticle spectrum of superfluid Fermi gases

We investigate the fermionic quasiparticle branch of superfluid Fermi gases in the BCS-BEC crossover and calculate the quasiparticle lifetime and energy shift due to its coupling with the collective mode. The only close-to-resonance process that low-energy quasiparticles can undergo at zero temperature is the emission of a bosonic excitation from the phononic branch. Close to the minimum of the branch we find that the quasiparticles remain undamped, allowing us to compute corrections to experimentally relevant quantities such as the energy gap, location of the minimum, effective mass, and Landau critical velocity.

cond-mat.quant-gas↗

arXiv2019

Feynman path-integral treatment of the Bose polaron beyond the Fröhlich model

An impurity immersed in a Bose-Einstein condensate is no longer accurately described by the Fröhlich Hamiltonian as the coupling between the impurity and the boson bath gets stronger. We study the dominant effects of the two-phonon terms beyond the Fröhlich model on the ground-state properties of the polaron using Feynman's variational path-integral approach. The previously reported discrepancy in the effective mass between the renormalization group approach and this theory is shown to be absent in the beyond-Fröhlich model on the positive side of the Feshbach resonance. Self-trapping, characterized by a sharp and dramatic increase of the effective mass, is no longer observed for the repulsive polaron once the two-phonon interactions are included. For the attractive polaron we find a divergence of the ground-state energy and effective mass at weaker couplings than previously observed within the Fröhlich model.

cond-mat.quant-gas↗

arXiv2019

Plasmonic Cooper pairing in single layer graphene

The dielectric function method (DFM), which uses a non-adiabatic approach to calculate the critical temperatures for superconductivity, has been quite successful in describing superconductors at low carrier densities. This regime of carrier densities causes other theories, such as BCS and Migdal-Eliashberg theory, to violate their assumption of a small Debye window. We investigate the application of DFM to the linear dispersion of single layer graphene. We derive the gap equation of DFM for a Dirac cone and calculate the critical temperature as a function of carrier density. This is done using an interaction potential that utilizes the Random Phase Approximation dielectric function and thus allows for plasmonic interactions. Our results show a significantly different behaviour of the critical temperature as a function of carrier density when compared to the BCS result. Thus, we find the DFM approach to be better suited when considering graphene systems at low carrier densities.

cond-mat.supr-con↗

arXiv2019

Finite element simulation of the liquid-liquid transition to metallic hydrogen

Hydrogen at high temperature and pressure undergoes a phase transition from a liquid molecular phase to a conductive atomic state, or liquid metallic hydrogen, sometimes referred to as the plasma phase transition (PPT). The PPT phase line was observed in a recent experiment studying laser-pulse heated hydrogen in a diamond anvil cell in the pressure range $\sim 100 - 170 \text{GPa}$ for temperatures up to $\sim 2000 \text{K}$. The experimental signatures of the transition are (i) a negative pressure-temperature slope, (ii) a plateau in the heating curve, assumed to be related to the latent heat of transformation, and (iii) an abrupt increase in the reflectance of the sample. We present a finite element simulation that accurately takes into account the position and time dependence of the heat deposited by the laser pulse. We calculate the heating curves and the sample reflectance and transmittance. This simulation confirms that the observed plateaus are related to the phase transition, however we find that large values of latent heat are needed and may indicate that dynamics at the transition are more complex than considered in current models. Finally, experiments are proposed that can distinguish between a change in optical properties due to a transition to a metallic state or due to closure of the bandgap in molecular hydrogen.

cond-mat.mtrl-sci↗