arXiv subjects

Jagadish Rajendran

Publications and source records attributed to Jagadish Rajendran.

3 recordsLinked to original sources

arXiv2026

Barium Hexaferrite Thin Films as a Scalable Magnetic-Insulator Platform for Proximity-Engineered Spintronics

Rare-earth iron garnets, such as yttrium iron garnet (YIG) and thulium iron garnet (TmIG), are the benchmark magnetic insulators for spintronic and magnonic devices, but achieving usable perpendicular magnetic anisotropy (PMA) in these materials typically relies on substrate strain- engineering, requiring careful lattice-matching and specific growth conditions that constrain ma- terial accessibility. Here we establish sputter grown barium hexaferrite (BaFe12O19, BaM) as a magnetic-insulator alternative with strong intrinsic perpendicular anisotropy, requiring no strain engineering. X-ray diffraction, transmission electron microscopy and Raman spectroscopy confirm stoichiometric films with atomically smooth surfaces, while first-principles calculations corroborate a robust ferrimagnetic ground state. The films exhibit square out-of-plane hysteresis with a coercive field of nearly 0.1 T. Unlike rare-earth garnets, the perpendicular anisotropy in BaM is intrinsic to its magnetoplumbite crystal structure, arising independent of highly ordered strain. Interfaced with Pt and with exfoliated BiSbTeSe2 (BSTS), BaM induces proximity induced anomalous Hall trans- port, confirming efficient interfacial exchange coupling, while the BSTS/BaM heterostructure shows an additional Hall contribution suggestive of non-collinear interfacial spin textures. These results position BaM thin films as a scalable magnetic-insulator platform for spintronic and topological heterostructure devices beyond the constraints of garnet chemistry.

cond-mat.mtrl-sci↗

arXiv2026

Crystallographic Orientation-Dependent Magnetotransport in the Layered Antiferromagnet -- CrSBr

Among two-dimensional magnetic materials, CrSBr has attracted considerable attention owing to its coexistence of ferromagnetic and antiferromagnetic ordering, which depends sensitively on crystallographic orientation. An additional distinguishing feature of CrSBr is its highly anisotropic Fermi surface in momentum space. In this work, we present a comprehensive investigation of magnetoresistance by systematically orienting the bias current and the applied magnetic field along all three crystallographic axes. We demonstrate that the magnetoresistance serves as a direct probe of electronic anisotropy, exhibiting pronounced variations when the current is applied along different crystallographic directions under a magnetic field perpendicular to the sample plane. For in-plane magnetic fields, we observe conventional anisotropic magnetoresistance accompanied by hysteresis, indicative of ferromagnetic behavior. Overall, our study provides a complete picture of electronic transport in CrSBr as a function of bias current and magnetic field orientation with respect to crystallographic directions, thereby opening pathways for future experiments requiring high sensitivity of electrical resistance to magnetic field gradients.

cond-mat.mtrl-sci↗

arXiv2025

Time Reversal Symmetry Broken Electronic Phases in Thin Films of Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$

High-temperature superconductors (high-Tc SCs) host a rich landscape of electronic phases encompassing the pseudogap, strange metal, superconducting, antiferromagnetic insulating, and Fermi-liquid regimes. The superconducting phase is notable for non-dissipative electronic functionality at relatively high temperatures. These phases are commonly probed in thermodynamic phase space by varying temperature or current through the sample. They can also be probed by breaking time-reversal symmetry (TRS) with an external magnetic field, which yields transition signatures distinct from those arising solely from temperature or current tuning. Here we show that electron transport in Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ is primarily governed by two-dimensional superconductivity consistent with a Berezinskii-Kosterlitz-Thouless (BKT) topological phase transition, as supported by current-voltage characteristics measured under temperature variation; these measurements preserve TRS. In contrast, when an external magnetic field is applied, the superconducting state is consistently preceded by weak antilocalization (WAL), where bound vortex-antivortex pairs dissociate into a normal metallic state through an intermediate localized phase. We further establish that highly disordered films exhibit transport dominated by three-dimensional weak localization, with superconductivity entirely suppressed.

cond-mat.supr-con↗